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Exploring formation mechanism and source attribution of ozone during the 2019 Wuhan Military World Games:Implications for ozone control strategies

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Journal of Environmental sciences 2024年第2期136卷 400-411页

作者： lei zhang lili wang Runyu wang Nan chen Yuan yang Ke li Jie Sun Dan Yao Yuesi wang Minghui Tao yang Sun Institute of Atmospheric Physics Chinese Academy of SciencesBeijing 100029China university of the Chinese Academy of sciences Beijing 100049China Hubei Ecological Environment Monitoring Center Station Wuhan 430072China Guizhou Research and Designing Institute of Environmental sciences Guizhou Academy of Environmental Science and DesignGuiyang 550081China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and EngineeringNanjing University of Information Science and TechnologyNanjing 210044China school of Environment Key Laboratory for Yellow River and Huai River Water Environment and Pollution ControlMinistry of EducationHenan Normal UniversityXinxiang 453007China Key Laboratory of Regional Ecology and Environmental Change School of Geography and Information EngineeringChina University of GeosciencesWuhan 430074China

A series of emission reduction measures were conducted in Wuhan,Central china,to ensure good air quality during the 7th Military World Games(MWG)in October *** better understand the implications for ozone(O_(3))pollution control strategies,we applied integrated analysis approaches based on the de-weathered statistical model,parameterization methods,chemical box model,and positive matrix factorization *** the MWG,concentrations of O_(3),NO_x,and volatile organic compound(VOCs),OFP(O_(3)formation potential),L_(OH)(OH radical loss rate)were 83μg/m^(3),43μg/m^(3),26 ppbv,188μg/m^(3),and 3.9 s^(-1),respectively,which were 26%,18%,3%,15%,and 13%lower than pre-MWG values and 6%,39%,30%,33%,and 50%lower than post-MWG values,*** removing meteorological influence,O_(3)and its precursors during the MWG decreased largely compared with post-MWG values,and only O_(3),NO_(2),and oxygenated VOCs(OVOCs)declined compared with pre-MWG values,which revealed the emission reduction measures during the MWG played an important role for O_(3)*** six VOCs sources,the mass contributions of biomass burning and solvents usage during the MWG decreased largely compared with pre-MWG values.O_(3)production was sensitive to VOCs and the key species were aromatics,OVOCs,and alkenes,which originated mainly from solvents usage,biomass burning,industrial-related combustion,and vehicle *** O_(3)concentration during the strict control was mainly caused by OVOCs reduction due to biomass burning ***,the O_(3)abatement strategies of Wuhan should be focused on the mitigation of high-reactivity VOCs.

关键词： VOCs Ozone Wuhan Military World Games Source apportionment Relative incremental reactivity Random forest

A semi-analytical model for coupled flow in stress-sensitive multi-scale shale reservoirs with fractal characteristics

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Petroleum science 2024年第1期21卷 327-342页

作者： Qian zhang Wen-Dong wang Yu-liang Su Wei chen zheng-Dong lei lei li Yong-Mao Hao Key Laboratory of Unconventional Oil&Gas Development(china university of Petroleum(East china)) Ministry of EducationQingdao266580ShandongChina school of Petroleum engineering China University of Petroleum(East China)Qingdao266580ShandongChina Shale Oil Development Branch Changqing Oilfield CompanyPetroChinaQingyang745708GansuChina Petrochina Research Institute of Petroleum Exploration&Development Beijing100083China

A large number of nanopores and complex fracture structures in shale reservoirs results in multi-scale flow of oil. With the development of shale oil reservoirs, the permeability of multi-scale media undergoes changes due to stress sensitivity, which plays a crucial role in controlling pressure propagation and oil flow. This paper proposes a multi-scale coupled flow mathematical model of matrix nanopores, induced fractures, and hydraulic fractures. In this model, the micro-scale effects of shale oil flow in fractal nanopores, fractal induced fracture network, and stress sensitivity of multi-scale media are considered. We solved the model iteratively using Pedrosa transform, semi-analytic Segmented Bessel function, Laplace transform. The results of this model exhibit good agreement with the numerical solution and field production data, confirming the high accuracy of the model. As well, the influence of stress sensitivity on permeability, pressure and production is analyzed. It is shown that the permeability and production decrease significantly when induced fractures are weakly supported. Closed induced fractures can inhibit interporosity flow in the stimulated reservoir volume (SRV). It has been shown in sensitivity analysis that hydraulic fractures are beneficial to early production, and induced fractures in SRV are beneficial to middle production. The model can characterize multi-scale flow characteristics of shale oil, providing theoretical guidance for rapid productivity evaluation.

关键词： Multi-scale coupled flow Stress sensitivity Shale oil Micro-scale effect Fractal theory

Co/N co-doped flower-like carbon-based phase change materials toward solar energy harvesting

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Aggregate 2024年第1期5卷 321-330页

作者： Xiao chen lei wang Yan Gao yang li Xiaowei zhang Yu Jiang Ge wang Institute of Advanced Materials Beijing Normal UniversityBeijingChina beijing Advanced Innovation Center for Materials Genome engineering Beijing Key Laboratory of Function Materials for Molecule and Structure ConstructionSchool of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijingChina

The photothermal conversion capacity of pristine organic phase change materials(PCMs)is inherently insufficient in solar energy *** upgrade their photothermal conversion capacity,we developed bimetallic zeolitic imidazolate framework(ZIF)derived Co/N co-doped flower-like carbon(Co/N-FLC)-based composite PCMs toward solar energy harvesting.3D interconnected carbon framework with low interfacial thermal resistance,abundant carbon defects and high content of nitrogen doping,excellent localized surface plasmon resonance(LSPR)effect of Co nanoparticles,and light absorber Co_(3)ZnC in Co/N-FLC synergistically upgrade the photothermal capacity of(polyethylene glycol)PEG@Co/N-FLC composite PCMs with an ultrahigh photothermal conversion efficiency of 94.8%under 0.16 W/cm^(2).Uniformly anchored Co and Co_(3)ZnC nanoparticles in carbon framework guarantee excellent photon capture *** carbon nanotubes(CNTs)in 2D carbon nanosheets further accelerate the rapid transport of phonons by constructing cross-connected heat transfer ***,PEG@Co/N-FLC exhibits a thermal energy storage density of 100.69 J/g and excellent thermal stability and durable ***,PEG@Co/N-FLC composite PCMs are promising candidates to accelerate the efficient utilization of solar energy.

关键词： bimetallic ZIF Co/N co-doped carbon phase change materials photothermal conversion thermal energy storage

Highly transparent anti-reflection coating enhances the underwater efficiency and stability of perovskite solar modules

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Nano Research 2024年第9期17卷 8126-8133页

作者： Feng Qian Shihao Yuan Ting zhang lei wang Xiaobo li Hualin zheng Qien Xu Zhi David chen Shibin li school of Optoelectronic science and engineering University of Electronic Science and Technology of ChinaChengdu 610054China Department of Electrical and computer engineering and Center for Nanoscale science and engineering University of KentuckyLexingtonKentucky 40506USA

Perovskite solar cells have shown great potential in the field of underwater solar cells due to their excellent optoelectronic properties;however,their underwater performance and stability still hinder their practical *** this research,a 1H,1H,2H,2H-heptadecafluorodecyl acrylate(HFDA)anti-reflection coating(ARC)was introduced as a high-transparent material for encapsulating perovskite solar modules(PSMs).Optical characterization results revealed that HFDA can effectively reduce reflection of light below 800 nm,aiding in the absorption of light within this wavelength range by underwater solar ***,a remarkable efficiency of 14.65%was achieved even at a water depth of 50 ***,the concentration of Pb^(2+)for HFDA-encapsulated film is significantly reduced from 186 to 16.5 ppb after being immersed in water for 347 ***,the encapsulated PSMs still remained above 80%of their initial efficiency after continuous underwater illumination for 400 ***,being exposed to air,the encapsulated PSMs maintained 94%of their original efficiency after 1000 h light *** highly transparent ARC shows great potentials in enhancing the stability of perovskite devices,applicable not only to underwater cells but also extendable to land-based photovoltaic devices.

关键词： underwater photovoltaics perovskite solar modules anti-reflection coating underwater stability

Nano-alumina@cellulose-coated separators with the reinforcedconcrete-like structure for high-safety lithium-ion batteries

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Chinese Journal of Chemical engineering 2024年第4期68卷 83-93页

作者： Zhihao yang li chen Jian Xue Miaomiao Su Fangdan zhang liangxin Ding Suqing wang Haihui wang Guangdong Provincial Key Lab of Green Chemical Product Technology School of Chemistry and Chemical EngineeringSouth China University of TechnologyGuangzhou 510640China beijing Key Laboratory of Membrane Materials and engineering Department of Chemical EngineeringTsinghua UniversityBeijing 100084China

Separators play a critical role in the safety and performance of lithium-ion ***,commercial polyolefin separators are limited by their poor affinity with electrolytes and low melting *** this work,we constructed a reinforced-concrete-like structure by homogeneously dispersing nano-Al_(2)O_(3) and cellulose on the separators to improve their stability and *** this reinforcedconcrete-like structure,the cellulose is a reinforcing mesh,and the nano-Al_(2)O_(3) acts as concrete to support the *** constructing the reinforced-concrete-like structure,the separators exhibit good stability even at 200℃(thermal shrinkage of 0.3%),enhanced tensile strain(tensile stress of 133.4 MPa and tensile strains of 62%),and better electrolyte wettability(a contact angle of 6.5°).Combining these advantages,the cells with nano-Al_(2)O_(3)@cellulose-coated separators exhibit stable cycling performance and good rate ***,the construction of the reinforced-concretelike structure is a promising technology to promote the application of lithium-ion batteries in extreme environments.

关键词： Alumina Nanomaterials lithium-ion batteries Membranes Cellulose Reinforced-concrete-like structure

Hierarchical Game Approach for Optimization of Regional Integrated Energy System Clusters Considering Bounded Rationality

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CSEE Journal of Power and Energy Systems 2024年第1期10卷 302-313页

作者： lei Dong Mengting li Junjie Hu Sheng chen Tao zhang Xinying wang Tianjiao Pu school of Electrical and Electronic engineering North China Electric Power UniversityBeijing 102206China Department of Artificial Intelligence Application Research China Electric Power Research InstituteBeijing 100192China Key Laboratory of Smart Grid of Ministry of Education Key Laboratory of Smart Energy&Information Technology of Tianjin MunicipalityTianjin UniversityTianjin 300072China

Regional integrated energy system(RIES)cluster,i.e.,multi-source integration and multi-region coordination,is an effective approach for increasing energy utilization *** hierarchical architecture and limited information sharing of RIES cluster make it difficult for traditional game theory to accurately describe their game ***,a hierarchical game approach considering bounded rationality is proposed in this paper to balance the interests of optimizing RIES cluster under privacy protection.A Stackelberg game with the cluster operator(CO)as the leader and multiple RIES as followers is developed to simultaneously optimize leader benefit and RIES utilization ***,a slight altruistic function is introduced to simulate the game behavior of each RIES agent on whether to cooperate or *** introducing an evolutionary game based on bounded rationality in the lower layer,the flaw of the assumption that participants are completely rational can be ***,for autonomous optimal dispatching,each RIES is treated as a prosumer,fexibly switching its market participation role to achieve cluster coordination *** studies on a RIES cluster verify effectiveness of the proposed approach.

关键词： Bounded rationality coordinated optimization evolutionary game regionaIilntegrated energysystem stackelberg game

Weakly supervised point cloud segmentation via deep morphological semantic information embedding

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CAAI Transactions on Intelligence Technology 2024年第3期9卷 695-708页

作者： Wenhao Xue yang yang lei li Zhongling Huang Xinggang wang Junwei Han Dingwen zhang school of Automation Northwestern Polytechnical UniversityXi'anChina Institute of Mechanical and Electrical engineering BeijingChina school of Electronic Information and Communications Huazhong University of Science and TechnologyWuhanChina

Segmenting the semantic regions of point clouds is a crucial step for intelligent agents to understand 3D *** supervised point cloud segmentation is highly desirable because entirely labelling point clouds is highly time-consuming and *** the low-costing labelling of 3D point clouds,the scene-level label is one of the most effortless label ***,due to the limitation of classifier discriminative capability and the orderless and structurless nature of the point cloud data,existing scene-level method is hard to transfer the semantic information,which usually leads to the under-activated or over-activated *** this end,a local semantic embedding network is introduced to learn local structural patterns and semantic ***,the proposed network contains graph convolution-based dilation and erosion embedding modules to implement‘inside-out’and‘outside-in’semantic information dissemination ***,the proposed weakly supervised learning framework could achieve the mutual propagation of semantic information in the foreground and *** experiments on the widely used ScanNet benchmark demonstrate the superior capacity of the proposed approach when compared to the current alternatives and baseline models.

关键词： artificial intelligence computer vision deep learning

Metal-organic framework-derived CoSe_(2)@N-doped carbon nanocubes for high-performance lithium-ion capacitors

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Rare Metals 2024年第5期43卷 2150-2160页

作者： lei wang Xiong zhang Yan-Yan Kong chen li Ya-Bin An Xian-Zhong Sun Kai wang Yan-Wei Ma Institute of Electrical engineering Chinese Academy of SciencesBeijing 100190China school of engineering sciences University of Chinese Academy of SciencesBeijing 100190China Institute of Electrical engineering and Advanced Electromagnetic Drive Technology Qilu ZhongkeJinan 250013China school of Materials science and engineering Zhengzhou UniversityZhengzhou 450001China

Cobalt selenide(CoSe_(2))has garnered considerable attention as a prospective anode candidate for advanced lithium-ion storage,prompting comprehensive ***,CoSe_(2)-based anodes usually suffer from significant volume variation upon lithiation leading to unsatisfactory cycling ***,a versatile synthesis route is proposed for the in-situ fabrication of CoSe2nanoparticles embedded in N-dope carbon skeleton(CoSe_(2)@NC)through annealing treatment and selenization of a metal–organic framework-derived(MOF)*** N-doped carbon derived from the MOF serves not only as an excellent conductive substrate but also as a confined reactor,effectively inhibiting the structural instability and alleviating the inevitable volume change of CoSe_(2).Owing to their unique nanostructure,the as-prepared CoSe_(2)@NC exhibits a high capacity of 745.9mAh·g^(-1)at 0.1 A·g^(-1),while maintaining excellent rate capability and an impressive ***,the assembled lithium-ion capacitor(liC)based on CoSe_(2)@NC demonstrates an energy density of 130Wh·kg^(-1),a power density of 24.6 kW·kg^(-1),and remarkable capacity retention of 90.8%after 8000 *** results highlight the great potential of CoSe_(2)@NC for practical applications.

关键词： lithium capacitors Cobalt selenide Metal-organic frameworks N-doped carbon

Improved simulation of winter wheat yield in North china Plain by using PRYM-Wheat integrated dry matter distribution coefficient

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Journal of Integrative Agriculture 2024年第4期23卷 1381-1392页

作者： Xuan li Shaowen wang Yifan chen Danwen zhang Shanshan yang Jingwen wang Jiahua zhang Yun Bai Sha zhang Research Center for Remote Sensing and Digital Earth College of Computer Science and TechnologyQingdao UniversityQingdao266071China Center for Geospatial Information Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China school of Geographical sciences Hebei Normal UniversityShijiazhuang 050024China

The accurate simulation of regional-scale winter wheat yield is important for national food security and the balance of grain supply and demand in ***,most remote sensing process models use the“biomass×harvest index(HI)”method to simulate regional-scale winter wheat ***,spatiotemporal differences in HI contribute to inaccuracies in yield simulation at the regional ***-series dry matter partition coefficients(Fr)can dynamically reflect the dry matter partition of winter *** this study,Fr equations were fitted for each organ of winter wheat using site-scale *** equations were then coupled into a process-based and remote sensingdriven crop yield model for wheat(PRYM-Wheat)to improve the regional simulation of winter wheat yield over the North china Plain(NCP).The improved PRYM-Wheat model integrated with the fitted Fr equations(PRYM-Wheat-Fr)was validated using data obtained from provincial yearbooks.A 3-year(2000-2002)averaged validation showed that PRYM-Wheat-Fr had a higher coefficient of determination(R^(2)=0.55)and lower root mean square error(RMSE=0.94 t ha^(-1))than PRYM-Wheat with a stable HI(abbreviated as PRYM-Wheat-HI),which had R^(2) and RMSE values of 0.30 and 1.62 t ha^(-1),*** PRYM-Wheat-Fr model also performed better than PRYM-Wheat-HI for simulating yield in verification years(2013-2015).In conclusion,the PRYM-Wheat-Fr model exhibited a better accuracy than the original PRYM-Wheat model,making it a useful tool for the simulation of regional winter wheat yield.

关键词： dry matter partition remote sensing model winter wheat yield North china Plain