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Double-confined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C toward ultra-stable Li-/Na-ion batteries

Rare Metals 2024年第5期43卷 2067-2079页

作者： Dan wang Qun Ma Huan He Zhi-Yuan wang Run-guo Zheng Hong-Yu Sun Yan-guo Liu Chun-Li Liu School of Materials Science and Engineering Northeastern UniversityShenyang110819China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province Qinhuangdao 066004China Department of Physics and Oxide Research Center Hankuk University of Foreign StudiesYongin 17035Korea

Antimony-based materials with high capacities and moderate potentials are promising anodes for lithium-/-sodium-ion ***,their tremendous volume expansion and inferior conductivity lead to poor structural stability and sluggish reaction ***,a doubleconfined nanoheterostructure Sb/Sb_(2)S_(3)@Ti_(3)C_(2)T_(x)@C has been fabricated through a solvothermal method followed by low-temperature heat *** dual protection of“MXene”and“carbon”can better accommodate the volume expansion of Sb/Sb_(2)S_(3).The strong covalent bond(Ti-S,Ti-O-Sb,C-O-Sb)can firmly integrate Sb-based material with Ti_(3)C_(2)T_(x)and carbon,which significantly improves the structure *** addition,the carbon layer can restrain the oxidation of MXenes,and the nano-Sb/Sb_(2)S_(3)can facilitate electron/ion transport and suppress the restacking of *** heterogeneous interface between Sb and Sb_(2)S_(3)can further promote interfacial charge *** MXene-Sb/Sb_(2)S_(3)@C-1 with the optimal Sb content shows high specific capacities,comparable rate properties and ultra-stable cycling performances(250 m Ah·g^(-1)after 2500 cycles at 1 A·g^(-1)for sodium-ion batteries).Ex situ X-ray diffractometer(XRD)test reveals the storage mechanism including the conversion and alloying process of MXene-Sb/Sb_(2)S_(3)@*** voltammetry(CV)test results demonstrate that the pseudocapacitance behavior is dominant in MXene-Sb/Sb_(2)S_(3)@C-1,especially at large *** design paves the way for exploring high-performance alloy-based/conversion-type anode for energy storage devices.

关键词： Sb/Sb_(2)S_(3) MXene Carbon Anode Lithium-ion batteries Sodium-ion batteries

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Mechanical response of a tunnel subjected to strike-slip faulting processes,based on a multi-scale modeling method

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Frontiers of Structural and Civil Engineering 2024年第8期18卷 1281-1295页

作者： guoguo LIU Ping GENG Tianqiang wang Xiangyu guo Jiaxiang wang Ti DING Key Laboratory of Transportation Tunnel Engineering Ministry of EducationChengdu 610031China College of Civil Engineering Huaqiao UniversityXiamen 361021China China Railway Design Corporation Tianjin 300308China

The stick-slip action of strike-slip faults poses a significant threat to the safety and stability of underground *** this study,the north-east area of the Longmenshan fault,Sichuan,provides the geological background;the rheological characteristics of the crustal lithosphere and the nonlinear interactions between plates are described by Burger’s viscoelastic constitutive model and the friction constitutive model,respectively.A large-scale global numerical model for plate squeezing analysis is established,and the seemingly periodic stick-slip action of faults at different crust depths is *** a second model at a smaller scale,a local finite element model(sub-model),the time history of displacement at a ground level location on the Longmenshan fault plane in a stick-slip action is considered as the displacement *** integration of these models,creating a multi-scale modeling method,is used to evaluate the crack propagation and mechanical response of a tunnel subjected to strike-slip *** determinations of the recurrence interval of stick-slip action and the cracking characteristics of the tunnel are in substantial agreement with the previous field investigation and experimental results,validating the multi-scale modeling *** can be concluded that,regardless of stratum stiffness,initial cracks first occur at the inverted arch of the tunnel in the footwall,on the squeezed side under strike-slip *** smaller the stratum stiffness is,the smaller the included angle between the crack expansion and longitudinal direction of the tunnel,and the more extensive the crack expansion *** the tunnel in a high stiffness stratum,both shear and bending failures occur on the lining under strike-slip faulting,while for that in the low stiffness stratum,only bending failure occurs on the lining.

关键词： stick-slip action plate squeezing analysis multi-scale modeling method lining cracking mechanical response

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Effect of heat treatment on corrosion behaviors of Mg-6Gd-3Y-0.5Zr alloy

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China Foundry 2024年第5期21卷 599-612页

作者： Fei wang Bin-guo Fu Yu-feng wang Tian-shun Dong guo-lu Li Jin-hai Liu Hebei Key Laboratory of New Functional Materials School of Materials Science and EngineeringHebei University of TechnologyTianjin 300401China Tianjin Institute of Aerospace Mechanical and Electrical Equipment Tianjin 300301China Tianjin Aerospace Long March Technology and Equipment Co. Ltd.Tianjin 300462China

The microstructures and corrosion behaviors of as-cast,T4-treated,and T6-treated Mg-6Gd-3Y-0.5Zr alloys were systematically investigated by SEM,TEM,immersion test,and electrochemical corrosion *** results show that the microstructure of the as-cast alloy is composed ofα-Mg and Mg_(24)(Gd,Y)_(5)eutectic phase,and in T4-treated alloy,Mg_(24)(Gd,Y)_(5)phase dissolves into theα-Mg matrix,leading to an increase in the(Y,Gd)H_(2)*** T6 treatment,nanoscale Mg_(24)(Gd,Y)_(5)phase dispersedly precipitates from theα-Mg matrix,and exhibits a specific orientation relationship with theα-Mg:(332)Mg_((24)(Gd,Y)_(5))//(1011)_(α-Mg),[136]Mg_((24)(Gd,Y)_(5))//[1210]_(α-Mg).The corrosion resistance of the Mg-6Gd-3Y-0.5Zr alloys can be ranked in the following order:T6-treated alloy exhibits the highest corrosion resistance,followed by the T4-treated alloy,and finally,the as-cast *** corrosion products of the alloys are all composed of MgO,Mg(OH)_(2),Gd_(2)O_(3),Y_(2)O_(3),and MgCl_(2).The corrosion behavior of Mg-6Gd-3Y-0.5Zr alloy is closely related to the precipitated *** establishing the relationship between corrosion rate,hydrogen evolution rate,and corrosion potential,it is further demonstrated that during the micro galvanic corrosion process,the coarse Mg_(24)(Gd,Y)_(5)phase in the as-cast alloy undergoes extensive dissolution,and(Y,Gd)H_(2)phase promotes the dissolution of theα-Mg matrix in the T4-treated alloy,intensifying the hydrogen evolution *** T6-treated alloy,with dispersive precipitation of nanoscale Mg_(24)(Gd,Y)_(5)phase,exhibits better corrosion resistance performance.

关键词： Mg-6Gd-3Y-0.5Zr alloy heat treatment microstructure precipitated phase corrosion resistance

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Robust video question answering via contrastive cross-modality representation learning

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Science China(Information Sciences) 2024年第10期67卷 211-226页

作者： Xun YANG Jianming ZENG Dan guo Shanshan wang Jianfeng DONG Meng wang School of Information Science and Technology University of Science and Technology of China Institute of Artificial Intelligence Hefei Comprehensive National Science Center School of Computer Science and Information Engineering Hefei University of Technology Institutes of Physical Science and Information Technology Anhui University School of Computer Science and Technology Zhejiang Gongshang University

Video question answering(VideoQA) is a challenging yet important task that requires a joint understanding of low-level video content and high-level textual semantics. Despite the promising progress of existing efforts, recent studies revealed that current VideoQA models mostly tend to over-rely on the superficial correlations rooted in the dataset bias while overlooking the key video content, thus leading to unreliable results. Effectively understanding and modeling the temporal and semantic characteristics of a given video for robust VideoQA is crucial but, to our knowledge, has not been well investigated. To fill the research gap, we propose a robust VideoQA framework that can effectively model the cross-modality fusion and enforce the model to focus on the temporal and global content of videos when making a QA decision instead of exploiting the shortcuts in datasets. Specifically, we design a self-supervised contrastive learning objective to contrast the positive and negative pairs of multimodal input, where the fused representation of the original multimodal input is enforced to be closer to that of the intervened input based on video perturbation. We expect the fused representation to focus more on the global context of videos rather than some static keyframes. Moreover, we introduce an effective temporal order regularization to enforce the inherent sequential structure of videos for video representation. We also design a Kullback-Leibler divergence-based perturbation invariance regularization of the predicted answer distribution to improve the robustness of the model against temporal content perturbation of videos. Our method is model-agnostic and can be easily compatible with various VideoQA backbones. Extensive experimental results and analyses on several public datasets show the advantage of our method over the state-of-the-art methods in terms of both accuracy and robustness.

关键词： video question answering cross-modality fusion contrastive learning cross-media reasoning

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Hypoxic tumor microenvironment:Destroyer of natural killer cell function

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Chinese Journal of Cancer Research 2024年第2期36卷 138-150页

作者： Yongfei Zhang Feifei guo Yufeng wang Cancer Center the First Hospital of Jilin UniversityChangchun 130021China

In recent years, immunotherapy has made remarkable progress in treating certain tumors and hematological malignancies. However, the efficacy of natural killer(NK) cells, which are an important subset of innate lymphocytes used in anticancer immunotherapy, remains limited. Hypoxia, a critical characteristic of the tumor microenvironment(TME), is involved in tumor development and resistance to radiotherapy, chemotherapy, and immunotherapy. Moreover, hypoxia contributes to the impairment of NK cell function and may be a significant factor that limits their therapeutic effects. Targeted hypoxia therapy has emerged as a promising research area for enhancing the efficacy of NK cell therapy. Therefore, understanding how the hypoxic TME influences NK cell function is crucial for improving antitumor treatment outcomes.

关键词： Hypoxia immunotherapy NK cell tumor microenvironment

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Preparation and Swelling Kinetic Analysis of Poly (HPMC-co-AA-co-AM) Super Absorbent Resin

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Journal of Wuhan University of Technology(Materials Science) 2024年第3期39卷 790-799页

作者：马砺 wang Xin LIU Xixi WEI Gaoming guo Ying School of Safety Science and Engineering Xi’an University of Science and TechnologyXi'an 710054China Key Laboratory of Coal Fire Disaster Prevention Xi’an University of Science and TechnologyXi'an 710054China School of Energy Engineering Xi’an Uni-versity of Science and TechnologyXi'an 710054China Yanzhou Coal Mining Co. Ltd.Zoucheng 237500China

Super absorbent resin(SAR)is prepared by aqueous high temperature polymerization using hydroxypropyl methylcellulose(HPMC)as monomer backbone material,acrylic acid(AA)and acrylamide(AM)as the graft copolymer monomer,potassium persulfate(KPS)as the initiator to generate free radicals,and N,N`-methylenebisacrylamide(MBA)as cross-linking agent for cross-linking ***,the influence of individual factors on the water absorption is investigated,and these factors are mainly AA,AM,KPS,MBA,HPMC,and reaction *** optimized conditions are obtained by the experiment repeating for several *** water absorption multiplicity and salt absorption multiplicity under the conditions are 782.4 and 132.5 g/g,***,the effects of different temperatures and salt concentrations on its water absorption,as well as the swelling kinetics of SAR are *** is indicated the water-absorbing swelling process is mainly caused by the difference in water osmotic pressure and Na+concentration inside and outside the cross-linked molecular structure of the resin,which is not only consistent with the quasi-secondary kinetic model,but also with the Fick diffusion model.

关键词： super absorbent resin swelling kinetics water absorption graft copolymerization hydroxypropyl methyl cellulose

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Double-branch forgery image detection based on multi-scale feature fusion

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Optoelectronics Letters 2024年第5期20卷 307-312页

作者： ZHANG Hongying guo Chunxing wang Xuyong College of Electronic Information and Automation Civil Aviation University of ChinaTianjin 300300China

Most of existing methods exhibit poor performance in detecting forged images due to the small size of tampered areas and the limited pixel difference between untampered and tampered regions. To alleviate the above problem, a double-branch tampered image detection based on multi-scale features is proposed. Firstly, we introduce a fusion module based on attention mechanism in the first branch to enhance the network's sensitivity towards tampered regions. Secondly, we construct a second branch specifically designed for detection, aiming to identify subtle differences between tampered and untampered areas by utilizing rich edge information from shallow features as guidance. Compared to the existing methods on the public benchmark datasets CASIA1.0, Columbia and NIST16, the values of F-score reached 0.766, 0.900 and 0.930 on those datasets, respectively. The experimental results show that our method could significantly improve the accuracy on detecting the tampered area.

关键词： branch image utilizing

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Effect of cerium on microstructure,texture and properties of ultrahigh-purity copper

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Journal of Rare Earths 2024年第1期42卷 220-227,I0008页

作者： Yunxiao Hua Haitao Liu Kexing Song Jiangwei wang Yin'gang guo Jing Tian Huiwen guo Provincial and Ministerial Co-construction of Collaborative Innovation Center for Non-ferrous Metal New Materials and Advanced Processing Technology School of Materials Science and EngineeringHenan University of Science and TechnologyLuoyang471023China Henan Academy of Sciences Zhengzhou450000China Center of Electron Microscopy and State Key Laboratory of Silicon Materials School of Materials Science and EngineeringZhejiang UniversityHangzhou310027China Henan Zhongyuan Gold Smelter Co. Ltd.Sanmenxia472100China Chinalco Luoyang Copper Processing Co. Ltd.Luoyang471039China

The effects of Ce addition(310 ppm and 1500 ppm)on the microstructure,texture and properties of ultrahigh-purity copper(99.99999%)were systematically studied using scanning electron microscopy(SEM),transmission electron microscopy(TEM)and electron backscattered diffraction(EBSD)analyses,combined with the microhardness and conductivity *** the microstructure of the as-cast and as-extruded samples,the addition of Ce refines the grain size of the ultrahigh-purity copper and the refinement effect of 310Ce alloy is greater than that of 1500Ce *** is due to the stronger compone nt supercooling and the accele rated recrystallization caused by lower Ce co *** addition,Ce can react with Cu to form the Cu-Ce eutectic phases,which are deformable during the hot ***,the added Ce can weaken the texture,showing a variation of brass recrystallization(BR),rotated cube,copper and S texture components,which depends on the recrystallization,the particle stimulated nucleation(PSN)as well as the stacking fault energy(SFE).Most remarkably,the introduction of Ce enhances the hardness of the ultrahigh-purity copper without obviously reducing its *** major{111}orientations and the stress distributions are responsible for such a superior conductivity of the Ce-containing alloys.

关键词： Ce addition Grain refinement Texture Conductivity Ultrahigh-purity copper Rare earths

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Thioacetamide Additive Homogenizing Zn Deposition Revealed by In Situ Digital Holography for Advanced Zn Ion Batteries

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Nano-Micro Letters 2024年第6期16卷 261-275页

作者： Kaixin Ren Min Li Qinghong wang Baohua Liu Chuang Sun Boyu Yuan Chao lai Lifang Jiao Chao wang School of Chemistry and Materials Science Jiangsu Normal UniversityXuzhou 221116JiangsuPeople’s Republic of China Jiangsu Key Laboratory of Advanced Laser Materials and Devices School ofPhysics and Electronic EngineeringJiangsu Normal UniversityXuzhou 221116JiangsuPeople’s Republic of China Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) Nankai University300071 TianjinPeople’s Republic of China

Zinc ion batteries are considered as potential energy storage devices due to their advantages of low-cost,high-safety,and high theoretical ***,dendrite growth and chemical corrosion occurring on Zn anode limit their *** problems can be tackled through the optimization of the ***,the screening of electrolyte additives using normal electrochemical methods is time-consuming and ***,a fast and simple method based on the digital holography is *** can realize the in situ monitoring of electrode/electrolyte interface and provide direct information concerning ion concentration evolution of the diffusion *** is effective and time-saving in estimating the homogeneity of the deposition layer and predicting the tendency of dendrite growth,thus able to value the applicability of electrolyte *** feasibility of this method is further validated by the forecast and evaluation of thioacetamide *** on systematic characterization,it is proved that the introduction of thioacetamide can not only regulate the interficial ion flux to induce dendrite-free Zn deposition,but also construct adsorption molecule layers to inhibit side reactions of Zn *** easy to operate,capable of in situ observation,and able to endure harsh conditions,digital holography method will be a promising approach for the interfacial investigation of other battery systems.

关键词： Digital holographic microscopy In situ observation Electrode/electrolyte interface Zn dendrites Screening electrolyte additives

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Recent advances in cobalt phosphide-based materials for electrocatalytic water splitting:From catalytic mechanism and synthesis method to optimization design

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Nano Materials Science 2024年第2期6卷 139-173页

作者： Rongrong Deng Mengwei guo Chaowu wang Qibo Zhang Key Laboratory of Ionic Liquids Metallurgy Faculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming650093PR China State Key Laboratory of Complex Nonferrous Metal Resources Cleaning Utilization in Yunnan Province Kunming650093PR China

Electrochemical water splitting has long been considered an effective energy conversion technology for trans-ferring intermittent renewable electricity into hydrogen fuel,and the exploration of cost-effective and high-performance electrocatalysts is crucial in making electrolyzed water technology commercially *** phosphide(Co-P)has emerged as a catalyst of high potential owing to its high catalytic activity and durability in water *** paper systematically reviews the latest advances in the development of Co-P-based materials for use in water *** essential effects of P in enhancing the catalytic performance of the hydrogen evolution reaction and oxygen evolution reaction are first ***,versatile synthesis techniques for Co-P electrocatalysts are summarized,followed by advanced strategies to enhance the electrocatalytic performance of Co-P materials,including heteroatom doping,composite construction,integration with well-conductive sub-strates,and structure control from the viewpoint of *** with these optimization strategies,the understanding of the inherent mechanism of enhanced catalytic performance is also ***,some existing challenges in the development of highly active and stable Co-P-based materials are clarified,and pro-spective directions for prompting the wide commercialization of water electrolysis technology are proposed.

关键词： Co-P electrocatalysts Water splitting Hydrogen production Catalytic mechanism Synthesis technique Optimization design

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