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Petroleum Science 2022年第4期19卷 1905-1914页

作者： yong-rui pi Mu-Tai Bao School of Ocean Yantai UniversityYantai264005China Key Laboratory of Marine Chemistry Theory and Technology Ministry of Education/Institute for Advanced Ocean StudyOcean University of China Qingdao266100China

The enzymes and the characteristics of the community of the petroleum-degrading bacteria play a crucial role in the crude oil biodegradation. The prediction of kinetics of the key groups of hydrocarbons in crude oil was important to evaluate the bioremediation speed and constant. Most of the n-alkanes(C9-C29) were degraded in 25 days, and the average degradation rates of C_(18)~C_(27) higher than 100 μg g^(-1) d^(-1).The hopanes, such as H_(30), had a biodegradation rate more than 10 μg g^(-1) d^(-1). The related enzymes activities changed along with the crude oil biodegradation, especially dehydrogenase. The 16 S rRNA gene amplicon sequencing revealed that Proteobacteria, Firmcutes, Bacteroidetes, Actinobacteria, Acidobacteria were the main petroleum hydrocarbon degraders during the crude oil biodegradation, and the top two highest relative abundance of the genera were Alcaligenes and Acinetobacter. Acinetobacter presented positive correlation to biodegradation of n-alkanes and PAHs. Based on COG analysis, the largest group involved in the general function was amino acid transport and metabolism. The functional categories of bacterial communities were mainly focused on the carbohydrate and amino acid metabolism, xenobiotics biodegradation and metabolism, membrane transport, and so on. Overall, these findings highlight the potential guideline for more adequate monitoring of microbial degradation of crude oil.

关键词： Crude oil Bioaugmentation Kinetics Enzyme activities Microbial functions

Boosting Oxygen Evolution Reaction Performance on NiFe‑Based Catalysts Through d‑Orbital Hybridization

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Nano-Micro Letters 2025年第1期17卷 281-292页

作者： Xing Wang Wei pi Sheng Hu Haifeng Bao Na Yao Wei Luo State Key Laboratory of New Textile Materials and Advanced Processing Technology Key Laboratory of New Textile Materials and Applications of Hubei ProvinceSchool of Materials Science and EngineeringWuhan Textile UniversityWuhan 430200People’s Republic of China College of Chemistry and Molecular Sciences Wuhan UniversityWuhan 430072People’s Republic of China

Anion-exchange membrane water electrolyzers(AEMWEs)for green hydrogen production have received intensive attention due to their feasibility of using earth-abundant NiFe-based *** introducing a third metal into NiFe-based catalysts to construct asymmetrical M-NiFe units,the d-orbital and electronic structures can be adjusted,which is an important strategy to achieve sufficient oxygen evolution reaction(OER)performance in ***,the ternary NiFeM(M:La,Mo)catalysts featured with distinct M-NiFe units and varying d-orbitals are reported in this *** and theoretical calculation results reveal that the doping of La leads to optimized hybridization between d orbital in NiFeM and 2p in oxygen,resulting in enhanced adsorption strength of oxygen intermediates,and reduced rate-determining step energy barrier,which is responsible for the enhanced OER *** critically,the obtained NiFeLa catalyst only requires 1.58 V to reach 1 A cm^(−2) in an anion exchange membrane electrolyzer and demonstrates excellent long-term stability of up to 600 h.

关键词： NiFe-based catalysts d-orbital coupling Oxygen evolution reaction Anion exchange membrane electrolyzer

Text-Image Feature Fine-Grained Learning for Joint Multimodal Aspect-Based Sentiment Analysis

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Computers, Materials & Continua 2025年第1期82卷 279-305页

作者： Tianzhi Zhang Gang Zhou Shuang Zhang Shunhang Li Yepeng Sun Qiankun pi Shuo Liu School of Data and Target Engineering Information Engineering UniversityZhengzhou450001China Information Engineering Department Liaoning Provincial College of CommunicationsShenyang110122China School of Computer and Artificial Intelligence Zhengzhou UniversityZhengzhou450000China

Joint Multimodal Aspect-based Sentiment Analysis(JMASA)is a significant task in the research of multimodal fine-grained sentiment analysis,which combines two subtasks:Multimodal Aspect Term Extraction(MATE)and Multimodal Aspect-oriented Sentiment Classification(MASC).Currently,most existing models for JMASA only perform text and image feature encoding from a basic level,but often neglect the in-depth analysis of unimodal intrinsic features,which may lead to the low accuracy of aspect term extraction and the poor ability of sentiment prediction due to the insufficient learning of intra-modal *** this problem,we propose a Text-Image Feature Fine-grained Learning(TIFFL)model for ***,we construct an enhanced adjacency matrix of word dependencies and adopt graph convolutional network to learn the syntactic structure features for text,which addresses the context interference problem of identifying different aspect ***,the adjective-noun pairs extracted from image are introduced to enable the semantic representation of visual features more intuitive,which addresses the ambiguous semantic extraction problem during image feature ***,the model performance of aspect term extraction and sentiment polarity prediction can be further optimized and *** on two Twitter benchmark datasets demonstrate that TIFFL achieves competitive results for JMASA,MATE and MASC,thus validating the effectiveness of our proposed methods.

关键词： Multimodal sentiment analysis aspect-based sentiment analysis feature fine-grained learning graph convolutional network adjective-noun pairs

High resolution wide swath revisit synthetic aperture radar imaging mode and algorithm

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Journal of Systems Engineering and Electronics 2015年第2期26卷 274-281页

作者： Weihua Zuo Yiming pi rui Min School of Electronic Engineering University of Electronic Science and Technology of China Department of Physics and Information Engineering Huaihua University

Based on the squint mode, a high resolution wide swath revisit synthetic aperture radar （SAR） imaging mode is pro- posed. The transmitting antennas are configured as the single phase center multiple azimuth beams （SPC MAB）. The formed two beams point to two different directions to obtain two images of the observed scenario. The receiving antennas are configured as displaced phase center multiple azimuth beams （DPC MAB） to decrease the required pulse repetition frequency （PRF）. The de- creased PRF can ensure the high resolution wide swath imaging. Based on the analysis of the character of the return signal, a pro- cessing method named multiple beam multiple channel algorithm （MBMCA） is proposed to separate the aliased sub-beams＇ echoes. The separated echoes are focused respectively to get the revisit imaging to the observed scenario. The simulation experiments ve- rify the validity and correctness of the proposed imaging mode and processing algorithm.

关键词： synthetic aperture radar(SAR) high resolution wide swath revisit

Stability and Stabilization of Sampled-Data Based LFC for Power Systems:A Data-Driven Method

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IEEE/CAA Journal of Automatica Sinica 2025年第1期 291-293页

作者： Yu-Long Fan Chuan-Ke Zhang yong He the School of Automation China University of Geosciences the Hubei Key Laboratory of Advanced Control and Intelligent Automation for Complex Systems the Engineering Research Center of Intelligent Technology for Geo-Exploration Ministry of Education IEEE

Dear Editor,This letter is concerned with stability analysis and stabilization design for sampled-data based load frequency control(LFC) systems via a data-driven method. By describing the dynamic behavior of LFC systems based on a data-based representation, a stability criterion is derived to obtain the admissible maximum sampling interval(MSI) for a given controller and a design condition of the pi-type controller is further developed to meet the required MSI. Finally, the effectiveness of the proposed methods is verified by a case study.

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EXISTENCE RESULTS FOR THE KIRCHHOFF TYPE EQUATION WITH A GENERAL NONLINEAR TERM

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Acta Mathematica Scientia 2022年第5期42卷 2063-2077页

作者： Huirong pi yong ZENG School of Mathematics and Information Guangci UniversityNanning 530004China

This paper is mainly concerned with existence and nonexistence results for solutions to the Kirchhoff type equation−(a+b∫_(R^(3))|∇u|^(2))Δu+V(x)u=f(u)in R^(3),with the general hypotheses on the nonlinearity f being as introduced by Berestycki and *** analysis introduces variational techniques to the analysis of the effect of the nonlinearity,especially for those cases when the concentration-compactness principle cannot be applied in terms of obtaining the compactness of the bounded Palais-Smale sequences and a minimizing problem related to the existence of a ground state on the Pohozaev manifold rather than the Nehari manifold associated with the equation.

关键词： Kirchhoff type equation general nonlinearity variational methods Pohozaev identity

A New Ensemble HDG Method for Parameterized Convection Diffusion PDEs

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Numerical Mathematics(Theory,Methods and Applications) 2021年第1期14卷 144-175页

作者： yong Yu Gang Chen Liangya pi Yangwen Zhang School of Mathematics Sichuan UniversityChengduChina Department of Mathematics and Statistical Missouri University of Science and TechnologyRollaMOUSA Department of Mathematics Science University of DelawareNewarkDEUSA

A new second order time stepping ensemble hybridizable discontinuous Galerkin method for parameterized convection diffusion PDEs with various initial and boundary conditions,body forces,and time depending coefficients is *** ensemble solutions in L_(∞)(0,T;L^(2)(Ω)),a superconvergent rate with respect to the freedom degree of the globally coupled unknowns for all the polynomials of degree k≥0 is *** results of numerical experiments are consistent with the theoretical findings.

关键词： HDG method ensemble methods parameterized convection diffusion PDEs nu-merical analysis

Synthesis and Crystal Structure of N,N′-4-aminomethyl-pyromellitic diimide

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Chinese Journal of Structural Chemistry 2005年第10期24卷 1176-1180页

作者： LU Xing-Qiang pi Xiang-Dong SU Cheng-yong School of Chemistry and Chemical Engineering Sun Yat-Sen University Guangzhou 510275 China Chemtcal Envtronmental Protectton Monitoring Station of Hubei Wuhan 430060 China

The title compound N,N′-4-aminomethyl-pyromellitic diimide （4-pmpmd） crystallizes in monoclinic, space group P21/c with a = 4.785（1）, b = 6.200（1）, c = 29.907（2） A, β = 93.583（11）°, V= 885.5（2） A^3, Dc = 1.494 g/cm^3, Z= 2, C22H14N4O4, Mr = 398.37,/t（MoKα） = 0.106 mm^-1 and F（000） = 412, and its structure was refined to R = 0.0469 and wR = 0.1017 for 1194 observed reflections （F0 〉 4σ（F0））. The X-ray diffraction shows the existence of the staggered strong intermolecular C-H…O （DA） hydrogen bonds between adjacent molecules, the intermo- lecular C-H…π hydrogen bonds and the weak π…π stacking interactions, leading to the formation of multi-dimensional supramolecular network based on the Z-mode conformation of the title compound.

关键词： N,N′-4-aminomethyl-pyromellitic diimide intermolecular weak interactions,supramolecular network

Formation, Structures and Electronic Properties of Silicene Oxides on Ag(111)

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Journal of Materials Science & Technology 2017年第7期33卷 751-757页

作者： Muhammad Ali Zhenyi Ni Stefaan Cottenier yong Liu Xiaodong pi Deren Yang Centerfor Molecular Modeling （CMM） and Department of Materials Science and Engineering （DMSE） Ghent University Zwijnaarde BE-9052. Belgium

The formation, structural and electronic properties of silicene oxides（SOs） that result from the oxidation of silicene on Ag（111） surface have been investigated in the framework of density functional theory（DFT）.It is found that the honeycomb lattice of silicene on the Ag（111） surface changes after the oxidation. SOs are strongly hybridized with the Ag（111） surface so that they possess metallic band structures. Charge accumulation between SOs and the Ag（111） surface indicates strong chemical bonding, which dramatically affects the electronic properties of SOs. When SOs are peeled off the Ag（111） surface, however, they may become semiconductors.

关键词： Silicene oxides Ag(111) Density functional theory Oxidation Hybridization Band gap

Formation,Stability,Geometry and Band Structure of Organically Surface-Modified Germanane

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Journal of Materials Science & Technology 2017年第1期33卷 59-64页

作者： Hui Jia Rong Wang Zhenyi Ni yong Liu Xiaodong pi Deren Yang State Key Laboratory of Silicon Materials and Department of Materials Science and Engineering Zhejiang University Key Laboratory of Interface Science and Engineering in Advanced Materials Ministry of EducationTaiyuan University of Technology

Surface modification may be an effective means for controlling the properties of germanane, i.e., hydrogenated germanene. In this work, we investigate the formation, stability, structure and electronic properties of surface-modified germanane that results from the hydrogermylation, alkoxylation, aminization or phenylation of germanane. By assuming the typical organic surface coverage of -33%, we have com- pared organically surface-modified germanane with germanene and germanane in the framework of density functional theory. It is found that organically surface-modified germanane may all stably exist despite the endothermic nature of organic surface modification. Organic surface modification leads to the de- crease of the Ge--Ge bond length and the Ge--Ge-Ge bond angle ofgermanane, while causing the buckling distance of germanane to increase. Hydrogenation makes germanene change from a semimetal to a direct- bandgap semiconductor. Organic surface modification further impacts the band structure of the resulting germanane. Hydrogermylated/alkoxylated germanane is a direct-bandgap semiconductor, while aminated/ phenylated germanane is an indirect-bandgap semiconductor. All the organic surface modification gives rise to the increase of the bandgap of germanane.

关键词： Germanane Surface modification Density functional theory Band structure