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[Progress in applications of ambient ionization mass spectrometry for lipids identification]

Se pu = Chinese journal of chromatography 2025年第1期43卷 22-32页

作者： Xiao-Rong wang Yi-Yan Yin Jin Ouyang Na Na Key Laboratory of Radiopharmaceuticals Ministry of Education College of Chemistry Beijing Normal University Beijing 100875 China. Department of Chemistry College of Arts and Sciences Beijing Normal University Zhuhai 519087 China.

Lipids are indispensable components of living organisms and play pivotal roles in cell-membrane fluidity, energy provision, and neurotransmitter transmission and transport. Lipids can act as potential biomarkers of diseases given their abilities to indicate cell-growth status. For example, the lipid-metabolism processes of cancer cells are distinct from those of normal cells owing to their rapid proliferation and adaptation to ever-changing biological environments. As a result, the ability to rapidly detect, identify, and monitor lipid components is critical for tracking life-related processes and may enhance cancer diagnosis and treatment efficacy. Mass spectrometry (MS) is regarded to be among the most efficient methods for directly obtaining molecular-structural information, and is distinctly advantageous for identifying lipids. Recent years have witnessed the emergence of ambient mass spectrometry (AMS), which enables direct analyte sampling and ionization without the need for sample preprocessing. These characteristics endow AMS with special advantages for identifying and monitoring lipids. Furthermore, the ongoing development of soft ionization technologies has led to the widespread use of AMS for the detection of complex and diverse lipid molecules. Electrospray ionization (ESI) is a gentle ionization method that can be used to detect medium-to-high-polarity compounds and provide detailed chemical information for lipids by producing a fine mist of charged droplets from a liquid sample. Consequently, a series of ESI-based ionization methods have been developed for fabricating different AMS systems capable of rapidly detecting lipids in a simple manner. For example, desorption electrospray ionization (DESI) is among the most extensively employed ambient ionization techniques, and has been used to detect a wide range of samples, including solids, liquids, and gases. DESI involves spraying a charged solvent onto the surface of a sample, after which the solvent is

关键词： ambient mass spectrometry (AMS) ionization techniques lipid lipid fine structure tandem mass spectrometry (MS/MS)

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高温高压对三元预混燃料爆炸特性的影响

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高压物理学报 2025年第1期39卷 64-78页

作者：朱源姜根柱王筱蓉郭宏展苏傲成江苏科技大学机械工程学院江苏镇江212003

乙醇/甲烷/氢气(C_(2)H_(5)OH/CH_(4)/H_(2))作为一种新型的替代燃料,研究其爆炸特性对于我国新能源的可持续发展具有重要意义。在不同的当量比(0.8~1.4)、初始压力(0.1、0.2和0.4 MPa)和初始温度(370、400和450 K)下,从实验和化学动力... 详细信息

乙醇/甲烷/氢气(C_(2)H_(5)OH/CH_(4)/H_(2))作为一种新型的替代燃料,研究其爆炸特性对于我国新能源的可持续发展具有重要意义。在不同的当量比(0.8~1.4)、初始压力(0.1、0.2和0.4 MPa)和初始温度(370、400和450 K)下,从实验和化学动力学角度分析了其对关键爆炸特性参数,如峰值爆炸压力、峰值爆炸压力上升速率、爆炸时间以及爆燃指数的影响。结果表明,爆炸特性参数在当量比为1.2~1.3之间时出现极值。峰值爆炸压力与初始压力呈线性正相关,而与初始温度呈线性负相关。增大初始压力,火焰锋面裂纹、胞化程度加深,峰值爆炸压力增大。此外,实验工况下评估的最大爆燃指数为20.83 MPa·m/s,表明预混燃料的燃烧处于相对安全水平。基元反应敏感性分析表明:爆燃反应与H和OH自由基密切相关,而R1、R8、R24、R96是影响爆炸反应强度最重要的4个基元反应。研究成果可为C_(2)H_(5)OH/CH_(4)/H_(2)三元混合燃料在实际燃烧装置中的应用、燃料安全性评估以及爆炸事故预防提供参考。

关键词：乙醇/甲烷/氢气爆炸特性线性相关 H和OH自由基

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基于改进YOLOv5的红花目标检测算法研究

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农机化研究 2025年第1期47卷 26-32,66页

作者：陈金荣许燕周建平王小荣新疆大学机械工程学院乌鲁木齐830047 新疆大学工程训练中心乌鲁木齐830047 新疆维吾尔自治区农牧机器人及智能装备工程研究中心乌鲁木齐830047

为实现农业非结构环境下采摘机器人对红花的准确识别,提出了一种基于改进YOLOv5的红花目标检测算法。将CBAM注意力机制嵌入到YOLOv5网络,提高了小尺寸目标物在高层次特征中的表现力;建立一种Alpha-IoU目标位置损失函数对原损失函数GIOU... 详细信息

为实现农业非结构环境下采摘机器人对红花的准确识别,提出了一种基于改进YOLOv5的红花目标检测算法。将CBAM注意力机制嵌入到YOLOv5网络,提高了小尺寸目标物在高层次特征中的表现力;建立一种Alpha-IoU目标位置损失函数对原损失函数GIOU存在的梯度消失问题进行改进,提高了被遮挡红花的预测率,并通过在目标检测网络中增加分割检测模块,提高宽和高小于最低像素的小目标物检测精度,利用图像扩增数据集对改进后的YOLOv5算法进行训练,再分别与改进前后YOLOv5网络和Faster R-CNN网络在不同红花品种、不同自然光照情况、不同天气条件和不同遮挡情况下进行对比。试验结果表明:改进后的YOLOv5算法P值、R值分别为90.45%和0.90,对非结构环境下盛开期的未采摘红花mAP值达到94.48%,在不同影响因素下都可以准确识别出红花且置信度较高,可为红花采摘机器人自动化作业中的红花识别提供技术支持。

关键词：红花目标检测改进YOLOv5 数据增强非结构环境

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深度学习方法在红花采摘机器人中的应用

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农机化研究 2025年第4期47卷 186-191页

作者：陈金荣许燕周建平王小荣崔超新疆大学机械工程学院乌鲁木齐830047 新疆维吾尔自治区农牧机器人及智能装备工程研究中心乌鲁木齐830047 新疆大学工程训练中心乌鲁木齐830047

为实现农业复杂环境中红花的快速准确识别,提出了一种基于深度学习方法的改进YOLOv5s红花目标检测算法。在YOLOv5s基础上融入适配GPU的轻量Ghost模块,获得复杂度更低、网络推理速度更快的基线模型,将CBAM注意力机制嵌入基线模型,增强了... 详细信息

为实现农业复杂环境中红花的快速准确识别,提出了一种基于深度学习方法的改进YOLOv5s红花目标检测算法。在YOLOv5s基础上融入适配GPU的轻量Ghost模块,获得复杂度更低、网络推理速度更快的基线模型,将CBAM注意力机制嵌入基线模型,增强了小目标物在高频特征中的表现力,并通过建立一种基于边界框宽和高差值的Focal-EIoU损失函数,提高红花在不同遮挡情况下的识别率。最后,在并联式红花采摘机器人上开展红花识别试验,验证改进算法的可行性和可靠性。结果表明:改进后的YOLOv5s模型相较于原始模型在mAP值上提高了1.94个百分点,模型参数量和单幅图像检测速度分别为3.52 MB和0.06 s/幅,红花采摘机器人视觉系统的平均识别成功率可达89.92%。

关键词：红花采摘机器人深度学习 YOLOv5s 识别成功率

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C30F12.4 influences oogenesis, fat metabolism, and lifespan in C. elegans

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Protein & Cell 2016年第10期7卷 714-721页

作者： Lu wang Fei Xu Guishuan wang xiaorong wang Ajuan Liang Hefeng Huang Fei Sun International Peace Maternity & Child Health Hospital Shanghai Key laboratory for Reproductive Medicine School of Medicine Institute of Embryo-Fetal Original Adult Disease Shanghai Jiaotong University Shanghai 200030 China School of Life Sciences University of Science and Technology of China Hefei 230026 China

Reproduction, fat metabolism, and longevity are inter- twined regulatory axes; recent studies in C. elegans have provided evidence that these processes are directly coupled. However, the mechanisms by which they are coupled and the reproductive signals modu- lating fat metabolism and lifaspan are poorly under- stood. Here, we find that an oogenesis-enriched gene, c30PI2.4, is specifically expressed and located in germ cells and early embryos; when the gene is knocked out, oogenesis is disrupted and brood size is decreased. In addition to the reproductive phenotype, we find that the loss of c30f12.4 alters fat metabolism, resulting in decreased fat storage and smaller lipid droplets. Mean- while, c30f12.4 mutant worms display a shortened lifaspan. Our results highlight an important role for c30f12.4 in regulating reproduction, fat homeostasis, and aging in C. elegans, which helps us to better understand the relationship between these processes.

关键词： C30F12.4 oogenesis fat metabolism,lifespan

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Effects of environmental factors on the production and release of matrix-bound phosphine from lake sediments

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Frontiers of Environmental Science & Engineering 2007年第1期1卷 120-124页

作者： GENG Jinju wang Qiang NIU Xiaojun wang xiaorong State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentNanjing UniversityNanjing 210093China South China University of Technology School of Environmental Science and EngineeringGuangzhou 510641China

Effects of pH,temperature,and oxygen on the production and release of phosphine in eutrophic lake sedi-ments were investigated under laboratory *** indi-cated that the elimination of matrix-bound phosphine was accelerated under initial pH 1 or *** levels could reach maximum under initial pH *** contents of phos-phine increased with the addition of alkali under pH *** rates of phosphine production and release from lake sed-iments varied with temperature.20°C was the most favorable temperature for the production of matrix-bound *** showed little effect on matrix-bound ***-bound phosphine concentrations in lake sediments were concluded to be dependent on a balance of natural generation and depletion processes.

关键词： phosphine production release lake sediments environmental factors

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Toxicological effects involved in risk assessment of rare earth lanthanum on roots of Vicia faba ***

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Journal of Environmental Sciences 2011年第10期23卷 1721-1728页

作者： Chengrun wang Mei He Wen Shi Jessie Wong Tao Cheng xiaorong wang Lingling Hu Fenfen Chen School of Life Science Huainan Normal University Huainan 232001 China State Key Laboratory of Pollution Control and Resources Reuse School of the Environment Nanjing University Nanjing 210046 China Department of Chemical and Biochemical Engineering University of Western Ontario London ON N6A5B9 Canada Department of Biology University of Western Ontario London ON N6A5B9 Canada

Combined chemical analyses and biological measurements were utilized to investigate potential toxicological effects and possible mechanisms involved in risk assessment of rare earth elements （REEs） on Viciafaba L. seedlings, which were hydroponically cultivated and exposed to various concentrations of lanthanum （La） for 15 days. The results showed that La contents in both the solution and roots increased with the increase of extraneous La, contributing to hormetic dose responses of superoxide dismutase （SOD）, catalase （CAT）, guaiacol peroxidase （GPX）, ascorbate peroxidase （APX） and endoprotease （EP） isozymes activities, and HSP 70 production enhanced at low doses but suppressed at higher doses of La. These physiological responses constituted antioxidant and detoxification systems against La-induced oxidative stress. The elevated La levels also contributed to oxidatively modified proteins, which were most responsible for subsequent cell death and growth retardation of the roots. By combination of hormetic and traditional threshold dose levels, the threshold dose range was deduced to be 108-195 μg La/g dry weight in the roots, corresponding to 0.90-3.12 mg/L of soluble La in the culture solution. It suggests that persistent applications of REEs may lead to potential ecological risk in the environment.

关键词： rare earth elements lanthanum heat shock protein 70 oxidatively modified proteins isoenzymes hormesis riskassessment

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MODEL AND PERFORMANCE ANALYSIS OF FMT SYSTEM AND ORTHOGONAL FILTERBANKS

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Journal of Electronics(China) 2009年第1期26卷 80-87页

作者： Xu xiaorong Zheng Baoyu wang Lei Institute of Signal Processing and Transmission Nanjing University of Posts and Telecommunications Nanjing 210003 China

An orthogonal multi-carrier modulation-Filtered Multi-Tone (FMT) modulation, is evaluated in this paper. The objective of this paper is to model the FMT system with polyphase fil- terbank network, design its synthesis/analysis orthogonal filterbanks and analyze their performance. Oversampled and critically sampled cases of FMT system are discussed in detail. Perfect Reconstruc- tion (PR) properties of M parallel orthogonal subchannels in the case of critically sampled is derived from filterbank polyphase decomposition. Diverse types of prototype filters which include Infinite Impulse Response (IIR) and Finite Impulse Response (FIR) are designed and analyzed. Performance analysis of orthogonal filterbanks which are implemented by these prototype filters are proposed and compared respectively. Simulation results of FMT orthogonal filterbanks are presented. In the end, the application prospect of FMT is discussed.

关键词： Filtered Multi-Tone (FMT) System modeling Orthogonal filterbanks Prototype filter Performance analysis

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Ethanol Evaporation Characteristics of the Blends of Fatty Acid Methyl Ester and Ethanol

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Journal of Shanghai Jiaotong university(Science) 2021年第2期26卷 210-217页

作者： wang xiaorong wang Gang wang Lihui ZHANG Jie YAN Jun School of Mechanical Engineering Jiangsu University of Science and TechnologyZhenjiang 212100JiangsuChina

The evaporation characteristics of fatty acid methyl ester(FAME)mixed with four concentrations of ethanol at 873 K and normal atmospheric pressure are studied *** is used as base oils,and et hanol mass fractions vary from 10%,20%,30%to 40%。The experimental results show that the evaporation process of the binary component droplets of FAME-ethanol can be divided into two stages:a fuctuation evaporation stage,and an equilibrium evaporation *** these four concentration gradients,micro-explosions occur in the droplet evaporation *** fuctuation evaporation stage is divided into two stages:a strong fuctuation stage and a weak fluctuation *** the micro-explosion,there is still a small amount of ethanol in the *** to the surface tension of the droplet,a small amount of ethanol cannot make the droplet violently *** results show that the earlier the droplet micro-explosion occurs,the more intense it is,and the shorter the lifetime of the droplet *** concentrations of ethanol have different improvements in droplet evaporation ***,the higher the ethanol concentration is,the shorter the lifetime of the droplet ***,increasing the ethanol concentration from 20%to 30%has the most obvious effect on the lifetime of the droplet.

关键词： ethanol micro-explosion fatty acid methyl ester(FAME) fluctuation evaporation stage equilibrium evaporation stage

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Production and emission of phosphine gas from wetland ecosystems

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Journal of Environmental Sciences 2010年第9期22卷 1309-1311页

作者： Chao Han Xueyuan Gu Jinju Geng Yuning Hong Rui Zhang xiaorong wang Shixiang Gao State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing 210093 China School of Chemistry and Environmental Science Nanjing Normal University Nanjing 210097 China

Phosphine is a part of an atmospheric link of phosphorus cycle on earth, which could be an important pathway for phosphorus transport in environment. Wetland ecosystems are important locations for global biogeochemical phosphorus cycle. In this study, production and emission fluxes of free phosphine from four wetlands types in southern China were observed in different seasons. The results showed that the concentration of phosphine liberated from wetlands was at pg/m^3·ng/m^3 level. The emission concentrations of different wetlands followed the sequence： paddy field （51.83 ± 3.06） ng/m^3 〉/marsh （46.54 ± 20.55） ng/m^3 〉 lake （37.05 ± 22.74） ng/m^3 〉〉 coastal wetland （1.71 ± 0.73） ng/m^3, the positive phosphine emission flux occurred in rice paddy field （6.67 ± 5.18） ng/（m^***） and marsh （6.23 ± 26.9） ng/（m^***）, while a negative phosphine flux of （-13.11 ± 35.04） ng/（m^***） was observed on the water-air interface of Lake Taihu, suggesting that paddy field and marsh may be important sources for phosphine gas in atmosphere, while lake may be a sink of atmospheric phosphine gas during the sampling period. Atmospheric phosphine levels and emission flux from Yancheng marsh and rice paddy field varied in different seasons and vegetational zones. Both diffusion resistance in aqueous phase and temperature were dominating factors for the production and transportation of phosphine to atmosphere.

关键词： phosphine flux wetland ecosystems

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