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Reversible Li plating regulation on graphite anode through a barium sulfate nanofibers-based dielectric separator for fast charging and high-safety lithium-ion battery

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Journal of Energy Chemistry 2025年第2期101卷 511-523页

作者： Yaxin Zhang Long Cheng ying-jie zhu Jin Wu Han-Ping Yu Sida Xie Dandan Li Zhaohui Wang Heng Li State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of Ceramics Chinese Academy of Sciences College of Materials Science and Engineering Hunan University Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences

Poor Li plating reversibility and high thermal runaway risks are key challenges for fast charging lithiumion batteries with graphite ***,a dielectric and fire-resistant separator based on hybrid nanofibers of barium sulfate（BS） and bacterial cellulose（BC） is developed to synchronously enhance the battery's fast charging and thermal-safety *** regulation mechanism of the dielectric BS/BC separator in enhancing the Li+ion transport and Li plating reversibility is revealed.（1） The Max-Wagner polarization electric field of the dielectric BS/BC separator can accelerate the desolvation of solvated Li+ions,enhancing their transport kinetics.（2） Moreover,due to the charge balancing effect,the dielectric BS/BC separator homogenizes the electric field/Li+ion flux at the graphite anode-separator interface,facilitating uniform Li plating and suppressing Li dendrite ***,the fast-charge graphite anode with the BS/BC separator shows higher Coulombic efficiency（99.0% vs.96.9%） and longer cycling lifespan（100 cycles vs.59 cycles） than that with the polypropylene（PP） separator in the constantlithiation cycling test at 2 mA *** high-loading LiFePO4(15.5 mg cm-2)//graphite(7.5 mg cm-2) full cell with the BS/BC separator exhibits excellent fast charging performance,retaining 70% of its capacity after 500 cycles at a high rate of 2C,which is significantly better than that of the cell with the PP separator（retaining only 27% of its capacity after 500 cycles）.More importantly,the thermally stable BS/BC separator effectively elevates the critical temperature and reduces the heat release rate during thermal runaway,thereby significantly enhancing the battery's safety.

关键词： Fast charging Graphite anode Ion transport Lithium-ion battery Separator

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Multifunctional Fire-Resistant Paper Based on Ultralong Hydroxyapatite Nanowires

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Chinese Journal of Chemistry 2021年第8期39卷 2296-2314页

作者： ying-jie zhu State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of Sciences1295 Ding-Xi RoadShanghai 200050China

Paper was one of the greatest inventions in ancient China,and it greatly promoted the rapid development of human *** in today's electronic information age,paper and paper-derived products are still indispensable to people's daily work and ***;the traditional paper based on cellulose fibers from plants has some *** instance:(1)papermaking consumes a large amount of precious natural resources such as trees;(2)the papermaking industry causes environmental pollution;(3)the traditional paper consisting of organic cellulose fibers is highly flammable and easy to burn;(4)the traditional paper based on cellulose fibers turns to yellow color with time;(5)the lifetime of the traditional paper is relatively short because of the degradation of cellulose *** efforts are needed to investigate and solve these problems facing the traditional *** recent years,a new kind of multifunctional fire-resistant paper based on ultralong hydroxyapatite nanowires has been developed and investigated for various applications,and many research findings have been documented in the *** review article provides a comprehensive summary and discussion on recent research advances for this new kind of multifunctional fire-resistant paper based on ultralong hydroxyapatite nanowires,including the synthesis,properties,applications,and future perspectives.

关键词： Nano wires Hydroxyapatite Fire-resistant paper Nanostructures Green chemistry

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Nanowires:Synthesis and Energy/Environmental Applications

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Energy & Environmental Materials 2021年第4期4卷 544-561页

作者： Heng Li ying-jie zhu State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

As the main inorganic component of human bones and teeth,hydroxyapatite(HAP)materials have been widely investigated for various applications especially in the biomedical ***,HAP nanowires(HAP NWs)have attracted research interest in the energy and environment-related fields owing to their advantages such as excellent biocompatibility and bioactivity,high-thermal stability,surface modification and functionalization,and selfassembly to form nanoscale porous networked *** this review,we first briefly discuss the synthesis of HAP *** we focus on summarizing the foremost advances in energy and environment-related applications of HAP NWs,including the battery,solar energy-assisted water evaporation,light-driven self-propelled device,thermal insulation,fireresistant inorganic paper,water purification,air purification,molecular detection,superhydrophobic surface,and high-strength nanocomposite *** addition,the future research directions on HAP NWs and their energy and environmental applications are *** review aims to provide inspiration and stimulate extensive future studies in the energy and environmental applications of HAP NWs and other inorganic NWs.

关键词： hydroxyapatite nanowire application energy environment

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Nanostructured Materials of Calcium Phosphates and Calcium Silicates： Synthesis, Properties and Applications

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Chinese Journal of Chemistry 2017年第6期35卷 769-790页

作者： ying-jie zhu State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of Ceramics Chinese Academy of Sciences Shanghai 200050 China

Calcium phosphates are a family of compounds with different chemical compositions, structures and properties containing calcium ions and functional groups of orthophosphate （ pO34- ）, metaphosphate （ PO3- ） or pyrophosphate （ P2O4-7 ） and sometimes hydrogen or hydroxide ions. Calcium phosphates can be widely found in nature as well as in hard tissues （bone and tooth） of the vertebrate. Owing to similar chemical composition and structure to the main inorganic constituents of bone and tooth, calcium phosphate-based materials are promising biomaterials with high biocompatibility, and have been investigated for applications in various biomedical areas. Calcium silicate-based materials have attracted much attention on their potential applications in various biomedical fields such as bone de- fect repair and drug delivery. In recent years, this research group has been focusing on the research in this exciting and rapidly evolving research field, and has published many papers. This article will provide a brief review on our main research work on the synthesis, characterization, properties and applications of nanostructured materials of calcium phosphates and calcium silicates. Finally, future perspectives and challenges for the research and applica- tions of nanostructured materials of calcium phosphates and calcium silicates are discussed.

关键词： calcium phosphate calcium silicate nanostructured materials biomaterials biomedical applications

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Bioinspired flexible,high-strength,and versatile hydrogel with the fiberboard-and-mortar hierarchically ordered structure

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Nano Research 2021年第10期14卷 3643-3652页

作者： Han-Ping Yu ying-jie zhu State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

The synthetic hydrogels with high water contents are promising for various applications,however,they usually exhibit low mechanical *** this work,inspired by the natural biological soft tissues,whose hierarchically ordered fibrous structures result in high strength and good flexibility,a flexible,high-strength,and versatile hydrogel with the fiberboard-and-mortar hierarchically ordered structure(HFMOS)is developed based on ultralong hydroxyapatite(HAP)nanowires and polyacrylic acid(PAA).The as-prepared HFMOS hydrogel has a high water content(~70 wt.%),dense structure,and excellent mechanical properties,and these properties are similar to those of the human cartilage and are superior to many hydrogels reported in the *** excellent mechanical properties of the HFMOS hydrogel originate from the combination of the fiberboard-and-mortar hierarchically ordered structure,reinforcement of ultralong HAP nanowires,strong interfacial strength,and multiple energy dissipation ***,thanks to the controllable components and injection procedure,the HFMOS hydrogel with a Janus structure is prepared for particular *** HFMOS hydrogel possesses abundant ordered water channels,and can be used for loading,release,and directed delivery of various functional ***,the as-prepared flexible,high-strength,and versatile HFMOS hydrogel possesses a great potential for various applications such as water purification,pollution treatment,biomedicine,nanofluidic devices,and high-performance structural materials.

关键词： hydrogel nanowire hydroxyapatite ordered structure

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Cysteine dioxygenase type 1 (CDO1): Its functional role in physiological and pathophysiological processes

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Genes & Diseases 2023年第3期10卷 877-890页

作者： Min Chen jie-ying zhu Wang-Jing Mu Liang Guo School of Kinesiology Shanghai University of SportShanghai 200438China Shanghai Frontiers Science Research Base of Exercise and Metabolic Health Shanghai University of SportShanghai 200438China

Cysteine dioxygenase type 1 (CDO1), belonging to the mammalian non-heme Fe(II) dioxygenases family, is a key enzyme for cysteine catabolism. Its activity and expression is regulated through multiple mechanisms. CDO1 is involved in a spectrum of physiological processes including lipid metabolism, adipogenesis, osteoblastic differentiation, redox homeostasis, fertility, bile acid metabolism, sulfide metabolism, and organismal growth and development. Many of these processes are regulated directly or indirectly by CDO1-mediated metabolism of cysteine. In pathophysiological processes, the degree of CDO1 promoter methylation is closely related to the progression and malignancy of tumors, and overexpression of CDO1 will promote ferroptosis of cancer cells. Moreover, CDO1 may ameliorate metabolic disorders through the taurine-mediated improvement of lipid metabolism and insulin sensitivity and improve neurodegenerative diseases by regulating cysteine level. Therefore, elucidation of the mechanisms underlying the role of CDO1 would provide a clearer view of the therapeutic potential and possible risks of targeting this important enzyme.

关键词： Anti-tumor Antioxidation Cysteine Promoter methylation Taurine

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The functional role of Higd1a in mitochondrial homeostasis and in multiple disease

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Genes & Diseases 2023年第5期10卷 1833-1845页

作者： jie-ying zhu Min Chen Wang-Jing Mu Hong-Yang Luo Liang Guo School of Kinesiology Shanghai University of SportShanghai 200438China Shanghai Frontiers Science Research Base of Exercise and Metabolic Health Shanghai University of SportShanghai 200438China

Higd1a is a conserved gene in evolution which is widely expressed in many tissues in *** evidence has revealed multiple functions of Higd1a,as a mitochon-drial inner membrane protein,in the regulation of metabolic *** plays an impor-tant role in anti-apoptosis and promotes cellular survival in several cell types under hypoxic *** the survival of porcine Sertoli cells facilitated by Higd1a helps to support *** some cases,Higd1a can serve as a sign of metabolic *** the past several years,a considerable amount of studies about how tumor fate is determined and how cancerous proliferation is regulated by Higd1a have been *** this review,we summarize the physiological functions of Higd1a in metabolic homeostasis and its pathophysiological roles in distinct diseases including cancer,nonalcoholic fatty liver disease(NAFLD),type Il diabetes and mitochondrial *** prospect of Higd1a with potential to preserve mammal health is also *** review might pave the way for Higd1a-based research andapplicationinclinicalpractice.

关键词： Apoptosis Cancer Diabetes Mitochondrial homeostasis NAFLD

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Krüppel-like factor 10 (KLF10) as a critical signaling mediator: Versatile functions in physiological and pathophysiological processes

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Genes & Diseases 2023年第3期10卷 915-930页

作者： Hong-Yang Luo jie-ying zhu Min Chen Wang-Jing Mu Liang Guo Shanghai Frontiers Science Research Base of Exercise and Metabolic Health Shanghai University of SportShanghai 200438China School of Kinesiology Shanghai University of SportShanghai 200438China

Krüppel-like factor 10 (KLF10), also known as TGFβ-inducible early gene-1 (TIEG1), was first found in human osteoblasts. Early studies show that KLF10 plays an important role in osteogenic differentiation. Through decades of research, KLF10 has been found to have complex functions in many different cell types, and its expression and function is regulated in multiple ways. As a downstream factor of transforming growth factor β (TGFβ)/SMAD signaling, KLF10 is involved in various biological functions, including glucose and lipid metabolism in liver and adipose tissue, the maintenance of mitochondrial structure and function of the skeletal muscle, cell proliferation and apoptosis, and plays roles in multiple disease processes, such as nonalcoholic steatohepatitis (NASH) and tumor. Besides, KLF10 shows gender-dependent difference of regulation and function in many aspects. In this review, the biological functions of KLF10 and its roles in disease states is updated and discussed, which would provide new insights into the functional roles of KLF10 and a clearer view of potential therapeutic strategies by targeting KLF10.

关键词： Adipose tissue Estrogen signaling Glucose and lipid metabolism NASH Obesity Skeletal muscle TGFβ/SMAD signaling Tumor

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Weichang'an and 5-fluorouracil suppresses colorectal cancer in a mouse model

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World Journal of Gastroenterology 2015年第4期21卷 1125-1139页

作者： Li Tao Jin-Kun Yang ying Gu Xin Zhou Ai-Guang Zhao Jian Zheng ying-jie zhu Department of Oncology Longhua Hospital Shanghai University of Traditional Chinese Medicine Department of Pharmacy Longhua HospitalShanghai University of Traditional Chinese Medicine

AIM: To examine the effect of Weichang'an(WCA) and 5-fluorouracil(5-Fu) on colorectal tumor and hepatic metastasis in a mouse model. METHODS: Quantitative determination of hesperidin, the effective component in WCA decoction, was performed using Hp LC. In vitro cytotoxicity of WCA was determined by treating HCT-116 cells with WCA diluents or serum extracted from rats that received WCA by oral gavage for 1 wk and MTT assays. Forty-eight nude mice received cecum implantation with tumor blocks subcutaneously amplified from human colon cancer cell line HCT-116. Mice were randomly divided into four treatment groups: control(CON), WCA, 5-Fu and combination(WCA + 5-Fu). pathological examination of tumors consisted of tissue sectioning and hematoxylin and eosin staining. Tumor weight and size were measured, and the number of metastatic l e s i o n s wa s c o u n t e d. S e r u m c a r c i n o e m b r yo n i c antigen(CEA) level was determined by ELISA. The expression levels of tumor genesis and metastasisrelated proteins β-catenin and matrix metalloproteinase(MMp)-7 were measured by real-time quantitative reverse transcriptase polymerase chain reaction(RTp CR), immunohistochemistry and immunoblotting. Cell fractionation was used to investigate intracellular distribution of β-***: parenchymal tumors were palpable in the abdomens of nude mice 2 wk post-implantation and orthotopic tumor formation rate was 100% in all groups. 5-Fu treatment alone significantly decreased tumor weight compared to the CON group(1.203 ± 0.284 g vs 1.804 ± 0.649 g, p < 0.01). WCA treatment alone reduced the rate of metastasis(50% vs 100%,p < 0.05). Combination treatment of WCA + 5-Fu was the most effective, reducing the tumor weight(1.140 ± 0.464 g vs 1.804 ± 0.649 g, p < 0.01) and size(1493.438 ± 740.906 mm3 vs 2180.259 ± 816.556 mm3, p < 0.05), the rate of metastases(40% vs 100%, p < 0.01), and serum CEA levels(31.263 ± 7.421 μg/L vs 43.040 ± 11.273 μg/L, p < 0.05). Expression of β-cat

关键词： Colorectal cancer Hepatic metastasis Weichang’an f

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Release of Endogenous Brain-derived Neurotrophic Factor into the Lateral Entorhinal Cortex from the Paraventricular Thalamus Ameliorates Social Memory Deficits in a Mouse Model of Alzheimer’s Disease

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Neuroscience Bulletin 2022年第11期38卷 1425-1430页

作者： Yun‑Long Xu Lin zhu Zi‑Jun Chen Xiao‑Fei Deng Pei‑Dong Liu Shan Li Bing‑Chun Lin Chuan‑Zhong Yang Wei Xu Kui-Kui Zhou ying‑jie zhu Shenzhen Key Laboratory of Drug Addiction Shenzhen Neher Neural Plasticity Laboratorythe Brain Cognition and Brain Disease Institute(BCBDI)Shenzhen Institute of Advanced TechnologyChinese Academy of Sciences(CAS)Shenzhen-Hong Kong Institute of Brain Science-Shenzhen Fundamental Research InstitutionsShenzhen 518055China University of Chinese Academy of Sciences Beijing 100049China Department of Neonatology Shenzhen Maternity&Child Healthcare HospitalThe First School of Clinical MedicineSouthern Medical UniversityShenzhen 518055China The First Afliated Hospital Sun Yat-sen UniversityGuangzhou 510080China Cheeloo College of Medicine Shandong UniversityJinan 250012China Faculty of Life and Health Sciences Shenzhen Institute of Advanced TechnologyCASShenzhen 518055China CAS Center for Excellence in Brain Science and Intelligence Technology CASShanghai 200031China CAS Key Laboratory of Brain Connectome and Manipulation BCBDIShenzhen Institute of Advanced Technology(SIAT)CASShenzhen 518055China

Dear Editor,Alzheimer's disease(AD)is one of the most devastating neurodegenerative disorders and the most common form of *** loss is a hallmark of AD pathology and exacerbates cognitive impairment[1].Synaptic loss,un... 详细信息

关键词： Alzheimer pathology impairment

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