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Scalable parallel ultrafast optical random bit generation based on a single chaotic microcomb

Light(Science & Applications) 2024年第4期13卷 637-644页

作者： Pu Li Qizhi Li Wenye Tang Weiqiang Wang wenfu zhang Brent ELittle Sai Tek Chu KAlan Shore Yuwen Qin Yuncai Wang Institute of Advanced Photonics Technology School of Information EngineeringGuangdong University of TechnologyGuangzhou 51006China. Key Laboratory of Photonic Technology for Integrated Sensing and Communication Ministry of Education of ChinaGuangdong University of TechnologyGuangzhou 51006China. Guangdong Provincial Key Laboratory of Information Photonics Technology Guangdong University of TechnologyGuangzhou 51006China. Key Laboratory of Advanced Transducers andIntelligent Control System Ministry of EducationTaiyuan University of TechnologyTaiyuan 030024China. State Key Laboratory of Transient Optics and Photonics Xi’an Institute of Optics and Precision MechanicsChinese Academy of SciencesXi’an 710119China. Department of Physics and Materials Science City University of Hong KongHong KongChina. School of Electronic Engineering Bangor UniversityBangorWales LL571UTUK

Random bit generators are critical for information security,cryptography,stochastic modeling,and simulations.Speed and scalability are key challenges faced by current physical random bit generation.Herein,we propose a massively parallel scheme for ultrafast random bit generation towards rates of order 100 terabit per second based on a single micro-ring resonator.A modulation-instability-driven chaotic comb in a micro-ring resonator enables the simultaneous generation of hundreds of independent and unbiased random bit streams.A proof-of-concept experiment demonstrates that using our method,random bit streams beyond 2 terabit per second can be successfully generated with only 7 comb lines.This bit rate can be easily enhanced by further increasing the number of comb lines used.Our approach provides a chip-scale solution to random bit generation for secure communication and high-performance computation,and offers superhigh speed and large scalability.

关键词： resonator random chaotic

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The structure-directing role of heterologous seeds in the synthesis of zeolite

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Green Energy & Environment 2024年第5期9卷 792-801页

作者： Haoyang zhang Binyu Wang wenfu Yan State Key Laboratory of Inorganic Synthesis&Preparative Chemistry College of ChemistryJilin UniversityChangchun130012China

Zeolites have been widely used as catalysts,ion-exchangers,and adsorbents in chemical industries,detergent industry,steel industry,glass industry,ceramic industry,medical and healthﬁeld,and environmentalﬁeld,and recently applied in energy storage.Seed-assisted synthesis is a very effective approach in promoting the crystallization of zeolites.In some cases,the target zeolite cannot be formed in the absence of seed zeolite.In homologous seed-assisted synthesis,the structure of the seed zeolite is the same to that of the target zeolite,while the structure of the seed zeolite is different to that of the target zeolite in the heterologous seed-assisted synthesis.In this review,we brieﬂy summarized the heterologous seed-assisted syntheses of zeolites and analyzed the structure-directing effect of heterologous seeds and surveyed the“common composite building units(CBUs)hypothesis”and the“common secondary building units(SBUs)hypothesis”.However,both hypotheses cannot explain all observations on the heterologous seed-assisted syntheses.Finally,we proposed that the formation of the target zeolite does need nuclei with the structure of target zeolite and the formation of the nuclei of the target zeolite can be promoted by either the undissolved seed crystals with the same CBUs or SBUs to the target zeolite or by the facilitated appropriate distribution of the speciﬁc building units due to the presence of the heterologous seed that does not have any common CBUs and SBUs with the target zeolite.

关键词： Zeolite Heterologous seed Synthesis Structure-directing effect

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Mechanism of interfacial effects in sodium-ion storage devices

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Nano Research 2024年第3期17卷 1313-1326页

作者： Yifan Wei Lingxing Zan Huicong Xia wenfu Yan Jia-Nan zhang College of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China Key Laboratory of Advanced Energy Catalytic and Functional Material Preparation of Zhengzhou City Zhengzhou 450001China Key Laboratory of Chemical Reaction Engineering of Shaanxi Province College of Chemistry&Chemical EngineeringYan’an UniversityYan’an 716000China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry and College of Chemistry Jilin UniversityChangchun 130012China

Rechargeable sodium-ion batteries(SIBs)are considered as the next-generation secondary batteries.The performance of SIB is determined by the behavior of its electrode surface and the electrode–electrolyte interface during charging and discharging.Thus,the characteristics of these surfaces and interfaces should be analyzed to realize large-scale energy storage systems with high energy density and long-cycle stability.Although various studies have investigated the properties of electrode materials,few studies have focused on the construction of stable and efficient SIB interfaces,and even fewer have explored the mechanisms of interfacial effects;however,the strategies of regulating interfacial effects are yet to be completely developed.Moreover,the results obtained thus far are insufficient to draw systematic conclusions.The present study reviews the literature on the mechanism of interfacial effects in Na+storage devices.The interfaces in a sodium-ion storage device include a heterogeneous interface between electrode materials,a solid electrolyte interphase,and a cathode electrolyte interphase.The interfacial effects during the intercalation,transformation,and alloy reactions and the resulting overall battery performance were theoretically analyzed.In this review,we aim to provide a theoretical basis for optimizing the structures of electrode surface and electrode–electrolyte interface to optimize the performance of SIBs.In addition,the challenges of investigating interfacial effects and several possible helpful methods and opportunities for studying the mechanisms of interfacial effects in SIBs will be presented.

关键词： sodium-ion storage interfacial effects solid electrolyte interphase cathode electrolyte interphase

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Zeolite-confined Fe-site Catalysts for the Hydrogenation of CO_(2) to Produce High-value Chemicals

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Chemical Research in Chinese Universities 2024年第1期40卷 78-95页

作者： HAN Xiaoyang XIA Huicong TU Weifeng WEI Yifan XUE Dongping LI Minhan YAN wenfu zhang Jia-Nan HAN Yi-Fan College of Materials Science and Engineering Zhengzhou UniversityZhengzhou450001P.R.China State Key Laboratory of Coking Coal Resources Green Exploitation Zhengzhou UniversityZhengzhou450001P.R.China Engineering Research Center of Advanced Functional Material Manufacturing of Ministry of Education School of Chemical EngineeringZhengzhou UniversityZhengzhou450001P.R.China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry and College of Chemistry Jilin UniversityChangchun130012P.R.China State Key Laboratory of Chemical Engineering East China University of Science and TechnologyShanghai200237P.R.China

Zeolite-confined Fe-site catalysts(ZFCs)have emerged as superior materials for sustainably producing high-value chemicals through CO_(2) hydrogenation,owing to their adaptable framework,customizable composition,and thermal robustness.They excel in activating,adsorbing,and converting CO_(2) with remarkable efficiency and consistency in performance.This has sparked a surge in research interest in recent years.The review delves into the latest advancements in CO_(2) catalytic hydrogenation to olefins,alcohols,aromatics,and other liquid hydrocarbons,examining the synthesis,modification tactics,and the correlation between structure and performance across various ZFCs.Additionally,it underscores the pivotal factors affecting performance and sheds light on the mechanisms behind selectivity control in the CO_(2) hydrogenation process facilitated by ZFCs.To conclude,it presents pressing challenges and strategic recommendations to inspire the development of high-performance,durable ZFCs for CO_(2) hydrogenation applications.

关键词： Zeolite-confined Fe-site catalyst CO_(2) hydrogenation Modification strategy High-value chemical

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Ultra-high-linearity integrated lithium niobate electro-optic modulators

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Photonics Research 2022年第10期10卷 2366-2373页

作者： HANKE FENG KE zhang WENZHAO SUN YANGMING REN YIWEN zhang wenfu zhang CHENG WANG Department of Electrical Engineering&State Key Laboratory of Terahertz and Millimeter Waves City University of Hong KongKowloonHong KongChina State Key Laboratory of Transient Optics and Photonics Xi’an Institute of Optics and Precision MechanicsChinese Academy of SciencesXi’an 710119China University of Chinese Academy of Sciences Beijing 100049China

Integrated lithium niobate(LN)photonics is a promising platform for future chip-scale microwave photonics systems owing to its unique electro-optic properties,low optical loss,and excellent scalability.A key enabler for such systems is a highly linear electro-optic modulator that could faithfully convert analog electrical signals into optical signals.In this work,we demonstrate a monolithic integrated LN modulator with an ultra-high spurious-free dynamic range(SFDR)of 120.04 dB·Hz^(4/5)at 1 GHz,using a ring-assisted Mach–Zehnder interferometer configuration.The excellent synergy between the intrinsically linear electro-optic response of LN and an optimized linearization strategy allows us to fully suppress the cubic terms of third-order intermodulation distortions(IMD3)without active feedback controls,leading to∼20 dB improvement over previous results in the thin-film LN platform.Our ultra-high-linearity LN modulators could become a core building block for future large-scale functional microwave photonic integrated circuits by further integration with other high-performance components like low-loss delay lines,tunable filters,and phase shifters available on the LN platform.

关键词： modulator interferometer lithium

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圆孔工字型蜂窝梁扭转模态自由振动研究

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振动与冲击 2024年第6期43卷 329-335,344页

作者：黄斌张文福南京工程学院建筑工程学院南京211167

从能量等效角度,提出了一种圆孔工字型截面蜂窝梁连续型模型,应用新的薄壁构件扭转理论:板-梁理论,建立了构件扭转模态自由振动能量泛函模型,明确了圆孔工字型截面蜂窝梁名义约束扭转惯性矩(翘曲常数)、自由扭转常数、转动惯量。通过变... 详细信息

从能量等效角度,提出了一种圆孔工字型截面蜂窝梁连续型模型,应用新的薄壁构件扭转理论:板-梁理论,建立了构件扭转模态自由振动能量泛函模型,明确了圆孔工字型截面蜂窝梁名义约束扭转惯性矩(翘曲常数)、自由扭转常数、转动惯量。通过变分运算,获得了平衡微分方程模型。基于扭转模态试函数,推导了圆孔工字型截面蜂窝梁自由振动扭转模态振动圆频率,并与有限元结果对比校验理论模型预测精度。开展了悬臂圆孔工字型蜂窝梁受集中扭矩作用的端部截面转角理论分析与有限元计算,进一步检验了基于板-梁理论建立的蜂窝梁连续模型的适用性。应用板-梁理论对圆孔工字型截面蜂窝梁自由振动扭转的分析过程及推导步骤,为其他开孔类型工字型蜂窝梁扭转模态自由振动研究提供了直接参考。

关键词：圆孔工字型截面蜂窝梁扭转自由振动板-梁理论蜂窝梁连续型模型能量泛函模型

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Hyperbolic resonant radiation of concomitant microcombs induced by cross-phase modulation

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Photonics Research 2023年第6期11卷 1075-1084页

作者： YANG WANG WEIQIANG WANG ZHIZHOU LU XINYU WANG LONG HUANG BRENT ELITTLE SAI TCHU WEI ZHAO wenfu zhang State Key Laboratory of Transient Optics and Photonics Xi’an Institute of Optics and Precision MechanicsChinese Academy of SciencesXi’an 710119China University of Chinese Academy of Sciences Beijing 100049China Chongqing United Microelectronics Center(CUMEC) Chongqing 401332China Department of Physics and Materials Science City University of Hong KongHong KongChina

A high-quality optical microcavity can enhance optical nonlinear effects by resonant recirculation,which provides a reliable platform for nonlinear optics research.When a soliton microcomb and a probe optical field are coexisting in a micro-resonator,a concomitant microcomb(CMC)induced by cross-phase modulation(XPM)will be formed synchronously.Here,we characterize the CMC comprehensively in a micro-resonator through theory,numerical simulation,and experimental verification.It is found that the CMCs spectra are modulated due to resonant radiation(RR)resulting from the interaction of dispersion and XPM effects.The group velocity dispersion induces symmetric RRs on the CMC,which leads to a symmetric spectral envelope and a dual-peak pulse in frequency and temporal domains,respectively,while the group velocity mismatch breaks the symmetry of RRs and leads to asymmetric spectral and temporal profiles.When the group velocity is linearly varying with frequency,two RR frequencies are hyperbolically distributed about the pump,and the probe light acts as one of the asymptotic lines.Our results enrich the CMC dynamics and guide microcomb design and applications such as spectral extension and dark pulse generation.

关键词： resonant symmetric dispersion

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Scanning dual-microcomb spectroscopy

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Science China(Physics,Mechanics & Astronomy) 2022年第9期65卷 65-71页

作者： Yang Wang Zhichuang Wang Xinyu Wang Wen Shao Long Huang Bo Liang Brent ELittle Sai TChu Wei Zhao Weiqiang Wang wenfu zhang State Key Laboratory of Transient Optics and Photonics Xi’an Institute of Optics and Precision MechanicsChinese Academy of SciencesXi’an 710119China University of Chinese Academy of Sciences Beijing 100049China Department of Physics and Materials Science City University of Hong KongHong Kong 999077China

Dual-comb spectroscopy(DCS) is a powerful tool in molecular spectroscopy benefiting from the advantages of high resolution and short measurement time. The recently developed soliton microcomb(SMC) can potentially transfer the dual-comb method to an on-chip platform. In this paper, we demonstrate DCS using two frequency scanning SMCs, termed scanning dual-microcomb spectroscopy(SDMCS). The two SMCs are generated by an auxiliary-assisted thermal balance scheme, and the pump laser frequency sweeps over one free spectral range of the microresonator(~49 GHz) using a feedback control system. The proposed SDMCS has a spectral resolution of 12.5 MHz, which is determined by the minimum sweeping step of the pump laser. Using this SDMCS system, we perform three types of gas molecule absorption spectroscopy recognition and gas concentration detection.This study paves the way for integrated DCS with a high signal-to-noise ratio, high spectral resolution, and fast acquisition rate.

关键词： microresonator soliton microcomb dual-comb spectroscopy molecular spectroscopy gas sensing

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Advances in soliton microcomb generation

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Advanced Photonics 2020年第3期2卷 2-28页

作者： Weiqiang Wang Leiran Wang wenfu zhang Chinese Academy of Sciences Xi’an Institute of Optics and Precision MechanicsState Key Laboratory of Transient Optics and PhotonicsXi’anChina University of Chinese Academy of Sciences BeijingChina

Optical frequency combs,a revolutionary light source characterized by discrete and equally spaced frequencies,are usually regarded as a cornerstone for advanced frequency metrology,precision spectroscopy,high-speed communication,distance ranging,molecule detection,and many others.Due to the rapid development of micro/nanofabrication technology,breakthroughs in the quality factor of microresonators enable ultrahigh energy buildup inside cavities,which gives birth to microcavity-based frequency combs.In particular,the full coherent spectrum of the soliton microcomb(SMC)provides a route to low-noise ultrashort pulses with a repetition rate over two orders of magnitude higher than that of traditional mode-locking approaches.This enables lower power consumption and cost for a wide range of applications.This review summarizes recent achievements in SMCs,including the basic theory and physical model,as well as experimental techniques for single-soliton generation and various extraordinary soliton states(soliton crystals,Stokes solitons,breathers,molecules,cavity solitons,and dark solitons),with a perspective on their potential applications and remaining challenges.

关键词： optical frequency comb soliton microcomb microcavity photonic integration Kerr effect four-wave mixing

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Emerging material platforms for integrated microcavity photonics

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Science China(Physics,Mechanics & Astronomy) 2022年第10期65卷 10-28页

作者： Jin Liu Fang Bo Lin Chang Chun-Hua Dong Xin Ou Blake Regan Xiaoqin Shen Qinghai Song Baicheng Yao wenfu zhang Chang-Ling Zou Yun-Feng Xiao State Key Laboratory of Optoelectronic Materials and Technologies School of PhysicsSun Yat-sen UniversityGuangzhou 510000China MOE Key Laboratory of Weak-Light Nonlinear Photonics TEDA Institute of Applied Physics and School of PhysicsNankai UniversityTianjin 300071China State Key Laboratory of Advanced Optical Communications System and Networks School of ElectronicsPeking UniversityBeijing 100871China CAS Key Lab of Quantum Information University of Science and Technology of ChinaHefei 230026China State Key Laboratory of Functional Material for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China School of Mathematical and Physical Sciences University of Technology SydneyUltimo 2007Australia School of Physical Science and Technology ShanghaiTech UniversityShanghai 201210China Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information System Harbin Institute of TechnologyShenzhen 518055China Key Laboratory of Optical Fiber Sensing and Communications(Ministry of Education) University of Electronic Science and Technology of ChinaChengdu 611731China State Key Laboratory of Transient Optics and Photonics Xi’an Institute of Optics and Precision MechanicsChinese Academy of SciencesXi’an 710119China State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics School of PhysicsPeking UniversityBeijing 100871China

Many breakthroughs in technologies are closely associated with the deep understanding and development of new material platforms.As the main material used in microelectronics,Si also plays a leading role in the development of integrated photonics.The indirect bandgap,absence ofχ(2)nonlinearity and the parasitic nonlinear absorptions at the telecom band of Si imposed technological bottlenecks for further improving the performances and expanding the functionalities of Si microcavities in which the circulating light intensity is dramatically amplified.The past two decades have witnessed the burgeoning of the novel material platforms that are compatible with the complementary metal-oxide-semiconductor(COMS)process.In particular,the unprecedented optical properties of the emerging materials in the thin film form have resulted in revolutionary progress in microcavity photonics.In this review article,we summarize the recently developed material platforms for integrated photonics with the focus on chip-scale microcavity devices.The material characteristics,fabrication processes and device applications have been thoroughly discussed for the most widely used new material platforms.We also discuss open challenges and opportunities in microcavity photonics,such as heterogeneous integrated devices,and provide an outlook for the future development of integrated microcavities.

关键词： microcavity integrated optics nonlinear optics

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