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Photocatalytic and Electrocatalytic Generation of Hydrogen Peroxide: Principles, Catalyst Design and Performance

Nano-Micro Letters 2023年第6期15卷 24-72页

作者： yan guo Xili Tong Nianjun yang State Key Laboratory of Coal Conversion Institute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001People’s Republic of China University of Chinese Academy of Sciences Beijing 100049People’s Republic of China Institute of Materials Engineering University of Siegen57076 SiegenGermany Department of Chemistry Hasselt University3590 DiepenbeekBelgium IMO‑IMOMEC Hasselt University3590 DiepenbeekBelgium

Hydrogen peroxide(H_(2)O_(2)) is a high-demand organic chemical reagent and has been widely used in various modern industrial applications. Currently,the prominent method for the preparation of H_(2)O_(2) is the anthraquinone ***, it is not conducive to economic and sustainable development since it is a complex process and involves unfriendly environment and potential hazards. In this context, numerous approaches have been developed to synthesize H_(2)O_(2). Among them, photo/electro-catalytic ones are considered as two of the most promising manners for on-site synthesis of H_(2)O_(2). These alternatives are sustainable in that only water or O_(2) is required. Namely, water oxidation(WOR) or oxygen reduction(ORR)reactions can be further coupled with clean and sustainable energy. For photo/electro-catalytic reactions for H_(2)O_(2) generation, the design of the catalysts is extremely important and has been extensively conducted with an aim to obtain ultimate catalytic performance. This article overviews the basic principles of WOR and ORR,followed by the summary of recent progresses and achievements on the design and performance of various photo/electro-catalysts for H_(2)O_(2) generation. The related mechanisms for these approaches are highlighted from theoretical and experimental aspects. Scientific challenges and opportunities of engineering photo/electro-catalysts for H_(2)O_(2) generation are also outlined and discussed.

关键词： H_(2)O_(2)generation Photocatalysts Electrocatalysts Reaction mechanisms

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DBST:a lightweight block cipher based on dynamic S-box

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Frontiers of Computer Science 2023年第3期17卷 177-185页

作者： Liuyan yan Lang LI Ying guo College of Computer Science and Technology Hengyang Normal UniversityHengyang 421002China Hunan Provincial Key Laboratory of Intelligent Information Processing and Application Hengyang Normal UniversityHengyang 421002China

IoT devices have been widely used with the advent of *** devices contain a large amount of private data during *** is primely important for ensuring their ***,we proposed a lightweight block cipher based on dynamic S-box named *** is introduced for devices with limited hardware resources and high throughput *** is a 128-bit block cipher supporting 64-bit key,which is based on a new generalized Feistel variant *** retains the consistency and significantly boosts the diffusion of the traditional Feistel *** SubColumns of round function is implemented by combining bit-slice technology with *** S-box is dynamically associated with the *** has been demonstrated that DBST has a good avalanche effect,low hardware area,and high *** S-box has been proven to have fewer differential features than RECTANGLE *** security analysis of DBST reveals that it can against impossible differential attack,differential attack,linear attack,and other types of attacks.

关键词： internet of things 5G dynamic S-box bit-slice technology lightweight block cipher

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The damage evolution behavior of polypropylene fiber reinforced concrete subjected to sulfate attack based on acoustic emission

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Frontiers of Structural and Civil Engineering 2022年第3期16卷 316-328页

作者： Ninghui LIANG Jinwang MAO ru yan Xinrong LIU Xiaohan ZHOU School of Civil Engineering Chongqing UniversityChongqing 400045China National Joint Engineering Research Center for Prevention and Control of Environmental Geological Hazards in the TGR Area Chongqing UniversityChongqing 400045China Power China Chengdu Engineering Corporation Ltd. Chengdu 610072China

To study the damage evolution behavior of polypropylene fiber reinforced concrete(PFRC)subjected to sulfate attack,a uniaxial compression test was carried out based on acoustic emission(AE).The effect of sulfate attack relative to time and fiber hybridization were analyzed and the compression damage factor was calculated using a mathematical *** changes to AE ringing counts during the compression could be divided into compaction,elastic,and AE signal hyperactivity *** the initial stage of sulfate attack,the concrete micropores and microcracks were compacted gradually under external load and a corrosion products filling effect,and this corresponded with detection of few AE signals and with concrete compression strength *** increasing sulfate attack time,AE activity *** cumulative AE ringing counts of PFRC at all corrosion ages were much higher than those for plain *** could still produce AE signals after peak load due to drawing effect of polypropylene *** 150 d of sulfate attack,the cumulative AE ringing counts of plain concrete went down by about an order of magnitude,while that for PFRC remained at a high *** initial damage factor of hybrid PFRC was-0.042 and-0.056 respectively after 150 d of corrosion,indicating that the advantage of hybrid polypropylene fiber was more obvious than plain concrete and single-doped *** on a deterioration equation,the corrosion resistance coefficient of hybrid PFRC would be less than 0.75 after 42 drying-wetting sulfate attack cycles,which was 40%longer than that of plain concrete.

关键词： polypropylene fiber reinforced concrete sulfate attack damage evolution behavior acoustic emission damage factor

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苗草专用型大麦品种鉴定及全基因组关联分析

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作物学报 2025年第1期51卷 91-102页

作者：马敏虎常华瑜陈朝燕仁增刘廷辉邢国芳郭刚刚山西农业大学农学院/杂粮种质创新与分子育种山西省重点实验室山西晋中030801 中国农业科学院作物科学研究所/农业农村部粮食作物基因资源评价利用重点实验室/农作物基因资源与基因改良国家重大科学工程北京100081 甘孜藏族自治州农业科学研究所四川甘孜626000

苗草工厂为实现草食动物的饲草周年供应提供了新的解决方案。针对苗草生产的品种需求,本研究对124份中国大麦育成品种(系)与种质开展了苗草转化率鉴定和生物量调控位点发掘。结果显示,大麦种子萌动后,水培条件下苗草生物量呈指数增长趋... 详细信息

苗草工厂为实现草食动物的饲草周年供应提供了新的解决方案。针对苗草生产的品种需求,本研究对124份中国大麦育成品种(系)与种质开展了苗草转化率鉴定和生物量调控位点发掘。结果显示,大麦种子萌动后,水培条件下苗草生物量呈指数增长趋势并在7 d后进入平台期。在植物工厂条件下,鉴定出冬青16、扎青6号等10个高苗草转化率品种且分析发现苗草生物量与籽粒千粒重呈一定的负相关。进一步通过全基因组关联分析,共鉴定到12个苗草生物量相关QTL位点,从中预测出8个调控苗草生物量的候选基因。本研究不仅为大麦苗草工厂化生产筛选出高转化率品种,同时也为苗草专用型大麦品种的遗传改良奠定了基础。

关键词：大麦苗草生物量调控位点全基因组关联分析

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Removal of phosphorus-rich phase from high-phosphorous iron ore by melt separation at 1573 K in a super-gravity field

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International Journal of Minerals,Metallurgy and Materials 2016年第7期23卷 743-750页

作者： Jin-tao Gao Lei guo Yi-wei Zhong Hong-ru Ren Zhan-cheng guo State Key Laboratory of Advanced Metallurgy University of Science and Technology Beijing

A new approach of removing the phosphorus-rich phase from high-phosphorous iron ore by melt separation at 1573 K in a super-gravity field was investigated. The iron？slag separation by super-gravity resulted in phosphorus being effectively removed from the iron-rich phase and concentrated as a phosphorus-rich phase at a temperature below the melting point of iron. The samples obtained by super-gravity exhibited obvious layered structures. All the iron grains concentrated at the bottom of the sample along the super-gravity direction, whereas the molten slag concentrated in the upper part of the sample along the opposite direction. Meanwhile, fine apatite crystals collided and grew into larger crystals and concentrated at the slag–iron interface. Consequently, in the case of centrifugation with a gravity coefficient of G = 900, the mass fractions of the slag phase and iron-rich phase were similar to their respective theoretical values. The mass fraction of MFe in the iron-rich phase was as high as 97.77wt% and that of P was decreased to 0.092wt%.

关键词： ironmaking super-gravity melt separation dephosphoration

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The leaching of additive-derived flame retardants(FRs) from plastics in avian digestive fluids:The significant risk of highly lipophilic FRs

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Journal of Environmental Sciences 2019年第11期31卷 200-207页

作者： Huiying guo Xiaobo Zheng Shuling ru Xiaojun Luo Bixian Mai State Key Laboratory of Organic Geochemistry and Guangdong Key Laboratory of Environmental Protection and Resources Utilization Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangzhou 510640 China College of Resources and Environment South China Agricultural University Guangzhou 510642 China University of the Chinese Academy of Sciences Beijing 100049 China

The exposure to plastic debris and associated pollutants for wildlife is of urgent concern,but little attention has been paid on the transfer of plastic additives from plastic debris to *** the present study,the leaching of incorporated flame retardants (FRs),including polybrominated diphenyl ethers (PBDEs),alternative brominated FRs (AFRs),and phosphate flame retardants (PFRs),from different sizes of recycled acrylonitrile-butadiene-styrene (ABS) polymer were investigated in avian digestive *** impact of co-ingested sediment on the leaching of additive-derived FRs in digestive fluids was also *** the recycled ABS,BDE 209 (715 μg/g) and 1,2-bis(2,4,6-tribromophenoxy) ethane (BTBPE,1766 μg/g) had the highest concentrations among all target *** leaching proportions of FRs were higher in finer sizes of *** leaching proportions of FRs from recycled ABS increased with elevated logKow of *** the tests with coexisted ABS and sediment,hexato deca-BDEs,BTBPE,and decabromodiphenyl ethane (DBDPE) migrated from ABS to sediment,which resulted in the less bioaccessible fractions of these FRs in gut *** lipophilic chemicals tended to be adsorbed by sediment from *** results suggest the migration of additive-derived FRs from plastics to other indigestible materials in digestive *** findings in this study provide insights into the transfer of additive-derived FRs from plastics to birds,and indicate the significant contribution of FR-incorporated plastics to bioaccumulation of highly lipophilic FRs.

关键词： Recycled plastics Digestive fluids Flame retardants Leaching

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Unraveling salt stress signaling in plants

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Journal of Integrative Plant Biology 2018年第9期60卷 796-804页

作者： Yongqing yang yan guo State Key Laboratory of Plant Physiology and Biochemistry College of Biological SciencesChina Agricultural UniversityBeijing 100193China

Salt stress is a maior environmental factor limiting plant growth and productivity. A better understanding of the mechanisms mediating salt resistance will help researchers design ways to improve crop performance under adverse environmental conditions. Salt stress can lead to ionic stress, osmotic stress and secondary stresses, particularly oxidative stress, in plants. Therefore, to adapt to salt stress, plants rely on signals and pathways that re-establish cellular ionic, osmotic, and reactive oxygen species （ROS） homeostasis. Over the past two decades, genetic and biochemical analyses have revealed several core stress signaling pathways that participate in salt resistance. The Salt Overly Sensitive signaling pathway plays a key role in maintaining ionic homeostasis, via extruding sodium ions into the apoplast. Mitogenactivated protein kinase cascades mediate ionic, osmotic, and ROS homeostasis. SnRK2 （sucrose nonfermenting l-related protein kinase 2） proteins are involved in maintaining osmotic homeostasis. In this review, we discuss recent progress in identifying the components and pathways involved in the plant＇s response to salt stress and their regulatory mechanisms. We also review progress in identifying sensors involved in salt-induced stress signaling in plants.

关键词： Unraveling salt stress signaling in plants ROS ABA MAPKKK SOS CBL

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Regional path moving horizon tracking controller design for autonomous ground vehicles

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Science China(Information Sciences) 2017年第1期60卷 201-207页

作者： Hongyan guo Feng LIU ru YU Zhenping SUN Hong CHEN State Key Laboratory of Automotive Simulation and Control Jilin University(Campus Nanling) College of Communication Engineering Jilin University (Campus Nanling) School of Mechatronic Engineering and Automation National University of Defense Technology

A novel regional path tracking description is presented in this manuscript, and the moving horizon control method that is model predictive control(MPC) is proposed to discuss the regional path tracking issue which could avoid colliding road boundary when tracking a more complex road effectively. The feasible region for autonomous ground vehicles(AGVs) running is determined first according to the detected road ***, in order to keep the actual trajectory of AGVs in the region and satisfy the safety requirements, MPC method is employed to design the path tracking controller considering actuator and road boundary *** order to verify the effectiveness of the proposed method, experiments based on Hongqi AGV HQ430 are carried out, and the results illustrate that the presented method could be successfully applied to Hongqi AGV vehicle HQ 430.

关键词： autonomous ground vehicles regional path tracking model predictive control road boundaries experimental validation

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The Degenerated Second Main Theorem and Schmidt's Subspace Theorem

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Science China Mathematics 2012年第7期55卷 1367-1380页

作者： CHEN ZhiHua ru Min yan QiMing Department of Mathematics Tongji University Shanghai 200092 China Department of Mathematics University of Houston Houston TX 77004 USA

In this paper, we establish a Second Main Theorem for an algebraically degenerate holomorphic curve f : C → Pn(C) intersecting hypersurfaces in general position. The related Diophantine problems are also considered.

关键词： Nevanlinna theory holomorphic curve Second Main Theorem Diophantine approximation Schmidt's Subspace Theorem

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Real-time Monitoring of Living Cationic Ring-opening Polymerization of THF and Direct Prediction of Equilibrium Molecular Weight of Poly THF

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Chinese Journal of Polymer Science 2015年第1期33卷 23-35页

作者： An-ru guo Fan yang rui Yu 吴一弦 State Key Laboratory of Chemical Resource Engineering Key Laboratory of Carbon Fiber and Functional Polymers(Ministry of Education) Beijing University of Chemical Technology

A convenient real-time monitoring of monomer concentration during living cationic ring-opening polymerizations of tetrahydrofuran（THF） initiated with methyl triflate（Me OTf） has been developed for kinetic investigation and determination of equilibrium monomer concentration（[M]e） via in situ FTIR spectroscopy in combination with a diamond tipped attenuated total reflectance（ATR） immersion probe. The polymerization rate was first order with respect to monomer concentration and initiator concentration from the linear slope of ln（[M]0-[M]e）/（[M]-[M]e） versus polymerization time at different temperatures in various solvents. [M]e decreased linearly with initial monomer concentration while increased exponentially with increasing polymerization temperature. The equilibrium also strongly depends on solvent polarity and its interaction with monomer. The equilibrium polymerization time（te） decreased with increasing solvent polarity and decreased linearly with increasing [M]0 in three solvents with different slopes to the same point of bulk polymerization in the absence of solvent. Equation of Mn,e = 72.1/（0.14–0.04[M]e） has been established to provide a simple and effective approach for the prediction for the number-average molecular weight of poly THFs at equilibrium state（Mn,e） in the equilibrium living cationic ring-opening polymerization of THF at 0 °C.

关键词： Cationic ring-opening polymerization Living polymerization Tetrahydrofuran Equilibrium Kinetics.

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