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Point-defect engineering of nanoporous CuBi_(2)O_(4) photocathode via rapid thermal processing for enhanced photoelectrochemical activity

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Journal of Energy Chemistry 2022年第8期31卷 201-209,I0007页

作者： Li Qu Runfa Tan Arumugam Sivanantham Min Je Kang yoo Jae Jeong Dong Hyun Seo Sungkyu kim In Sun Cho Department of Materials Science&Engineering Ajou UniversitySuwon 16499South Korea Department of Energy Systems Research Ajou UniversitySuwon 16499South Korea Department of Nanotechnology and Advanced Materials Engineering Sejong UniversitySeoul 05006South Korea

Engineering point defects such as metal and oxygen vacancies play a crucial role in manipulating the electrical,optical,and catalytic properties of oxide semiconductors for solar water ***,we synthesized nanoporous CuBi_(2)O_(4)(np-CBO)photocathodes and engineered their surface point defects via rapid thermal processing(RTP)in controlled atmospheres(O_(2),N_(2),and vacuum).We found that the O_(2)-RTP treatment of np-CBO increased the charge carrier density effectively without hampering the nanoporous morphology,which was attributed to the formation of copper vacancies(VCu).Further analyses revealed that the amounts of oxygen vacancies(Vo)and Cu^(1+)were reduced simultaneously,and the relative electrochemical active surface area increased after the O_(2)-RTP ***,the point defects(VC_(u),Cu^(1+),and Vo)regulated np-CBO achieved a superb water-splitting photocurrent density of-1.81 m A cm^(-2) under simulated sunlight illumination,which is attributed to the enhanced charge transport and transfer properties resulting from the regulated surface point ***,the reversibility of the formation of the point defects was checked by sequential RTP treatments(O_(2)-N_(2)-O_(2)-N_(2)),demonstrating the strong dependence of photocurrent response on the RTP ***,the surface point defect engineering via RTP treatment in a controlled atmosphere is a rapid and facile strategy to promote charge transport and transfer properties of photoelectrodes for efficient solar water-splitting.

关键词： Nanoporous Copper bismuth oxide Rapid thermal processing Copper vacancy Charge transport

Tonicity response element binding protein associated with neuronal cell death in the experimental diabetic retinopathy

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International Journal of Ophthalmology(English edition) 2014年第6期7卷 935-940页

作者： Seong-Jae kim Hwajin kim Jeongsook Park Inyoung Chung Hyug-Moo Kwon Wan-Sung Choi Ji-Myong yoo Department of Ophthalmology School of MedicineGyeongsang National University Institute of Health Science Gyeongsang National University Department of Anatomy and Neurobiology BK21 Biomedical CenterSchool of MedicineGyeongsang National University School of Nano-Bioscience and Chemical Engineering Ulsan National Institute and Science and Technology

AIM: To study the contribution of tonicity response element binding protein(Ton EBP) in retinal ganglion cell(RGC) death of diabetic retinopathy(DR).METHODS: Diabetes was induced in C57BL/6 mice by five consecutive intraperitoneal injections of 55 mg/kg streptozotocin(STZ). Control mice received vehicle(phosphate-buffered saline). All mice were killed 2mo after injections, and the extent of cell death and the protein expression levels of Ton EBP and aldose reductase(AR) were ***: The Ton EBP and AR protein levels and the death of RGC were significantly increased in the retinas of diabetic mice compared with controls 2mo after the induction of diabetes. Terminal deoxynucleotidyl transferase(Td T)-mediated d UTP nick end labeling(TUNEL)-positive signals co-localized with Ton EBP immunoreactive RGC. These changes were increased in the diabetic retinas compared with ***: The present data show that AR and Ton EBP are upregulated in the DR and Ton EBP may contribute to apoptosis of RGC in the DR.

关键词： aldose reductase diabetes tonicity response element binding protein retinopathy

Mimicking a Superhydrophobic Insect Wing by Argon and Oxygen Ion Beam Treatment on Polytetrafluoroethylene Film

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Journal of Bionic Engineering 2009年第4期6卷 365-370页

作者： Youngjong Lee Yonghoon yoo Jihoon kim Sriyulianti Widhiarini Baeho Park Hoon Cheol Park Kwang Joon yoon Doyoung Byun Department of Aerospace Information Engineering Konkuk UniversitySeoul 143-701Republic of Korea Department of Physics Konkuk UniversitySeoul 143-701Republic of Korea Department of Advanced Technology Fusion Konkuk UniversitySeoul 143-701Republic of Korea

Biological tiny structures have been observed on many kinds of surfaces such as lotus leaves and insect wings,which enhance the hydrophobicity of the natural surfaces and play a role of *** presented the fabrication technology of a superhydrophobic surface using high energy ion *** insect wings that mimic the morphology and the superhydrophobocity of cicada's wings were successfully fabricated using argon and oxygen ion beam treatment on a polytetrafluoroethylene (PTFE)*** wing structures were supported by carbon/epoxy fibers as artificial flexible veins that were bonded through an autoclave *** morphology of the fabricated surface bears a strong resemblance to the wing surface of a cicada,with contact angles greater than 160°,which could be sustained for more than two months.

关键词： superhydrophobic insect wing mimicry of the wing ion beam treatment artificial flapper dynamic contact angle

Curved copper nanowires-based robust flexible transparent electrodes via all-solution approach

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Nano Research 2017年第9期10卷 3077-3091页

作者： Zhenxing Yin Seung Keun Song Sanghun Cho Duck-Jae You Jeeyoung yoo Suk Tai Chang Youn Sang kim Program in Nano Science and Technology Graduate School of Convergence Science and Technology Seoul National University Seoul 08826 Republic of Korea School of Chemical Engineering and Materials Science Chung-Ang University Seou106974 Republic of Korea Advanced Institutes of Convergence Technology 145 Gwanggyo-ro Yeongtong-gu Suwon-si Gyeonggi-do 16229 Republic of Korea

Curved Cu nanowire (CCN)-based high-performance flexible transparent conductive electrodes (FTCEs) were fabricated via a fully solution-processed approach, involving synthesis, coating, patterning, welding, and transfer. Each step involved an innovative technique for completing the all-solution processes. The high-quality and well-dispersed CCNs were synthesized using a multi-polyol method through the synergistic effect of specific polyol reduction. To precisely control the optoelectrical properties of the FTCEs, the CCNs were uniformly coated on a polyimide (PI) substrate via a simple meniscus-dragging deposition method by tuning several coating parameters. We also employed a polyurethane (PU)-stamped patterning method to effectively produce 20 μm patterns on CCN thin films. The CCN thin films exhibited high electrical performance, which is attributed to the deeply percolated CCN network formed via a solvent-dipped welding method. Finally, the CCN thin films on the PI substrate were partially embedded and transferred to the PU matrix to reduce their surface roughness. Through consecutive processes involving the proposed methods, a highly percolated CCN thin film on the PU matrix exhibited high optoelectrical performance (R s = 53.48 Ω/□ at T = 85.71%), excellent mechanical properties (R/R 0 < 1.10 after the 10th repetition of tape peeling or 1,000 bending cycles), and a low root-mean-square surface roughness (R rms = 14.36 nm).

关键词： curved Cu nanowires all-solution processes 20 μm patterns high performance transparent electrode

Transanal excision of a malignant fibrous histiocytoma of anal canal:A case report and literature review

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World Journal of Gastroenterology 2008年第9期14卷 1459-1462页

作者： Beom Gyu kim In Taik Chang Jun Seok Park yoo Shin Choi Gi Hyeon kim Eon Sub Park Chang Hwan Choi Department of Surgery College of MedicineChung-Ang University Seoul 156-755Korea Department of Radiology College of MedicineChung-Ang University Seoul 156-755Korea Department of Pathology College of MedicineChung-Ang University Seoul 156-755 Korea Department of Internal Medicine College of Medicine Chung-Ang UniversitySeoul 156-755Korea

Malignant fibrous histiocytoma, which is composed of spindle-shaped cells arranged in a pleomorphic and storiform pattern, is rarely found in the colorectum. Although complete surgical excision remains the main stem of therapy, an optimal treatment strategy according to the stage has not been elucidated. We report a case of a 63-year-old woman with an ulcerative lesion in the anorectal junction and a final diagnosis of malignant fibrous histiocytoma. We introduced an access for transanal local excision and adjuvant radiotherapy because the patient refused abdominoperineal resection. No local recurrences or distant metastases were observed 15 mo after the operation. To our knowledge, this is the first case reported in the English literature of a malignant fibrous histiocytoma treated with the transana local excision and adjuvant radiotherapy. This report showed that this approach is selectively reserved for early-stage malignant fibrous histiocytoma and for those patients who refuse radical surgery because of the risk in a permanent colostomy.

关键词： Malignant fibrous histiocytoma Anorectal junction Transanal local excision

Time- and cell-type specific changes in iron, ferritin, and transferrin in the gerbil hippocampal CA1 region after transient forebrain ischemia

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Neural Regeneration Research 2016年第6期11卷 924-930页

作者： Dae Young yoo Ki-Yeon yoo Joon Ha Park Hyun Jung Kwon Hyo Young Jung Jong Whi kim Goang-Min Choi Seung Myung Moon Dae Won kim Yeo Sung yoon Moo-Ho Won In Koo Hwang Department of Anatomy and Cell Biology College of Veterinary Medicine and Research Institute for Veterinary Science Seoul National University Department of Oral Anatomy Research Institute of Oral Sciences College of Dentistry Gangneung-Wonju National University Department of Neurobiology School of Medicine Kangwon National University Department of Biochemistry and Molecular Biology Research Institute of Oral Sciences College of Dentistry Gangneung-Wonju National University Department of Thoracic and Cardiovascular Surgery Chuncheon Sacred Heart Hospital College of Medicine Hallym University Department of Neurosurgery Dongtan Sacred Heart Hospital College of Medicine Hallym University

In the present study, we used immunohistochemistry and western blot analysis to examine changes in the levels and cellular localization of iron, heavy chain ferritin（ferritin-H）, and transferrin in the gerbil hippocampal CA1 region from 30 minutes to 7 days following transient forebrain ischemia. Relative to sham controls, iron reactivity increased significantly in the stratum pyramidale and stratum oriens at 12 hours following ischemic insult, transiently decreased at 1–2 days and then increased once again within the CA1 region at 4–7 days after ischemia. One day after ischemia, ferritin-H immunoreactivity increased significantly in the stratum pyramidale and decreased at 2 days. At 4–7 days after ischemia, ferritin-H immunoreactivity in the glial components in the CA1 region was significantly increased. Transferrin immunoreactivity was increased significantly in the stratum pyramidale at 12 hours, peaked at 1 day, and then decreased significantly at 2 days after ischemia. Seven days after ischemia, Transferrin immunoreactivity in the glial cells of the stratum oriens and radiatum was significantly increased. Western blot analyses supported these results, demonstrating that compared to sham controls, ferritin H and transferrin protein levels in hippocampal homogenates significantly increased at 1 day after ischemia, peaked at 4 days and then decreased. These results suggest that iron overload-induced oxidative stress is most prominent at 12 hours after ischemia in the stratum pyramidale, suggesting that this time window may be the optimal period for therapeutic intervention to protect neurons from ischemia-induced death.

关键词： ferritin transferrin hippocampal stratum minutes glial Ferritin hippocampus rabbit reactivity

Effects of prostaglandin F_(2α) on small intestinal interstitial cells of Cajal

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World Journal of Gastroenterology 2011年第9期17卷 1143-1151页

作者： Chan Guk Park Young Dae kim Man yoo kim Jae Woong Koh Jae Yeoul Jun Cheol Ho Yeum Insuk So Seok Choi Department of Internal Medicine College of MedicineChosun University Department of Ophthalmology College of MedicineChosun University Department of Physiology College of MedicineChosun University Department of Physiology and Biophysics College of MedicineSeoul National University

AIM：To explore the role of prostaglandin F2α（PGF2α） on pacemaker activity in interstitial cells of Cajal（ICC）from mouse small intestine. METHODS：In this study,effects of PGF2αin the cultured ICC cells were investigated with patch clamp technology combined with Ca 2＋ image analysis. RESULTS：Externally applied PGF2α（10μmol/L）produced membrane depolarization in current-clamp mode and increased tonic inward pacemaker currents in voltage-clamp *** application of flufenamic acid（a non-selective cation channel inhibitor）or niflumic acid（aCl channel inhibitor）abolished the generation of pacemaker currents but only flufenamic acid inhibited the PGF2α-induced tonic inward *** addition,the tonic inward currents induced by PGF2αwere not inhibited by intracellular application of 5’-[-thio]diphosphate trilithium *** with Ca 2＋ free solution, U-73122,an active phospholipase C inhibitor,and thapsigargin,a Ca 2＋ -ATPase inhibitor in endoplasmic reticulum,abolished the generation of pacemaker currents and suppressed the PGF2α-induced tonic inward ***,chelerythrine or calphostin C,protein kinase C inhibitors,did not block the PGF2α-induced effects on pacemaker *** recording intracellular Ca 2＋（[Ca 2＋ ]i）concentration using fluo-3/AM,PGF2α broadly increased the spontaneous[Ca 2＋ ]i oscillations. CONCLUSION：These results suggest that PGF2αcan modulate pacemaker activity of ICC by acting non-selective action channels through phospholipase C-dependent pathway via[Ca2＋]i regulation

关键词： Prostaglandin F2α Interstitial cells of Cajal Tonic inward currents Intestinal motility

Insights into the pathogenesis of cystoid macular edema: leukostasis and related cytokines

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International Journal of Ophthalmology(English edition) 2019年第7期12卷 1202-1208页

作者： yoo-Ri Chung Young Ho kim Seung Yeop Lee Hye-Eun Byeon Kihwang Lee Department of Ophthalmology Ajou University School of Medicine Suwon 16499 Korea Institute of Medical Science Ajou University School of Medicine Suwon 16499 Korea

Cystoid macular edema(CME) is the abnormal collection of intraretinal fluid in the macular region, especially in the inner nuclear and outer plexiform layers. CME leads to severe visual impairment in patients with various retinal diseases, such as diabetic retinopathy, retinal vascular occlusion, choroidal neovascularization, and uveitis. Although various retinal conditions lead to CME, a shared pathogenesis of CME is involved in these diseases. Accordingly, the pathogenesis of CME based on vasogenic mechanisms is first discussed in this review, including vascular hyperpermeability, leukostasis, and inflammation. We then describe cytotoxic mechanisms based on retinal Müller cell dysfunction. This comprehensive review will provide an understanding of the pathogenesis of CME for potential therapeutic strategies.

关键词： cystoid macular edema cytokine leukostasis pathogenesis

Microstructure,Elastic Modulus and Tensile Properties of Ti-Nb-O Alloy System

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Journal of Materials Science & Technology 2008年第1期24卷 33-36页

作者： H.S.kim T.Y.Ra I.D.Yeo H.J.Bang Y.G.yoo W.Y.kim Advanced Materials R＆D Division Korea Institute of Industrial Technology Incheon 406-800 Korea

In the present study Ti-Nb binary alloy system was chosen because it has excellent biocompatibility as well as reasonable mechanical properties,aiming at understanding oxygen content on microstructural formation, elastic modulus and tensile properties in Ti-Nb alloy *** alloy buttons of 50 mm in diameter were prepared by arc melting on a water-cooled copper hearth under an argon gas atmosphere with a non-consumable tungsten *** button ingots were then heat treated in a vacuum atmosphere at 1273 K for 0.5 h followed by water quenching in a specially designed heat treatment ***,elastic modulus and tensile properties were investigated in order to understand the effect of oxygen content in quenched Ti- Nb alloy *** orthorhombic structuredα″martensite was changed to bcc structuredβ-phase with increasing Nb ***,it was found that oxygen makesβ-phase stable in quenched Ti-Nb alloy *** modulus values were sensitive to phase stability of constituent *** strength increased with increasing oxygen *** will be explained by phase formation and stability behavior.

关键词： Ti-Nb-O alloy Phase stability Elastic modulus Mechanical properties