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Carbon dots anchored NiAl-LDH@In_(2)O_(3) hierarchical nanotubes for promoting selective CO_(2) photoreduction into CH_(4)

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Chinese Chemical Letters 2024年第6期35卷 404-408页

作者： Xiuzheng Deng Changhai liu xiaotong Yan Jingshan Fan Qian Liang Zhongyu Li Advanced Catalysis and Green Manufacturing Collaborative Innovation Center CNPC-CZU Innovation AllianceSchool of Petrochemical EngineeringChangzhou UniversityChangzhou 213164China School of Materials Science&Engineering Changzhou UniversityChangzhou 213164China

The efficient conversion of CO_(2) into hydrocarbon fuels(CH_(4))with high selectivity is considered as a great challenge in photocatalysis owing to the multiple-electron transfer pathway and competitive H_(2) ***,we developed carbon dots(CDs)-modulated S-scheme heterojunction of CDs/NiAl-LDH@In_(2)O_(3)(C-DH@IN)through a facile in-situ hydrothermal *** to the multi-shell nanotube structure,the C-DH@IN shows an enhanced CH_(4) evolution rate of 10.67μmol h^(-1)g^(-1)and higher selectivity of CH_(4)(85.70%)compared with In_(2)O_(3) and Ni Al-LDH@In_(2)O_(3) binary catalyst in the pure water without sacrificial *** spin resonance(ESR)and in situ Fourier transform infrared spectra verify that the constructed S-scheme heterojunction can possess the strong redox capability and the HCOOand CH_(3)O-as critical intermediates play an important role in selective CO_(2) reduction to generate CH_(4).Furthermore,CDs with superior photoabsorption can boost the electron transfer and absorb H^(+),thus improving the integration of H^(+)and CO_(2) ***,this work emphasizes a facile strategy to achieve efficient CO_(2)-to-CH_(4) conversion based on construction of CDs-based heterojunction catalysts.

关键词： Carbon dots In_(2)O_(3) Layered double hydroxides Photocatalytic CO_(2) reduction S-scheme

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Revealing the role of honokiol in human glioma cells by RNA-seq analysis

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BIOCELL 2024年第6期48卷 945-958页

作者： YUNBAO GUO XU liu QI XU xiaotong ZHOU JIAWEI liu YANYAN XU YAN LU HAIYAN liu The Department of Neurosurgery First Hospital of Jilin UniversityChangchun130021China The Department of Anatomy College of Basic Medical SciencesJilin UniversityChangchun130021China The Third College of Clinical Medicine Jilin UniversityChangchun130021China

Background:Glioma is a kind of tumor that easily deteriorates and originates from glial cells in nerve *** is a bisphenol compound that is an essential monomeric compound extracted from the roots and bark of Magnoliaceae *** also has anti-infection,antitumor,and immunomodulatory *** this study,we found that honokiol induces cell apoptosis in the human glioma cell lines U87-MG and ***,the mechanism through which honokiol regulates glioma cell apoptosis is still ***:We performed RNA-seq analysis of U251-MG cells treated with honokiol and control ***-protein interaction(PPI)network analysis was performed,and the 10 top hub unigenes were examined via real-time quantitative ***,MAPK signaling and ferroptosis were detected via western ***:332 differentially expressed genes(DEGs)were found,comprising 163 increased and 169 decreased *** of the DEGs revealed that various biological processes were enriched,including‘response to hypoxia’,‘cerebellum development cellular response to hypoxia,’‘iron ion binding,’‘oxygen transporter activity,’‘oxygen binding,’‘ferric iron binding,’and‘structural constituent of cytoskeleton.’Kyoto Encyclopedia of Genes and Genomes(KEGG)pathway analysis revealed that the DEGs were enriched in the following pathways:‘mitogen-activated protein kinases(MAPK)’,‘Hypoxia-inducible factor 1(HIF-1)’,‘ferroptosis,’‘Peroxisome proliferator-activated receptor(PPAR),’‘Phosphatidylinositol-4,5-bisphosphate 3-kinase(PI3K)-protein kinase B(Akt),’and‘phagosome.’Among these pathways,the MAPK signaling pathway and ferroptosis were veriﬁ***:This study revealed the potential mechanism by which honokiol induces apoptosis and provided a comprehensive analysis of DEGs in honokiol-treated U251-MG cells and the associated signaling *** data could lead to new ideas for future research and therapy for patients with glioma.

关键词： Human glioma Honokiol RNA-seq Apoptosis Ferroptosis MAPK

Effect of land use on soil nematode community composition and co-occurrence network relationship

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Journal of Integrative Agriculture 2024年第8期23卷 2807-2819页

作者： xiaotong.liu Siwei Liang Yijia Tian Xiao Wang Wenju Liang Xiaoke Zhang Institute of Applied Ecology Chinese Academy of SciencesShenyang 110016China Tillage and Cultivation Research Institute Liaoning Academy of Agricultural SciencesShenyang 110161China University of Chinese Academy of Sciences Beijing 100049China Key Lab of Conservation Tillage and Ecological Agriculture in Liaoning Province Shenyang 110016China

Land use influences soil biota community composition and diversity,and then belowground ecosystem processes and *** characterize the effect of land use on soil biota,soil nematode communities in crop land,forest land and fallow land were investigated in six regions of northern *** richness,diversity,abundance and biomass of soil nematodes was the lowest in crop *** richness and diversity of soil nematodes were 28.8and 15.1%higher in fallow land than in crop land,*** significant differences in soil nematode indices were found between forest land and fallow land,but their network keystone genera composition was *** the keystone genera,50%of forest land genera were omnivores-predators and 36%of fallow land genera were *** proportion of fungivores in forest land was 20.8%lower than in fallow *** network complexity and the stability were lower in crop land than forest land and fallow *** pH,NH_(4)^(+)-N and NO_(3)^(–)-N were the major factors influencing the soil nematode community in crop land while soil organic carbon and moisture were the major factors in forest *** nematode communities in crop land influenced by artificial management practices were more dependent on the soil environment than communities in forest land and fallow *** use induced soil environment variation and altered network relationships by influencing trophic group proportions among keystone nematode genera.

关键词： soil nematode trophic groups community composition co-occurrence network land use

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Neural-based inexact graph de-anonymization

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High-Confidence Computing 2024年第1期4卷 52-59页

作者： Guangxi Lu Kaiyang Li xiaotong Wang Ziyue liu Zhipeng Cai Wei Li Department of Computer Science Georgia State UniversityAtlantaUSA St.George’s School VancouerCanada

Graph de-anonymization is a technique used to reveal connections between entities in anonymized graphs,which is crucial in detecting malicious activities,network analysis,social network analysis,and *** its paramount importance,conventional methods often grapple with inefficiencies and challenges tied to obtaining accurate query graph *** paper introduces a neural-based inexact graph de-anonymization,which comprises an embedding phase,a comparison phase,and a matching *** embedding phase uses a graph convolutional network to generate embedding vectors for both the query and anonymized *** comparison phase uses a neural tensor network to ascertain node *** matching procedure employs a refined greedy algorithm to discern optimal node ***,we comprehensively evaluate its performance via well-conducted experiments on various real *** results demonstrate the effectiveness of our proposed approach in enhancing the efficiency and performance of graph de-anonymization through the use of graph embedding vectors.

关键词： Graph de-anonymization Graph convolutional network Neural tensor network

Upcycling the spent graphite/LiCoO_(2) batteries for high-voltage graphite/LiCoPO_(4)-co-workable dual-ion batteries

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1745-1751页

作者： Miao Du Hongyan Lü Kaidi Du Shuohang Zheng xiaotong Wang xiaotong Deng Ronghua Zeng Xinglong Wu Key Laboratory for UV Light-Emitting Materials and Technology of Ministry of Education Northeast Normal UniversityChangchun 130024China Faculty of Chemistry Northeast Normal UniversityChangchun 130024China School of Chemistry South China Normal UniversityGuangzhou 510006China

The worldwide proliferation of portable electronics has resulted in a dramatic increase in the number of spent lithium-ion batteries(LIBs).However,traditional recycling methods still have limitations because of such huge amounts of spent ***,we proposed an ecofriendly and sustainable double recycling strategy to concurrently reuse the cathode(LiCoO_(2))and anode(graphite)materials of spent LIBs and recycled LiCoPO_(4)/graphite(RLCPG)in Li^(+)/PF^(-)_(6) co-de/intercalation dual-ion *** recycle-derived dualion batteries of Li/RLCPG show impressive electrochemical performance,with an appropriate discharge capacity of 86.2 mAh·g^(-1) at25 mA·g^(-1) and 69%capacity retention after 400 *** recycling of the cathode and anode from spent LIBs avoids wastage of resources and yields cathode materials with excellent performance,thereby offering an ecofriendly and sustainable way to design novel secondary batteries.

关键词： recycle lithium cobalt oxide lithium cobalt phosphate graphite dual-ion batteries spent lithium-ion batteries

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Low-Strain and High-Energy KVPO4F Cathode with Multifunctional Stabilizer for Advanced Potassium-Ion Batteries

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Energy & Environmental Materials 2024年第5期7卷 144-153页

作者： Yongli Heng Zhenyi Gu Jinzhi Guo Haojie Liang Yan liu Wei Guo Xinxin Zhao xiaotong Wang Xinglong Wu MOE Key Laboratory for UV Light-Emitting Materials and Technology Northeast Normal University Key Laboratory of Organo-Pharmaceutical Chemistry of Jiangxi Province Gannan Normal University Department of Chemistry Northeast Normal University

KVPO4F with excellent structural stability and high operating voltage has been identified as a promising cathode for potassium-ion batteries （PIBs）,but limits in sluggish ion transport and severe volume change cause insufficient potassium storage ***,a high-energy and low-strain KVPO4F composite cathode assisted by multifunctional K2C4O4electrode stabilizer is exquisitely *** electrochemical investigations demonstrate that this composite cathode can deliver a remarkable energy density up to 530 Wh kg-1with 142.7 mAh g-1of reversible capacity at25 mA g-1,outstanding rate capability of 70.6 mAh g-1at 1000 mA g-1,and decent cycling ***,slight volume change （-5%） and increased interfacial stability with thin and even cathode-electrolyte interphase can be observed through in situ and ex situ characterizations,which are attributed to the synergistic effect from in situ potassium compensation and carbon deposition through self-sacrificing K2C4O4additive.

关键词： high energy density K2C4O4 KVPO4F composite cathode low strain potassium-ion batteries

Interfacial mechanism of hydrogel with controllable thickness for stable drag reduction

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Friction 2024年第2期12卷 231-244页

作者： xiaotong WU Ying liu Yunlei ZHANG Xingwei WANG Wufang YANG Lang JIANG Shuanhong MA Meirong CAI Feng ZHOU School of Advanced Manufacturing Nanchang UniversityNanchang 330031China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China Yantai Zhongke Research Institute of Advanced Materials and Green Chemical Engineering Shandong Laboratory of Yantai Advanced Materials and Green ManufactureYantai 264006China

Surface wettability plays a significant role in reducing solid–liquid frictional resistance,especially the superhydrophilic/hydrophilic interface because of its excellent thermodynamic *** this work,poly(acrylic acid)-poly(acrylamide)(PAA–PAM)hydrogel coatings with different thicknesses were prepared in situ by polydopamine(PDA)-UV assisted surface catalytically initiated radical *** drag reduction performance of hydrogel surface was measured using a rotational rheometer by the plate–plate *** experimental results showed that the average drag reduction of hydrogel surface could reach up to about 56%in Couette flow,which was mainly due to the interfacial polymerization phenomenon that enhanced the ability of hydration layer to delay the momentum dissipation between fluid layers and the diffusion behavior of *** proposed drag reduction mechanism of hydrogel surface was expected to shed new light on hydrogel–liquid interface interaction and provide a new way for the development of steady-state drag reduction methods.

关键词： steady state drag reduction hydrogel interface hydration hydrophilic

Adaptive Predefined-Time Backstepping Control for Grid Connected Photovoltaic Inverter

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Energy Engineering 2024年第8期121卷 2065-2083页

作者： Jiarui Zhang Dan liu Kan Cao Ping Xiong xiaotong Ji Yanze Xu Yunfei Mu Key Laboratory of Smart Grid of Ministry of Education Tianjin UniversityTianjin300072China State Grid Hubei Electric Power Research Institute Wuhan430077China State Grid Hubei Electric Power Co. Ltd.Wuhan430077China

The system performance of grid-connected photovoltaic(PV)has a serious impact on the grid *** improve the control performance and shorten the convergence time,a predefined-time controller based on backstepping technology and dynamic surface control is formulated for the inverter in the grid-connected *** time-varying tuning functions are introduced into state-tracking errors to realize the predefined-time control *** address the“computational explosion problem”in the design process of backstepping control,dynamic surface control is adopted to avoid the analytical calculations of virtual *** disturbances of the PV system are estimated and compensated by adaptive *** control parameters are chosen and the global stability of the closed-loop is ensured by Lyapunov *** results confirm the effectiveness of the proposed controller and ensure the predefined time control in the photovoltaic inverter.

关键词： Photovoltaic inverter system backstepping technology predefined-time control adaptive control

Evaluation of suitability of university ladder classroom environment on humans

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Energy and Built Environment 2024年第4期5卷 615-627页

作者： Xin liu Xiu Geng Kailiang Huang Guohui Feng He Zhao xiaotong Wang Jianing He School of Municipal and Environment Engineering Shenyang Jianzhu UniversityShenyang 100168China Jianke EET Co. Ltd.Beijing 100013China

Evaluation of the suitability of university ladder classroom environment on humans is an effective approach to improve the quality of the indoor environment and protect human ***,there are unresolved issues regarding the suitability of university ladder classroom environment for *** example,the design of en-closure structure and heating ventilation and air conditioning(HVAC)system is unreasonable,and the indoor air quality does not meet the required *** this study,the suitability of university ladder classroom environ-ment on humans was considered the research *** evaluation indices of indoor environment were selected from indoor air quality,indoor thermal and humid environments,light environment,and sound *** the health and comfort of users were taken as the evaluation indices of *** to the results of expert investigations and case measurements,the index weight was determined by the expert-entropy weight method,and a complete evaluation system of indices was *** were two first-level,six second-level,and fourteen third-level indices in the evaluation *** evaluation indices of each level with the largest weight were indoor environment(0.5940),user health(0.2530),and indoor temperature(0.1175)*** comparing the actual learning effect to the evaluation results,the applicability of the evaluation system was *** evaluation system of the suitability of university ladder classroom environment on humans is convenient for operators to identify the weak points between humans and the *** evaluation system is endowed with important theoretical and practical significance to realize the green development of colleges and universities and build an environment-friendly campus.

关键词： Severe cold region Suitability of environment on humans Natural ventilation Expert-entropy weight method Evaluation system