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3D‑Printed Carbon‑Based Conformal Electromagnetic Interference Shielding Module for Integrated Electronics

Nano-Micro Letters 2024年第5期16卷 87-101页

作者： Shaohong Shi yuheng jiang Hao Ren Siwen Deng Jianping Sun Fangchao Cheng Jingjing Jing Yinghong Chen State Key Laboratory of Featured Metal Materials and Life‑Cycle Safety for Composite Structures School of ResourcesEnvironment and MaterialsGuangxi UniversityNo.100Daxuedong RoadNanning 530004People’s Republic of China State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversitySichuan UniversityNo.24 South Section 1Yihuan RoadChengdu 610065People’s Republic of China

Electromagnetic interference shielding(EMI SE)modules are the core com-ponent of modern electronics.However,the tra-ditional metal-based SE modules always take up indispensable three-dimensional space inside electronics,posing a major obstacle to the integra-tion of electronics.The innovation of integrating 3D-printed conformal shielding(c-SE)modules with packaging materials onto core electronics offers infinite possibilities to satisfy ideal SE func-tion without occupying additional space.Herein,the 3D printable carbon-based inks with various proportions of graphene and carbon nanotube nanoparticles are well-formulated by manipulating their rheological peculiarity.Accordingly,the free-constructed architectures with arbitrarily-customized structure and multifunctionality are created via 3D printing.In particular,the SE performance of 3D-printed frame is up to 61.4 dB,simultaneously accompanied with an ultralight architecture of 0.076 g cm^(-3) and a superhigh specific shielding of 802.4 dB cm3 g^(-1).Moreover,as a proof-of-concept,the 3D-printed c-SE module is in situ integrated into core electronics,successfully replacing the traditional metal-based module to afford multiple functions for electromagnetic compatibility and thermal dissipa-tion.Thus,this scientific innovation completely makes up the blank for assembling carbon-based c-SE modules and sheds a brilliant light on developing the next generation of high-performance shielding materials with arbitrarily-customized structure for integrated electronics.

关键词： 3D printing Carbon-based nanoparticles Conformal electromagnetic interference shielding Integrated electronics

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Hybrid assembly of conducting nanofiber network for ultra-stretchable and highly sensitive conductive hydrogels

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Journal of Materials Science & Technology 2024年第2期169卷 1-10页

作者： Yalei Wang Shulong Zeng Shaohong Shi yuheng jiang Zhiwei Du Bingzhen Wang Xiurong Li State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures School of ResourcesEnvironment and MaterialsGuangxi UniversityNanning 530004China State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversitySichuan UniversityChengdu 610065China

Conductive hydrogels have attracted extensive attention owing to their promising application prospects in flexible and wearable electronics.However,achieving both high sensitivity and mechanical robustness remains challenging.Herein,a novel and versatile conductive hydrogel based on the hybrid assem-bly of conductive cellulose nanofiber(CNF)networks has been designed and fabricated.Assisted by the templating effect of CNFs and stabilizing effect of negatively charged poly(styrene sulfonate)(PSS),conducting polymer poly(3,4-ethylenedioxythiophene)(PEDOT)was self-organized into three-dimensional nanostructures which constructed a robust conductive network after in-situ oxidative polymerization.The unique structure derived from CNF bio-template endowed polyacrylamide(PAM)hydrogels with improved electrical conductivity and excellent mechanical performance.As a result,the as-fabricated CNF/PEDOT:PSS/PAM hydrogel exhibited an ultimate tensile strain of 1881%and toughness of 3.72 MJ/m^(3),which were 4.07 and 8.27 times higher than the CNF-free hydrogel,respectively.More significantly,the resultant hydrogel sensor showed highly desirable sensing properties,including remarkable sensing range(1100%),high gauge factor(GF=5.16),fast response time(185 ms),and commendable durability,as well as good adhesiveness.Moreover,the hydrogel sensor was able to distinguish subtle physiological activities including phonation and facial expression,and monitor large human body motions such as finger flexion and elbow blending.Besides,it was feasible to integrate the strain sensor on the joints of robots to recognize complicated machine motion signals,showing potential in advanced human-machine interactions.

关键词： Strain sensor Cellulose nanofibers PEDOT:PSS Conductive hydrogel Templating method

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Flexible pressure sensors with ultrahigh stress tolerance enabled by periodic microslits

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Microsystems & Nanoengineering 2024年第1期10卷 301-311页

作者： Song Wang Chenying Wang Yifan Zhao Yujing Zhang Yaxin Zhang Xiangyue Xu Qijing Lin Kai Yao yuheng Wang Feng Han Yu Sun Zhuangde jiang State Key Laboratory for Manufacturing Systems Engineering International Joint Laboratory for Micro/Nano Manufacturing and Measurement TechnologiesSchool of Mechanical EngineeringXi’an Jiaotong UniversityXi’anChina State Key Laboratory for Manufacturing Systems Engineering International Joint Laboratory for Micro/Nano Manufacturing and Measurement TechnologiesSchool of Instrument Science and TechnologyXi’an Jiaotong UniversityXi’anChina The Faculty of Electrical Engineering and Computer Science Ningbo UniversityNingboChina Department of Mechanical and Industrial Engineering University of TorontoTorontoCanada

Stress tolerance plays a vital role in ensuring the effectiveness of piezoresistive sensing films used in flexible pressure sensors.However,existing methods for enhancing stress tolerance employ dome-shaped,wrinkle-shaped,and pyramidal-shaped microstructures in intricate molding and demolding processes,which introduce significant fabrication challenges and limit the sensing performance.To address these shortcomings,this paper presents periodic microslits in a sensing film made of multiwalled carbon nanotubes and polydimethylsiloxane to realize ultrahigh stress tolerance with a theoretical maximum of 2.477 MPa and a sensitivity of 18.092 kPa−1.The periodic microslits permit extensive deformation under high pressure(e.g.,400 kPa)to widen the detection range.Moreover,the periodic microslits also enhance the sensitivity based on simultaneously exhibiting multiple synapses within the sensing interface and between the periodic sensing cells.The proposed solution is verified by experiments using sensors based on the microslit strategy for wind direction detection,robot movement sensing,and human health monitoring.In these experiments,vehicle load detection is achieved for ultrahigh pressure sensing under an ultrahigh pressure of over 400 kPa and a ratio of the contact area to the total area of 32.74%.The results indicate that the proposed microslit strategy can achieve ultrahigh stress tolerance while simplifying the fabrication complexity of preparing microstructure sensing films.

关键词： robot shaped stress

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Recent advances on aerobic photocatalytic methane conversion under mild conditions

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Nano Research 2023年第11期16卷 12558-12571页

作者： yuheng jiang Siyang Li Xiaoyu Fan Zhiyong Tang Chinese Academy of Science(CAS)Key Laboratory of Nanosystem and Hierarchy Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190China Center for Nanoscale Science and Technology Academy for Advanced Interdisciplinary StudiesPeking UniversityBeijing 100871China University of Chinese Academy of Sciences Beijing 100049China Sino-Danish College University of Chinese Academy of SciencesBeijing 100049China

Photocatalytic methane conversion to high value-added chemicals under mild conditions acts as a promising approach to utilize natural gas and renewable energy.Specifically,aerobic photocatalytic methane conversion that uses molecular oxygen as oxidant has attracted much attention because it is thermodynamic favorable and could generate various reactive oxygen species,resulting in many value-added products like methanol,formaldehyde,ethane,and ethylene.In this review,we classify the aerobic photocatalytic methane conversion into aerobic photocatalytic partial oxidation of methane(APPOM)and aerobic photocatalytic coupling of methane(APCM).We particularly focus on the fundamentals of oxygen activation and methane reaction modes in these conversions.Finally,we provide a brief summary for current challenges and future prospects towards aerobic photocatalytic methane conversion.

关键词： photocatalysis oxygen methane oxidation coupling mild conditions

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In situ reconstruction induced oxygen-deficient multiphase Cu based species hybridized with Ni single atoms as tandem platform for CO_(2) electroreduction

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Nano Research 2024年第5期17卷 3888-3894页

作者： Juzhe Liu yuheng Wang Pengpeng Mo Feng Yang Kaiqi jiang Zhixiang Cheng Yuxuan Liu Zhiyi Sun Zheng Liu Yimei Zhang Wenxing Chen The Key Laboratory of Resources and Environmental System Optimization Ministry of EducationCollege of Environmental Science and EngineeringNorth China Electric Power UniversityBeijing 102206China Energy&Catalysis Center School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China SEPA Key Laboratory of Eco-Industry Chinese Research Academy of Environmental SciencesBeijing 100012China

Tandem catalysis,capable of decoupling individual steps,provides a feasible way to build a high-efficiency CO_(2) electro-conversion system for multicarbons(C_(2+)).The construction of electrocatalytic materials is one of focusing issues.Herein,we fabricated a single atom involved multivalent oxide-derived Cu composite material and found it inclined to reconstruct into oxygen-deficient multiphase Cu based species hybridized with monatomic Ni on N doped C matrix.In this prototype,rapid CO generation and C-C coupling are successively achieved on NiN4 sites and surface amorphized Cu species with defects,resembling a micro-production line.In this way,the in situ formed tandem catalyst exhibited a high Faradaic efficiency(FE)of~78%for C_(2+)products along with satisfactory durability over 50 h.Particularly,the reconstruction-induced amorphous layer with abundant asymmetric sites should be favorable to improve the ethanol selectivity(FE:63%),which is about 10 times higher than that of the non-tandem Cu-based contrast material.This work offers a new approach for manipulating tandem catalyst systems towards enhancing C_(2+)products.

关键词： tandem catalysis single atom reconstruction amorphous CO_(2)reduction reaction

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Photocatalytic Methane Conversion:Insight into the Mechanism of C(sp^(3))-H Bond Activation

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CCS Chemistry 2023年第1期5卷 30-54页

作者： yuheng jiang Yingying Fan Siyang Li Zhiyong Tang Chinese Academy of Science(CAS)Key Laboratory of Nanosystem and Hierarchy Fabrication CAS Center for Excellence in NanoscienceNational Center for Nanoscience and TechnologyBeijing 100190 Center for Advanced Analytical Science School of Chemistry and Chemical EngineeringSchool of Civil EngineeringAnalytical and Testing CenterGuangzhou UniversityGuangzhou 510006 Center for Nanoscale Science and Technology Academy for Advanced Interdisciplinary StudiesPeking UniversityBeijing 100871 University of Chinese Academy of Sciences Beijing 100049

Mild and direct conversion of methane into high value-added products is a desired goal for chemistry,energy,and environment.The active species generated in the photocatalytic reaction system under mild conditions activate the inert C-H bond in methane and promote methane conversion.This review focuses on the developed mechanisms for C(sp^(3))-H bond activation in photocatalytic methane conversion,including radical and active site mechanisms.Particular emphasis is placed on the detailed summary of mechanism,characterization method,and corresponding application in photocatalytic methane conversion.We also discuss the challenges and prospects for future direction on C(sp^(3))-H bond activation mechanism in photocatalytic methane conversion.This review aims to promote the development of photocatalytic methane conversion and provides guidance for the design of high-efficiency photocatalysts.

关键词： photocatalysis methane C-H bonds radical active site

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Chemical construction and anti-HCoV-OC43 evaluation of novel 10,12-disubstituted aloperine derivatives as dual cofactor inhibitors of TMPRSS2 and SR-B1

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Chinese Chemical Letters 2024年第5期35卷 201-206页

作者： Yulong Shi Fenbei Chen Mengyuan Wu Xin Zhang Runze Meng Kun Wang Yan Wang yuheng Mei Qionglu Duan Yinghong Li Rongmei Gao Yuhuan Li Hongbin Deng Jiandong jiang Yanxiang Wang Danqing Song Beijing Key Laboratory of Antimicrobial Agents Institute of Medicinal BiotechnologyChinese Academy of Medical Sciences and Peking Union Medical CollegeBeijing 100050China Department of Pharmacy Affiliated Hospital of Jining Medical UniversityJining Medical UniversityJining 272000China

Thirty-one new 10,12-disubstituted aloperine derivatives were subtly constructed through a selective oxidation on the 10-α-C-H induced by sulfonyl and a nucleophilic substitution with the stereoselectivity and scalability.Of them,compound 6b displayed a moderate anti-human coronavirus OC43(HCoV-OC43)potency and blocked the viral entry stage through a host mechanism of action.Using chemoproteomic techniques,both transmembrane serine protease 2(TMPRSS2)and scavenger receptor class B type 1(SR-B1)proteins,which act as host cofactors of viral entry,were identified to be the direct targets of 6b against HCoV-OC43.Furthermore,6b may deactivate the TMPRSS2 by inducing a change in protein conformation,rather than binding to its catalytic center,thus suppressing the viral membrane fusion.Accordingly,our study provided key scientific data for the development of aloperine derivatives into a new class of antiviral candidates against humanβ-coronavirus,including severe acute respiratory syndrome coronavirus 2(SARS-CoV-2).

关键词： Aloperine SARS-CoV-2 TMPRSS2 SR-B1 Synthesis

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基于自然容错开关表的五相永磁同步电机直接转矩控制

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中国电机工程学报 2024年第4期44卷 1618-1628,I0031页

作者：周华伟陈铖赵宇恒江光耀张多江苏大学电气信息工程学院江苏省镇江市212013

五相永磁同步电机(permanent-magnetsynchronous motor,PMSM)传统直接转矩控制(direct torque control,DTC)存在相电流畸变严重、共模电压(common-modevoltage,CMV)高、转矩和磁链脉动大等问题,且无法实现相开路故障情况下的无扰运行。为解决上述问题,提出一种基于自然容错开关表的DTC策略。该策略根据PMSM开路故障前后基电压矢量的特点以及三次平面合成电压矢量为零的原则,构建虚拟矢量(virtual vector,VV),设计故障前后同一套自然容错开关表,进而不但抑制了故障导致的转矩脉动,而且在故障前后均能降低三次谐波电流、减小转矩和磁链脉动、抑制CMV。实验结果验证所提策略的可行性。

关键词：共模电压直接转矩控制容错开关表单相开路故障永磁同步电机虚拟矢量

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Advances in the Treatment of Acute ITP

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Journal of Integrative Medicine（双语） 2022年第1期11卷 22-28页

作者： yuheng jiang Jiahao Gu Zai Gu Yifeng Xu Bin Jia Jing Yang School of Emergency Trauma Hainan Medical UniversityHaikouHainan570100China School of Nursing Hainan Medical UniversityHaikouHainan570100China

Immune thrombocytopenia(ITP),also known as idiopathic thrombocytopenic purpura,is a hematologic disease in which platelet destruction increases and production decreases,mainly mediated by immunity.However,up to now,the pathogenesis of ITP is not clear,which has caused great trouble in treatment.Therefore,this paper intends to review the recent literature on ITP treatment to provide some reference for clinical treatment.This paper combines the evidence of ASH immune thrombocytopenia and the Chinese Guidelines for the Diagnosis and Treatment of Adult primary immune thrombocytopenia(2020 edition).In this paper,the treatment process of ITP was divided into first-line treatment and second-line treatment,and it was concluded that first-line treatment was often used when newly diagnosed with ITP:combination of high-dose dexamethasone and low-dose gamma globulin.However,it should be noted that only 60%-80%of patients responded to first-line treatment,and most of them relapsed during dosing reduction or drug withdrawal.Second-line treatment is recommended in this case.The standard treatment is splenectomy,but due to its uncontrollable nature and side effects,it should be used cautiously.A new treatment approach,thrombogenin receptor agonist,has great development potential,and multidrug combination therapy for ITP has positive clinical significance.

关键词： ITP Hormone therapy IVIg treatment Splenectomy Thrombopoietin receptor agonist

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渤东凹陷新生代伸展-走滑叠合断裂时空差异演化模式及控藏效应

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岩性油气藏 2024年第3期36卷 106-116页

作者：董柔李坤殷际航薛煜恒江涛徐国盛中国石油长庆油田分公司第十一采油厂甘肃庆阳745000 油气藏地质及开发工程国家重点实验室(成都理工大学) 成都610059 中海石油(中国)有限公司天津分公司天津300452

以三维地震精细解释为基础,通过构造剖面恢复,系统分析了渤东凹陷新生代伸展-走滑叠合断裂的时空差异演化特征及控藏作用。研究结果表明:(1)渤东凹陷新生代广泛发育以NNE向为主干、NE向为派生、NW向为叠加的伸展-走滑叠合断裂体系,可划... 详细信息

以三维地震精细解释为基础,通过构造剖面恢复,系统分析了渤东凹陷新生代伸展-走滑叠合断裂的时空差异演化特征及控藏作用。研究结果表明:(1)渤东凹陷新生代广泛发育以NNE向为主干、NE向为派生、NW向为叠加的伸展-走滑叠合断裂体系,可划分为强伸展-弱走滑断裂和强走滑-弱伸展断裂2类;整体具有深浅分层、南北分段的特征,纵向上,古近系主要发育强伸展-弱走滑断裂,断裂大而稀,新近系—第四系主要发育强走滑-弱伸展断裂,断裂小而密;平面上,同一断裂在不同段的构造组合样式存在差异。(2)研究区新生代伸展-走滑叠合断裂的演化主要表现为北部断裂活动强度“早强晚弱”,中部断裂继承性持续发育,南部断裂活动强度“早弱晚强”;演化模式分为初始断陷(孔店组—沙四段沉积期)、强烈断陷(沙三段—东营组沉积期)和走滑坳陷(馆陶组—平原组沉积期)3个阶段,初始断陷阶段,NNE—NE向强伸展与弱走滑叠合,NE向强伸展-弱走滑断裂为主控,NW向先存断裂活化,分割凹陷;强烈断陷阶段,NNE—NE向强伸展与弱走滑叠合,NNE向强伸展-弱走滑断裂变为主控,NW向断裂活动减弱或停止;走滑坳陷阶段,NNE向强走滑与弱伸展叠合,断裂不控制沉积,但对地层展布具有调整作用。(3)研究区伸展-走滑叠合断裂的发育演化与油气成藏密切相关,整体具有“早期伸展控源、晚期走滑控运、多期叠加控圈”的特征,东部斜坡带是油气运聚的有利区。

关键词：伸展-走滑叠合断裂断裂演化油气运聚断裂控藏沙河街组东营组新生代渤东凹陷

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