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Feasible synthesis of porous h-BN by Mg^(2+)induced lattice dislocations for hydrogen and ammonia storage

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Nano Research 2025年第1期18卷 94-99页

作者： xiaojia Huang Zihao wang Yihan Kong Li Jiang Baolin wang Jiangtao Jia Heping Ma Guangshan Zhu Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Northeast Normal UniversityChangchun 130024China School of Chemical Engineering and Technology Xi’an Jiaotong university Xi’an 710049China

Hexagonal boron nitride(h-BN)is a two-dimensional(2D)layered material with a structure similar to graphite and it has potential as a hydrogen and ammonia storage ***,dense packing in the standard h-BN structure limits its surface area and prevents the B and N from being adsorption *** this study,the addition of Mg^(2+)during h-BN synthesis facilitated the growth of lattice dislocations and led to a crosslinked three-dimensional(3D)porous structure.A proposed formation mechanism for porous h-BN was confirmed by several characterization routes,most clearly by high-resolution transmission electron microscopy(HRTEM).Porous Mg/BNs exhibited high H_(2)and NH_(3)uptakes and showed potential for H_(2)and NH_(3)storage.

关键词： hexagonal boron nitride porous material dislocation gas storage

高静压联合天然抑制剂处理对浑浊苹果汁多酚氧化酶活性及相关品质的影响

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食品科学 2025年第2期46卷 1-7页

作者：田学智曹智鸿江乃相肖志剑唐征王永涛中国农业大学食品科学与营养工程学院国家果蔬加工工程技术研究中心农业农村部果蔬加工重点实验室食品非热加工北京市重点实验室北京100083 山东泰乐源农业科技有限公司山东泰安271411

探究高静压(high hydrostatic pressure,HHP)联合阿魏酸(ferulic acid,FA)、表没食子儿茶素没食子酸酯(epigallocatechin gallate,EGCG)处理对浑浊苹果汁中多酚氧化酶(polyphenol oxidase,PPO)活性及相关品质的影响。结果表明,添加0.1 g/100 mL的FA或者0.2 g/100 mL的EGCG均能显著降低样品中PPO活性,并显著提高其亮度(P<0.05)。单独HHP处理(550 MPa、5 min)样品的PPO相对残余活性高达82.70%,而经过HHP+FA或HHP+EGCG处理后,样品的PPO相对残余活性分别降至66.35%和41.50%。在冷藏2周期间,样品的PPO活性持续下降,而颜色参数保持稳定。贮藏第14天,HHP+FA组的褐变指数最小,仅有4.37,而HHP+EGCG组的PPO相对残余活性最低(24.71%)。此外,两组样品都保留了80%以上的总酚和90%以上的抗氧化能力。综上,HHP与FA/EGCG的联合处理可以有效抑制浑浊苹果汁的酶促褐变,具有进一步推广应用的潜力。

关键词：高静压天然抑制剂浑浊苹果汁多酚氧化酶品质

Study of the seismic response of a recycled aggregate concrete frame structure

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Earthquake Engineering and Engineering Vibration 2013年第4期12卷 669-680页

作者： wang Changqing xiao Jianzhuang Department of Building Engineering Tongji University College of Civil Engineering and Architecture Nanyang Normal University State Key Lab.for Disaster Reduction in Civil Engineering Tongji University

Based on six-degree-of-freedom three-dimensional shaking table tests, the seismic response of a recycled aggregate concrete （RAC） frame was obtained. The analysis results indicate that the maximum story shear force and overturning moment reduce proportionally along the height of the model under the same earthquake wave. The story shear force, base shear coefficient and overturning moment of the structure increase progressively as the acceleration amplitude increases. The base shear coefficient is primarily controlled by the peak ground acceleration （PGA）. The relationships between the PGA and the shear coefficient as well as between the PGA and the dynamic amplification factor are obtained by mathematical fitting. The dynamic amplification factor decreases rapidly at the elastic-plastic stage, but decreases slowly with the development of the elastic-plasticity stage. The results show that the RAC frame structure has reasonable deformability when compared with natural aggregate concrete frame structures. The maximum inter-story drift ratios of the RAC frame model under frequent and rare intensity 8 test phases are 1/266 and 1/29, respectively, which are larger than the allowable value of 1/500 and 1/50 according to Chinese seismic design requirements. Nevertheless, the RAC frame structure does not collapse under base excitations with PGAs from 0.066 g up to 1.170 g.

关键词： recycled aggregate concrete (RAC) frame structure seismic response shear coefficient dynamicamplification factor

An improved multiple model GM-PHD filter for maneuvering target tracking

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Chinese Journal of Aeronautics 2013年第1期26卷 179-185页

作者： wang xiao Han Chongzhao The Flight Automatic Control Research Institute of AVIC School of Electronic and Information Engineering Xi'an Jiaotong University

In this paper, an improved implementation of multiple model Gaussian mixture probability hypothesis density （MM-GM-PHD） filter is proposed. For maneuvering target tracking, based on joint distribution, the existing MM-GM-PHD filter is relatively complex. To simplify the filter, model conditioned distribution and model probability are used in the improved MM-GM-PHD filter. In the algorithm, every Gaussian components describing existing, birth and spawned targets are estimated by multiple model method. The final results of the Gaussian components are the fusion of multiple model estimations. The algorithm does not need to compute the joint PHD distribution and has a simpler computation procedure. Compared with single model GM-PHD, the algorithm gives more accurate estimation on the number and state of the targets. Compared with the existing MM-GM-PHD algorithm, it saves computation time by more than 30%. Moreover, it also outperforms the interacting multiple model joint probabilistic data association （IMMJPDA） filter in a relatively dense clutter environment.

关键词： Estimation Gaussian mixture Maneuvering target racking Multiple model Probability hypothesis density

ultrafiltration with in-line coagulation for the removal of natural humic acid and membrane fouling mechanism

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Journal of Environmental Sciences 2006年第5期18卷 880-884页

作者： wang Jin wang xiao-chang Department of Municipal and Environmental Engineering Beijing Jiaotong University Beijing 100044 China School of Environmental and Municipal Engineering Xi＇an University of Architecture and Technology Xi＇an 710055 China

Experimental and theoretical analysis were made on the natural humic acid removal and the membrane fouling of ultrafiltration （uF） with in-line coagulation. The results showed dissolved organic carbon （DOC） and uV254 removals by the uF with in-line coagulation at pH 7 were increased from 28% to 53% and 40% to 78% in comparison with direct uF treatment respectively. At the same time, the analysis of high performance liquid chromatography showed that uF with coagulation had significant improvement of removal of humic acid with molecular weights less than 6000 Da in particular. Compared to direct uF, the in-line coagulation uF also kept more constant permeate flux and very slight increase oftransmembrane pressure during a filtration circle. Two typical membrane fouling models were used by inducing two coefficients Kc and Kp corresponding to cake filtration model and pore narrowing model respectively. It was found that membrane fouling by pore-narrowing effect was effectively alleviated and that by cake-filtration was much decreased by in-line coagulation. under the condition of coagulation prior to ultrafiltration at pH 7, the cake layer formed on the membrane surface became thicker, but the membrane filtration resistance was lower than that at pH 5 with the extension of operation time.

关键词： natural humic acid ultrafiltration (uF) in-line coagulation high performance liquid chromatography (HPLC) membrane fouling

Case-Based Reasoning(CBR) Model for ultra-Fast Cooling in Plate Mill

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Chinese Journal of Mechanical Engineering 2014年第6期27卷 1264-1271页

作者： Hu xiao wang Zhaodong wang Guodong State Key Laboratory of Rolling and Automation Northeastern University

New generation thermo-mechanical control process（TMCP） based on ultra-fast cooling is being widely adopted in plate mill to product high-performance steel material at low cost. ultra-fast cooling system is complex because of optimizing the temperature control error generated by heat transfer mathematical model and process parameters. In order to simplify the system and improve the temperature control precision in ultra-fast cooling process, several existing models of case-based reasoning（CBR） model are reviewed. Combining with ultra-fast cooling process, a developed R5 CBR model is proposed, which mainly improves the case representation, similarity relation and retrieval module. Certainty factor is defined in semantics memory unit of plate case which provides not only internal data reliability but also product performance reliability. Similarity relation is improved by defined power index similarity membership function. Retrieval process is simplified and retrieval efficiency is improved apparently by windmill retrieval algorithm. The proposed CBR model is used for predicting the case of cooling strategy and its capability is superior to traditional process model. In order to perform comprehensive investigations on ultra-fast cooling process, different steel plates are considered for the experiment. The validation experiment and industrial production of proposed CBR model are carried out, which demonstrated that finish cooling temperature（FCT） error is controlled within±25℃ and quality rate of product is more than 97%. The proposed CBR model can simplify ultra-fast cooling system and give quality performance for steel product.

关键词： ultra-fast cooling plate mill case-based reasoning case representation similarity relation retrieval module

Phase constitution of the noble metal thin-film complex solid solution system Ag-Ir-Pd-Pt-Ru in dependence of elemental compositions and annealing temperatures

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Nano Research 2022年第6期15卷 4827-4836页

作者： Bin xiao xiao wang Alan Savan Alfred Ludwig Materials Discovery and Interfaces Institute for MaterialsRuhr University Bochum44780 BochumGermany Zentrum für Grenzflächendominierte Höchstleistungswerkstoffe(ZGH) Ruhr University Bochum44780 BochumGermany

Multiple-principal element alloys hold great promise for multifunctional material discovery(e.g.,for novel electrocatalysts based on complex solid solutions)in a virtually unlimited compositional ***,the phase constitution of the noble metal system Ag-Ir-Pd-Pt-Ru was investigated over a large compositional range in the quinary composition space and for different annealing temperatures from 600 to 900°C using thin-film materials ***-dependent X-ray diffraction mapping of the asdeposited thin-film materials library indicates different phases being present across the composition space(face-centered cubic(fcc),hexagonal close packed(hcp)and mixed fcc+hcp),which are strongly dependent on the Ru *** general,low Ru contents promote the fcc phase,whereas high Ru contents favor the formation of an hcp solid-solution ***,a temperature-induced phase transformation study was carried out for a selected measurement area of fcc-Ag_(5)Ir_(8)Pd_(56)Pt_(8)Ru_(23).With increasing temperature,the initial fcc phase transforms to an intermediate C14-type Laves phase at 360°C,and then to hcp when the temperature reaches 510°*** formation and disappearance of the hexagonal Laves phase,which covers a wide temperature range,plays a crucial role of bridging the fcc to hcp phase *** obtained composition,phase and temperature data are transformed into phase maps which could be used to guide theoretical studies and lay a basis for tuning the functional properties of these materials.

关键词： noble metal high-entropy alloys phase transformation combinatorial synthesis and high-throughput characterization

Decentralized Optimal Control and Stabilization of Interconnected Systems With Asymmetric Information

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IEEE/CAA Journal of Automatica Sinica 2024年第3期11卷 698-707页

作者： Na wang xiao Liang Hongdan Li xiao Lu the College of Electrical Engineering and Automation Shandong University of Science and TechnologyQingdao 266000China the School of Automation and Electrical Engineering Linyi UniversityLinyi 276000China the College of Energy Storage Technology Shandong University of Science and TechnologyQingdao 266000China

The paper addresses the decentralized optimal control and stabilization problems for interconnected systems subject to asymmetric *** with previous work,a closed-loop optimal solution to the control problem and sufficient and necessary conditions for the stabilization problem of the interconnected systems are given for the first *** main challenge lies in three aspects:Firstly,the asymmetric information results in coupling between control and estimation and failure of the separation ***,two extra unknown variables are generated by asymmetric information(different information filtration)when solving forward-backward stochastic difference ***,the existence of additive noise makes the study of mean-square boundedness an *** adopted technique is proving and assuming the linear form of controllers and establishing the equivalence between the two systems with and without additive noise.A dual-motor parallel drive system is presented to demonstrate the validity of the proposed algorithm.

关键词： Asymmetric information decentralized control forwardbackward stochastic difference equations interconnected system stalibization

The codes of matter and their applications

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Science Bulletin 2015年第19期60卷 1661-1673页

作者： xiao-Lin wang Spintronic and Electronic Materials Group Institute for Superconducting and Electronic Materials Australia Institute for Innovative Materials University of Wollongong

The elements in the periodic table are the building blocks used to form substances with different compositions. Nevertheless, it is the properties of substances that are decisive for their existence and practical applications. Searching for new class of materials with exotic properties has always been challenging because of the complexity of both the theoretical and the experimental approaches developed so far. Here, we propose that the three ubiquitous and paramount attributes of all existing matter charge(Q), spin(S) or rotational motion, and linear motion(K) can be used to account for the formation of different types of matter/materials and their properties that have been or will be known to us. The three attributes or original codes can produce six primary codes which can further produce another sixty codes. The physical meanings represented by each code are unlocked. The table consisting of the 60 codes is introduced as the table of properties of codes of matter. We demonstrate that these codes can be used as building blocks to form new properties and new materials. Many new types of quasiparticles and new classes of materials with exotic properties of Q, S and K are predicted. Their possible experimental realizations are proposed. The possible applications of the codes of matter in other fields such as elementary particles, photonics and chemistry are briefly discussed. We know that there should be more new materials and new electronic, spin and photonic states to be discovered, but we do not know what they are. The codes of matter clearly reveal to us how many and what they are and how easily we can recognize what they are. Experimental and theoretical exploration for new forms of matter, new quasiparticles, or new electronic and spin states, or new states of photon or properties of light, as well as macroscopic entities with exotic properties represented by the codes of matter, is imminent.

关键词： New materials New electronic state New method Materials design