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Polymer-to-Monomers Chemically Recyclable Poly(imide-imine)Plastics with Extreme-Condition Resistance and Flame Retardancy

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Chinese Journal of Polymer Science 2024年第10期42卷 1525-1535,I0012页

作者： Zhen-Yu wang xiao-Kong Liu State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchun130012China

Polyimides are a family of high-tech plastics that have irreplaceable applications in the fields of aerospace,defense,and opto-electronics,but polyimides are difficult to be reprocessed and recycled at the end of their service life,resulting in a significant waste of ***,it is of great significance to develop recyclable polyimides with comparable properties to the commercial ***,we report a novel polymer-to-monomers chemically recyclable poly(imide-imine)(PtM-CR-PII)plastic,synthesized by cross-linking the amine-terminated aromatic bisimide monomer and the hexa-vanillin terminated cyclophosphazene monomer via dynamic imine *** PtM-CR-PII plastic exhibits comparable mechanical and thermal properties as well as chemical stability to the commercial *** PtM-CR-PII plastic possesses a high Young’s modulus of≈3.2 GPa and a tensile strength as high as≈108 MPa,which also exhibits high thermal stability with a glass transition temperature of≈220℃.Moreover,the PtM-CR-PII plastic exhibits outstanding waterproofness,acid/alkali-resistance,and solvent-resistance,its appearance and mechanical properties can be well maintained after long-term soaking in water,highly concentrated acid and base,and various organic ***,the cyclophosphazene moieties endow the PtM-CR-PII plastic with excellent flame *** PtM-CR-PII plastic exhibits the highest UL-94 flame-retarding rating of V-0 and a limiting oxygen index(LOI)value of 45.5%.Importantly,the PtM-CR-PII plastic can be depolymerized in an organic solvents-acid mixture medium at room temperature,allowing easy separation and recovery of both monomers in high *** recovered pure monomers can be used to regenerate new PtM-CR-PII plastics,enabling sustainable polymer-monomers-polymer circulation.

关键词： Chemical recyclability Polyimides Polyimines Dynamic imine bonds Mechanical properties Chemical stability

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Identification of residues in Lassa virus glycoprotein 1 involved in receptor switch

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Virologica Sinica 2024年第4期39卷 600-608页

作者： Jiao Guo Yi Wan yang Liu xiaoying Jia Siqi Dong Gengfu xiao Wei wang State Key Laboratory of Virology Wuhan Institute of VirologyCenter for Biosafety Mega-ScienceChinese Academy of SciencesWuhan 430071China University of the Chinese Academy of Sciences Beijing 100049China The Xi'an Key Laboratory of Pathogenic Microorganism and Tumor Immunity School of Basic MedicineXi'an Medical UniversityXi'an 710021China

Lassa virus(LASV)is an enveloped,negative-sense RNA virus that causes Lassa hemorrhagic *** entry of LASV requires the viral glycoprotein 1(GP1)to undergo a receptor switch from its primary receptor alpha-dystroglycan(α-DG)to its endosomal receptor lysosome-associated membrane protein 1(LAMP1).A conserved histidine triad in LASV GP1 has been reported to be responsible for receptor *** test the hypothesis that other non-conserved residues also contribute to receptor switch,we constructed a series of mutant LASV GP1 proteins and tested them for binding to *** residues,L84,K88,L107,and H170,were identified as critical for receptor *** any of the four residues with the corresponding lymphocytic choriomeningitis virus(LCMV)residue(L84 N,K88E,L10F,and H170S)reduced the binding affinity of LASV GP1 for ***,all mutations caused decreases in glycoprotein precursor(GPC)-mediated membrane fusion at both pH 4.5 and *** infectivity of pseudotyped viruses bearing either GPCL84N or GPCK88E decreased sharply in multiple cell types,while L107F and H170S had only mild effects on *** biolayer light interferometry assay,we found that all four mutants had decreased binding affinity to LAMP1,in the order of binding affinity being L84 N>L107F>K88E>*** four amino acid loci identified for the first time in this study have important reference significance for the in-depth investigation of the mechanism of receptor switching and immune escape of LASV occurrence and the development of reserve anti-LASV infection drugs.

关键词： Lassa virus(LASV) Lysosome-associated membrane protein 1 (LAMP1) Glycoprotein Receptor switch Membrane fusion

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Incremental Data Stream Classification with Adaptive Multi-Task Multi-View Learning

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Big Data Mining and Analytics 2024年第1期7卷 87-106页

作者： Jun wang Maiwang Shi xiao Zhang Yan Li Yunsheng Yuan Chengei yang Dongxiao Yu School of Computer Science and Technology Shandong UniversityQingdao 266237China School of Software Shandong UniversityJinan 250101China

With the enhancement of data collection capabilities,massive streaming data have been accumulated in numerous application ***,the issue of classifying data streams based on mobile sensors can be formalized as a multi-task multi-view learning problem with a specific task comprising multiple views with shared features collected from multiple *** incremental learning methods are often single-task single-view,which cannot learn shared representations between relevant tasks and *** adaptive multi-task multi-view incremental learning framework for data stream classification called MTMVIS is proposed to address the above challenges,utilizing the idea of multi-task multi-view ***,the attention mechanism is first used to align different sensor data of different *** addition,MTMVIS uses adaptive Fisher regularization from the perspective of multi-task multi-view learning to overcome catastrophic forgetting in incremental *** reveal that the proposed framework outperforms state-of-the-art methods based on the experiments on two different datasets with other baselines.

关键词： data stream classification mobile sensors multi-task multi-view learning incremental learning

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LncRNAs are involved in regulating ageing and age-related disease through the adenosine monophosphate-activated protein kinase signalling pathway

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Genes & Diseases 2024年第5期11卷 183-197页

作者： Jiamei Li Feng xiao Siqi wang xiaolan Fan Zhi He Taiming Yan Jia Zhang Mingyao yang Deying yang College of Animal Science and Technology Sichuan Agricultural UniversityChengduSichuan 611130China Farm Animal Genetic Resources Exploration and Innovation Key Laboratory of Sichuan Province Sichuan Agricultural UniversityChengduSichuan 611130China Chengdu Women’s and Children’s Central Hospital School of MedicineUniversity of Electronic Science and Technology of ChinaChengduSichuan 610017China

A long noncoding RNA(lncRNA)is longer than 200 *** regulates various biological processes mainly by interacting with DNA,RNA,or protein in multiple kinds of biological *** monophosphate-activated protein kinase(AMPK)is activated during nutrient starvation,especially glucose starvation and oxygen deficiency(hypoxia),and exposure to toxins that inhibit mitochondrial respiratory chain complex *** is an energy switch in organisms that controls cell growth and multiple cellular processes,including lipid and glucose metabolism,thereby maintaining intracellular energy homeostasis by activating catabolism and inhibiting *** AMPK signalling pathway consists of AMPK and its upstream and downstream *** upstream targets include proteins such as the transforming growth factor b-activated kinase 1(TAK1),liver kinase B1(LKB1),and calcium/calmodulindependent protein kinase b(CaMKKb),and its downstream targets include proteins such as the mechanistic/mammalian target of rapamycin(mTOR)complex 1(mTORC1),hepatocyte nuclear factor 4a(HNF4a),and silencing information regulatory 1(SIRT1).In general,proteins function relatively independently and *** this article,a review of the currently known lncRNAs involved in the AMPK signalling pathway is presented and insights into the regulatory mechanisms involved in human ageing and age-related diseases are provided.

关键词： Age-related diseases Ageing AMPK signalling pathway Long noncoding RNA microRNA

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On Minor Left Prime Factorization Problem for Multivariate Polynomial Matrices

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Journal of Systems Science & Complexity 2024年第3期37卷 1295-1307页

作者： LU Dong wang Dingkang xiao Fanghui School of Mathematics Southwest Jiaotong UniversityChengdu 610031China KLMM Academy of Mathematics and Systems ScienceChinese Academy of SciencesBeijing 100190China School of Mathematical Sciences University of Chinese Academy of SciencesBeijing 100049China MOE-LCSM School of Mathematics and StatisticsHunan Normal UniversityChangsha 410081China

A new necessary and sufficient condition for the existence of minor left prime factorizations of multivariate polynomial matrices without full row rank is *** key idea is to establish a relationship between a matrix and any of its full row rank *** on the new result,the authors propose an algorithm for factorizing matrices and have implemented it on the computer algebra system *** examples are given to illustrate the effectiveness of the algorithm,and experimental data shows that the algorithm is efficient.

关键词： Free modules Grobner bases minor left prime(MLP) multivariate polynomial matrices polynomial matrix factorizations

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Optimal Nonlinear Robust Sliding Mode Control of an Excitation System Based on Mixed Linear H_(2)/H_(∞) Matrix Inequalities

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Protection and Control of Modern Power Systems 2024年第4期9卷 1-22页

作者： Yidong Zou Yunhe wang Jinbao Chen Wenqing Hu yang Zheng Wenhao Sun Zhihuai xiao the School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072China

In this paper,an optimal nonlinear robust sliding mode control(ONRSMC)based on mixed H_(2)/H_(∞)linear matrix inequalities(LMIs)is designed for the excitation system in a“one machine-infinite bus system”(OMIBS)to enhance system ***,the direct feedback linearization method is used to establish a mathematical model of the OMIBS incorporating *** is then designed for this model,employing the mixed H_(2)/H_(∞)*** chaos mapping-based adaptive salp swarm algorithm(CASSA)is introduced to fully optimize the parameters of the sliding mode control,ensuring optimal performance under a specified *** demonstrates rapid convergence and reduced like-lihood of falling into local optima during ***,ONRSMC is obtained through inverse transformation,exhibiting the advantages of simple structure,high reliability,and independence from the accuracy of system *** simulation scenarios are employed to validate the effectiveness and robustness of ONRSMC,including mechanical power variation,generator three-phase short circuit,transmission line short circuit,and generator parameter *** results indicate that ONRSMC achieves optimal dynamic performance in various operating conditions,facilitating the stable operation of power systems following faults.

关键词： Excitation sliding mode linear matrix inequality salp swarm algorithm

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A data-assisted physics-informed neural network(DA-PINN)for fretting fatigue lifetime prediction

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International Journal of Mechanical System Dynamics 2024年第3期4卷 361-373页

作者： Can wang Qiqi xiao Zhikun Zhou Yongyu yang Gregor Kosec Lihua wang Magd Abdel Wahab Soete Laboratory Department of Electrical EnergyMetalsMechanical Constructions and SystemsFaculty of Engineering and ArchitectureGhent UniversityGentBelgium Department of Engineering Mechanics School of Aerospace EngineeringHuazhong University of Science and TechnologyWuhanChina Key Laboratory for Mechanics Anhui Polytechnic UniversityWuhuChina Parallel and Distributed Systems Laboratory Jožef Stefan InstituteLjubljanaSlovenia School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghaiChina College of Engineering Yuan Ze UniversityTaiwanChina

In this study,we present for the first time the application of physics-informed neural network(PINN)to fretting fatigue *** PINN has recently been applied to pure fatigue lifetime prediction,it has not yet been explored in the case of fretting *** propose a data-assisted PINN(DA-PINN)for predicting fretting fatigue crack initiation *** traditional PINN that solves partial differential equations for specific problems,DA-PINN combines experimental or numerical data with physics equations as part of the loss function to enhance prediction *** DA-PINN method,employed in this study,consists of two main ***,damage parameters are obtained from the finite element method by using critical plane method,which generates a data set used to train an artificial neural network(ANN)for predicting damage parameters in other ***,the predicted damage parameters are combined with the experimental parameters to form the input data set for the DA-PINN models,which predict fretting fatigue *** results demonstrate that DA-PINN outperforms ANN in terms of prediction accuracy and eliminates the need for high computational costs once the damage parameter data set is ***,the choice of loss-function methods in DA-PINN models plays a crucial role in determining its performance.

关键词： crack initiation data-assisted fretting fatigue finite element method physics-informed neural network

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A Polarization-Adjustable Picosecond Deep-Ultraviolet Laser for Spin- and Angle-Resolved Photoemission Spectroscopy

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Chinese Physics Letters 2012年第6期29卷 149-151页

作者： ZHANG Feng-Feng yang Feng ZHANG Shen-Jin wang Zhi-Min XU Feng-Liang PENG Qin-Jun ZHANG Jing-Yuan wang xiao-yang CHEN Chuang-Tian XU Zu-Yan RCLPT Key Lab of Functional Crystal and Laser TechnologyTechnical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190 Beijing Center for Crystal R&D Key Lab of Functional Crystal and Laser TechnologyTechnical Institute of Physics and ChemistryChinese Academy of SciencesBeijing 100190 Graduate University of Chinese Academy of Sciences Beijing 100190

We report on a polarization-adjustable picosecond deep-ultraviolet (DUV) laser at 177.3 *** DUV laser was produced by second harmonic generation from a mode-locked laser at 355 nm in nonlinear optical crystal *** laser delivered a maximum average output power of 1.1 m W at 177.3 *** polarization of the 177.3nm beam was adjusted with linear and circular polarization by means of λ/4 and λ/2 wave *** the best of our knowledge,the laser has been employed as the circularly polarized and linearly polarized DUV light source for a spin- and angle-resolved photoemission spectroscopy with high resolution for the first time.

关键词： polarization polarized circular

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Predicted lower limit of normal reduces misclassification risk of airflow limitation in asymptomatic elderly never-smokers

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Chinese Medical Journal 2013年第18期126卷 3486-3492页

作者： wang yang xiao Wei MA De-dong JIANG Yuan-yuan Department of Respiratory Medicine Qilu Hospital Shandong University Jinan Shandong 250012 China

Background It remains controversial what better defines abnormal lung function at the extremes of age. This study aimed to establish new spirometric reference equations for residents in Jinan and compare the most accepted two spirometric definitions of chronic obstructive pulmonary disease （COPD）--a fixed post-bronchodilator ratio of forced expiratory volume in one second to forced vital capacity （FEVJFVC） below 70% vs. FEV1/FVC 〈lower limit of normal （LLN）-in an elderly population （age 〉60 years）. Methods Among 10 002 cases, only never-smokers who had no respiratory symptoms or diagnoses of cardio- pulmonary diseases and whose lung function measurements strictly followed the American Thoracic Society guidelines, were included in the statistical analysis. For each gender, prediction equations of FEV1, FVC, FEV1/FVC and corresponding LLN values were developed using multiple regression models. Results In this cross-sectional study, spirometric reference values were statistically derived from a sample of 1328 healthy never-smokers （672 males, 656 females）, age 56-84 years. As expected, age and height were the main predictors for all lung function parameters. Using the two spirometric definitions, the number of pulmonary function test results interpreted as obstructed varied markedly in the elderly population for both genders （males： X2=19.59, P 〈0.01; females： X2=5.67, P=0.017）. Conclusions The Global Initiative for Chronic Obstructive Lung Disease （GOLD） criterion probably leads to over- diagnosis in asymptomatic elderly never-smokers. Our study suggests that the predicted LLN values will reduce the misclassification risk instead. However, cohort studies are urgently needed for clinical validation.

关键词： pulmonary disease chronic obstructive spirometry FEV/FVC lower limit of normal

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Stabilizing high-efficiency iridium single atoms via lattice confinement for acidic oxygen evolution

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Nano Research 2024年第4期17卷 2492-2498页

作者： Yibo wang Jiadong Jiang Zhaoping Shi Hongxiang Wu Jiahao yang Pengbo wang Shuai Hou Meiling xiao Junjie Ge Changpeng Liu Wei Xing Laboratory of Advanced Power Sources Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China School of Applied Chemistry and Engineering University of Science and Technology of ChinaHefei 230026.China State Key Laboratory of Electroanalytical Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Jilin Province Key Laboratory of Low Carbon Chemical Power Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Key Laboratory of Physics and Technology for Advanced Batteries Ministry of EducationCollege of PhysicsJilin UniversityChangchun 130012China

Stable and efficient single atom catalysts(SACs)are highly desirable yet challenging in catalyzing acidic oxygen evolution reaction(OER).Herein,we report a novel iridium single atom catalyst structure,with atomic Ir doped in tetragonal PdO matrix(IrSAs-PdO)via a lattice-confined *** optimized IrSAs-PdO-0.10 exhibited remarkable OER activity with an overpotential of 277 mV at 10 mA·cm^(-2) and long-term stability of 1000 h in 0.5 M H_(2)SO_(4).Furthermore,the turnover frequency attains 1.6 s^(-1) at an overpotential of 300 mV with a 24-fold increase in the intrinsic *** high activity originates from isolated iridium sites with low valence states and decreased Ir–O bonding covalency,and the excellent stability is a result of the effective confinement of iridium sites by Ir–O–Pd ***,we demonstrated for the first time that SACs have great potential in realizing ultralow loading of iridium(as low as microgram per square center meter level)in a practical water electrolyzer.

关键词： lattice confinement iridium single atoms ultralow iridium loading acidic oxygen evolution proton exchange membrane water electrolysis

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