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Micelle-directed self-assembly of single-crystal-like mesoporous stoichiometric oxides for high-performance lithium storage

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National Science Review 2024年第4期11卷 195-205页

作者： Yanhua wan Changyao wang Xingmiao Zhang Yang Yin Mengmeng Liu bing Ma Linlin Duan Yuzhu Ma Wei Zhang Changlin Zheng Dongliang Chao Fei wang Yongyao Xia Wei Li Department of Chemistry Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials State Key Laboratory of Molecular Engineering of Polymers College of Chemistry and Materials ScienceFudan University State Key Laboratory of Surface Physics and Department of Physics Fudan University

Due to their uncontrollable assembly and crystallization process,the synthesis of mesoporous metal oxide single crystals remains a formidable ***,we report the synthesis of single-crystal-like mesoporous Li2TiSiO5by using soft micelles as *** key lies in the atomic-scale self-assembly and step-crystallization processes,which ensure the formation of single-crystal-like mesoporous Li2TiSiO5microparticles via an oriented attachment growth mechanism under the confinement of an in-situ formed carbon *** mesoporous Li2TiSiO5anode achieves a superior rate capability(148 mAh g-1at5.0 A g-1) and outstanding long-term cycling stability(138 mAh g-1after 3000 cycles at 2.0 A g-1) for lithium storage as a result of the ultrafast Li+diffusion caused by penetrating mesochannels and nanosized crystal frameworks（5-10 nm）.In comparison,bulk Li2TiSiO5exhibits poor rate capability and cycle performance due to micron-scale diffusion *** method is very simple and reproducible,heralding a new way of designing and synthesizing mesoporous single crystals with controllable frameworks and chemical functionalities.

关键词： mesoporous materials micelles single-crystal-like Li2TiSiO5 lithium-ion batteries

Upwelling current and its relationship to the enrichment of organic matter in the Lower Silurian Longmaxi Formation, northern Chongqing-western Hubei area, southern China

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Journal of Palaeogeography 2024年第4期13卷 993-1015页

作者： Jun-Jun Shen Jia-Kai Yan Peng-wan wang Yu-Man wang Lin Zhou Yu-bing Ji Min Xu Hubei Cooperative Innovation Center of Unconventional Oil and Gas of Yangtze University Hydrogeology and Engineering Geology Institute of Hubei Geological Bureau PetroChina Hangzhou Institute of Petroleum Geology PetroChina Research Institute of Petroleum Exploration and Development Exploration and Production Research Institute Zhejiang Oilfield Company Integrated Center of Exploration and Development

Upwelling currents play a crucial role in the enrichment of organic matter, yet the mechanisms driving this process remain incompletely understood due to methodological and data resolution limitations. In this paper, we employ a combination of biostratigraphic classification, qualitative methods, and quantitative methods to systematically analyze the sedimentological and geochemical characteristics of the Lower Silurian Longmaxi Formation in the northern Chongqing-western Hubei area, southern China. The relationship between the upwelling currents and organic matter enrichment in the shale of the Longmaxi Formation is investigated. Results indicate that the upwelling currents in the study area were primarily influenced by the foreland flexure process. From the Rhuddanian(flexure-sedimentation stage) to the Aeronian(flexure-migration stage), the more intense tectonic activity led to gradual opening of the barrier between the South Qinling Ocean and the Yangtze Platform, resulting in an increase in the influx of the oceanic current. The upwelling currents significantly contributed to the organic matter production, albeit without substantially affecting the preservation conditions. Throughout the succession of the Longmaxi Formation, the organic matter content decreased gradually from the passive continental margin to the foreland flexural stagnant basin, which was mainly due to deterioration of the preservation conditions as a result of sea level fall and increased terrigenous input. Despite the increase in the upwelling currents, they did not decisively control the organic matter enrichment. Spatially, during the Rhuddanian to Aeronian period, the organic matter content decreased similarly from the passive continental margin to the foreland flexural stagnant basin, influenced by reduced organic matter production caused by weakening of the upwelling currents and the worsening preservation conditions caused by sea-level fall. The terrigenous input had a relatively minor

关键词： Middle–Upper Yangtze Ordovician–Silurian transition Black shale Passive continental margin Foreland flexural stagnant basin Sedimentary paleoenvironment

Self-assembled high-entropy nitride multilayer coating

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Rare Metals 2024年第6期43卷 2876-2883页

作者： Xiang-Yu Zhang Yan Liu Vasiliy Pelenovich Xiao-Mei Zeng Jie Liu Qiang wan Alexander Pogrebnjak Long-Jian Xue Zhi-Wen Chen Yan Lei bing Yang School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072China Hubei JiuFengShan Future Science and Technology Laboratory Wuhan 420000China Institute of Technological Sciences of Wuhan University Wuhan 430072China Hubei Key Laboratory of Electronic Manufacturing and Packaging Integration Wuhan UniversityWuhan 430072China College of Engineering Huazhong Agricultural UniversityWuhan 430070China Sumy State University Sumy 40007Ukraine Institute of Materials Science Slovak University of Technology in BratislavaJána Bottu2591724 TrnavaSlovak Republic Shenzhen Research Institute of Wuhan University Shenzhen 518057China

The development of advanced materials and construction of multilayer structure contribute to enhancing the performance of protective coatings,further improving the industrial productivity and conserving *** this paper,the self-assembled high-entropy nitride(heN)AlCrNbSiTiN multilayer coating was designed by harnessing the plasma distribution characteristics and depos-ited by arc ion plating using single target.

关键词： coating energy multilayer

Measurement of Br(n,γ)cross sections up to stellar s-process temperatures at the CSNS Back‑n

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Nuclear Science and Techniques 2023年第11期34卷 226-241页

作者： Gao‑Le Yang Zhen‑Dong An Wei Jiang Xian‑Kai Li Wei‑Wei Qiu Zheng‑Fa Liao Zi‑Yue Zhuang Xiao‑Ping Zhang Sheng‑Li Chen Chen‑Chen Guo Er‑Xi Xiao Xiao Fang Xin‑Xiang Li Xin‑Rong Hu bing Jiang Jin‑Cheng wang Jie Ren Wen Luo Zhi‑Chao Zhu Hao‑Yang Lan Zong‑Wei Cao Xu Ma Ying‑Du Liu Pu‑Sen wang Yi Yang Ping Su Xian‑Gai Deng wan‑bing he Chun‑wang Ma Yu‑Ting wang Zhi‑Tao Dai Peng‑Qin he Ren‑Guang Tang Tao Zhou Jing wang Han Yi Yue Zhang Yong‑Hao Chen Rui‑Rui Fan Ke‑Qing Gao Qiang Li Kang Sun Zhi‑Xin Tan Min‑Hao Gu Han‑Tao Jing Jing‑Yu Tang School of Physics and Astronomy Sun Yat-sen UniversityZhuhai 519082China Shanghai Institute of Applied Physics Chinese Academy of SciencesShanghai 201800China State Key Laboratory of Lunar and Planetary Sciences Macao University of Science and TechnologyMacao 999078China CNSA Macao Center for Space Exploration and Science Macao 999078China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China Spallation Neutron Source Science Center Dongguan 523803China School of Nuclear Science and Technology University of South ChinaHengyang 421001China Sino‑French Institute of Nuclear Engineering and Technology Sun Yat-sen UniversityZhuhai 519082China University of Chinese Academy of Sciences Beijing 100049China Key Laboratory of Nuclear Data China Institute of Atomic EnergyBeijing 102413China School of Materials Science and Engineering Xiangtan UniversityXiangtan 411100China Key Laboratory of Nuclear Physics and Ion‑beam Application(MOE) Institute of Modern PhysicsDepartment of Nuclear Science and TechnologyFudan UniversityShanghai 200433China Institute of Particle and Nuclear Physics Henan Normal UniversityXinxiang 453007China School of Physics Henan Normal UniversityXinxiang 453007China Shenzhen Center Cancer hospitalChinese Academy of Medical SciencesShenzhen 518100China School of Nuclear Science and Technology University of Science and Technology of ChinaHefei 230027China

The neutron capture cross sections(n,γ)of bromine were obtained using the time-of-flight technique at the Back-n facility of the China Spallation Neutron ***γ-rays originating from neutron-induced capture events were detected using four C_(6)D_(6) *** pulse-height weighting technique and double-bunch unfolding method based on Bayesian theory were used in the data *** deductions,normalization,and corrections were carefully considered to obtain reliable measurement *** multilevel R-matrix Bayesian code SAMMY was used to extract the resonance parameters in the resolved resonance region(RRR).The average cross sections in the unresolved resonance region(URR)were obtained from 10 to 400 *** experimental results were compared with data from several evaluated libraries and previous experi-ments in the RRR and *** TALYS code was used to describe the average cross sections in the *** astrophysical Maxwell average cross sections(MACSs)of ^(79,81)Br from kT=5 to 100 keV were calculated over a sufficiently wide range of neutron *** a thermal energy of kT=30 keV,the MACS value for ^(79)Br 682±68 mb was in good agreement with the KADoNiS v1.0 recommended *** contrast,the value of 293±29 mb for ^(81)Br was substantially higher than that of the evaluated database and the KADoNiS v1.0 recommended value.

关键词： Time-of-flight technique Neutron capture cross sections Maxwell average cross sections

Novel miR-490-3p/hnRNPA1-b/PKM2 axis mediates the Warburg effect and proliferation of colon cancer cells via the PI3K/AKT pathway

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World Journal of Gastrointestinal Oncology 2024年第5期16卷 2038-2059页

作者： Xiang-Hui wan Guo-bing Jin Qun Yang Ji-Long Hu Zhi-Liang Liu Jun Rao Can Wen Peng-Ling Li Xi-Mei Yang Bo Huang Xiao-Zhong wang Jiangxi Medical College Nanchang UniversityNanchang 330029Jiangxi ProvinceChina Department of Clinical Laboratory Jiangxi Cancer HospitalNanchang 330029Jiangxi ProvinceChina Jiangxi Key Laboratory of Translational Research for Cancer Jiangxi Cancer HospitalNanchang 330029Jiangxi ProvinceChina Department of Abdominal Surgery Jiangxi Cancer HospitalNanchang 330029Jiangxi ProvinceChina Department of Pathology Jiangxi Cancer HospitalNanchang 330029Jiangxi ProvinceChina Science and Education Section Jiangxi Cancer HospitalNanchang 330029Jiangxi ProvinceChina Department of Clinical Laboratory Jiangxi Children’s HospitalNanchang 330006Jiangxi ProvinceChina Department of Clinical Laboratory The Second Affiliated Hospital of Nanchang UniversityNanchang 330006Jiangxi ProvinceChina Jiangxi Province Key Laboratory of Laboratory Medicine The Second Affiliated Hospital of Nanchang UniversityNanchang 330006Jiangxi ProvinceChina

BACKGROUND heterogeneous ribonucleoprotein A1(hnRNPA1)has been reported to enhance the Warburg effect and promote colon cancer(CC)cell proliferation,but the role and mechanism of the miR-490-3p/hnRNPA1-b/PKM2 axis in CC have not yet been *** To investigate the role and mechanism of a novel miR-490-3p/hnRNPA1-b/PKM2 axis in enhancing the Warburg effect and promoting CC cell proliferation through the PI3K/AKT *** Paraffin-embedded pathological sections from 220 CC patients were collected and subjected to immunohistochemical analysis to determine the expression of *** relationship between the expression values and the clinicopathological features of the patients was *** in mRNA expression were analyzed using quantitative real-time polymerase chain reaction,while differences in protein expression were analyzed using western *** proliferation was evaluated using the cell counting kit-8 and 5-ethynyl-2’-deoxyuridine assays,and cell cycle and apoptosis were detected using flow cytometric *** targeted binding of miR-490-3p to hnRNPA1-b was validated using a dual luciferase reporter *** Warburg effect was evaluated by glucose uptake and lactic acid production *** The expression of hnRNPA1-b was significantly increased in CC tissues and cells compared to normal controls(Phemical results demonstrated significant variations in the expression of the hnRNPA1-b antigen in different stages of CC,including stage I,II-III,and ***,the clinicopathologic characterization revealed a significant correlation between hnRNPA1-b expression and clinical stage as well as T ***1-b was found to enhance the Warburg effect through the PI3K/AKT pathway,thereby promoting proliferation of HCT116 and SW620 ***,the proliferation of HCT116 and SW620 cells was inhibited when miR-490-3p targeted and bound to hnRNPA1-b,effectively blocking the Warburg ***

关键词： heterogeneous ribonucleoprotein A1-b MiR-490-3p Colon cancer Alternative splicing Warburg effect

技术进步能有效促进粮食安全与农民增收双目标实现吗?——来自全国省级面板数据的经验证据

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农村金融研究 2024年第7期 3-15页

作者：马晓河周婉冰中国宏观经济研究院中国社会科学院大学经济学院

技术进步能显著提高粮食安全与农民增收双目标实现的有效性。论文基于2002—2022年全国31省的面板数据,通过耦合协调度模型、DEA-Malmquist指数模型及面板数据双向固定效应模型等进行实证分析。研究表明:技术进步能明显提高粮食安全与... 详细信息

技术进步能显著提高粮食安全与农民增收双目标实现的有效性。论文基于2002—2022年全国31省的面板数据,通过耦合协调度模型、DEA-Malmquist指数模型及面板数据双向固定效应模型等进行实证分析。研究表明:技术进步能明显提高粮食安全与农民收入一致性水平,其中,技术变化对粮食安全与农民收入一致性水平的影响更为显著,该结论在经过一系列稳健性检验后依旧成立。在经济发展水平相对落后的西部地区以及地形更为崎岖的丘陵地区,技术进步对粮食安全与农民收入一致性水平的促进作用更强。此外,技术进步可以通过促进农业适度经营规模水平提升进而间接作用于粮食安全与农民增收双目标的实现。以此为基础,论文提出了相应的政策建议,以充分发挥技术进步对粮食安全与农民增收双目标实现的促进作用。

关键词：技术进步粮食安全与农民增收耦合协调度适度规模经营

hemolysis attributed to high dose vitamin C:Two case reports

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World Journal of Clinical Cases 2024年第17期12卷 3168-3176页

作者： Shi-wan wang Xiao-Wei Zhang Jin-Xiu Qu Yi-Zhong Rao Shuai Lu bing wang Jia he Yuan Zhao Ben-Qiang Rao Center for Oncology Nutrition and Metabolism Beijing Shijitan HospitalCapital Medical University/Key Laboratory of Cancer FSMP for State Market RegulationBeijing 100038China

BACKGROUND High-dose vitamin C treatment(HVCT)can reduce the adverse effect of chemotherapy and enhance the effect of antitumor therapy,which has been considered one of the safest alternative ***,the severity of its adverse effects may have been *** most serious adverse effect is hemolysis,which may result in acute kidney injury or *** glucose-6-phosphate dehydrogenase(G6PD)deficiency is considered to be the main cause,the probability and pathological mechanism are not completely understood,leading to a lack of effective and standardized treatment *** SUMMARY Two patients with colorectal cancer developed hemolytic anemia after using 1 g/kg *** contrast to previous cases,the lowest hemoglobin level in the two cases washepatitis B for many years,which caused abnormal liver reserve function,and Case 2 had grade II bone marrow *** patients improved and were discharged after blood replacement *** cases had the most severe degree of hemolysis but the best prognosis,suggesting that our treatment may be helpful for rescue of drug-induced *** is the first review of the literature on hemolysis caused by HVCT,and we found that all patients with G6PD deficiency developed hemolysis after *** G6PD deficiency should be considered as a contraindication to HVCT,and it is not recommended for patients with bone marrow suppression,moderate-tosevere anemia,hematopoietic abnormalities,or abnormal liver and kidney *** blood purification and steroid therapy may avoid acute kidney injury or death caused by HVCT-related hemolytic anemia.

关键词： hemolysis Vitamin C Adverse effects Acute kidney injury Cancer Case report

RBCC模态特征与热力循环分析样本全覆盖策略

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推进技术 2024年第4期45卷 20-34页

作者：万冰白菡尘陈军中国空气动力研究与发展中心高超声速冲压发动机技术重点实验室四川绵阳621000

为了获得样本全覆盖的RBCC全模态热力循环分析策略,针对目前尚有争议的低速阶段,采用数值模拟方法研究了支板式RBCC构型在Ma=0~2的流场演化特性,基于对流场演化的认识,区分了火箭-冲压联合工作阶段的模态,提出了除纯火箭模态以外的RBCC... 详细信息

为了获得样本全覆盖的RBCC全模态热力循环分析策略,针对目前尚有争议的低速阶段,采用数值模拟方法研究了支板式RBCC构型在Ma=0~2的流场演化特性,基于对流场演化的认识,区分了火箭-冲压联合工作阶段的模态,提出了除纯火箭模态以外的RBCC样本全覆盖的热力循环分析方法策略。研究结果表明,火箭-冲压联合工作阶段时,RBCC的工作模态包括引射模态、“火箭冲压协同”模态和“加力冲压”模态;在亚声速范围,只要正确赋值来流总温、总压,零速引射分析方法可以用于确定有速度条件的进气道入流流量和混合室出口条件;存在“扫掠激波”的超声速阶段与高亚声速阶段的流场特征相似,零速引射分析方法可用于存在“扫掠激波”的超声速阶段,输入条件取“扫掠激波”后的滞止参数;将零速引射分析方法和以燃烧区特征马赫数为表征的等效热力过程分析方法结合,可以实现RBCC除纯火箭模态以外的各模态样本全覆盖的热力循环分析。

关键词： RBCC 低速段模态样本全覆盖热力循环

基于等效热力过程的宽域冲压全流道性能设计方法

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航空学报 2024年第4期45卷 157-171页

作者：万冰陈军白菡尘中国空气动力研究与发展中心空天技术研究所高超声速冲压发动机技术重点实验室绵阳621000

为了开展宽域冲压发动机的全流道设计工作,将双模态冲压发动机等效热力过程分析方法拓展到全流道设计,建立了基于等效热力过程的宽域冲压全流道性能设计方法。将该方法应用于带几何可调进气道的宽域冲压发动机全流道方案设计,分析了进... 详细信息

为了开展宽域冲压发动机的全流道设计工作,将双模态冲压发动机等效热力过程分析方法拓展到全流道设计,建立了基于等效热力过程的宽域冲压全流道性能设计方法。将该方法应用于带几何可调进气道的宽域冲压发动机全流道方案设计,分析了进气道调节、燃烧室尺寸对发动机性能潜力的影响。研究结果表明:马赫数2.0~3.5范围,在比冲和流量2个因素之间,流量对发动机推力性能影响更大,所以在低速段应尽力增大进气道流量;与第2级转折角相比,第2级折转角对比冲和推力的影响权重更大,采用较小的2级折转角有利于提高性能;获得最优推力和比冲性能需要不同的进气道方案。在所研究的马赫数范围,燃烧室需用面积相差很大,飞行马赫数越低、需用面积越大。若以低马赫数的高推力要求为设计依据,需要付出横向尺寸的代价,意味着阻力和重量的增大;若以高马赫数的高推力要求为选择依据,需要在低马赫数时付出推力性能的代价,意味着加速时间和耗油量的增大。本文发展的方法可以快速筛选获得最优推力性能或比冲性能的全流道方案,为宽域高性能冲压发动机的全流道性能初步设计提供有力支撑。

关键词：等效热力过程宽域冲压几何可调进气道全流道设计方法参数化分析性能潜力