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Pb induced dislocation defects of PtCo systems: Strain-triggered oxygen reduction reaction for PEMFC

Nano Research 2024年第4期17卷 2462-2472页

作者： chun Jin Qiheng wang Jingjun liu Beijing Key Laboratory of Electrochemical Process and Technology for Materials Beijing 100029China Beijing University of Chemical Technology Beijing 100029China

Design and development of advanced electrocatalysts with high performance and low Pt consumption are crucial for reducing the kinetic energy barrier of the cathode oxygen reduction reaction(ORR)and improving the efficiency of proton exchange membrane fuel cells(PEMFC).In this study,we demonstrate a Pb-modulated PtCo system for efficient ORR,in which the inclusion of Pb in ternary alloys induces dislocation defects due to the significant difference in atomic ***-PtCoPb was confirmed to exhibit significantly higher ORR activity and stability in acidic *** practical PEMFC applications,it outperforms the corresponding commercial Pt/C with a mass activity of 0.58 A·mgPt^(-1),making it a promising alternative to state-of-the-art Pt-based *** combination of experimental results and density functional theory(DFT)calculations offers valuable atomic-level insights into the dislocation *** with a larger atomic radius is located in the lattice stretching region below the dislocation slip plane,forming a structure similar to a Cottrell atmosphere,which reduces the dislocation energy and puts the system in a lower energy *** Cottrell atmosphere pins the dislocation structure and stabilizes the ternary *** adjusting the amount of added Pb,a moderate level of dislocation density induces a tuned strain effect,thereby enhancing the electrocatalytic mechanism by optimizing the electronic structure of the alloy surface and the adsorption and desorption of oxygen *** work provides valuable insights into the design and development of lattice dislocation defect structures to trigger strain effects for improving ORR performance.

关键词： dislocation defect strain effect Pb-modulated oxygen reduction reaction

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Cathepsin B protease is required for metamorphism in silkworm, Bombyx moil

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Insect Science 2008年第3期15卷 201-208页

作者： Gen-Hong wang chun liu Qing-You Xia Xing-Fu Zha Jie Chen Liang Jiang Key Sericultural Laboratory of the Agricultural Ministry College of Biotechnology Southwest University Chongqing China

Cathepsin B belongs to lysosomal cysteine protease of the papain family. Temporal and spatial expression analysis of cathepsin B of Bombyx mori （BmCtB） was carried out based on Expression Sequence Tags （ESTs） data, oligonucleotide microarray, reverse transcription polymerase chain reaction （RT-PCR） and quantitative real-time PCR. Expression of BmCtB was observed in all of the tissues and stages. Among the 10 tested tissues, the fat body and posterior silk gland are the two most enriched tissues with BmCtB. During Bombyx development, there was an expression fastigium of BmCtB during metamorphosis. RNA interference was used to suppress the expression of cathepsin B during metamorphosis. Significant developmental defective phenotypes were obtained in the RNAi treated group. The dramatically reduced expression of BmCtB was con^rmed by Northern blot and quantitative real-time PCR. These evidences strongly suggest cathepsin B proteinase was predominantly involved in the metabolism process of fat body and the posterior silk gland and was critical for metamorphism and development of silkworm, Bombyx mori.

关键词： cathepsin B RNA interference quantitative real-time PCR Bombyx mori

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Reconstruction of Gene Regulatory Networks Based on Two-Stage Bayesian Network Structure Learning Algorithm

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Journal of Bionic Engineering 2009年第1期6卷 86-92页

作者： Gui-xia liu, Wei Feng, Han wang, Lei liu, chun-guang ZhouCollege of Computer Science and Technology, Jilin University, Changchun 130012,P.R. China College of Computer Science and Technology Jilin University Changchun P. R. China

In the post-genomic biology era,the reconstruction of gene regulatory networks from microarray gene expression data is very important to understand the underlying biological system,and it has been a challenging task in *** Bayesian network model has been used in reconstructing the gene regulatory network for its advantages,but how to determine the network structure and parameters is still important to be *** paper proposes a two-stage structure learning algorithm which integrates immune evolution algorithm to build a Bayesian *** new algorithm is evaluated with the use of both simulated and yeast cell cycle *** experimental results indicate that the proposed algorithm can find many of the known real regulatory relationships from literature and predict the others unknown with high validity and accuracy.

关键词： gene regulatory networks two-stage learning algorithm Bayesian network immune evolutionary algorithm

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Relationship Between Short-chain Fatty Acids and Parkinson’s Disease:A Review from Pathology to Clinic

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Neuroscience Bulletin 2024年第4期40卷 500-516页

作者： Wen-Xiang Duan Fen wang Jun-Yi liu chun-Feng liu Department of Neurology and Clinical Research Center of Neurological Disease The Second Affiliated Hospital of Soochow UniversitySuzhou215004China Department of Neurology Dushu Lake Hospital affiliated to Soochow UniversitySuzhou215125China Jiangsu Key Laboratory of Neuropsychiatric Diseases and Institute of Neuroscience Soochow UniversitySuzhou215123China

Parkinson’s disease(PD)is a complicated neurodegenerative disease,characterized by the accumulation ofα-synuclein(α-syn)in Lewy bodies and neurites,and massive loss of midbrain dopamine *** evidence suggests that gut microbiota and microbial metabolites are involved in the development of *** these,short-chain fatty acids(SCFAs),the most abundant microbial metabolites,have been proven to play a key role in brain-gut *** this review,we analyze the role of SCFAs in the pathology of PD from multiple dimensions and summarize the alterations of SCFAs in PD patients as well as their correlation with motor and non-motor *** research should focus on further elucidating the role of SCFAs in neuroinflammation,as well as developing novel strategies employing SCFAs and their derivatives to treat PD.

关键词： Parkinson’s disease Short-chain fatty acids Microbial metabolites Brain-gut-microbiota axis

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A method to interpret fracture aperture of rock slope using adaptive shape and unmanned aerial vehicle multi-angle nap-of-the-object photogrammetry

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第3期16卷 924-941页

作者： Mingyu Zhao Shengyuan Song Fengyan wang chun Zhu Dianze liu Sicong wang College of Construction Engineering Jilin UniversityChangchun130026China College of Geo-Exploration Science and Technology Jilin UniversityChangchun130026China Institute of Engineering Geology and Geohazards Hohai UniversityNanjing210098China

The aperture of natural rock fractures significantly affects the deformation and strength properties of rock masses,as well as the hydrodynamic properties of fractured rock *** conventional measurement methods are inadequate for collecting data on high-steep rock slopes in complex mountainous *** study establishes a high-resolution three-dimensional model of a rock slope using unmanned aerial vehicle(UAV)multi-angle nap-of-the-object photogrammetry to obtain edge feature points of *** opening morphology is characterized using coordinate projection and *** central axis is determined using vertical measuring lines,allowing for the interpretation of aperture of adaptive fracture *** feasibility and reliability of the new method are verified at a construction site of a railway in southeast Tibet,*** study shows that the fracture aperture has a significant interval effect and size *** optimal sampling length for fractures is approximately 0.5e1 m,and the optimal aperture interpretation results can be achieved when the measuring line spacing is 1%of the sampling *** fractures in the study area generally have larger apertures than shear fractures,and their tendency to increase with slope height is also greater than that of shear *** aperture of tensile fractures is generally positively correlated with their trace length,while the correlation between the aperture of shear fractures and their trace length appears to be *** of different orientations exhibit certain differences in their distribution of aperture,but generally follow the forms of normal,log-normal,and gamma *** study provides essential data support for rock and slope stability evaluation,which is of significant practical importance.

关键词： Unmanned aerial vehicle(UAV) photogrammetry High-steep rock slope Fracture aperture Interval effect Size effect Parameter interpretation

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Double-confined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C toward ultra-stable Li-/Na-ion batteries

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Rare Metals 2024年第5期43卷 2067-2079页

作者： Dan wang Qun Ma Huan He Zhi-Yuan wang Run-Guo Zheng Hong-Yu Sun Yan-Guo liu chun-Li liu School of Materials Science and Engineering Northeastern UniversityShenyang110819China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province Qinhuangdao 066004China Department of Physics and Oxide Research Center Hankuk University of Foreign StudiesYongin 17035Korea

Antimony-based materials with high capacities and moderate potentials are promising anodes for lithium-/-sodium-ion ***,their tremendous volume expansion and inferior conductivity lead to poor structural stability and sluggish reaction ***,a doubleconfined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C has been fabricated through a solvothermal method followed by low-temperature heat *** dual protection of“MXene”and“carbon”can better accommodate the volume expansion of Sb/Sb_(2)S_(3).The strong covalent bond(Ti-S,Ti-O-Sb,C-O-Sb)can firmly integrate Sb-based material with Ti_(3)C_(2)T_(x)and carbon,which significantly improves the structure *** addition,the carbon layer can restrain the oxidation of MXenes,and the nano-Sb/Sb_(2)S_(3)can facilitate electron/ion transport and suppress the restacking of *** heterogeneous interface between Sb and Sb_(2)S_(3)can further promote interfacial charge *** MXene-Sb/Sb_(2)S_(3)@C-1 with the optimal Sb content shows high specific capacities,comparable rate properties and ultra-stable cycling performances(250 m Ah·g^(-1)after 2500 cycles at 1 A·g^(-1)for sodium-ion batteries).Ex situ X-ray diffractometer(XRD)test reveals the storage mechanism including the conversion and alloying process of MXene-Sb/Sb_(2)S_(3)@*** voltammetry(CV)test results demonstrate that the pseudocapacitance behavior is dominant in MXene-Sb/Sb_(2)S_(3)@C-1,especially at large *** design paves the way for exploring high-performance alloy-based/conversion-type anode for energy storage devices.

关键词： Sb/Sb_(2)S_(3) MXene Carbon Anode Lithium-ion batteries Sodium-ion batteries

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Reactive oxygen species:Multidimensional regulators of plant adaptation to abiotic stress and development

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Journal of Integrative Plant Biology 2024年第3期66卷 330-367页

作者： Pengtao wang Wen-Cheng liu Chao Han Situ wang Ming-Yi Bai chun-Peng Song State Key Laboratory of Crop Stress Adaptation and Improvement School of Life SciencesHenan UniversityKaifeng 475004China The Key Laboratory of Plant Development and Environmental Adaptation Biology Ministry of EducationSchool of Life SciencesShandong UniversityQingdao 266237China Faculty of Science McGill UniversityMontreal H3B1X8Canada

Reactive oxygen species(ROS)are produced as undesirable by-products of metabolism in various cellular compartments,especially in response to unfavorable environmental conditions,throughout the life cycle of *** ROS production disrupts normal cellular function and leads to oxidative *** cope with excessive ROS,plants are equipped with a sophisticated antioxidative defense system consisting of enzymatic and non-enzymatic components that scavenge ROS or inhibit their harmful effects on ***,when maintained at relatively low levels,ROS act as signaling molecules that regulate plant growth,development,and adaptation to adverse ***,we provide an overview of current approaches for detecting *** also discuss recent advances in understanding ROS signaling,ROS metabolism,and the roles of ROS in plant growth and responses to various abiotic stresses.

关键词： abiotic stress growth and development plant reactive oxygen species

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Molecular mechanism for the unusual enhancement of the second-step chemiluminescence production from the carcinogenic tetrabromohydroquinone and H2O_(2)

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Journal of Environmental Sciences 2024年第7期141卷 330-342页

作者： Zi-Han wang chun-Hua Huang Zhi-Sheng liu Li Mao Ben-Zhan Zhu State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China College of Environment and Resources University of Chinese Academy of SciencesBeijing 100049China

We have found recently that two-step intrinsic hydroxyl radical(·OH)-dependent chemiluminescence(CL)could be produced by carcinogenic tetrahaloquinone and H_(2)O_(2).However,the first-step CL was too fast to clearly detect the stepwise generation of·OH and CL,and to distinguish the exact dividing point between the first-step and second-step *** we found that,extremely clear two-step intrinsic CL could be produced by the relative slow reaction of tetrabromohydroquinone(TBHQ)with H_(2)O_(2),which was directly dependent on the two-step·OH ***,the second-step,but not the first-step CL production of TBHQ/H_(2)O_(2)(CRET donor)was markedly enhanced by fluorescein(a typical xanthene dye,CRET acceptor)through a unique chemiluminescence resonance energy transfer(CRET)*** novel CRET system of TBHQ/H_(2)O_(2)/fluorescein was successfully applied for the sensitive detection of TBHQ with the detection limit as low as 2.5μmol/*** findings will help to develop more sensitive and highly efficient CL or CRET systems and specific CL sensor to detect the carcinogenic haloquinones,which may have broad environmental applications.

关键词： Two-step chemiluminescence Bromohydroquinone Hydrogen peroxide Hydroxyl radical CRET

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Constructing highly safe and long-life calcium ion batteries based on hydratedvanadium oxide cathodes featuring a pillar structure

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Rare Metals 2024年第6期43卷 2597-2612页

作者： chun-Fang wang Shi-Wei Zhang Lan Huang Yuan-Min Zhu Feng liu Jian-Chuan wang Li-Ming Tan chun-Yi Zhi Cui-Ping Han Powder Metallurgy Research Institute Central South UniversityChangsha410083China Songshan Lake Materials Laboratory Dongguan 523808China Research Institute of Interdisciplinary Science and School of Materials Science and Engineering Dongguan University of TechnologyDongguan 523808China Department of Materials Science and Engineering City University of Hong KongHong Kong 999077China Faculty of Materials Science and Energy Engineering/Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China

Calcium-ion batteries(CIBs)have generated intense interest due to the growing demand for safer,cheaper,and large-scale energy storage ***,their development is still in its infancy,owing to the lack of suitable cathodes for sustaining reversiblc Ca^(2+)intercalation/***,layered H_(2)V_(3)O_(8)(HVO)with Zn^(2+)pre-insertion(ZHVO)is reported as a high-rate and highly durable cathode material for *** existence of Zn^(2+)and H_(2)O pillars could expand the interlayer spacing up to 1.8 nm,which is favorable for the diffusion of bulky Ca^(2+).The formation of Zn-O bonds facilitates electron transfer and enhances electrical ***,the ZHVO cathode achieves superior capacity performance(213.9 mAh·g^(-1)at 0.2 A·g^(-1))and long lifespan(78.3%for 1,000 cycles at 5 A·g^(-1))compared to pristine *** functional theory(DFT)calculations revealed that Zn^(2+)moved during Ca^(2+)intercalation,thereby reducing the diffusion energy barrier and facilitating Ca^(2+)***,a safe aqueous calcium ion cell was successfully assembled.

关键词： Multivalent batteries Calcium-ion batteries Layered structure Vanadium oxide Cathode materials

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Systematic bibliometric and visualized analysis of research hotspots and trends on the application of artificial intelligence in glaucoma from 2013 to 2022

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International Journal of Ophthalmology(English edition) 2024年第9期17卷 1731-1742页

作者： chun liu Lu-Yao wang Ke-Yu Zhu chun-Meng liu Jun-Guo Duan Eye School of Chengdu University of TCM Chengdu 610072Sichuan ProvinceChina Ineye Hospital of Chengdu University of TCM Chengdu 610084Sichuan ProvinceChina Key Laboratory of Sichuan Province Ophthalmopathy Prevention&Cure and Visual Function Protection with TCM Laboratory Chengdu 610072Sichuan ProvinceChina

AIM:To conduct a bibliometric analysis of research on artificial intelligence(AI)in the field of glaucoma to gain a comprehensive understanding of the current state of research and identify potential new directions for future ***:Relevant articles on the application of AI in the field of glaucoma from the Web of Science Core Collection were retrieved,covering the period from January 1,2013,to December 31,*** order to assess the contributions and co-occurrence relationships among different countries/regions,institutions,authors,and journals,CiteSpace and VOSviewer software were employed and the research hotspots and future trends within the field were ***:A total of 750 English articles published between 2013 and 2022 were collected,and the number of publications exhibited an overall increasing *** majority of the articles were from China,followed by the United States and *** University of Singapore,Chinese Academy of Sciences,and Sun Yat-sen University made significant contributions to the published *** RN and Fu HZ ranked first among authors and cited *** Journal of Ophthalmology is the most impactful academic journal in the field of AI application in *** disciplinary scope of this field includes ophthalmology,computer science,mathematics,molecular biology,genetics,and other related *** clustering and identification of keyword nodes in the co-occurrence network reveal the evolving landscape of AI application in the field of ***,the hot topics in this field were primarily“segmentation”,“classification”and“diagnosis”.However,in recent years,the focus has shifted to“deep learning”,“convolutional neural network”and“artificial intelligence”.CONCLUSION:With the rapid development of AI technology,scholars have shown increasing interest in its application in the field of ***,the application of AI in assisting treatment and predicting prognosis in glaucom

关键词： glaucoma ar tificial intelligence bibliometrics

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