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A facile strategy to construct MOF-based nanocatalyst with enhanced activity and selectivity in oxytetracycline degradation

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Nano Research 2024年第7期17卷 5863-5871页

作者： Yanjing Ke Jiaxing Zhang xin Peng Zhiyi Zhang xu Wang Wei Qi Mengfan Wang School of Life Sciences Faculty of MedicineSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China The Co-Innovation Centre of Chemistry and Chemical Engineering of Tianjin Tianjin 300072China Tianjin Key Laboratory of Membrane Science and Desalination Technology Tianjin 300350China

Recently,many efforts have been dedicated to construct artificial catalysts with enzyme-like ***,it is still a big challenge to endow artificial catalysts with specific substrate *** this study,we developed a facile strategy to construct a MIL-53(Fe)-based nanocatalyst with designable selectivity in the degradation of oxytetracycline(OTC).Through the Fe–O–P conjunction,oxytetracycline aptamer(OA)can be easily anchored on MIL-53(Fe)to provide the specific site for OTC *** verified that the obtained MIL-53(Fe)-Apt nanocatalyst displayed enhanced catalytic ability in the degradation of OTC,whereas obvious suppression toward other substrate *** performance therefore brings about an anticipated selectivity toward ***,we highlighted that the configuration of aptamers on MIL-53(Fe)can be modulated through varying conjunction ***–function analysis revealed that aptamer configuration affects the local concentration of substrate around catalytic site,which thus decides the catalytic performance toward *** work presented a facile and promising strategy for developing artificial catalysts with designable selectivity.

关键词： MIL-53(Fe) aptamer Fe-O-P catalytic selectivity oxytetracycline

Identification and effective regulation of scarb1 gene involved in pigmentation change in autotetraploid Carassius auratus

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Zoological Research 2024年第2期45卷 381-397页

作者： Xi-Dan xu Yue Zhou Chong-Qing Wang xu Huang Kun Zhang Xiao-Wei xu Li-Wen He xin-Yue Zhang xin-Zhu Fu Ming Ma Qin-Bo Qin Shao-Jun Liu State Key Laboratory of Developmental Biology of Freshwater Fish Engineering Research Center of Polyploid Fish Reproduction and Breeding of the State Education MinistryCollege of Life SciencesHunan Normal UniversityChangshaHunan 410081China Nansha-South China Agricultural University Fishery Research Institute GuangzhouGuangdong 511458China Hunan Yuelu Mountain Science and Technology Co.Ltd.for Aquatic Breeding ChangshaHunan 410081China College of Chemistry and Chemical Engineering Hunan Normal UniversityChangshaHunan 410081China

The autotetraploid Carassius auratus(4nRR,4n=200,RRRR)is derived from whole-genome duplication of Carassius auratus red var.(RCC,2n=100,RR).In the current study,we demonstrated that chromatophores and pigment changes directly caused the coloration and variation of 4nRR skin(red in RCC,brownish-yellow in4nRR).To further explore the molecular mechanisms underlying coloration formation and variation in 4nRR,we performed transcriptome profiling and molecular functional verification in RCC and *** revealed that scarb1,associated with carotenoid metabolism,underwent significant down-regulation in *** editing of this candidate pigment gene provided clear evidence of its significant role in RCC ***,we identified four divergent scarb1 homeologs in 4nRR:two original scarb1 homeologs from RCC and two duplicated ***,three of these homeologs possessed two highly conserved alleles,exhibiting biased and allelespecific expression in the ***,after precise editing of both the original and duplicated scarb1homeologs and/or alleles,4nRR individuals,whether singly or multiply mutated,displayed a transition from brownishyellow skin to a cyan-gray ***,the proportional areas of the cyan-gray regions displayed a gene-dose *** findings illustrate the subfunctionalization of duplicated scarb1,with all scarb1genes synergistically and equally contributing to the pigmentation of *** is the first report concerning the functional differentiation of duplicated homeologs in an autopolyploidfish,substantiallyenrichingour understanding of coloration formation and change within this group of organisms.

关键词： Autopolyploidization Coloration change scarb1 Functional differentiation Genetic changes

Oligopeptide Self-Assembly:Mechanisms,Stimuli-Responsiveness,and Biomedical Applications

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CCS Chemistry 2024年第1期6卷 69-90页

作者： Lei Ge Hanyan xu xin Jiang Jing Yu School of Materials Science and Engineering Nanyang Technological UniversitySingapore 637553 Institute for Digital Molecular Analytics and Science Nanyang Technological UniversitySingapore 637553

Oligopeptide self-assembly materials have emerged as a promising class of biomaterials with diverse applications in *** review highlights the recent progress in comprehending the selfassembly mechanisms intrinsic to oligopeptides and their behavior in response to specific *** methodically structuring the amino acid sequence and managing external stimuli such as pH levels,redox conditions,or enzymatic activity,we can exercise unprecedented control over the self-assembly *** controlling the self-assembly process of oligopeptides,various structures with extraordinary versatility can be obtained,including micelles,nanofibers,and coacervate droplets,each possessing modifiable mechanical and chemical ***,these self-assembled constructs demonstrate immense potential within varied biomedical *** stimuli-sensitive nature of oligopeptide assembly materials facilitates timely encapsulation and release of therapeutic cargos,consequently eliciting desired cellular *** approach paves the way for more precise tumor targeting,personalized medicinal treatments,and well-regulated drug *** innate biocompatibility and proficiency in replicating the extracellular matrix(ECM)render them ideally suited for applications such as tissue engineering,wound remediation,and regenerative *** summary,oligopeptide self-assembling materials show tremendous potential as adaptable platforms for cutting-edge biomedical applications,thereby bridging the divide between fundamental research and practical clinical application.

关键词： oligopeptides self-assembly nonequilibrium stimuli-responsive behavior biomedical applications

TP-PROFILE: Monitoring the Thermodynamic Structure of the Troposphere over the Third Pole

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Advances in Atmospheric Sciences 2024年第6期41卷 1264-1277页

作者： xuelong CHEN Yajing LIU Yaoming MA Weiqiang MA Xiangde xu xinghong CHENG Luhan LI xin xu Binbin WANG Land-Atmosphere Interaction and its Climatic Effects Group State Key Laboratory of Tibetan Plateau Earth SystemEnvironment and Resources(TPESER)Institute of Tibetan Plateau ResearchChinese Academy of SciencesBeijing 100101China College of Earth and Planetary Sciences University of Chinese Academy of SciencesBeijing 100049China National Observation and Research Station for Qomolongma Special Atmospheric Processes and Environmental Changes Dingri 858200China China-Pakistan Joint Research Center on Earth Sciences Chinese Academy of SciencesIslamabad 45320Pakistan College of Atmospheric Science Lanzhou UniversityLanzhou 730000China Kathmandu Center of Research and Education Chinese Academy of SciencesBeijing 100101China State Key Laboratory of Disastrous Weather China Academy of Meteorological SciencesBeijing 100081China

Ground-based microwave radiometers(MWRs)operating in the K-and V-bands(20–60 GHz)can help us obtain temperature and humidity profiles in the *** from some soundings from local meteorological observatories,the tropospheric atmosphere over the Tibetan Plateau(TP)has never been continuously *** part of the Chinese Second Tibetan Plateau Scientific Expedition and Research Program(STEP),the Tibetan Plateau Atmospheric Profile(TPPROFILE)project aims to construct a comprehensive MWR troposphere observation network to study the synoptic processes and environmental changes on the *** initiative has collected three years of data from the MWR *** paper introduces the data information,the data quality,and data *** applications of the data obtained from these MWRs were also *** comparisons of MWR against the nearest radiosonde observation demonstrate that the TP-PROFILE MWR system is adequate for monitoring the thermal and moisture variability of the troposphere over the *** continuous temperature and moisture profiles derived from the MWR data provide a unique perspective on the evolution of the thermodynamic structure associated with the heating of the *** TP-PROFILE project reveals that the low-temporal resolution instruments are prone to large uncertainties in their vapor estimation in the mountain valleys on the TP.

关键词： microwave radiometer thermodynamic structure vertical profile Tibetan Plateau

Precipitating thermally reinforcement phase in aluminum alloys for enhanced strength at 400℃

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Journal of Materials Science & Technology 2024年第5期172卷 71-82页

作者： Xiang Su Yuan Lei Yang Chen Hongjie Qu Zhixiang Qi Gong Zheng xu Liu Henggao Xiang guang Chen National Key Laboratory of Advanced Casting Technologies MIIT Key Laboratory of Advanced Metallic and Intermetallic Materials TechnologyEngineering Research Center of Materials Behavior and DesignMinistry of EducationNanjing University of Science and TechnologyNanjing 210094China School of Aviation and Mechanical Engineering Changzhou Institute of TechnologyChangzhou 213032China

Heat-resistant aluminum alloys are widely used in aerospace and automotive fields for manufacturing hot components due to their advantages in lightweight design and energy ***,the high-temperature strength of existing cast aluminum alloys is always limited to about 100 MPa at 350℃due to coarsening and transformation of strengthening ***,we reveal that the yield strength and ultimate tensile strength of the T6 state Al-8.4Cu-2.3Ce-1.0Mn-0.5Ni-0.2Zr alloy at 400◦C increase by 34%and 44%after re-aging at 300℃for 100 h,and its thermal strength exhibits distinguished ad-vantage over traditional heat-resistant aluminum *** enhanced elevated-temperature strength is attributed to the reprecipitation of the Ni-bearing T-Al_(20)Cu_(2)Mn_(3)phase,whose number density increases over one *** significant segregation of Ni,Ce,and Zr elements at the interfaces helps improve the thermal stability of the T *** thermostable T phase effectively strengthens the matrix by in-hibiting dislocation ***,a highly interconnected 3D intermetallic network along the grain boundaries can still remain after long-term re-aging at 300℃,which is conducive to imposing a drag on the grain boundaries at high *** finding offers a viable route for enhancing the elevated-temperature strength of heat-resistant aluminum alloys,which could provide expanded opportunities for higher-temperature applications.

关键词： Aluminum alloys Precipitation Thermally reinforcement phase Re-aging treatment High-temperature strength

Rotating Massive Strangeon Stars and X-Ray Plateau of Short GRBs

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Research in Astronomy and Astrophysics 2024年第3期24卷 47-57页

作者： Xi-Yan Yang Xiao-Yu Lai Wei-Wei Tan Ren-xin xu School of Physics and Optoelectronic Engineering Yangtze UniversityJingzhou 434023China Research Center for Astronomy Hubei University of EducationWuhan 4300205China Key Laboratory of Quark and Lepton Physics Central China Normal UniversityMinistry of EducationWuhan 430079China School of Physics Peking UniversityBeijing 100871China Kavli Institute for Astronomy and Astrophysics Peking UniversityBeijing 100871China

Strangeon stars,which are proposed to describe the nature of pulsar-like compact stars,have passed various observational *** maximum mass of a non-rotating strangeon star could be high,which implies that the remnants of binary strangeon star mergers could even be long-lived massive strangeon *** study rigidly rotating strangeon stars in the slowly rotating approximation,using the Lennard-Jones model for the equation of *** can significantly increase the maximum mass of strangeon stars with unchanged baryon numbers,enlarging the mass-range of long-lived strangeon *** spin-down after merger,the decrease of radius of the remnant will lead to the release of gravitational *** into account the efficiency of converting the gravitational energy luminosity to the observed X-ray luminosity,we find that the gravitational energy could provide an alternative energy source for the plateau emission of X-ray *** fitting results of X-ray plateau emission of some short gamma-ray bursts suggest that the magnetic dipole field strength of the remnants can be much smaller than that of expected when the plateau emission is powered only by spin-down luminosity of magnetars.

关键词： dense matter-(stars) pulsars general-(stars) gamma-ray burst general

Variability of urban fractional vegetation cover and its driving factors in 328 cities in China

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Science China Earth Sciences 2024年第2期67卷 466-482页

作者： Fei FENG xin YANG Baoquan JIA Xiaoting LI Xianwen LI Chengyang xu Kaicun WANG Research Centre of Urban Forestry Key Laboratory for Silviculture and Forest Ecosystem of State Forestry and Grassland AdministrationBeijing Forestry UniversityBeijing100083China State Key Laboratory of Earth Surface Processes and Resource Ecology Beijing Normal UniversityBeijing100875China Research Institute of Forestry Chinese Academy of ForestryBeijing100091China School of Architecture Tsinghua UniversityBeijing100084China College of Urban and Environmental Sciences Sino-French Institute for Earth System ScienceInstitute of Carbon NeutralityPeking UniversityBeijing100871China

Urban green space promotes the health of urban residents,enhances urban ecosystem biodiversity,mitigates environmental pollution,and attenuates urban heat island ***,urban vegetation cover is highly heterogeneous and difficult to *** this study,the variation of urban fractional vegetation cover(FVC)in 328 cities in China from 1990 to2022 was quantified based on Landsat satellite data at a 30-m *** was found that from 1990 to 2005,due to increases in building density and impervious surfaces in cities,the national mean urban vegetation cover decreased from 0.38 to ***2005,urban vegetation cover began to reverse,reaching 0.45 in *** increasing trend was most pronounced in newly built urban *** decrease in average urban vegetation cover before 2005 was mainly due to the expansion of low vegetation cover areas,while the increase in urban vegetation cover after 2005 manifested as the expansion of high vegetation cover *** reversal in the trend of urban vegetation cover change after 2004 is related to the gradual implementation of national policies requiring increased urban green space *** urban gross domestic product(GDP)showed the highest correlation with changes in urban vegetation *** large and medium-sized cities,the top three factors influencing vegetation cover were GDP,urban population,and ***,for cities in arid/semi-arid regions,changes in vegetation cover were more sensitive to climatic factors(such as precipitation).Although the urban vegetation cover in China has substantially increased in recent years,the urban green space in small-sized cities and in the old urban districts of large-sized cities still have room to improve.

关键词： Urban vegetation Urban vegetation cover Urbanization Remote sensing

Understanding Simulated Causes of Damaging Surface Winds in a Derecho-Producing Mesoscale Convective System near the East China Coast Based on Convection-Permitting Simulations

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Advances in Atmospheric Sciences 2024年第11期41卷 2112-2130页

作者： Liping LUO Ming xuE xin xu Lijuan LI Qiang ZHANG Ziqi FAN College of Civil Aviation Nanjing University of Aeronautics and AstronauticsNanjing 211106China State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Key Laboratory of Mesoscale Severe Weather/Ministry of Education and School of Atmospheric Sciences Nanjing UniversityNanjing 210023China Center for Analysis and Prediction of Storms and School of Meteorology University of OklahomaNormanOklahoma 73072USA Civil Aviation North China Air Traffic Management Bureau Meteorological Center Beijing 100621China

A mesoscale convective system(MCS) occurred over the East China coastal provinces and the East China Sea on 30April 2021, producing damaging surface winds near the coastal city Nantong with observed speeds reaching 45 m s^(–1). A simulation using the Weather Research and Forecasting model with a 1.5-km grid spacing generally reproduces the development and subsequent organization of this convective system into an MCS, with an eastward protruding bow segment over the sea. In the simulation, an east-west-oriented high wind swath is generated behind the gust front of the MCS. Descending dry rear-to-front inflows behind the bow and trailing gust front are found to feed the downdrafts in the main precipitation regions. The inflows help to establish spreading cold outflows and enhance the downdrafts through evaporative cooling. Meanwhile, front-to-rear inflows from the south are present, associated with severely rearward-tilted updrafts initially forming over the gust front. Such inflows descend behind(north of) the gust front, significantly enhancing downdrafts and near-surface winds within the cold pool. Consistently, calculated trajectories show that these parcels that contribute to the derecho originate primarily from the region ahead(south) of the east-west-oriented gust front, and dry southwesterly flows in the low-to-middle levels contribute to strong downdrafts within the MCS. Moreover, momentum budget analyses reveal that a large westward-directed horizontal pressure gradient force within the simulated cold pool produced rapid flow acceleration towards Nantong. The analyses enrich the understanding of damaging wind characteristics over coastal East China and will prove helpful to operational forecasters.

关键词： damaging surface winds convection-permitting simulations mesoscale convective system gust front cold pool

Production traits and fertility of reciprocal hybrids between Argopecten irradians irradians and ***

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Journal of Oceanology and Limnology 2024年第1期42卷 304-315页

作者： Jinjing WANG Junhao NING Xia LU Min CHEN Guilong LIU xin xu Quanchao WANG He xu Chunde WANG Research and Development Center for Efficient Utilization of Coastal Bioresources Yantai Institute of Coastal Zone ResearchChinese Academy of SciencesYantai 264003China College of Marine Science and Engineering Qingdao Agricultural UniversityQingdao 266109China University of Chinese Academy of Sciences Beijing 100049China Yantai Spring-Sea AquaSeed Co. Ltd.Yantai 264006China Jiangsu Baoyuan Biotechnology Co. Ltd.Lianyungang 222144China Jiangsu Haitai MariTech Co. Ltd.Lianyungang 222144China

The two bay scallop subspecies,Argopecten irradians irradians(NN)and ***(SS),are fast growing and major cultured bivalves in ***,their relatively small sizes and decreasing production traits caused by long-term inbreeding have been major concerns to the industry in the last two *** between the two bay scallop subspecies may provide a new approach to breed a new variety with superior production traits for the *** this end,in this study,we hybridized the two bay scallop subspecies in order to obtain a new strain that incorporates the genes of both *** significant difference was found in fertilization rate,hatching rate and metamorphosis rate between the purebred and crossbred cohorts(NN♀×SS♂,denoted as NS;SS♀×NN♂,denoted as SN).Both mating strategy(***-population crosses)and egg origin had significant effects on growth and survival at the larval *** was observed in the crossbred and was more pronounced in older *** diversity of the reciprocal hybrids,especially that of SN,was increased compared with the purebred *** all hybrids were completely fertile and able to reproduce by selffertilization or by backcrossing with either ***,male sterile individuals whose gonads were fully occupied by the ovary part at mature stage were found in the hybrids for the first *** hybrids,especially SN,may provide precious germplasm resources for the production of ternary hybrids with the Peruvian scallop,***.

关键词： bay scallop hybridization growth survival heterosis fertility ternary hybrids