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Light(Science & Applications) 2024年第4期13卷 738-746页

作者： Zongliang Xie zhu Mao Hailan Wang Yuxin Xiao Xiayu Zhang Tao Yu Zhongfu An wei Huang Frontiers Science Center for Flexible Electronics Xi’an Institute of Flexible Electronics&Xi’an Institute of Biomedical Materials and EngineeringNorthwestern Polytechnical University127 West Youyi RoadXi’an 710072China. Research&Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518100China. Shenzhen Institutes of Advanced Electronic Materials Shenzhen 518100China. Key Laboratory of Flexible Electronics&Institute of Advanced Materials Nanjing Tech University30 South Puzhu RoadNanjing 211816China

Organic mechanoluminescence materials,featuring dual emission and ultralong phosphorescence characteristics,exhibit significant potential for applications in real-time stress sensing,pressure-sensitive lighting,advanced security marking techniques,and material breakage ***,due to immature molecular design strategies and unclear luminescence mechanisms,these materials remain rarely *** this study,we propose a valuable molecular design strategy to achieve dual-channel *** introducing the arylphosphine oxide group into a highly twisted molecular framework,enhanced intra-and intermolecular interactions could be achieved within rigid structures,leading to dual-channel mechanoluminescence with greatly promoted ultralong *** investigations reveal the substantial boosting effect of intra-and intermolecular interactions on mechanoluminescence and ultralong phosphorescence properties by locking the highly twisted molecular *** work provides a concise and guiding route to develop novel smart responsive luminescence materials for widespread applications in material science.

关键词： channel luminescence locking

Pd/N-doped carbon dots@dendritic mesoporous silica nanospheres:A highly efficient catalyst for the hydrogenation of 4-nitrophenol

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Nano Research 2024年第9期17卷 7967-7974页

作者： weiruo Liu Yanbin zhu Jiwei Wang Haisong Feng Yunpu Zhai wei Li Dongyuan Zhao College of Chemistry Zhengzhou University100 Kexue AvenueZhengzhou 450001China Department of Chemistry Laboratory of Advanced MaterialsShanghai Key Laboratory of Molecular Catalysis and Innovative Materialsand State Key Laboratory of Molecular Engineering of PolymersFudan UniversityShanghai 200433China State Key Laboratory of Chemical Resource Engineering Beijing Advanced Innovation Center for Soft Matter Science and EngineeringBeijing University of Chemical TechnologyBeijing 100029China

Highly dispersed Pd/N-doped carbon dots(Pd/NCDs)were successfully immobilized in the mesoporous channels of amino-functionalized dendritic mesoporous silica nanospheres(NMS).The synthesized Pd/NCDs@NMS catalyst exhibits outstanding performance in the catalytic reduction of 4-nitrophenol(4-NP),achieving a turnover frequency of 1461.8 mol·molPd^(-1)·h^(-1),with the conversion rate remaining above 80%after 11 *** and density functional theory calculations reveal that the NCDs significantly affect the electronic structure of Pd nanoparticles,leading to changes in the energy barriers for the adsorption of 4-NP at the Pd sites and the conversion of 4-NP reaction intermediates,which is a key factor contributing to the catalytic *** study offers a new strategy for synthesizing carbon-dot-modified metal-based catalysts.

关键词： palladium nanoparticles nitrogen-doped carbon dots dendritic mesoporous silica catalytic hydrogenation 4-nitrophenol reduction

Straw addition increases enzyme activities and microbial carbon metabolism activities in bauxite residue

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Journal of Environmental Sciences 2024年第1期135卷 332-344页

作者： Hao Wu wei Sun Feng zhu Yifan Jiang Shiwei Huang Johnvie Goloran Shengguo Xue School of Minerals Processing and Bioengineering Central South UniversityChangsha 410083China School of Metallurgy and Environment Central South UniversityChangsha 410083China School of Environment and Science Griffith UniversityBrisbaneQLD 4072Australia

Recovery of microbial functions is one of the critical processes in the nutrient cycling of bauxite residue for improving *** is considered to be effective to increase microbial diversity and drive the development of the microbial community,but its effect on microbial carbon metabolism has not been *** present study evaluated the effects of phosphogypsum(PG),straw(SF)and phosphogypsum plus straw(PGSF)on physicochemical properties,enzyme activities,and microbial carbon metabolism activities in bauxite *** 180 days incubation,PG,SF and PGSF treatment significantly reduced the residue pH from 10.85 to 8.64,9.39 and 8.06,*** to CK treatment,SF treatment significantly increased the content of total organic carbon(TOC)and organic carbon fractions(DOC,MBC,EOC,and POC).In addition,straw addition significantly increased glucosidase,cellulose,urease,and alkaline phosphatase by 7.2-9.1 times,5.8-7.1 times,11.1-12.5 times,and 1.1-2.2 times,*** Biolog results showed that straw addition significantly increased microbial metabolic activity(AWCD)and diversity in bauxite *** analysis indicated total nitrogen(TN)and carbon fractions(POC,MBC and DOC)were the most important environmental factors affecting microbial metabolic activity and diversity in bauxite *** findings provided us with a biogeochemical perspective to reveal soil formation in bauxite residue and suggested that nutrient supplement and regulation of salinity-alkalinity benefit the establishment of microbial communities and functions in bauxite residue.

关键词： Bauxite residue Labile organic carbon fractions Enzyme activities Community-level physiological profiles Soil formation in bauxite residue

Well-controlled Organocatalytic Ring-opening Polymerization of Seven-membered Cyclic Carbonates with Cyclohexyl Fusion

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CHEMICAL RESEARCH IN CHINESE UNIVERSITIES 2024年第5期40卷 856-862页

作者： Zhang, wei Shan, Si-Yi Dai, Jiang Cai, Zhongzheng zhu, Jian-Bo Tianjin Univ Sci & Technol Coll Chem Engn & Mat Sci Tianjin Key Lab Brine Chem Engn & Resource Ecoutil Tianjin 300457 Peoples R China Sichuan Univ Coll Chem Natl Engn Lab Ecofriendly Polymer Mat Sichuan Chengdu 610064 Peoples R China

Developing green and well-controlled polymerization methods is of great significance for the preparation of biomedical polymer materials. In this contribution, an efficient organocatalytic ring-opening polymerization (ROP) of a class of seven-membered cyclic carbonates (T6DO, T6HDO, C6DO, C6HDO) containing cis- or trans-cyclohexane structure was established. Organic catalyst 1,5,7-triazabicyclo[4.4.0]dec-5-ene (TBD) promoted living polymerization of these cyclic carbonates to deliver polycarbonate and block copolymer products with predictable molecular weights and narrow dispersity. The robust TBD-mediated ROP at 90 degrees C showcased turnover frequency (TOF) up to 10(3) h(-1). The resulting amorphous polycarbonates displayed good thermal stability.

关键词： CO2 Organic catalyst Living ring-opening polymerization Aliphatic polycarbonate KINETIC RESOLUTION POLYMERIZATION RAC-LACTIDE

The Astrometric Performance of the China Space Station Telescope(CSST)Sky Survey in Extending the Gaia Celestial Reference Frame

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Research in Astronomy and Astrophysics 2024年第8期24卷 133-140页

作者： Jun Yao Jia-Cheng Liu Niu Liu Zi zhu Zhen-wei Wang School of Astronomy and Space Science Key Laboratory of Modern Astronomy and Astrophysics(Ministry of Education)Nanjing UniversityNanjing 210023China University of Chinese Academy of Sciences Nanjing 211135China

The multi-color imaging sky survey conducted by the China Space Station Telescope(CSST)holds significant promise for advancing the development of the celestial reference *** this study,we focus on assessing the astrometric performance of the CSST celestial reference frame(CSST-CRF)in extending the Gaia Celestial Reference Frame 3(Gaia-CRF3).First,the orientation precision of the CSST reference frame is evaluated using a simulated set of extragalactic sources with CSST g magnitudes ranging from 18 to 25 *** estimated orientation uncertainty caused by random error insignificantly affects the alignment between Gaia-CRF3 and the ***,the systematic effect of incomplete CSST sky coverage on the alignment between CSST-CRF and Gaia-CRF3 is discussed by analyzing the differences between the subset of Gaia-CRF3 in the CSST observation region(Gaia-CRF3′)and Gaia-CRF3 as a *** the third International Celestial Reference Frame(ICRF3)S/X band as an intermediate reference frame,the orientation offset between Gaia-CRF3′and GaiaCRF3 is estimated to be 20μ*** offset is marginally larger than the orientation offset between Gaia-CRF3 and the ICRF3,approximately 15μ*** residual spin and glide rate of Gaia-CRF3′are derived from the proper motions,consistent with that of Gaia-CRF3 within the formal ***,we explore the role of CSST in establishing a multi-band celestial reference frame by comparing its limiting magnitude and observation accuracy with existing catalogs in the infrared and ultraviolet *** to its broad wavelength coverage and highprecision measurements,CSST is well-positioned to make significant contributions to the development of a multiband celestial reference frame.

关键词： astrometry-reference systems-surveys

Potential clinical application of microRNAs in bladder cancer

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Journal of Biomedical Research 2024年第4期38卷 289-306页

作者： Pei Wang Xiaowei wei Xiaojun Qu Yefei zhu Laboratory Medicine Center the Second Affiliated Hospital of Nanjing Medical UniversityNanjingJiangsu 210011China School of Biological Science and Medical Engineering Southeast UniversityNanjingJiangsu 210096China

Bladder cancer(BC)is the tenth most prevalent malignancy globally,presenting significant clinical and societal challenges because of its high incidence,rapid progression,and frequent ***,cystoscopy and urine cytology serve as the established diagnostic methods for ***,their efficacy is limited by their invasive nature and low ***,the development of highly specific biomarkers and effective noninvasive detection strategies is imperative for achieving a precise and timely diagnosis of BC,as well as for facilitating an optimal tumor treatment and an improved ***(miRNAs),short noncoding RNA molecules spanning around 20–25 nucleotides,are implicated in the regulation of diverse carcinogenic *** altered miRNAs form robust functional regulatory networks that exert a notable influence on the tumorigenesis and progression of *** into aberrant miRNAs derived from blood,urine,or extracellular vesicles indicate their potential roles as diagnostic biomarkers and prognostic indicators in BC,enabling miRNAs to monitor the progression and predict the recurrence of the ***,the investigation centered on miRNA as a potential therapeutic agent presents a novel approach for the treatment of *** review comprehensively analyzes biological roles of miRNAs in tumorigenesis and progression,and systematically summarizes their potential as diagnostic and prognostic biomarkers,as well as therapeutic targets for ***,we evaluate the progress made in laboratory techniques within this field and discuss the prospects.

关键词： bladder cancer microRNAs biomarker diagnosis detection method

A real-time calibration method based on time-to-digital converter for accelerator timing system

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Nuclear Science and Techniques 2024年第9期35卷 127-140页

作者： Qi-Hao Duan Liang Ge Yan-Hao Jia Jie-Yu zhu wei Zhang Institute of modern physics Chinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100049China

The high-intensity heavy-ion accelerator facility(HIAF)is a scientific research facility complex composed of multiple cas-cade accelerators of different types,which pose a scheduling problem for devices distributed over a certain range of 2 km,involving over a hundred *** white rabbit,a technology-enhancing Gigabit Ethernet,has shown the capability of scheduling distributed timing devices but still faces the challenge of obtaining real-time synchronization calibration param-eters with high *** study presents a calibration system based on a time-to-digital converter implemented on an ARM-based System-on-Chip(SoC).The system consists of four multi-sample delay lines,a bubble-proof encoder,an edge controller for managing data from different channels,and a highly effective calibration module that benefits from the SoC *** performance was evaluated with an average RMS precision of 5.51 ps by measuring the time intervals from 0 to 24,000 ps with 120,000 data for every *** design presented in this study refines the calibration precision of the HIAF timing *** eliminates the errors caused by manual calibration without efficiency loss and provides data support for fault *** can also be easily tailored or ported to other devices for specific applications and provides more space for developing timing systems for particle accelerators,such as white rabbits on HIAF.

关键词： HIAF White rabbit Calibration system Time-to-digital converter(TDC)

Efficient conversion of acoustic vortex using extremely anisotropic metasurface

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Frontiers of physics 2024年第4期19卷 257-264页

作者： Zhanlei Hao Haojie Chen Yuhang Yin Cheng-wei Qiu Shan zhu Huanyang Chen Institute of Electromagnetics and Acoustics and Department of Physics College of Physical Science and TechnologyXiamen UniversityXiamen 361005China Department of Electrical and Computer Engineering National University of Singapore4 Engineering Drive 3117583Singapore Department of Mechanical and Electrical Engineering Xiamen UniversityXiamen 361005China Pen-Tung Sah Institute of Micro-Nano Science and Technology Xiamen UniversityXiamen 361005China

Vortex wave and plane wave,as two most fundamental forms of wave propagation,are widely applied in various research ***,there is currently a lack of basic mechanism to enable arbitrary conversion between *** this paper,we propose a new paradigm of extremely anisotropic acoustic metasurface(AM)to achieve the efficient conversion from 2D vortex waves with arbitrary orbital angular momentum(OAM)to plane *** underlying physics of this conversion process is ensured by the symmetry shift of AM medium parameters and the directional compensation of ***,this novel phenomenon is further verified by analytical calculations,numerical demonstrations,and acoustic experiments,and the deflection angle and direction of the converted plane waves are qualitatively and quantitatively confirmed by a simple *** work provides new possibilities for arbitrary manipulation of acoustic vortex,and holds potential applications in acoustic communication and OAM-based devices.

关键词： efficient wave conversion vortex wave plane wave orbital angular momentum acoustic metasurface

Timp1 Deletion Induces Anxiety-like Behavior in Mice

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Neuroscience Bulletin 2024年第6期40卷 732-742页

作者： Xiaotong Wang wei Zheng Ziyi zhu Biyu Xing weijie Yan Ke zhu Lingli Xiao Chaojuan Yang Mengping wei Lei Yang Zi-Bing Jin Xueyun Bi Chen Zhang State Key Laboratory of Neurology and Oncology Drug Development Nanjing210000China School of Basic Medical Sciences Wenzhou Medical UniversityWenzhou325035China School of Basic Medical Sciences Beijing Key Laboratory of Neural Regeneration and RepairAdvanced Innovation Center for Human Brain ProtectionBeijing Laboratory of Oral HealthCapital Medical UniversityBeijing100069China Beijing Institute of Ophthalmology Beijing Tongren Eye CenterBeijing Tongren HospitalCapital Medical UniversityBeijing100005China Chinese Institute for Brain Research Beijing102206China Key Laboratory for Biomechanics and Mechanobiology of the Ministry of Education Beijing Advanced Innovation Center for Biomedical EngineeringSchool of Engineering MedicineBeihang UniversityBeijing100191China

The hippocampus is essential for learning and memory,but it also plays an important role in regulating emotional behavior,as hippocampal excitability and plasticity affect anxiety and *** synaptic plasticity may be regulated by tissue inhibitor of matrix metalloproteinase 1(TIMP1),a known protein inhibitor of extracellular matrix(ECM),and the expression of TIMP1 in the hippocampus can be induced by neuronal excitation and various ***,the involvement of Timp1 in fear learning,anxiety,and hippocampal synaptic function remains to be *** study of Timp1 function in vivo revealed that Timp1 knockout mice exhibit anxiety-like behavior but normal fear *** results suggested that Timp1 knockout mice showed hyperactivity in the ventral CA1 region,but the basic synaptic transmission and plasticity were normal in the Schaffer collateral *** together,our results suggest that deletion of Timp1 in vivo leads to the occurrence of anxiety behaviors,but that Timp1 is not crucial for fear learning.

关键词： Timp1 Anxiety Fear Synaptic transmission Synaptic plasticity

Deformation of Rigid Conjugate Self-dual Galois Representations

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Acta Mathematica Sinica,English Series 2024年第7期40卷 1599-1644页

作者： Yi Feng LIU Yi Chao TIAN Liang XIAO wei ZHANG Xin Wen zhu Institute for Advanced Study in Mathematics Zhejiang UniversityHangzhou 310058P.R.China Morningside Center of Mathematics AMSSChinese Academy of SciencesBeijing 100190P.R.China New Cornerstone Lab Beijing International Center for Mathematical ResearchPeking Ui Beijing 100871P.R.China Department of Mathematics Massachusetts Institute of TechnologyCambridge MA 02139United States Department of Mathematics Stanford UniversityStanfordCA 94305United States

In this article,we study deformations of conjugate self-dual Galois *** study is ***,we prove an R=T type theorem for a conjugate self-dual Galois representation with coefficients in a finite field,satisfying a certain property called ***,we study the rigidity property for the family of residue Galois representations attached to a symmetric power of an elliptic curve,as well as to a regular algebraic conjugate self-dual cuspidal representation.

关键词： Galois deformation rigid conjugate self-dual Galois representations