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Influence of tectonic preservation conditions on the nanopore structure of shale reservoir: A case study of Wufeng-Longmaxi Formation shale in western Hubei area, south China

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Petroleum Science 2024年第4期21卷 2203-2217页

作者： Meng Xiang Shang xu ya-Ru Wen Qi-yang Gou Bing-Chang Liu National Key Laboratory of Deep Oil and Gas China University of Petroleum (East China) Hubei Key Laboratory of Resources and Eco-environment Geology Hubei Geological Survey Key Laboratory of Tectonics and Petroleum Resources Ministry of Education China University of Geosciences

Tectonism is one of the dominant factors affecting the shale pore structure. However, the control of shale pore structure by tectonic movements is still controversial, which limits the research progress of shale gas accumulation mechanism in the complex tectonic region of southern China. In this study, 34 samples were collected from two exploratory wells located in different tectonic locations. Diverse experiments,e.g., organic geochemistry, XRD analysis, FE-SEM, low-pressure gas adsorption, and high-pressure mercury intrusion, were conducted to fully characterize the shale reservoir. The TOC, Ro, and mineral composition of the shale samples between the two wells are similar, which reflects that the shale samples of the two wells have proximate pores-generating capacity and pores-supporting ***, the pore characteristics of shale samples from two wells are significantly different. Compared with the stabilized zone shale, the porosity, pore volume, and specific surface area of the deformed zone shale were reduced by 60.61%, 64.85%, and 27.81%, respectively. Moreover, the macroscopic and fine pores were reduced by 54.01% and 84.95%, respectively. Fault activity and uplift denudation are not conducive to pore preservation, and the rigid basement of Huangling uplift can promote pore preservation. These three factors are important reasons for controlling the difference in pore structure between two wells shales. We established a conceptual model of shale pores evolution under different tectonic preservation conditions. This study is significant to clarify the scale of shale gas formation and enrichment in complex tectonic regions, and helps in the selection of shale sweet spots.

关键词： Shale gas Pore structure Tectonic preservation conditions Shale gas enrichment mechanism

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Introducing urea into tirapazamine derivatives to enhance anticancer therapy

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National Science Review 2024年第4期11卷 245-253页

作者： yajun xu Jianlin Lv Chaoying Kong ya Liu Kun Wang Zhaohui Tang xuesi Chen Key Laboratory of Polymer Ecomaterials Changchun Institute of Applied ChemistryChinese Academy of Sciences School of Applied Chemistry and Engineering University of Science and Technology of China

Tirapazamine（TPZ） has been approved for multiple clinical trials relying on its excellent anticancer ***,as a typical hypoxia-activated prodrug（HAP）,TPZ did not exhibit survival advantages in Phase Ⅲ clinical trials when used in combination therapy due to the insufficient hypoxia levels in patients' *** this study,to improve the therapeutic effects of TPZ,we first introduced urea to synthesize a series of urea-containing derivatives of *** urea-containing TPZ derivatives showed increased hypoxic cytotoxicity（9.51-30.85-fold） compared with TPZ,while maintaining hypoxic ***,one of these derivatives,showed 20-fold higher cytotoxicity than TPZ while maintaining a similar hypoxic cytotoxicity *** highly efficiently deliver TPZP to the tumors and reduce its side effects on healthy tissues,we further prepared TPZP into a nanodrug with fibrin-targeting ability:***4-NPs,a vascular disrupting agent,was used to increase the fibrin level within tumors and exacerbate tumor *** being combined with CA4-NPs,FT11-TPZP-NPs can accumulate in the hypoxia-aggravated tumors and activate sufficiently to kill tumor *** a single-dose treatment,FT11-TPZP-NPs+CA4-NPs showed a high inhibition rate of 98.1% against CT26 tumor models with an initial volume of ～480 mm3and four out of six tumors were completely eliminated;it thereby exerted a significant antitumor *** study provides a new strategy for improving the therapeutic effect of TPZ and other HAPs in anticancer therapy.

关键词： tirapazamine vascular disrupting agent hypoxia-activated prodrug combretastatin A4 urea

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Simultaneously enhancing ionic conductivity and interfacial stability by Fe_(2)O_(3) for solid-state sodium metal batteries

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Journal of Materiomics 2024年第6期10卷 1243-1251页

作者： Jicheng xu Huachao Tao Zerong Deng xuelin yang Li-zhen Fan College of Electrical Engineering&New Energy China Three Gorges UniversityYichangHubei443002China College of Materials and Chemical Engineering Hubei Provincial Collaborative Innovation Center for New Energy MicrogridChina Three Gorges UniversityYichangHubei443002China Beijing Advanced Innovation Center for Materials Genome Engineering Institute of Advanced Materials and TechnologyUniversity of Science and Technology BeijingBeijing100083China

NASICON-structured Na_(3)Zr_(2)Si_(2)PO_(12)(NZSP)has been considered as one of the ideal electrolytes for all-solid-state sodium metal batteries(ASSSB).However,the practical application of NZSP-based ASSSB is hindered by the low ionic conductivity and large interfacial resistance caused by the poor contact between NZSP and Na ***,the introduction of Fe_(2)O_(3) not only improves ionic conductivity and reduces activation energy by the doping of Fe^(3+)in the crystal structure of NZSP,but also reduces the interfacial resistance and enhances interface stability between NZSP and Na metal *** synergistic effects significantly enhance the cycling stability,rate capability,and critical current density of the symmetrical solid-state *** interfacial reaction mechanism indicates that Fe3+in the interface is reduced Fe2+by Na anode,which effectively even the electric-filed distribution and suppresses the dendrite ***,the symmetric solid-state cells exhibit stable cycling performance for 1,500 h at 0.1 mA·cm−1/0.1 mA·h·cm−1 and over 900 h at 0.2 mA·cm−1/0.2 mA·h·cm−*** Na|NZSP-0.075%Fe_(2)O_(3)|Na_(2)FePO_(4)F solid-state full cells display high capacity retention of 94.2%after 100 cycles at 0.5 *** stable interface of NZSP/Na and improved ionic conductivity contribute to excellent electrochemical performance,which accelerates the practical application of ASSSB.

关键词： Solid-state electrolyte Na_(3)Zr_(2)Si_(2)PO_(12) Fe_(2)O_(3) Ionic conductivity Interfacial stability

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SG-NeRF:Sparse-Input Generalized Neural Radiance Fields for Novel View Synthesis

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Journal of Computer Science & Technology 2024年第4期39卷 785-797页

作者： Kuo xu Jie Li zhen-Qiang Li yang-Jie Cao School of Cyber Science and Engineering Zhengzhou UniversityZhengzhou 450002China Intelligent Big Data System(iBDSys)Lab Shanghai Jiao Tong UniversityShanghai 200240China School of Computer and Artificial Intelligence Zhengzhou UniversityZhengzhou 450001China

Traditional neural radiance fields for rendering novel views require intensive input images and pre-scene optimization,which limits their practical *** propose a generalization method to infer scenes from input images and perform high-quality rendering without pre-scene optimization named SG-NeRF(Sparse-Input Generalized Neural Radiance Fields).Firstly,we construct an improved multi-view stereo structure based on the convolutional attention and multi-level fusion mechanism to obtain the geometric features and appearance features of the scene from the sparse input images,and then these features are aggregated by multi-head attention as the input of the neural radiance *** strategy of utilizing neural radiance fields to decode scene features instead of mapping positions and orientations enables our method to perform cross-scene training as well as inference,thus enabling neural radiance fields to generalize for novel view synthesis on unseen *** tested the generalization ability on DTU dataset,and our PSNR(peak signal-to-noise ratio)improved by 3.14 compared with the baseline method under the same input *** addition,if the scene has dense input views available,the average PSNR can be improved by 1.04 through further refinement training in a short time,and a higher quality rendering effect can be obtained.

关键词： Neural Radiance Fields(NeRF) multi-view stereo(MVS) new view synthesis(NVS)

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Insight into vertical piezoelectric characteristics regulated thermal transport in van der Waals two-dimensional materials

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Rare Metals 2024年第2期43卷 770-779页

作者： Dong-Hai Wei E Zhou Jin-Yuan xu Hui-Min Wang Chen Shen Hong-Bin Zhang zhen-zhen Qin Guang-Zhao Qin State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body College of Mechanical and Vehicle EngineeringHunan UniversityChangsha410082China Hunan Key Laboratory for Micro-Nano Energy Materials and Device and School of Physics and Optoelectronics Xiangtan UniversityXiangtan411105China Institute of Materials Science Technical University of DarmstadtAlarich-Weiss-Str.264287DarmstadtGermany School of Physics and Microelectronics Zhengzhou UniversityZhengzhou450001China

The urgent demand of extreme(ultra-high/low)thermal conductivity materials is triggered by the high-power device,where exploring the theories and mechanisms of regulating thermal transport properties plays a key ***,we elaborately investigate the effect of vertical(out-of-plane)piezoelectric characteristics on thermal transport,which is historically *** different stacking-order(AA and AB)bilayer boron nitride(Bi-BN)in two-dimensional(2D)materials are selected as study *** performing state-of-the-art first-principles calculations,it is found that the polarization charge along the out-of-plane orientation ascends significantly with the increasing piezoelectric response in AB stacked Bi-BN(Bi-BN-AB)followed by the enhanced interlayer B–N atomic ***,the amplitude of phonon anharmonicity in Bi-BN-AB increases larger than that in the AA stacked Bi-BN(Bi-BN-AA),resulting in the dramatic weakening of the thermal conductivity by 20.34%under 18%*** research reveals the significant role of the vertical(out-of-plane)piezoelectric characteristic in regulating thermal transport and provides new insight into accurately exploring the thermal transport performance of 2D van der Waals materials.

关键词： Thermal conductivity Piezoelectric effect 2D materials Bilayer BN Strain engineering

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Associations between the use of red yeast rice preparations and adverse health outcomes:An umbrella review of meta-analyses of randomized controlled trials

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Journal of Integrative Medicine 2024年第2期22卷 126-136页

作者： zhen-yu Ma Shu-ping yang Ying Li Tian-tian xu ya-lin yang Hui-yong yang Heng-bing Li Le-jin Zhou Yong Diao Su-yun Li School of Medicine Huaqiao UniversityQuanzhou 362021Fujian ProvinceChina College of Traditional Chinese Medicine Shandong University of Traditional Chinese MedicineJinan 250355Shandong ProvinceChina Second Clinical Medical College Nanjing Medical UniversityNanjing 211166Jiangsu ProvinceChina

Background:Red yeast rice(RYR),a natural lipid-lowering agent,is widely used in clinical ***,the existing meta-analyses concerning the safety of RYR preparations have yielded inconsistent results,and the credibility of the evidence has not been ***:This study was designed to evaluate the existing evidence and offer a comprehensive understanding of the associations between the use of RYR preparations and various adverse health *** strategy:Seven literature databases were searched from inception to May 5,2023,using medical subject headings and free-text terms(e.g.,“red yeast rice,”“xuezhikang,”and“Zhibitai”).Inclusion criteria:Meta-analyses that investigated and quantitatively estimated associations between the use of RYR preparations and adverse health outcomes were included in this *** extraction and analysis:Two researchers independently extracted data using a standardized data collection table;any disagreements were resolved by consulting a third *** on the participant,intervention,comparator and outcome(PICO)framework in each eligible meta-analysis,a series of unique associations between the use of RYR preparations and adverse health outcomes were *** associations’effect estimates were re-evaluated using random-effect ***:Fifteen meta-analyses,comprising 186(164 unique)randomized controlled trials,were *** on A Mea Surement Tool to Assess Systematic Reviews version 2,3(20%)and 12(80%)of these meta-analyses had low and critically low confidence,respectively.A total of 61 unique associations between the use of RYR preparations and adverse health outcomes were extracted from eligible *** on the random-effect models,10(16.4%)associations indicated a significant protective effect of RYR preparations against adverse health outcomes,while 5(8.2%)indicated an increased risk of adverse health outcomes related to uric acid,alanine transaminase and aspartate trans

关键词： Red yeast rice Safety Adverse health outcomes Umbrella review Meta-analysis Systematic review

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Multicolor upconversion reversible modulations in YNbO_(4):Er^(3+)/Tm^(3+)/Yb^(3+) photochromic materials

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Journal of Rare Earths 2024年第2期42卷 270-277,I0002页

作者： zhen Zhang Peng Li Ziyi xu Zhihao Zhang Qiwei Zhang Haiqin Sun Xihong Hao Inner Mongolia Key Laboratory of Ferroelectric-related New Energy Materials and Devices Schoolof Materials and MetallurgyInner Mongolia University of Science and TechnologyBaotou014010China College of Physics and Technology Guangxi Normal UniversityGuilin541004China

Photochromic materials with multicolor upconversion reversible modulations are attractive in optical switching ***,the fabricated YNbO_(4):Er^(3+)/Tm^(3+)/Yb^(3+) materials exhibit excellent photochromism and multicolor upconversion properties from green,red to near infrared(NIR) emissions with increasing Yb *** multiband upconversion modulations are achieved by alternating light(365 and 405 nm) or thermal *** 365 nm irradiation,the luminescence color changes from yellow to red,the luminescent photoswitching contrast reaches up to 86.21%(green),82.12%(red) and 77.38%(NIR) in the Y_(0.83)Er_(0.01)Tm_(0.01)NbO_(4):0.15 Yb ***,the upconversion emission intensity before and after photochromic reaction shows remarkable change in a wide temperature range of 298-718 *** results indicate that the Er^(3+)/Tm^(3+)/Yb^(3+) tri-doped YNbO_(4) materials can be a good candidate in optical switching and data storage applications.

关键词： Photochromic materials Luminescence modulation Multicolor emission Photoswitching contrast Rare earths

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Shallow sub-lakes are essential for sustaining the successful wintering of waterbirds in Poyang Lake,China

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Avian Research 2024年第2期15卷 219-228页

作者： Mengjie Lu zhen Zhang Peng Chen Changxin xu Bin Gao Luzhang Ruan School of Life Sciences Nanchang UniversityNanchang330031China Jiangxi Province Key Laboratory of Watershed Ecosystem Change and Biodiversity Center for Watershed EcologyInstitute of Life Science and School of Life SciencesNanchang UniversityNanchang330031China

For migratory waterbirds,the quality of wintering habitat is related to spring migration and successful breeding in the next *** availability of food resources in the habitat is critical and varies within water *** the water-level fluctuations in Poyang Lake have been extremely variable interannually in recent years,the wintering waterbird populations have remained relatively ***,the mechanism of maintaining the stability is worth *** study aimed to compare the distribution of vegetation and herbivorous wa-terbirds in 2015-2016 and 2016-2017,focusing on three shallow sub-lakes and one main lake *** results showed that the emergence of tubers and the growth of Carex *** a continuous food supply and habitat for wintering waterbirds with a gradual decline in the water *** sub-lakes supported almost all of the tuber-eating waterbirds(1.42-1.62×10^(5))and most geese(1.34-1.53×10^(6)).However,the main lake area,covered with Persicaria hydropiper,did not provide adequate and accessible *** resulted in almost no distribution of tuber-eating waterbirds,with only a few geese congregating in early *** results demonstrated that the shallow sub-lakes under human control provided a different environment from the main lake and are key to sustaining the successful wintering of hundreds of thousands of migratory waterbirds in Poyang ***,we recommend refining the anthropogenic management of the shallow sub-lakes to regulate the water level to ensure the carrying capacity of Poyang Lake.

关键词： Anthropogenic management Carrying capacity Seasonal lake Water level Wintering habitat

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Analysis of risk factors of suicidal ideation in adolescent patients with depression and construction of prediction model

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World Journal of Psychiatry 2024年第3期14卷 388-397页

作者： Jun-Chao Zhou yan Cao xu-Yuan xu zhen-Ping Xian Department of Psychosomatic Medicine The Affiliated Lianyungang Hospital of Xuzhou Medical UniversityThe First People's Hospital of LianyungangLianyungang 222000Jiangsu ProvinceChina

BACKGROUND Major depressive disorder is a common mental illness among adolescents and is the largest disease burden in this age *** adolescent patients with depression have suicidal ideation(SI);however,few studies have focused on the factors related to SI,and effective predictive models are *** To construct a risk prediction model for SI in adolescent depression and provide a reference assessment tool for *** The data of 150 adolescent patients with depression at the First People's Hospital of Lianyungang from June 2020 to December 2022 were retrospectively *** on whether or not they had SI,they were divided into a SI group(n=91)and a non-SI group(n=59).The general data and laboratory indices of the two groups were *** regression was used to analyze the factors influencing SI in adolescent patients with depression,a nomogram prediction model was constructed based on the analysis results,and internal evaluation was *** operating characteristic and calibration curves were used to evaluate the model’s efficacy,and the clinical application value was evaluated using decision curve analysis(DCA).RESULTS There were differences in trauma history,triggers,serum ferritin levels(SF),highsensitivity C-reactive protein levels(hs-CRP),and high-density lipoprotein(HDLC)levels between the two groups(P<0.05).Logistic regression analysis showed that trauma history,predisposing factors,SF,hs-CRP,and HDL-C were factors influencing SI in adolescent patients with *** area under the curve of the nomogram prediction model was 0.831(95%CI:0.763–0.899),sensitivity was 0.912,and specificity was *** higher net benefit of the DCA and the average absolute error of the calibration curve were 0.043,indicating that the model had a good *** The nomogram prediction model based on trauma history,triggers,ferritin,serum hs-CRP,and HDL-C levels can effectively predict the risk of SI in adolescent patients

关键词： Adolescents Depression Suicidal ideation Risk factors Prediction model Ferritin

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Viscosity and structure of CaO-BaO-SiO_(2)-Al_(2)O_(3)-based mold slags for continuous casting of high titanium steel with different Tio2 absorption

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Journal of Iron and Steel Research International 2024年第8期31卷 1936-1946页

作者： ya-tao Cui xue-you Wang xu-bin Zhang Qiang-qiang Wang Sheng-ping He College of Materials Science and Engineering Chongqing UniversityChongqing 400044China

The effect of TiO_(2) absorption into two different CaO-BaO-SiO_(2)-Al_(2)O_(3)-based mold slags from the steel plant on the viscosity,melting performance and microstructure of slags was investigated through the measurement of the viscosity-temperature relationship,melting temperature and Raman *** parameter of the number of non-bridging oxygen per tetrahedrally-coordinated atom(NBO/T)was also calculated to explain the microstructure variation of molten slags with different TiO_(2) *** variation of the actual slag consumption and the depth of the liquid slag in mold was explained through the comparison of the viscosity and the melting temperature of two different *** viscosity of mold slags(basicity=0.6)decreased from 1.1 to 0.68 Pa s with the increase in the Ti0_(2) absorption from 0 to 10%,while that of slags(basicity=0.7)decreased from 0.76 to 0.56 Pa s with the Ti0_(2) absorption from 0 to 6%.The activation energy of both two groups of slags had the tendency to decrease with the increasing TiO_(2) *** network structure of both two groups of slags measured by the Raman spectra showed that the fraction of complex structure units(Q^(1),Q^(2),Q^(3) and A1-O-Al)decreased and simple structure units(Al-O-and Q^(0))increased with the increase in TiO_(2) ***/T also increased with the increase in the TiO2 absorption,indicating that the absorption of TiO_(2) into slags resulted in the destruction of silicate/aluminate ***,the absorption of TiO_(2) into the current CaO-BaO-SiO_(2)-Al_(2)O_(3) mold slags decreased the degree of polymerization of these slags and then led to the decrease of viscosity.

关键词： Mold slag Viscosity Melting temperature Slag consumption Liquid slag depth Structure

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