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Halogen-free Polymer Donors Based on 3,4-Dicyanothiophene for High-performance Polymer Solar Cells

Chinese Journal of Polymer Science 2022年第8期40卷 905-913,I0008页

作者： Yun-Li Zhao Yue Zhang Xi-Yue yuan wan-yuan deng Bo Zhang Shu-Ting Pang Bing-Yan Yin Hong-Bin Wu Kai-Wen Lin Zhi-Tian Liu Chun-Hui Duan Fei Huang Yong Cao Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and DevicesSouth China University of TechnologyGuangzhou510640China Hubei Engineering Technology Research Center of Optoelectronic and New Energy Materials Wuhan Institute of TechnologyWuhan430205China Department of Materials and Food University of Electronic Science and Technology of China Zhongshan InstituteZhongshan528402China

Polymer solar cells(PSCs)consisting of a polymer donor and a small molecular acceptor is a promising photovoltaic technology,whose device performance is determined by both polymer donor and small molecular *** atoms such as fluorine or chlorine atoms were usually introduced onto the polymer donors to downshift the highest occupied molecular orbital(HOMO)energy levels and improve the open-circuit voltage(VOC)of the ***,the introduction of the halogen atoms especially fluorine atoms greatly complicates the polymer ***,we report the use of a structural simple and easily synthesized building block,3,4-dicyanothiophene(DCT),to construct a set of halogen-free polymer donors PBCNTx(x=25,50,75)via ternary random *** introduction of DCT units not only simplified the synthesis,but also downshifted the HOMO energy levels of the polymers and improved the V_(OC) of PSCs ***,the PBCNT75 afforded a power conversion efficiency up to 15.7%with a V_(OC) of 0.83 V,which are among the top values for halogen-free polymer *** work shows that the introduction of DCT units is a simple yet effective strategy to construct halogen-free and low-cost polymer donors for high-performance PSCs.

关键词： Polymer solar cells Polymer donors Halogen-free Open-circuit voltage Energy loss

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A Data Intrusion Tolerance Model Based on an Improved Evolutionary Game Theory for the Energy Internet

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Computers, Materials & Continua 2024年第6期79卷 3679-3697页

作者： Song deng Yiming yuan Institute of Advanced Technology Nanjing University of Posts and TelecommunicationsNanjing210003China College of Automation Nanjing University of Posts and TelecommunicationsNanjing210003China

Malicious attacks against data are unavoidable in the interconnected,open and shared Energy Internet(EI),Intrusion tolerant techniques are critical to the data security of *** intrusion tolerant techniques suffered from problems such as low adaptability,policy lag,and difficulty in determining the degree of *** address these issues,we propose a novel adaptive intrusion tolerance model based on game theory that enjoys two-fold ideas:(1)it constructs an improved replica of the intrusion tolerance model of the dynamic equation evolution game to induce incentive weights;and (2)it combines a tournament competition model with incentive weights to obtain optimal strategies for each stage of the game *** experiments are conducted in the IEEE 39-bus system,whose results demonstrate the feasibility of the incentive weights,confirm the proposed strategy strengthens the system’s ability to tolerate aggression,and improves the dynamic adaptability and response efficiency of the aggression-tolerant system in the case of limited resources.

关键词： Energy Internet Intrusion tolerance game theory racial competition adaptive intrusion response

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Nonlinear robust adaptive control for bidirectional stabilization system of all-electric tank with unknown actuator backlash compensation and disturbance estimation

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Defence Technology（防务技术） 2024年第2期32卷 144-158页

作者： Shusen yuan Wenxiang deng Jianyong Yao Guolai Yang School of Mechanical Engineering Nanjing University of Science and TechnologyNanjing210094China

Since backlash nonlinearity is inevitably existing in actuators for bidirectional stabilization system of allelectric tank,it behaves more drastically in high maneuvering *** this work,the accurate tracking control for bidirectional stabilization system of moving all-electric tank with actuator backlash and unmodeled disturbance is *** utilizing the smooth adaptive backlash inverse model,a nonlinear robust adaptive feedback control scheme is *** unknown parameters and unmodelled disturbance are addressed separately through the derived parametric adaptive function and the continuous nonlinear robust *** the unknown backlash parameters are updated via adaptive function and the backlash effect can be suppressed successfully by inverse operation,which ensures the system ***,the system disturbance in the high maneuverable environment can be estimated with the constructed adaptive law online improving the engineering ***,Lyapunov-based analysis proves that the developed controller can ensure the tracking error asymptotically converges to zero even with unmodeled disturbance and unknown actuator *** co-simulations and experiments illustrate the advantages of the proposed approach.

关键词： Bidirectional stabilization system Robust control Adaptive control Backlash inverse Disturbance estimation

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Synthesis of multifunctional additives for solid propellants:Structure,properties and mechanism

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Defence Technology（防务技术） 2024年第3期33卷 308-316页

作者： Pingan Zhang Lina Sun Jianmin yuan Jianru deng College of Chemistry and Chemical Engineering Hunan UniversityChangsha 410082PR China College of Material Science and Engineering Hunan UniversityChangsha 410082PR China Hu Bei Sanjiang Aerospace Jianghe Chemical Technology Co. LtdYichang 444200PR China

To simplify the composite propellant formulation and address the current issue of the single-functionality present in existing additives,the multi-cyano,amine-based polybutadiene(AEHTPB-CN)was prepared based on AEHTPB by adopting appropriate synthesis *** replacing 10% of HTPB binder in the propellant formulation,it can effectively enhance the interfacial bond strength between the propellant binder matrix and solid fillers(AP(ammonium perchlorate)and RDX(cyclotrimethylene-trinitramine)),the mechanical properties of the HTPB/AP/RDX/Al propellant were superior to blank control propellant with an improvement of 35.4% in tensile strength,62.0% enhancement in elongation at break,and reduce the propellant burn rate by 10.7% with any energy *** function mechanism of AEHTPB-CN was systematically elucidated through experiments and computer simulation *** results show that the tertiary amine group in AEHTPB-CN can react with AP to form ammonium ionic bonds,and the hydroxyl and cyano groups can form hydrogen bonding interactions with AP,which enables AEHTPB-CN to be firmly adsorbed on the AP surface through chemical and physical *** RDX,the interfacial bonding effect of AEHTPB-CN is attributed to their ability to form C-H···N≡C weak hydrogen bonding interaction between the cyano group and RDX methylene group.

关键词： Hydroxyl-terminated polybutadiene(HTPB) HTPB propellant Chemical modification Bonding agent Mechanism

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Constructions of optimal binary locally repairable codes via intersection subspaces

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Science China(Information Sciences) 2024年第6期67卷 418-432页

作者： Wenqin ZHANG deng TANG Chenhao YING yuan LUO School of Electronic Information and Electrical Engineering Shanghai Jiao Tong University

Locally repairable codes（LRCs）, which can recover any symbol of a codeword by reading only a small number of other symbols, have been widely used in real-world distributed storage systems, such as Microsoft Azure Storage and Ceph Storage Cluster. Since binary linear LRCs can significantly reduce coding and decoding complexity, constructions of binary LRCs are of particular interest. The aim of this paper is to construct dimensional optimal binary LRCs with disjoint local repair groups. We introduce a method to connect intersection subspaces with binary LRCs and construct dimensional optimal binary linear LRCs with locality 2b（b 3） and minimum distance d 6 by employing intersection subspaces deduced from the direct sum. This method will sufficiently increase the number of possible repair groups of dimensional optimal LRCs, thus efficiently expanding the range of the construction parameters while keeping the largest code rates compared with all known binary linear LRCs with minimum distance d 6 and locality 2b.

关键词： locally repairable codes disjoint local repair groups distributed storage systems intersection subspaces direct sum

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All-inorganic ultrathin high-sensitivity transparent temperature sensor based on a Mn-Co-Ni-O nanofilm

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Microsystems & Nanoengineering 2024年第3期10卷 195-205页

作者： yuanyuan Cui Mengwei Sun Changbo Liu yuan deng Research Institute for Frontier Science Beihang UniversityBeijing 100191China School of Materials Science and Engineering Beihang UniversityBeijing 100191China Key Laboratory of Intelligent Sensing Materials and Chip Integration Technology of Zhejiang Province Hangzhou Innovation Institute of Beihang UniversityHangzhou 310051China

The demand for optically transparent temperature sensors in intelligent devices is ***,the performance of these sensors,particularly in terms of their sensitivity and resolution,must be further *** study introduces a novel transparent and highly sensitive temperature sensor characterized by its ultrathin,freestanding design based on a Mn-Co-Ni-O *** Mn-Co-Ni-O-based sensor exhibits remarkable sensitivity,with a temperature coefficient of resistance of−4%℃^(−1),and can detect minuscule temperature fluctuations as small as 0.03℃.Additionally,the freestanding sensor can be transferred onto any substrate for versatile application while maintaining robust structural stability and excellent resistance to interference,indicating its suitability for operation in challenging *** practical utility in monitoring the surface temperature of optical devices is demonstrated through vertical integration of the sensor and a micro light-emitting diode on a polyimide ***,an experiment in which the sensor is implanted in rats confirms its favorable biocompatibility,highlighting the promising applications of the sensor in the biomedical domain.

关键词： transparent sensor versatile

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Metarelation2vec:A Metapath-Free Scalable Representation Learning Model for Heterogeneous Networks

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Tsinghua Science and Technology 2024年第2期29卷 553-575页

作者： Lei Chen yuan Li Yong Lei Xingye deng School of Information and Electrical Engineering Hunan University of Science and TechnologyXiangtan 411201China School of Computer Science and Engineering Hunan University of Science and TechnologyXiangtan 411201China

Metapaths with specific complex semantics are critical to learning diverse semantic and structural information of heterogeneous networks(HNs)for most of the existing representation learning ***,any metapaths consisting of multiple,simple metarelations must be driven by domain *** sensitive,expensive,and limited metapaths severely reduce the flexibility and scalability of the existing models.A metapath-free,scalable representation learning model,called Metarelation2vec,is proposed for HNs with biased joint learning of all metarelations in a bid to address this ***,a metarelation-aware,biased walk strategy is first designed to obtain better training samples by using autogenerating cooperation probabilities for all metarelations rather than using expert-given ***,grouped nodes by the type,a common and shallow skip-gram model is used to separately learn structural proximity for each node ***,grouped links by the type,a novel and shallow model is used to separately learn the semantic proximity for each link ***,supervised by the cooperation probabilities of all meta-words,the biased training samples are thrown into the shallow models to jointly learn the structural and semantic information in the HNs,ensuring the accuracy and scalability of the *** experimental results on three tasks and four open datasets demonstrate the advantages of our proposed model.

关键词： metarelation random walk heterogeneous network metapath representation learning

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Spatial correlations in time and frequency domains between chlorophyll-a concentration and environmental factors in the Bohai Sea

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Journal of Oceanology and Limnology 2024年第4期42卷 1143-1156页

作者： wan XU Di MU Zhenteng YANG Dekui yuan Department of Mechanics Tianjin UniversityTianjin 300350China Engineering Research Center of Seawater Utilization of Ministry of Education School of Chemical Engineering and TechnologyHebei University of TechnologyTianjin 300130China State Key Laboratory of Hydraulic Engineering Simulation and Safety Tianjin UniversityTianjin 300072China

Based on the reconstructed MODIS data and ECMWF reanalysis data from 2003 to 2021,spatial correlations between chlorophyll a(Chl a)and sea surface temperature(SST),photosynthetically available radiation(PAR),aerosol optical thickness(AOT),and wind speed(WS)in the Bohai Sea were analyzed from the perspective of time domain and frequency *** indicate that the frequency domain analysis was more conducive to revealing the correlations between Chl a and environmental *** spatial pattern of time-domain correlations was similar to the isobaths of the Bohai Sea,which was positive in shallow waters and negative in deep waters for SST,PAR,and AOT,and was reversed for ***-domain correlations were obtained by performing Fourier Transform and were higher than correlations in time *** spatial distributions indicated that the effects of SST and PAR on Chl a were greater than AOT and WS in the Bohai ***,cross-spectrum analysis was applied to explore the response relationships.A depth-dependent pattern was shown in correlations and time lags,indicating that the influential mechanism of environmental factors on Chl-a concentration is related to seawater depth.

关键词： chlorophyll a(Chl a) frequency domain spatial correlation Bohai Sea

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Role of Stokes Drift in Ocean Dynamics Under Typhoon Conditions in the Bohai Sea

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Journal of Ocean University of China 2024年第1期23卷 33-45页

作者： LI Haoqian wan Kai wanG Menghan deng Zeng’an CAO Yu North China Sea Marine Forecasting Center Qingdao 266061China Shandong Provincial Key Laboratory of Marine Ecology and Environment&Disaster Prevention and Mitigation Qingdao 266061China North China Sea Offshore Engineering Survey Institute Qingdao 266061China School of Marine Science and Technology Tianjin UniversityTianjin 300072China South China Sea Marine Forecasting Center Guangzhou 510006China

The effect of Stokes drift production(SDP),which includes Coriolis-Stokes forcing,Langmuir circulation,and Craik-Lei-bovich vortexes,on the upper ocean during typhoon passage in the Bohai Sea(BS),China,is investigated by using a coupled wave-current *** role of SDP in turbulent mixing and the further dynamics during the entire typhoon period are comprehensively *** results show that SDP greatly increases turbulent mixing at all depths under typhoon conditions by up to seven times that under normal weather *** generally strengthens sea surface cooling by more than 0.4℃,with the maximum reduction in sea surface temperature(SST)at the during-typhoon stage exceeding 2℃,which is approximately seven times larger than that under normal weather *** SDP-induced decrease in current speed can exceed 0.2ms^(-1),and the change in current direction is generally opposite the wind *** results suggest that Stokes drift depresses the effect of strong winds on currents by intensifying turbulent *** layer depth(MLD)is distinctly increased by O(1)during typhoons due to SDP and can deepen by more than *** addition,the continuous effects of SDP on SST,current,and MLD at the after-typhoon stage indi-cate a hysteretic response between SDP and typhoon actions.

关键词： Stokes drift production Langmuir turbulence rurbulent mixing typhoon coupled model

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Tuning the surface electronic structure of noble metal aerogels to promote the electrocatalytic oxygen reduction

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Journal of Energy Chemistry 2024年第2期89卷 557-564,I0013页

作者： Hongxing yuan Wei Gao Xinhao wan Jianqi Ye Dan Wen State Key Laboratory of Solidification Processing School of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072ShaanxiChina

The sluggish kinetics of the oxygen reduction reaction(ORR)is the bottleneck for various electrochemical energy conversion *** the electronic structure of electrocatalysts by ligands has received particular attention in deriving valid ORR ***,the surface electronic structure of Ptbased noble metal aerogels(NMAs)was modulated by various organic ligands,among which the electron-withdrawing ligand of 4-methylphenylene effectively boosted the ORR *** calculations suggested the smaller energy barrier for the transformation of O^(*) to OH^(*) and downshift the d-band center of Pt due to the interaction between 4-methylphenylene and the surface metals,thus enhancing the ORR intrinsic *** Pt3Ni and Pt Pd aerogels with 4-methylphenylene decoration performed significant enhancement in ORR activity and durability in different ***,the 4-methylphenylene modified Pt Pd aerogel exhibited the higher halfwave potential of 0.952 V and the mass activity of 10.2 times of commercial Pt/*** work explained the effect of electronic structure on ORR electrocatalytic properties and would promote functionalized NMAs as efficient ORR electrocatalysts.

关键词： Noble metal aerogels Surface electronic structure ORR Electrocatalyst Organic ligands

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