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Ore Geology,H-O-C Isotopes and 40Ar-39Ar dating of the Wutonggou Iron deposit,Eastern Tianshan,NW China:Implications for the Source,Timing,and Genesis of Hydrothermal Mineralization in a Sedimentary Iron deposit

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Journal of Earth Science 2024年第4期35卷 1170-1185页

作者： Chun-Long wang Yi-Tian wang State Key Laboratory of Geological Processes and Mineral Resources Collaborative Innovation Center for Exploration of Strategic Mineral ResourcesSchool of Earth ResourcesChina University of GeosciencesWuhan430074China MNR Key Laboratory of Metallogeny and Mineral Assessment Institute of Mineral ResourcesChinese Academy of Geological SciencesBeijing100037China

The Wutonggou iron deposit is located in the well-known iron metallogenic belt in the eastern Tianshan,NW China,and has been regarded as a sedimentary iron *** hydrothermal overprinting could play indispensable roles in the formation of high-grade iron ores in sedimentary iron deposits,previous studies mainly focused on sedimentary-related iron mineralization,while the nature and contribution of hydrothermal fluids are poorly ***,an integrated study of ore geology,H-O-C isotopes and^(40)Ar-^(39)Ar dating,is conducted on the Wutonggou deposit,in order to reveal the features,source,and timing of hydrothermal *** studied deposit includes two mining sections namely the Jianshan and ***δ^(18)O values of early magnetite from the Jianshan section range from+3.0‰to+5.8‰that nearly consistent with classic magmatic magnetite,while increase to 6.3‰-8.0‰in the late *** from the two sections shows comparable H-O isotopic compositions and identical fractionation trends,and is plotted in or periphery to the primary magmatic water *** from the two sections are broadly similar in carbon and oxygen isotopic compositions,and siderite from the Wutonggou section is plotted in the same ***,comparable stable isotopic compositions and evolution trends indicate similar magmatic fluids contributed hydrothermal iron mineralization in the two mining ***,water-rock interactions of varying degrees generated distinct mineralization styles in the Jianshan and Wutonggou sections,and caused the isotopic fractionation in late *** extracted from a hydrothermal siderite ore yielded a^(40)Ar-^(39)Ar plateau age of 299.5±2.0 Ma,indicates the timing of hydrothermal iron mineralization is correspond.ng to the emplacement of vicinity *** together,the hydrothermal mineralization in the Wutonggou iron deposit was the product of remobilization and upgrad.ng of early sedimentary iron ores,a

关键词： iron deposits H-O-C isotopes 40Ar-39Ar dating sedimentary iron deposits Wutonggou iron deposit eastern Tianshan

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Self-supervised recalibration network for person re-identification

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defence Technology（防务技术） 2024年第1期31卷 163-178页

作者： Shaoqi Hou Zhiming wang Zhihua d.ng Ye Li Zhiguo wang Guangqiang Yin Xinzhong wang Shenzhen Institute of Information Technology Shenzhen518172China University of Electronic Science and Technology of China Chengdu611731China Kash Institute of Electronics and Information Industry Kashi844099China

The attention mechanism can extract salient features in images,which has been proved to be effective in improving the performance of person re-identification(Re-Id).However,most of the existing attention modules have the following two shortcomings:On the one hand,they mostly use global average pooling to generate context descriptors,without highlighting the guid.ng role of salient information on descriptor generation,resulting in insufficient ability of the final generated attention mask representation;On the other hand,the design of most attention modules is complicated,which greatly increases the computational cost of the *** solve these problems,this paper proposes an attention module called self-supervised recalibration(SR)block,which introduces both global and local information through adaptive weighted fusion to generate a more refined attention *** particular,a special"Squeeze-Excitation"(SE)unit is designed in the SR block to further process the generated intermediate masks,both for nonlinearizations of the features and for constraint of the resulting computation by controlling the number of ***,we combine the most commonly used Res Net-50 to construct the instantiation model of the SR block,and verify its effectiveness on multiple Re-Id datasets,especially the mean Average Precision(m AP)on the Occluded-duke dataset exceeds the state-of-the-art(SOTA)algorithm by 4.49%.

关键词： Person re-identification Attention mechanism Global information Local information Adaptive weighted fusion

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Conditioning treatments mitigate the levels of fecal pollution indicators in soil during land-application of sewage sludge

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Science China Technological Sciences 2024年第10期67卷 3091-3102页

作者： wang YuHang LI Hua FAng WenHao wang Ru wang XinXin ZHEng GuanYu ZHOU LiXiang department of Environmental Engineering College of Resources and Environmental SciencesNanjing Agricultural University College of Materials and Chemical Engineering Pingxiang University Jiangsu Collaborative Innovation Center for Solid Organic Waste Resource Utilization

Sewage sludge is a major source of fecal pathogens in the environment, and its application to land can result in a significant release of these pathogens into the soil. While conditioning treatments are crucial for improving the dewatering process of sludge, their impact on the presence and behavior of fecal pathogens in soil remains unclear. This study aims to assess four extraction methods for recovering fecal pollution indicators from soil amended with unconditioned and conditioned sludge. The indicators include Escherichia coli(EC), human-specific HF183 Bacteroides(HF183), human adenovirus(HAdV), human BK polyomavirus(BKPyV), human JC polyomavirus(JCPyV), and cross-assembly phage(crAssphage). This study also examines how soil moisture content affects the decay of these fecal pollution indicators in soil amended with raw sludge and investigates the influence of conditioning treatments with cationic polyacrylamide(PAM), Fenton's reagents, Fe[Ⅲ]/CaO on their persistence in soil. The results indicated that the direct extraction method was the most effective and unbiased for recovering fecal pollution indicators from sludge-amended soil compared with the three elution-concentration methods. All fecal pollution indicators, except HAdV, remained stable under dry soil conditions, while high soil moisture content(48.39%-53.14%) slowed the decay rates of these indicators. during the application of sludge to soil, effective control of fecal pollution indicators was observed, with JCPyVand HAdV becoming undetectable within a short period. The log reduction values of HF183, BKPyV, and crAssphage ranged from 0.1 to 2.8 logs after 30 d of cultivation. The application of conditioned sludge, especially Fenton's reagent-conditioned sludge, resulted in a reduction in human fecal contamination in the receiving soil. Therefore, implementing appropriate conditioning methods, such as using Fenton's reagent, can effectively mitigate the health risks associated with fecal pathogens.

关键词： fecal pollution indicators sewage sludge conditioning treatment land application soil

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Spatial light modulation for femtosecond laser manufacturing:Current developments and challenges

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Science China(Technological Sciences) 2024年第1期67卷 60-72页

作者： ZAng Xue LIU ZiTing XU YiShi wang Yi wang Qing LI ZhenZe wang Lei State Key Laboratory of Integrated Optoelectronics College of Electronic Science and EngineeringJilin UniversityChangchun 130012China State Key Laboratory of Precision Measurement and Instruments Department of Precision InstrumentTsinghua UniversityBeijing 100084China

Since the invention of lasers,spatial-light-modulated laser processing has become a powerful tool for various *** enables multidimensional and dynamic modulation of the laser beam,which significantly improves the processing efficiency,accuracy,and flexibility,and presents wider prospects over traditional mechanical technologies for machining three-dimensional,hard,brittle,or transparent *** this review,we introduce:(1)The role of spatial light modulation technology in the development of femtosecond laser manufacturing;(2)the structured light generated by spatial light modulation and its generation methods;and(3)representative applications of spatial-light-modulated femtosecond laser manufacturing,includ.ng aberration correction,parallel processing,focal field engineering,and polarization ***,we summarize the present challenges in the field and possible future research.

关键词： femtosecond laser manufacturing spatial light modulation structured light aberration correction parallel processing focal field engineering polarization control

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Study on the spatial and temporal evolutionary characteristics of ozone concentration and the impact of human activities in China in 2019

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Acta Geochimica 2024年第5期43卷 985-995页

作者： Yongchun wang wang Zhang Yu’an Liu Yazhu wang Yuting Fu Zhaohui Feng Lingqing wang School of Geography South China Normal UniversityGuangzhou 510631China College of Urban and Environmental Sciences Hunan University of TechnologyZhuzhou 412007China Nanjing Institute of Geography and Limnology Chinese Academy of SciencesNanjing 210008China Institute of Geographical Sciences and Natural Resources Research Chinese Academy of SciencesBeijing 100101China

Ozone(O_(3))pollution has a profound impact on human health,vegetation development,and the ecological environment,making it a critical focus of global academic *** recent years,O_(3)pollution in China has been on a steady rise,with ozone emerging as the sole conventional pollutant to consistently increase in concentration without any *** study conducted a quantitative analysis of O_(3)concentrations across 367 Chinese cities in 2019,examining spatial autocorrelation and local clustering of O_(3)levels,and investigated the diverse relationships between human activity factors and O_(3)*** seasonal fluctuation of O_(3)exhibited the“M-type”pattern,with peak concentrations in winter and the lowest levels in *** center of O_(3)pollution migrated southeastward,with the area of highest concentration progressively shifting south along the eastern ***,O_(3)concentration showed a strong positive correlation with population density,road freight volume,and industrial emissions,suggesting that human activities,vehicle emissions,and industrial operations are significant contributors to O_(3)*** results provide comprehensive information on the characteristics,causes,and occurrence mechanism of O_(3)in Chinese cities that can be utilized by global government departments to formulate strategies to prevent and control O_(3)pollution.

关键词： Ozone concentration Urban agglomerations Human activities Spatial heterogeneity

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Atomically dispersed materials:Ideal catalysts in atomic era

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Nano Research 2024年第1期17卷 18-38页

作者： Tao Gan d.ngsheng wang department of Chemistry Tsinghua UniversityBeijing 100084China

Catalysts can accelerate the chemical reaction rate and effectively promote the molecules transformation,which is of great significance in the research of chemical industry and material *** extreme utilization of reactive sites has led to the emergence and development of atomically dispersed materials(AdMs).The highly active coordination unsaturated metal sites and fully utilized metal atoms make AdMs show great potential in catalytic *** adjustment of coordination environment and electronic structure provides more possibilities for constructing reactive centers with different *** review summarized the application and research progress of AdMs in different *** design strategy and structure–activity relationship of AdMs for specific reactions were summarized and ***,we also provided advices for the challenges and opportunities faced by AdMs in catalytic reactions.

关键词： atomically dispersed materials catalysis organic synthesis battery sensor enzyme

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Collective Molecular Machines: Multidimensionality and Reconfigurability

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Nano-Micro Letters 2024年第8期16卷 309-340页

作者： Bin wang Yuan Lu department of Chemical Engineering Tsinghua UniversityBeijing 100084People’s Republic of China Key Laboratory of Industrial Biocatalysis Ministry of EducationTsinghua UniversityBeijing 100084People’s Republic of China

Molecular machines are key to cellular activity where they are involved in converting chemical and light energy into efficient mechanical *** the last 60 years,designing molecular structures capable of generating unidirectional mechanical motion at the nanoscale has been the topic of intense *** progress has been made,attributed to advances in various fields such as supramolecular chemistry,biology and nanotechnology,and ***,individual molecular machines are only capable of producing nanometer work and generally have only a single *** order to address these problems,collective behaviors realized by integrating several or more of these individual mechanical units in space and time have become a new *** this review,we comprehensively discuss recent developments in the collective behaviors of molecular *** particular,collective behavior is divided into two *** is the appropriate integration of molecular machines to efficiently amplify molecular motions and deformations to construct novel functional *** other is the construction of swarming modes at the supramolecular level to perform nanoscale or microscale *** discuss design strategies for both modes and focus on the modulation of features and ***,in order to address existing challenges,the idea of transferring experience gained in the field of micro/nano robotics is presented,offering prospects for future developments in the collective behavior of molecular machines.

关键词： Molecular machines Collective control Collective behaviors dNA Biomolecular motors

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CFd-based hull optimization in calm water using adaptive grid deformation method

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Journal of Hydrodynamics 2024年第2期36卷 241-262页

作者： Shuguang wang Yonghwan Kim department of Naval Architecture and Ocean Engineering Seoul National UniversitySeoulKorea

This paper presents an adaptive grid deformation technique for optimizing ship hull forms using computational fluid dynamics(CFd).The proposed method enables accurate and smooth updates of the hull surface and 3-d CFd grids in response to design *** technique incorporates a two-level point-transformation approach to move the grid points by a few design ***,generic B-splines are utilized to transform grid points accord.ng to the displacements of the control points within a defined control *** ensures surface modification accuracy and smoothness,similar to those provided by non-uniform rational ***,radial basis functions are used to interpolate the movements of the control points with a limited set of design *** developed method effectively maintains the mesh quality and simulation *** applying this method to surface and grid adaptation,a regression model is proposed in the form of a second-order polynomial to represent the relationship between the geometric parameters and design *** polynomial is then used to introduce geometric ***,a radial basis function surrogate model for the calm-water resistance is constructed to approximate the objective *** enhanced optimization framework is proposed for CFd–based hull optimization and applied to KVLCC2 to validate its feasibility and efficiency.

关键词： Hull-form optimization adaptive grid deformation ship resistance OpenFOAM radial basis function(RBF)surrogate model

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Composition Engineering Opens an Avenue Toward Efficient and Sustainable Nitrogen Fixation

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Energy & Environmental Materials 2024年第1期7卷 313-325页

作者： Xiaolin wang Liming Yang Key Laboratory of Material Chemistry for Energy Conversion and Storage Ministry of EducationWuhan 430074China Hubei Key Laboratory of Materials Chemistry and Service Failure Wuhan 430074China Hubei Key Laboratory of Bioinorganic Chemistry and Materia Medica Wuhan 430074China Hubei Engineering Research Center for Biomaterials and Medical Protective Materials Wuhan 430074China School of Chemistry and Chemical Engineering Huazhong University of Science and TechnologyWuhan 430074China

In this work,we open an avenue toward rational design of potential efficient catalysts for sustainable ammonia synthesis through composition engineering strategy by exploiting the synergistic effects among the active sites as exemplified by diatomic metals anchored graphdiyne via the combination of hierarchical high-throughput screening,first-principles calculations,and molecular dynamics *** 43 highly efficient catalysts feature ultralow onset potentials(|U_(onset)|≤0.40 V)with Rh-Hf and Rh-Ta showing negligible onset potentials of 0 and-0.04 V,*** high catalytic activities of Rh-Hf and Rh-Ta can be ascribed to the synergistic *** forming heteronuclears,the combinations of relatively weak(such as Rh)and relatively strong(such as Hf or Ta)components usually lead to the optimal strengths of adsorption Gibbs free energies of reaction *** origin can be ascribed to the mediate d-band centers of Rh-Hf and Rh-Ta,which lead to the optimal adsorption strengths of intermediates,thereby bringing the high catalytic *** work provides a new and general strategy toward the architecture of highly efficient catalysts not only for electrocatalytic nitrogen reduction reaction(eNRR)but also for other important *** expect that our work will boost both experimental and theoretical efforts in this direction.

关键词： composition engineering strategy diatomic catalysts electrocatalytic nitrogen reduction reaction first-principles calculations graphdiyne hierarchical high-throughput screening synergistic effects

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Hollow structured Fe@C nanorods for boosting dehydrogenation properties of α-AlH_(3)

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Nano Research 2024年第9期17卷 8184-8191页

作者： Yuan Zhao Qingshuang wang d.ngming Yin Xiaoli wang Shouliang Li Chunli wang Long Liang Shaolei Zhao Limin wang Yong Cheng School of Materials Science and Engineering Changchun University of Science and TechnologyChangchun 130022China State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China Shand.ng Provincial Key Laboratory of Monocrystalline Silicon Semiconductor Materials and Technology College of Chemistry and Chemical EngineeringDezhou UniversityDezhou 253023China Henan Nayu New Material Co. Ltd.Xinxiang 453000China

α-AlH_(3)is regarded as one of the most promising hydrogen storage materials due to its high hydrogen storage capacity(10.1 wt.%,148 kg·m^(-3)).However,in practical applications,the associated hydrogen release temperature remains relatively *** effectively address this issue,hollow structured Fe@C nanorods derived from Fe-MOF are introduced as highly efficient catalyst to optimize the dehydrogenation properties ofα-AlH_(3).Comparatively,the initial hydrogen release temperature ofα-AlH_(3)+3 wt.%Fe@C is reduced to 94.2℃,which is significantly lower than that of pureα-AlH_(3)(137.8℃).At 100 and 120℃,it exhibits hydrogen capacities of 5.38 wt.%and 7.47 wt.%,respectively,whereas pureα-AlH_(3)only delivers hydrogen capacities of 0.24 wt.%and 5.94 wt.%under the same *** density functional theory(dFT)calculations further indicate that the existence of Fe@C catalyst can make the length of Al-H bond increase,which is more conducive to the release of *** results show that the synergistic effect of Fe and porous carbon in Fe@C nanorods can improve the hydrogen desorption kinetics ofα-AlH_(3),provid.ng a good prospect for the application ofα-AlH_(3)in hydrogen storage fields.

关键词： Fe@C α-AlH_(3) dehydrogenation catalyst

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