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Effect of hafnium and molybdenum addition on inclusion characteristics in Co-based dual-phase high-entropy alloys

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1639-1650页

作者： Yong wang Wei wang Joo Hyun Park wangzhong Mu Key Laboratory for Ferrous Metallurgy and Resources Utilization of Ministry of Education&Hubei Provincial Key Laboratory for New Processes of Ironmaking and Steelmaking Wuhan University of Science and TechnologyWuhan 430081China Department of Materials Science and Engineering KTH Royal Institute of TechnologySE-10044StockholmSweden Department of Chemical Engineering Northeast Electric Power UniversityJilin 132012China Department of Materials Science and Chemical Engineering Hanyang UniversityAnsan 15588Korea Engineering Materials Division of Materials ScienceDepartment of Engineering Science and MathematicsLuleå University of Technology97187 LuleåSweden

Specific grades of high-entropy alloys(HEAs)can provide opportunities for optimizing properties toward high-temperature *** this work,the Co-based HEA with a chemical composition of Co_(47.5)Cr_(30)Fe_(7.5)Mn_(7.5)Ni_(7.5)(at%)was *** refractory metallic elements hafnium(Hf)and molybdenum(Mo)were added in small amounts(1.5at%)because of their well-known positive effects on high-temperature *** characteristics were comprehensively explored by using a two-dimensional cross-sectional method and extracted by using a three-dimensional electrolytic extraction *** results revealed that the addition of Hf can reduce Al_(2)O_(3)inclusions and lead to the formation of more stable Hf-rich inclusions as the main *** addition cannot influence the inclusion type but could influence the inclusion characteristics by affecting the physical parameters of the HEA *** calculated coagulation coefficient and collision rate of Al_(2)O_(3)inclusions were higher than those of HfO_(2)inclusions,but the inclusion amount played a larger role in the agglomeration behavior of HfO_(2)and Al_(2)O_(3)*** impurity level and active elements in HEAs were the crucial factors affecting inclusion formation.

关键词： high-entropy alloy non-metallic inclusion agglomeration thermodynamics alloying

Superhydrophilic nickel hydroxide ultrathin nanosheets enable high-performance asymmetric supercapacitors

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Rare Metals 2024年第1期43卷 138-147页

作者： Yi-Ran wang Fei Zhang Jian-Min Gu Xiao-Yu Zhao Ran Zhao Xing wang Tian-Hui Wu Jing wang Ji-Dong wang De-Song wang State Key Laboratory of Metastable Materials Science and Technology(MMST) Hebei Key Laboratory of Applied ChemistryYanshan UniversityQinhuangdao 066004China Department of Food and Pharmaceutical Engineering Suihua UniversitySuihua 152000China School of Chemical Science and Engineering Tongji UniversityShanghai 200092China School of Sciences Hebei University of Science and TechnologyShijiazhuang 050018China

Superhydrophilic surfaces have been applied for supercapacitor;however,during energy storage reaction,how the wettability affects the process of electrochemical reaction specifically is still ***,we demonstrate superhydrophilic surface for promotion of electrochemical reactions by liquid affinity and further explain the mechanism,where the transition of the wettability state caused by the change in surface free energy is the main reason for the obvious increase in specific *** citric acid assistance strategy,an intrinsically hydrophobic Ni(OH)_(2)thick nanosheets(HNHTNs,16 nm)can be transitioned into superhydrophilic Ni(OH)_(2)ultrathin nanosheets(SNHUNs,6.8 nm),where the water contact angle was 0°and the surface free energy increased from 8.6to 65.8 mN·m^(-1),implying *** with HNHTNs,the specific capacitance of SNHUNs is doubled:from 1230 F·g^(-1)(HNHTNs)to 2350 F·g^(-1)(2A·g^(-1))and,even at 20 A·g^(-1),from 833 F·g^(-1)(HNHTNs)to 1670 F·g^(-1).The asymmetric capacitors assembled by SNHUNs and activated carbon show 52.44 Wh·kg^(-1)at 160W·kg^(-1)and excellent stability with~90%retention after5000 cycles(~80%retention after 9500 cycles).The promotion of electrochemical performances is ascribed to the change of surface wettability caused by surface free energy,which greatly increase affinity of electrode to the surrounding liquid environment to reduce the interface resistance and optimize the electron transport path.

关键词： Asymmetric supercapacitor Superhydrophilic interface Transition metal hydroxides Ultrathin nanosheets High specific capacitance

Broadening environmental research in the era of accurate protein structure determination and predictions

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Frontiers of Environmental Science & Engineering 2024年第7期18卷 169-178页

作者： Mingda Zhou Tong wang Ke Xu Han wang Zibin Li Wei-xian Zhang Yayi wang State Key Laboratory of Pollution Control and Resources Reuse Shanghai Institute of Pollution Control and Ecological SecurityCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China Translational Research Institute of Brain and Brain-Like Intelligence Shanghai Fourth People's HospitalSchool of MedicineTongji UniversityShanghai 200434China

The deep-learning protein structure prediction method AlphaFold2 has garnered enormous attention beyond the realm of structural biology,for its groundbreaking contribution to solving the"protein foiding problem"In this perspective,we explore the connection between protein structure studies and environmental research,delving into the potential for addressing specific environmental *** are promising for environmental applications because of the functional diversity endowed by their structural ***,structural studies on proteins with environmental significance remain ***,we present the opportunity to study proteins by advancing experimental determination and deep-learning prediction ***,the latest progress in environmental research via cryogenic electron microscopy is *** allows us to determine the structure of protein complexes in their native state within cells at molecular resolution,revealing environmentally-associated structural *** the remarkable advancements in computational power and experimental resolution,the study of protein structure and dynamics has reached unprecedented depth and *** advancements will undoubtedly accelerate the establishment of comprehensive environmental protein structural and functional *** opportunities for protein engineering exist to enable innovative solutions for environmental applications,such as the degradation of persistent contaminants,and the recovery of valuable metals as well as rare earth elements.

关键词： Environmental proteins Protein structure Cryogenic electron microscopy Protein structure prediction Protein engineering Artificial Intelligence

Computational Experiments for Complex Social Systems:Integrated Design of Experiment System

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IEEE/CAA Journal of Automatica Sinica 2024年第5期11卷 1175-1189页

作者： Xiao Xue Xiangning Yu Deyu Zhou Xiao wang Chongke Bi Shufang wang Fei-Yue wang College of Intelligence and Computing Tianjin UniversityTianjin 300350China School of Software Shandong UniversityJinan 250101China School of Artificial Intelligence Anhui UniversityHefei 230601China School of Geographic and Environmental Sciences Tianjin Normal UniversityTianjin 300387China Institute of Automation Chinese Academy of Sciences Beijing 100190China

Powered by advanced information industry and intelligent technology,more and more complex systems are exhibiting characteristics of the cyber-physical-social systems(CPSS).And human factors have become crucial in the operations of complex social *** mechanical analysis and social simulations alone are powerless for analyzing complex social *** this backdrop,computational experiments have emerged as a new method for quantitative analysis of complex social systems by combining social simulation(e.g.,ABM),complexity science,and domain ***,in the process of applying computational experiments,the construction of experiment system not only considers a large number of artificial society models,but also involves a large amount of data and *** a result,how to integrate various data,model and knowledge to achieve a running experiment system has become a key *** paper proposes an integrated design framework of computational experiment system,which is composed of four parts:generation of digital subject,generation of digital object,design of operation engine,and construction of experiment ***,this paper outlines a typical case study of coal mine emergency management to verify the validity of the proposed framework.

关键词： artificial system operations

Achieving exceptionally high strength and rapid degradation rate of Mg-Er-Ni alloy by strengthening with lamellar γ' and bulk LPSO phases

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Journal of Materials Science & Technology 2024年第1期168卷 88-102页

作者： Chaoneng Dai Jingfeng wang Yuanlang Pan Kai Ma Yinhong Peng Ye wang Danqian wang Chunhua Ran Jinxing wang Yanlong Ma College of Chemistry and Chemical Engineering Chongqing UniversityChongqing 401331China College of Materials Science and Engineering Chongqing UniversityChongqing 400044China National Engineering Research Center for Magnesium Alloys Chongqing 400044China College of Materials Science and Engineering Chongqing University of TechnologyChongqing 400054China

As-extruded Mg-Er-Ni alloys with different volume fractions of long-period stacking ordered(LPSO)phase and density of lamellar γ' phase were prepared,and the microstructure,mechanical,and degradation properties were *** the bulk LPSO phase and the lamellar γ' phase,and controlling the dynamic recrystallization processes during deformation by adjusting the volume fraction of LPSO and the density of the γ' phase,a synergistic increase in strength and degradation rate can be *** the one hand,the increase in corrosion rate was related to the increased volume fraction of the bulk LPSO phase and the densities of the lamellar γ' phase,which provide more galvanic ***,high densities of the lamellar γ' phase can provide more corrosion interface by inhibiting the recrystallization process to refine dynamic recrystallized(DRXed)grains during the hot *** the other hand,the ultimate tensile strength(UTS)and tensile yield strength(TYS)of the Mg-Er-Ni alloy increased from 345 and 265 MPa to 514 MPa and 358 MPa,respectively,which was mainly attributed to grain boundary and texture strengthening,bulk LPSO phase and lamellar γ' phase ***,Mg^(-1)4Er-4Ni alloy,which contains the highest volume fraction bulk LPSO phase and the densities of lamellar γ' phase,re-alized a synergistic enhancement of strength and degradation *** UTS,TYS,and degradation rate of Mg^(-1)4Er-4Ni were 514 MPa,358 MPa,and 142.5 mg cm^(-2)h^(-1)(3 wt%KCl solution at 93◦C),*** research provides new insight into developing Mg alloys with high strength and degradation rates for fracturing tool materials in the application of oil and gas exploitation in harsh environments.

关键词： Mg-Er-Ni alloy Lamellarγ'and bulk LPSO phases Rapid degradation rate High strength Mechanical and corrosion mechanism

Conditioning treatments mitigate the levels of fecal pollution indicators in soil during land-application of sewage sludge

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Science China Technological Sciences 2024年第10期67卷 3091-3102页

作者： wang YuHang LI Hua FANG WenHao wang Ru wang XinXin ZHENG GuanYu ZHOU LiXiang Department of Environmental Engineering College of Resources and Environmental SciencesNanjing Agricultural University College of Materials and Chemical Engineering Pingxiang University Jiangsu Collaborative Innovation Center for Solid Organic Waste Resource Utilization

Sewage sludge is a major source of fecal pathogens in the environment, and its application to land can result in a significant release of these pathogens into the soil. While conditioning treatments are crucial for improving the dewatering process of sludge, their impact on the presence and behavior of fecal pathogens in soil remains unclear. This study aims to assess four extraction methods for recovering fecal pollution indicators from soil amended with unconditioned and conditioned sludge. The indicators include Escherichia coli(EC), human-specific HF183 Bacteroides(HF183), human adenovirus(HAdV), human BK polyomavirus(BKPyV), human JC polyomavirus(JCPyV), and cross-assembly phage(crAssphage). This study also examines how soil moisture content affects the decay of these fecal pollution indicators in soil amended with raw sludge and investigates the influence of conditioning treatments with cationic polyacrylamide(PAM), Fenton's reagents, Fe[Ⅲ]/CaO on their persistence in soil. The results indicated that the direct extraction method was the most effective and unbiased for recovering fecal pollution indicators from sludge-amended soil compared with the three elution-concentration methods. All fecal pollution indicators, except HAdV, remained stable under dry soil conditions, while high soil moisture content(48.39%-53.14%) slowed the decay rates of these indicators. During the application of sludge to soil, effective control of fecal pollution indicators was observed, with JCPyVand HAdV becoming undetectable within a short period. The log reduction values of HF183, BKPyV, and crAssphage ranged from 0.1 to 2.8 logs after 30 d of cultivation. The application of conditioned sludge, especially Fenton's reagent-conditioned sludge, resulted in a reduction in human fecal contamination in the receiving soil. Therefore, implementing appropriate conditioning methods, such as using Fenton's reagent, can effectively mitigate the health risks associated with fecal pathogens.

关键词： fecal pollution indicators sewage sludge conditioning treatment land application soil

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Single Fe atom-anchored manganese dioxide for efficient removal of volatile organic compounds in refrigerator

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Nano Research 2024年第5期17卷 3927-3933页

作者： Yiwen wang Jun Zhang Yongfei Zhang Yu Zhang Zhe wang Jing wang Yuen Wu Department of Endocrinology the First Affiliated Hospital of USTCDivision of Life Science and MedicineUniversity of Science and Technology of ChinaHefei 230001China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China Hefei Hualing Co. LtdHefei 230088China Linkway Technology Co. LtdResearch Institute of Single Atom Catalysts Industry TechnologyNanning 530000China

The efficient and rapid removal of volatile organic compounds(VOCs)holds significant importance for ensuring food quality and human health,particularly within the low-temperature confined spaces in ***,achieving effective VOCs degradation under such conditions poses challenges in terms of activating inert bonds and facilitating mass *** this study,we propose a novel solution by designing a cleaner module that incorporates 1.07%single Fe atom-anchored manganese dioxide catalysts(FeSAs-MnO_(2)).The combination of single Fe atoms and defect-rich MnO_(2) substrate efficiently activates molecular oxygen,leading to enhanced generation of highly reactive oxygen species(ROS).Non-thermal plasma(NTP)and circulating fan are introduced to facilitate the regeneration of catalytic activity and improve mass *** FeSAs-MnO_(2) cleaner module demonstrates exceptional performance in trimethylamine(TMA)removal,achieving a conversion efficiency of 98.9%for 9 ppm within just 9 ***,accelerated aging tests predict an extended service life of up to 45 years for the FeSAs-MnO_(2) cleaner module,surpassing the expected lifespan of refrigerators significantly.

关键词： single atom catalysts volatile organic compounds(VOCs) trimethylamine(TMA) non-thermal plasma(NTP) refrigerator

Analysis of SF6 decomposed products by fibre-enhanced Raman spectroscopy for gas-insulated switchgear diagnosis

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High Voltage 2024年第1期9卷 206-216页

作者： Jianxin wang Weigen Chen Pinyi wang Fu Wan Zhixian Zhang Shoufei Gao Yingying wang School of Electrical Engineering Chongqing UniversityChongqingChina State Key Laboratory of Power Transmission Equipment&System Security and New Technology Chongqing UniversityChongqingChina Institute of Photonics Technology Jinan UniversityGuangzhouChina

Sulphur hexafluoride(SF6)decomposed products analysis is highly critical in the earlystage fault diagnosis of gas-insulated switchgear(GIS).Spectrum technology outperforms traditional methods on non-invasiveness,no sample preparation,and no ***,the authors present an improved fibre-enhanced Raman spectroscopy(FERS)as a comprehensive analytical tool to detect a suite of SF_(6)decomposed products(SO_(2)F_(2),SOF_(2),SO_(2),H_(2)S,CF_(4),OCS,CO_(2),and CO).The FERS approach is combined with two iris diaphragms for spatial filtering and a rear-end reflector for additional Raman signal *** of detection down to 1×10^(−6)–8×10^(−6)are achieved for different SF6 decompositions,and quantification of an undefined multigas,sampled from an 800 kV GIS in service,is realised utilising SF6 as the internal standard gas and with a maximum error of 5.5%.The GIS is diagnosed according to the results and confirmed by an on-site *** authors foresee that this technique will provide a route for trace gas analysis in the power industry.

关键词： SF6 diagnosis fibre

Spatial light modulation for femtosecond laser manufacturing:Current developments and challenges

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Science China(Technological Sciences) 2024年第1期67卷 60-72页

作者： ZANG Xue LIU ZiTing XU YiShi wang Yi wang Qing LI ZhenZe wang Lei State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China State Key Laboratory of Precision Measurement and Instruments Department of Precision InstrumentTsinghua UniversityBeijing 100084China

Since the invention of lasers,spatial-light-modulated laser processing has become a powerful tool for various *** enables multidimensional and dynamic modulation of the laser beam,which significantly improves the processing efficiency,accuracy,and flexibility,and presents wider prospects over traditional mechanical technologies for machining three-dimensional,hard,brittle,or transparent *** this review,we introduce:(1)The role of spatial light modulation technology in the development of femtosecond laser manufacturing;(2)the structured light generated by spatial light modulation and its generation methods;and(3)representative applications of spatial-light-modulated femtosecond laser manufacturing,including aberration correction,parallel processing,focal field engineering,and polarization ***,we summarize the present challenges in the field and possible future research.

关键词： femtosecond laser manufacturing spatial light modulation structured light aberration correction parallel processing focal field engineering polarization control