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Anomalous quality factor evolution of induced transparency in a virtualized coupled-oscillator system

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 148-155页

作者： Yunhan Yang han Jia Tuo Liu Yuzhen Yang jun Yang Key Laboratory of Noise and Vibration Research Institute of Acoustics Chinese Academy of Sciences University of Chinese Academy of Sciences State Key Laboratory of Acoustics Institute of Acoustics Chinese Academy of Sciences

The phenomenon of induced transparency, characterized by a high quality(Q) factor, holds significant importance in the fields of high-precision sensing, energy storage and wave manipulation. Conventional transparency systems are often constrained by the limited experimentally accessible parameter space and the lack of independent control over intrinsic parameters, thereby hindering advanced research on high-Q effects. Here we propose a virtualized coupled-oscillator system that enables reconfigurable induced transparency in the reflection spectrum. By virtually incorporating a pair of coupled oscillators into an individual acoustic meta-atom, we achieve the manipulation of induced transparency in a decoupled, wide-ranging, and elaborate manner. Exploiting the diverse evolutions across the intrinsic parameter space, we show experimentally a counter-intuitive increase in the Q-factor of the transparency window, which is attributed to the enhanced dissipation of the bright ***, a constant group delay at the center frequency is observed accompanying this evolution. Our work demonstrates an intriguing platform as well as a novel strategy to engineer high-Q induced transparency phenomenon, and paves the way towards applications in programmable acoustic sensors, filters and slow-wave devices.

关键词： induced transparency acoustic meta-atom high quality-factor scattering programmable intrinsic parameter

Crystallization Modulation and Holistic Passivation Enables Efficient Two‑Terminal Perovskite/CuIn(Ga)Se_(2)Tandem Solar Cells

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Nano-Micro Letters 2025年第1期17卷 205-215页

作者： Cong Geng Kuanxiang Zhang Changhua Wang Chung Hsien Wu Jiwen Jiang Fei Long Liyuan han Qifeng han Yi‑Bing Cheng yong Peng State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070People’s Republic of China Triumph Photovoltaic Materials Co. Ltd.No.1001 Yannan AvenueHigh‑Tech Development DistrictBengbuAnhui 233000People’s Republic of China College of Materials Science and Engineering Guilin University of TechnologyGuilin 541004People’s Republic of China State Key Laboratory of Metal Matrix Composites Shanghai Jiao Tong UniversityShanghai 200240People’s Republic of China

Two-terminal(2-T)perovskite(PVK)/CuIn(Ga)Se_(2)(CIGS)tandem solar cells(TSCs)have been considered as an ideal tandem cell because of their best bandgap matching regarding to Shockley–Queisser(S–Q)***,the nature of the irregular rough morphology of commercial CIGS prevents people from improving tandem device *** this paper,D-homoserine lactone hydrochloride is proven to improve coverage of PVK materials on irregular rough CIGS surfaces and also passivate bulk defects by modulating the growth of PVK *** addition,the minority carriers near the PVK/C60 interface and the incompletely passivated trap states caused interface recombination.A surface reconstruction with 2-thiopheneethylammonium iodide and N,N-dimethylformamide assisted passivates the defect sites located at the surface and grain ***,LiF is used to create this field effect,repelling hole carriers away from the PVK and C60 interface and thus reducing *** a result,a 2-T PVK/CIGS tandem yielded a power conversion efficiency of 24.6%(0.16 cm^(2)),one of the highest results for 2-T PVK/CIGS TSCs to our *** validation underscores the potential of our methodology in achieving superior performance in PVK/CIGS tandem solar cells.

关键词： PVK/CIGS TSCs Irregular rough surfaces Modulating the growth PVK/C60 interface recombination

Effect of ^(103)Pd on proliferation and apoptosis of vascular smoothmuscle cells

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Nuclear Science and Techniques 2003年第4期14卷 253-256页

作者： LUO Quan-yong, ZHU jun, LU han-Kui, ZHU Rui-Sen(Department of Nuclear Medicine, Shanghai Sixth People’s Hospital, Shanghai Jiaotong University, Shanghai 200233) Department of Nuclear Medicine Shanghai Sixth People's Hospital Shanghai Jiaotong University 上海 200233

This study aimed at the effect of γ -emitting radionuclide 103Pd on the proliferation and apoptosis ofvascular SMCs (smooth muscle cells) in vitro. The cavy aortic SMCs were cultured with culture medium M-199. Theexperiments were carried out in two groups, one for proliferation test and the other for apoptosis test. In each group,103Pd solutions with various radioactivities were respectively added to the culture solution to irradiate SMCs for 72 h,while non-radioactive palladium solution was added to the control. 3H-thymidine incorporation test and liquid scin-tillator were used to detect the effect of 103Pd on the proliferation of SMCs. Flow cytometer was used to detect theapoptotic SMCs. The inhibition rate of SMCs proliferation by 1.85 MBq 103Pd solution was 2.3%, which was not sig-nificant, while the inhibition rate increased from 41.6% to 91.3% as the 103Pd activity increased from 7.40 MBq to 37MBq. The apoptosis rate of SMCs was extremely low (less than 4.0%) by 103Pd with activity from 1.85 MBq to 37MBq. The results suggest that the proliferation of SMCs can be repressed effectively in a dose-dependent fashion by103Pd in vitro. The mechanism of its inhibiting over neointima proliferation is likely to inhibite SMCs proliferationrather than to induce its apoptosis by 103Pd. 103Pd can be used as a γ -emitting intravascular brachytherapy radionu-clide to inhibit SMCs proliferation.

关键词：钯血管平滑肌细胞细胞增殖细胞凋亡冠状动脉成形术

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含锡易切削中碳钢的切削加工性能

钢铁研究学报 2018年第1期30卷 66-70页

作者：张永军韩静涛北京科技大学材料科学与工程学院

含锡易切削钢是一种环境友好的钢铁材料。对利用真空感应炉冶炼锡的质量分数为0.16%的试验用含锡易切削中碳钢,经过热锻成型直径100 mm的圆钢。之后,在C6140无极调速机床上对其进行切削加工性能试验研究,同时利用二次离子质谱仪对Sn、S... 详细信息

含锡易切削钢是一种环境友好的钢铁材料。对利用真空感应炉冶炼锡的质量分数为0.16%的试验用含锡易切削中碳钢,经过热锻成型直径100 mm的圆钢。之后,在C6140无极调速机床上对其进行切削加工性能试验研究,同时利用二次离子质谱仪对Sn、S、Mn合金元素在试验用含锡易切削钢中的分布进行表面线、面扫描的质谱分析。研究结果表明,试验钢的相对切削系数为1.75;切屑的形状主要呈C型,并伴有少量螺旋屑,说明该钢具有良好的切削加工性,能够满足高速切削加工的要求。锡在晶界和Mn S界面上偏聚的这种分布特点以及锡的低熔点特性而引起的晶界脆化,熔融金属脆性,以及切削刀具与切屑、工件界面之间的润滑剂——熔融锡的润滑作用,可以认为是该钢易切削的主要机理。

关键词：含锡易切削钢切削加工性能晶界脆化熔融金属脆性润滑作用

Trinuclear gold-catalyzed site-selective alkylation of peptides

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Science China Chemistry 2025年第1期68卷 249-256页

作者： Qing-Yun Fang Chengyihan Gu Yinghan Chen Wencheng Yan yong Liang Weipeng Li Chengjian Zhu Jie han Jin Xie State Key Laboratory of Coordination Chemistry Jiangsu Key Laboratory of Advanced Organic Materials Chemistry and Biomedicine Innovation Center (Chem BIC) School of Chemistry and Chemical Engineering Nanjing University Green Catalysis Center College of Chemistry Zhengzhou University State Key Laboratory of Natural Medicines China Pharmaceutical University

Selective modification of peptides has always been a challenging issue. The selective alkylation of peptides can alter the biological activity and physical properties of molecules, and it has gained significant research interest. We herein disclose an intriguing gold-catalyzed alkylation of peptides using bench-stable unactivated alkyl bromides under photoredox catalysis. A wide range of structurally diverse primary, secondary and tertiary alkyl bromides serve as effective coupling partners to precisely connect with the α-C(sp3)–H in glycine residue of peptides. This protocol demonstrates an exceptionally broad scope for alkyl halides and excellent tolerance for a wide range of useful functional groups. A series of relay transformations to construct cyclic peptides, to proceed click reaction and to realize peptide fluorescence labeling further enhance its synthetic practicality. In addition, mechanistic studies and density functional theory(DFT) calculations reveal an inner-sphere and subsequent outersphere single electron transfer(SET) mechanism.

关键词： gold catalysis peptide alkylation C-C coupling radical

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De novo synthesis of atropisomeric benzofurans via Cu/SPDO complex catalyzed asymmetric formal [3 + 2] annulation

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Science China Chemistry 2025年第1期68卷 174-180页

作者： Fan-Xiao Meng Xing-Yu Wang Ka Lu Ju-Song Yang Fu-Min Zhang Ai-jun Ma Bao Du yong-Qiang Tu State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical Engineering Lanzhou University School of Chemistry and Chemical Engineering Shanghai Jiao Tong University School of Biotechnology and Health Sciences Wuyi University

Herein, the de novo synthesis of atropisomeric benzofurans through the Cu/spirocyclic-pyrrolidine-oxazoline(SPDO) complex catalyze asymmetric formal [3 + 2] cycloaddition between quinones and ynamides is explored, producing a range of structurally diverse axially chiral benzofurans in satisfactory yields with good to excellent enantioselectivities. Furthermore, density functional theory calculations were applied to explain the possible reaction mechanism.

关键词： benzofuran atropisomers novel de novo synthetic strategy asymmetric formal [3 + 2] cycladdition Cu/SPDO complex DFT calculations

Mechanistic insight into the synergy between nickel single atoms and nanoparticles on N-doped carbon for electroreduction of CO2

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Journal of Energy Chemistry 2025年第1期100卷 327-336页

作者： Mingdong Sun Wenwen Guan Cailing Chen Chao Wu Xiaoling Liu Biao Meng Tao Chen Yu han jun Wang Shibo Xi Yu Zhou State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Advanced Membranes and Porous Materials Center Physical Sciences and Engineering Division King Abdullah University of Science and Technology Institute of Sustainability for Chemicals Energy and Environment A*STAR (Agency for Science Technology and Research) College of Materials Science and Engineering Sichuan University

The synergy of single atoms （SAs） and nanoparticles （NPs） has demonstrated great potential in promoting the electrocatalytic carbon dioxide reduction reaction （CO2RR）;however,the rationalization of the SAs/NPs proportion remains one challenge for the catalyst ***,a Ni2+-loaded porous poly（ionic liquids）(PIL) precursor synthesized through the free radical self-polymerization of the ionic liquid monomer,1-allyl-3-vinylimidazolium chloride,was pyrolyzed to prepare the Ni,N co-doped carbon materials,in which the proportion of Ni SAs and NPs could be facilely modulated by controlling the annealing *** catalyst Ni-NC-1000 with a moderate proportion of Ni SAs and NPs exhibited high efficiency in the electrocatalytic conversion of CO2into *** Ni K-edge X-ray absorption near-edge structure （XANES） spectra and theoretical calculations were conducted to gain insight into the synergy of Ni SAs and *** charge transfer from Ni NPs to the surrounding carbon layer and then to the Ni SAs resulted in the electron-enriched Ni SAs active *** the electroreduction of CO2,the coexistence of Ni SAs and NPs strengthened the CO2activation and the affinity towards the key intermediate of*COOH,lowering the free energy for the potential-determining*CO2→*COOH step,and therefore promoted the catalysis efficiency.

关键词： Activation energy

不同手术入路椎体成形术治疗老年性骨质疏松压缩性骨折的临床效果对比

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解放军医药杂志 2018年第10期30卷 55-57,62页

作者：陈勇韩俊蒋现永陈吉滨武汉科技大学附属汉阳医院重症医学科湖北汉阳430050

目的对比不同手术入路椎体成形术治疗老年性骨质疏松压缩性骨折的临床疗效。方法选择2013年7月—2016年1月收治的经皮椎弓根椎体成形术(PVP)治疗的老年骨质疏松性椎体压缩性骨折80例,根据手术入路方式分为单侧组和双侧组,每组40例。比较... 详细信息

目的对比不同手术入路椎体成形术治疗老年性骨质疏松压缩性骨折的临床疗效。方法选择2013年7月—2016年1月收治的经皮椎弓根椎体成形术(PVP)治疗的老年骨质疏松性椎体压缩性骨折80例,根据手术入路方式分为单侧组和双侧组,每组40例。比较2组手术时间、骨水泥量、椎体高度重建率、后凸Cobb角改善、手术前及术后1年疼痛视觉模拟评分(VAS)和Oswestry功能障碍指数(ODI)评分等。结果单侧组手术时间短于双侧组(P <0. 05)。双侧组注入骨水泥量、骨水泥渗漏率、邻近椎体骨折率均少于或低于单侧组(P <0. 05)。2组术后1 d、术后1年VAS及ODI评分均低于术前,术后1年低于术后1 d(P <0. 05)。结论不同手术入路PVP治疗老年性骨质疏松压缩性骨折均能取得较好临床疗效,但是PVP双侧入路可降低骨水泥的渗漏率及远期相邻椎体的再发骨折率。

关键词：骨折压缩性骨质疏松性骨折椎体成形术预后

Electro-optic tuning in ferroelectric capacitor with photonic crystal nanobeam cavity

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Science China(Information Sciences) 2025年

作者： Tongtong WANG yong ZhanG Danyang YAO Zhi JIANG Dongxin TAN Jie WEN Qiyu YANG Xuetao GAN Yan LIU Yue HAO Genquan han State Key Discipline Laboratory of Wide Band Gap Semiconductor Technology School of MicroelectronicsXidian University Key Laboratory of Light Field Manipulation and Information Acquisition Ministry of Industry and Information TechnologyShaanxi Key Laboratory of Optical Information Technology School of Physical Science and TechnologyNorthwestern Polytechnical University hangzhou Institute of Technology Xidian University

Silicon photonics has provided a platform for the convergency of photonic devices and electronic circuits, facilitating the development of optical telecommunications and optical interconnects on chip[1]. As the basic building block of optical communication systems, electro-optic tuning is expected to be more compact, high bandwidth, energy efficient, and allow for CMOS-compatible fabrication in the future[2]. Resonator-based electro-optic tuning has attracted more and more interest due to the small footprint, enhanced light-matter interactions and high energy efficiency. Compared with microring and microdisk resonators, photonic crystal nanobeam cavities （PCNBCs） realize higher quality factors, stronger light-matter interactions, ultrasmall mode volume and a much larger free spectral range （FSR）[3].

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