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Acetylacetone-TiO_(2) Promoted Large Area Compatible Cascade Electron Transport Bilayer for Efficient Perovskite Solar Cells

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Energy & Environmental Materials 2024年第2期7卷 221-228页

作者： hyong Joon Lee Jin Kyoung Park Jin hyuck heo Sang hyuk im Department of Chemical and Biological Engineering Korea University145 Anam-ro Seongbuk-guSeoul 17104Korea

In designing efficient perovskite solar cells(PSCs),the selection of suitable electron transport layers(ETLs)is critical to the final device performance as they determine the driving force for selective charge ***_(2)nanoparticles(NPs)based ETLs have been a popular choice for PSCs due to superior electron mobility,but their relatively deep-lying conduction band energy levels(ECB)result in substantial potential ***,TiO_(2)NPs establish favorable band alignment owing to shallower ECB,but their low intrinsic mobility and abundant surface trap sites impede the final *** this reason,constructing a cascaded bilayer ETL is highly desirable for efficient PSCs,as it can rearrange energy levels and exploit on advantages of an individual *** this study,we prepare SnO_(2)NPs and acetylacetone-modified TiO_(2)(Acac-TiO_(2))NPs and implement them as bilayer SnO_(2)/Acac-TiO_(2)(BST)ETL,to assemble cascaded energy band ***_(2)contributes to rapid charge carrier transport from high electron mobility while Acac-TiO_(2)minimizes band-offset and effectively suppresses interfacial ***,the optimized BST ETL generates synergistic influence and delivers power conversion efficiency(PCE)as high as 23.14%with open-circuit voltage(V_(oc))reaching 1.14 ***,the BST ETL is transferred to a large scale and the corresponding mini module demonstrates peak performance of 18.39%PCE from 25 cm^(2)aperture ***,the BST-based mini module exhibit excellent stability,maintaining 83.1%of its initial efficiency after 1000 h under simultaneous 1 Sun light-soaking and damp heat(85℃/Rh 85%)environment.

关键词： acetylacetone large area perovskite solar cells TiO_(2)

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Interfacial modulation of bifunctional electrolyte additive engineering for dendrite-free and robust lithium metal anode

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Journal of Energy Chemistry 2024年第10期97卷 120-127,I0003页

作者： Mahammad Rafi Shaik yongmin Park young-Kwang Jung Won Bin im Division of Materials Science and Engineering Hanyang University222Wangsimni-roSeongdongguSeoul 0473Republic of Kor Department of Chemical Engineering and Biotechnology University of CambridgeCambridge CB3 OASUK

Anode materials for rechargeable electric car batteries are obtained from Li-metal owing to their extremely high specific capacity and low redox ***,safety concerns related to dendrite formation on the anode surface caused by the uneven distribution of Li-ions during the discharge process interfere with the use of Li-metal in industrial *** this study,methyl vinyl sulfone(MVS),a sulfone-based functional electrolyte additive,is used in an additive engineering strategy to control Lielectrolyte interactions and address the aforementioned *** dendrite growth may be restricted,and transition metal degradation on the surface of the cathode can be reduced by the MVS-derived functional electrolyte additive interfacial *** electrochemical performance of an ethylene carbonate/dimethyl carbonate(EC/DMC)+1 wt% MVS Li-metal anode of a Li||Li symmetric cell exhibits remarkable cycle stability,maintaining a low overvoltage for over 750 h at 1 mA cm^(-2),and capacity of 1 mA h cm^(-2).Additionally,LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811) full cells with the MVS additive exhibit enhanced electrochemical stability for 250 cycles at a current density of 100 mA g^(-1).This study provides an innovative approach for stabilizing the metal-electrolyte interfacial layer that may be used for practical applications in metal-based rechargeable batteries.

关键词： Lithium rechargeable battery Dendrite-free Electrolyte additive Bifunctional electrolyte Interfacial layer

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Biomimetic Fe_(7)S_(8)/Carbon electrocatalyst from[FeFe]-hydrogenase for improving ph-Universal electrocatalytic hydrogen production Special Collection:Aggregation-Induced Processes and Functions

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Aggregate 2024年第1期5卷 451-459页

作者： Dohun Kim Subramani Surendran Sejin im Jaehyoung Lim Kyoungsuk Jin Ki Tae Nam Uk Sim Department of Energy Science&Engineering Daegu Gyeongbuk Institute of Science&Technology(DGIST)DaeguRepublic of Korea hydrogen Energy Technology Laboratory Korea Institute of Energy Technology(KENTECH)NajuRepublic of Korea Department of Chemistry Korea UniversitySeoulRepublic of Korea Department of Materials Science and Engineering Seoul National UniversitySeoulRepublic of Korea

Efficient and cost-effective electrocatalysts that can operate across a wide range of ph conditions are essential for green hydrogen *** by biological systems,Fe_(7)S_(8)nanoparticles incorporated on polydopamine matrix electrocatalyst were synthesized by co-precipitation and annealing *** resulting Fe_(7)S_(8)/C electrocatalyst possesses a three-dimensional structure and exhibits enhanced electrocatalytic performance for hydrogen production across various ph ***,the Fe_(7)S_(8)/C electrocatalyst demonstrates exceptional activity,achieving low overpotentials of 90.6,45.9,and 107.4 mV in acidic,neutral,and alkaline environments,*** impedance spectroscopy reveals that Fe_(7)S_(8)/C exhibits the lowest charge transfer resistance under neutral conditions,indicating an improved proton-coupled electron transfer ***-wave electron paramagnetic resonance results confirm a change in the valence state of Fe from 3+to 1+during the hydrogen evolution reaction(hER).These findings closely resemble the behavior of natural[FeFe]-hydrogenase,known for its superior hydrogen production in neutral *** remarkable performance of our Fe_(7)S_(8)/C electrocatalyst opens up new possibilities for utilizing bioinspired materials as catalysts for the hER.

关键词： biomimetic electrocatalyst hydrogen production renewable energy

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Anode surface engineering of zinc-ion batteries using tellurium nanobelt as a protective layer for enhancing energy storage performance

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Journal of Energy Chemistry 2024年第5期92卷 113-123页

作者： Soobeom Lee yeonjin Je Boeun Seok hyun Tae Kim yong-Ryun Jo Soong Ju Oh Byoungyong im Dae Guen Kim Sang-Soo Chee Geon-hyoung An Department of Energy System Engineering Gyeongsang National UniversityJinju 52725Republic of Korea Nano Convergence Materials Center Korea Institute of Ceramic Engineering and Technology(KICET)Jinju 52851Republic of Korea Department of Materials Science and Engineering Korea UniversitySeoul 02841Republic of Korea School of Materials Science and Engineering Gyeongsang National UniversityJinju 52828Republic of Korea GIST Advanced Insitute of Instrumental Analysis(GAIA) Electron Microscopy LaboratoryGwangju Institute of Science and TechnologyGwangju 61005Republic of Korea Center for Advanced Materials and Processing Institute for Advanced EngineeringYongin 17180Republic of Korea Department of Energy Engineering Gyeongsang National UniversityJinju 52725Republic of Korea

Over the years,zinc-ion batteries(ZIBs)have attracted attention as a promising next-generation energy storage technology because of their excellent safety,long cycling performance,eco-friendliness,and high-power ***,issues,such as the corrosion and dissolution of the Zn anode,limited wet-tability,and lack of sufficient nucleation sites for Zn plating,have limited their practical *** introduction of a protective layer comprising of tellurium(Te)nanobelts onto the surface of Zn anode has emerged as a promising approach to overcome these limitations and improve the electrochemical behav-ior by enhancing the safety and wettability of ZIBs,as well as providing numerous nucleation sites for Zn *** the presence of a Te-based protective layer,the energy power density of the surface-engineered Zn anode improved significantly(ranging from 310 to 144 W h kg^(-1),over a power density range of 270 to 1,800 W kg^(-1)),and the lifespan capability was *** results demonstrate that the proposed strategy of employing Te nanobelts as a protective layer holds great promise for enhancing the energy storage performance of zIBs,making them even more attractive as a viable energy storage solution forthefuture.

关键词： Zn ion battery Anode Protective layer Tellurium Nanobelt

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乳腺癌新辅助化疗后基于体积的代谢性肿瘤反应与复发风险增高相关

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国际医学放射学杂志 2015年第3期 283-283页

作者： S.h.hyun h.K.Ahn y.h.Park y.h.im W.h.Kil J.E.Lee 施益洁 Department of Nuclear Medicine Samsung Medical Center Sungkyunkwan University School of Medicine50 Irwon-dongGangnam-gu Seoul 135-710Republic of Korea

目的评估局部晚期乳腺癌病人新辅助化疗后以基于体积的代谢性肿瘤反应预测预后的价值。材料与方法本研究获伦理委员会批准,免除知情同意。选取2006年7

关键词：新辅助化疗乳腺癌乳腺肿瘤代谢性反应

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A data-driven reduced-order model for stiff chemical kinetics using dynamics-informed training

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Energy and AI 2024年第1期15卷 181-192页

作者： Vijayamanikandan Vijayarangan harshavardhana A.Uranakara Shivam Barwey Riccardo Malpica Galassi Mohammad Rafi Malik Mauro Valorani Venkat Raman hong G.im CCRC King Abdullah University of Science and TechnologyThuwalSaudi Arabia Argonne Leadership Computing Facility Argonne National LaboratoryLemontIL 60439USA Mechanical and Aerospace Engineering Department Sapienza University of RomeVia Eudossiana18Rome 00184Italy Department of Aerospace Engineering University of MichiganAnn ArborMI 48109USA

A data-based reduced-order model(ROM)is developed to accelerate the time integration of stiff chemically reacting systems by effectively removing the stiffness arising from a wide spectrum of chemical time ***,the objective of this work is to develop a ROM that acts as a non-stiff surrogate model for the time evolution of the thermochemical state vector(temperature and species mass fractions)during an otherwise highly stiff and nonlinear ignition *** model follows an encode-forecast-decode strategy that combines a nonlinear autoencoder(AE)for dimensionality reduction(encode and decode steps)with a neural ordinary differential equation(NODE)for modeling the dynamical system in the AE-provided latent space(forecasting step).By means of detailed timescale analysis by leveraging the dynamical system Jacobians,this work shows how data-based projection operators provided by autoencoders can inherently construct the latent spaces by removing unnecessary fast timescales,even more effectively than physics-based counterparts based on an eigenvalue analysis.A key finding is that the most significant degree of stiffness reduction is achieved through an end-to-end training strategy,where both AE and neural ODE parameters are optimized simultaneously,allowing the discovered latent space to be *** addition to end-to-end training,this work highlights the vital contribution of AE nonlinearity in the stiffness reduction *** the prediction of homogeneous ignition phenomena for h2-air and C2h4-air mixtures,the proposed ROM achieves several ordersof-magnitude increase in the integration time step size when compared to(a)a baseline CVODE solver for the full-chemical system,(b)statistical technique–principal component analysis(PCA),and(c)computational singular perturbation(CSP),a vetted physics-based stiffness-reducing modeling framework.

关键词： Stiff system Chemical kinetics Reacting flows Autoencoders Neural ODE

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Superior antibody and membrane protein‑specific T‑cell responses to CoronaVac by intradermal versus intramuscular routes in adolescents

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World Journal of Pediatrics 2024年第4期20卷 353-370页

作者： Jaime S.Rosa Duque Samuel M.S.Cheng Carolyn A.Cohen Daniel Leung Xiwei Wang Xiaofeng Mu yuet Chung Tsun Ming Lau Manni Wang Wenyue Zhang yanmei Zhang howard h.W.Wong Leo C.h.Tsang Sara Chaothai Tsz Chun Kwan John K.C.Li Karl C.K.Chan Leo L.h.Luk Jenson C.h.ho Wing yan Li Amos M.T.Lee Jennifer h.y.Lam Sau Man Chan Wilfred h.S.Wong Issan y.S.Tam Masashi Mori Sophie A.Valkenburg Malik Peiris Wenwei Tu yu Lung Lau Department of Paediatrics and Adolescent Medicine The University of Hong KongHong KongChina School of Public health The University of Hong KongHong KongChina hKU‑Pasteur Research Pole School of Public HealthThe University of Hong KongHong KongChina Research Institute for Bioresources and Biotechnology Ishikawa Prefectural UniversityNonoichiJapan Department of Microbiology and immunology Peter Doherty Institute for Infectionand ImmunityUniversity of MelbourneMelbourneVICAustralia Center for immunology and Infection C2i Hong KongChina

Background Optimising the immunogenicity of COVID-19 vaccines to improve their protection against disease is *** dosing by intradermal(ID)administration has been shown to be equally immunogenic as intramuscular(im)administration for several vaccines,but the immunogenicity of ID inactivated whole severe acute respiratory syndrome coronavirus 2(SARS-CoV-2)at the full dose is *** study(NCT04800133)investigated the superiority of antibody and T-cell responses of full-dose CoronaVac by ID over im administration in *** Participants aged 11–17 years received two doses of im or ID vaccine,followed by the 3rd dose 13–42 days *** and cellular immunogenicity outcomes were measured post-dose 2(im-CC versus ID-CC)and post-dose 3(imCCC versus ID-CCC).Doses 2 and 3 were administered to 173 and 104 adolescents,*** Spike protein(S)immunoglobulin G(IgG),S-receptor-binding domain(RBD)IgG,S IgG Fcγreceptor IIIa(FcγRIIIa)-binding,SNM[sum of individual(S),nucleocapsid protein(N),and membrane protein(M)peptide pool]-specific interleukin-2(IL-2)+CD4^(+),SNM-specific IL-2^(+)CD8^(+),S-specific IL-2^(+)CD8^(+),N-specific IL-2^(+)CD4^(+),N-specific IL-2^(+)CD8^(+)and M-specific IL-2^(+)CD4^(+)responses fulfilled the superior and non-inferior criteria for ID-CC compared to im-CC,whereas IgG avidity was *** ID-CCC,S-RBD IgG,surrogate virus neutralisation test,90%plaque reduction neutralisation titre(PRNT90),PRNT50,S IgG avidity,S IgG FcγRIIIa-binding,M-specific IL-2^(+)CD4^(+),interferon-γ+CD8^(+)and IL-2^(+)CD8^(+)responses were superior and non-inferior to *** estimated vaccine efficacies were 49%,52%,66%and 79%for im-CC,ID-CC,im-CCC and ID-CCC,*** ID groups reported more local,mild adverse *** This is the first study to demonstrate superior antibody and M-specific T-cell responses by ID inactivated SARSCoV-2 vaccination and serves as the basis for future research to improve the

关键词： CoronaVac Coronavirus disease 2019 immunity Intradermal Vaccine

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improved rate-distortion optimized video coding using non-integer bit estimation and multiple Lambda search

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Frontiers of Computer Science 2016年第1期10卷 157-166页

作者： Sio Kei im Mohammad Mahdi GhANDI MPI-QMUL Information Systems Research Centre Macao Polytechnic Institute Macao China Department of Electronic Systems Engineering University of Essex Colchestey CO4 3SQ UK

Many modern video encoders use the Lagrangian rate-distortion optimization （RDO） algorithm for mode deci- sions during the compression procedure. For each encoding stage, this approach involves minimizing a cost, which is a function of rate, distortion and a multiplier called Lambda. This paper proposes to improve the RDO process by applying two modifications. The first modification is to increase the ac- curacy of rate estimation, which is achieved by computing a non-integer number of bits for arithmetic coding of the syntax elements. This leads to a more accurate cost computation and therefore a better mode decision. The second modification is to search and adjust the value of Lambda based on the char- acteristics of each coding stage. For the encoder used, this paper proposes to search multiple values of Lambda for the intra-4x4 mode decision. Moreover, a simple shift in Lambda value is proposed for motion estimation. Each of these modi- fications offers a certain gain in RDO performance, and, when all are combined, an average bit-rate saving of up to 7.0% can be achieved for the h.264/AVC codec while the same concept is applicable to the h.265/hEVC codec as well. The extra added complexity is contained to a certain level, and is also adjustable according to the processing resources available.

关键词： rate distortion optimization Lambda adjust-ment non-integer bit estimation h.264/AVC h265/hEVCvideo coding

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Structure-activity relationship of lysophosphatidylcholines in hL-60 human leukemia cells

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Acta Pharmacologica Sinica 2004年第11期 137-140页

作者： Eun-hee LEE,Jee h JUNG,Dong-soon im Laboratories of Pharmacology and Marine Natural Product Laboratories of Pharmacology and Marine Natural Product Laboratories of Pharmacology and Marine Natural Product College of Pharmacy Pusan National University Busan 609-735 Korea College of Pharmacy Pusan National University Busan 609-735 Korea College of Pharmacy Pusan National University Busan 609-735 Korea

Aim: To explore the structure-activity relationship of lysophosphatidylcholine (LPC) and lysolipid molecules from a marine sponge and ladybirds. METhODS: We tested three synthetic LPCs and four natural lysolipids on Ca2+ mobilization in hL-60 human leukemia cells. RESULTS: We observed lysolipid-mediated Ca2+ mobilization. The activity was the same in both ester- and ether-linked lysolipids, and introduction of a double bond or methoxy group on the alkyl chain did not significantly modulate the activity. however, replacement of trimethylammonium moiety in the choline structure with ammonium moiety reduced the activity. Furthermore, change of the alkyl chain length influenced the Ca2+ response. CONCLUSION: LPC-induced Ca2+ mobilization might be dependent on the length of alkyl chain and the presence of choline moiety in hL-60 leukemia cells.

关键词： lysophosphatidylcholines leukemia calcium signaling structure-activity relationship platelet activating factor

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Comparison of the probiotic characteristics of Lactic Acid Bacteria (LAB) isolated from sourdough and infant feces

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Food Bioscience 2022年第3期47卷 992-997页

作者： yasemin Kaya Tayyibe Erten Melike Vurmaz hümeyra İspirli Ömer Şimşek Enes Dertli Bayburt University Central Research LaboratoryBayburtTurkey Bayburt University Department of Nutrition and DieteticsFaculty of Heath SciencesBayburtTurkey Pamukkale University Department of Food EngineeringFaculty of EngineeringDenizliTurkey yıldız Technical University Department of Food EngineeringFaculty of Chemical and Metallurgical EngineeringİstanbulTurkey

Probiotics are beneficial microorganisms with certain characteristics such as survival under gastrointestinal conditions,adhesion to intestinal surface and different functions which result in several health benefits to *** this regards,this study aimed to isolate Lactic Acid Bacteria (LAB) from sourdough and human feces as two different environments and to test their potential probiotic *** total nine distinct isolates were assessed with several probiotic functions such as in vitro adhesion to human colon cells,antimicrobial activities and survival under harsh gastrointestinal *** general,distinct strains showed strong antimicrobial activity against the pathogenic and fungal strains tested in this ***,the adhesion levels to hT29 cells were determined between 0.29 % and 9.54% and Lactobacillus paracasei F7B showed the highest *** isolates tolerated the bile salt after 24 h and the infant feces isolates showed good survival characteristics at ph 4.

关键词： Probiotic Sourdough Infant feces Adhesion

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