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Efficient and Stable Photoassisted Lithium‑Ion Battery Enabled by Photocathode with Synergistically Boosted Carriers Dynamics

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Nano-Micro Letters 2025年第3期17卷 440-454页

作者： Zelin Ma Shiyao wang Zhuangzhuang Ma Juan Li Luomeng Zhao Zhihuan Li Shiyuan wang Yazhou Shuang Jiulong wang Fang wang Weiwei Xia Jie Jian Yibo He Junjie wang Pengfei Guo Hongqiang wang State Key Laboratory of Solidification Processing Center for Nano Energy MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical University and Shaanxi Joint Laboratory of Graphene(NPU)Xi’an 710072People’s Republic of China State Key Laboratory of Solidification Processing School of Materials Science and Engineering DepartmentNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072People’s Republic of China Research and Development Institute of Northwestern Polytechnical University in Shenzhen Shenzhen 518063People’s Republic of China Key Laboratory of Applied Surface and Colloid Chemistry Shaanxi Key Laboratory for Advanced Energy DevicesShaanxi Engineering Lab for Advanced Energy TechnologySchool of Materials Science and EngineeringNational Ministry of EducationShaanxi Normal UniversityXi’an 710119People’s Republic of China

Efficient and stable photocathodes with versatility are of significance in photoassisted lithium-ion batteries(PLIBs),while there is always a request on fast carrier transport in electrochemical active *** work proposes a general approach of creating bulk heterojunction to boost the carrier mobility of photocathodes by simply laser assisted embedding of plasmonic *** employed in PLIBs,it was found effective for synchronously enhanced photocharge separation and transport in light charging ***,experimental photon spectroscopy,finite difference time domain method simulation and theoretical analyses demonstrate that the improved carrier dynamics are driven by the plasmonic-induced hot electron injection from metal to TiO_(2),as well as the enhanced conductivity in TiO2 matrix due to the formation of oxygen vacancies after Schottky *** from these merits,several benchmark values in performance of TiO2-based photocathode applied in PLIBs are set,including the capacity of 276 mAh g^(−1)at 0.2 A g^(−1)under illumination,photoconversion efficiency of 1.276%at 3 A g^(−1),less capacity and Columbic efficiency loss even through 200 *** results exemplify the potential of the bulk heterojunction strategy in developing highly efficient and stable photoassisted energy storage systems.

关键词： Photoassisted lithium-ion batteries Bulk heterojunction Carrier dynamics TiO2 nanofiber Plasmonic metal nanocrystals

面向不同电流工况的锂离子电池改进EECM研究

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电力工程技术 2023年第4期42卷 2-12页

作者：张志行韩雪冰冯旭宁卢兰光王贺武欧阳明高清华大学车辆与运载学院北京100084

锂离子电池是新能源汽车动力系统的核心,基于模型的电池管理系统(battery management system,BMS)是保证电池性能充分发挥的关键。然而现有BMS主要采用等效电路模型(equivalent circuit model,ECM),尚未考虑放电倍率对可用容量的影响机... 详细信息

锂离子电池是新能源汽车动力系统的核心,基于模型的电池管理系统(battery management system,BMS)是保证电池性能充分发挥的关键。然而现有BMS主要采用等效电路模型(equivalent circuit model,ECM),尚未考虑放电倍率对可用容量的影响机制,导致模型在不同放电倍率下以及低荷电状态(state of charge,SOC)区域会存在明显的端电压仿真误差,影响算法精度;尤其是BMS无法准确估计电池放电截止条件,剩余放电电量(remaining discharge capacity,RDC)估计误差大,可能导致电池电压骤降甚至整车抛锚等严重后果。针对以上问题,文中以考虑内部扩散机制的扩展等效电路模型(extended equivalent circuit model,EECM)为基础,对不同倍率的放电电压容量增量(incremental capacity,IC)曲线进行对比分析,利用能斯特方程构造不同放电倍率下的容量-开路电压曲线,提出改进的EECM。所提改进EECM在不同电流倍率和动态工况下的端电压仿真误差均小于传统ECM和EECM,可以提高RDC估计的准确性,有应用于实际BMS的潜力。

关键词：锂离子电池等效电路模型(ECM) 电池管理系统(BMS) 电动汽车剩余放电电量(RDC)估计改进的扩展等效电路模型(EECM)

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储能电池簇液流冷却温控性能优化仿真研究

低温与超导 2023年第11期51卷 37-43,73页

作者：李许一王炎李涵闫涵超王禹王贺武卢兰光李德胜李连强青岛理工大学机械与汽车工程学院青岛266525 清华大学汽车安全与能源国家重点实验室北京100084 清安储能技术(重庆)有限公司重庆400050 一汽解放青岛汽车有限公司青岛266043

为了提高储能电站中电池簇的散热效果、改善电池表面温度分布的不均匀性,本文按照实际尺寸建立了电池簇的液冷仿真模型。利用Fluent仿真软件研究了出水口布置在不同位置时的散热效果,选定了最佳的布置方案,最大温差由16 K降低到13 K,降... 详细信息

为了提高储能电站中电池簇的散热效果、改善电池表面温度分布的不均匀性,本文按照实际尺寸建立了电池簇的液冷仿真模型。利用Fluent仿真软件研究了出水口布置在不同位置时的散热效果,选定了最佳的布置方案,最大温差由16 K降低到13 K,降低了18.8%。进一步研究分析了冷板布置在底面和侧面时的散热效果,结果表明,采用冷板布置在电池侧面的方案,电池表面温度分布的不均匀性得到改善,最大温差由13 K减小到3.7 K,减小了71.5%,温差被控制在规定范围内。

关键词：储能电站电池簇液冷 Fluent

Rational modulation of fluorophosphate cathode by anionic groups to reduce the polarization behavior for fast-charging sodium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 509-521页

作者： Xinyuan wang Fan Zhang Xingyu Zhou Qian wang Changyu Liu Yangyang Liu Hui wang Xiaojie Liu Key Laboratory of Synthetic and Natural Functional Molecule of the Ministry of Education College of Chemistry & Materials Science Northwest University

Na3V2（PO4）2O2F （VP） is recognized as a promising cathode material for sodium-ion batteries due to its stable structural framework and high specific *** functional theory （DFT） and finite element simulations show that incorporating SO42-into VP decreases its band gap,lowers the migration energy barrier,and ensures a uniform Na+concentration gradient and stress distribution during charge and discharge ***,the average Na+diffusion coefficient of Na3V2（PO4）1.95（SO4）0.05O2F（VPS-1） is roughly double that of VP,leading to enhanced rate capability (80 C,75.5 mAh g-1) and cycling stability (111.0 mAh g-1capacity after 1000 cycles at 10 C current density) for ***-1 exhibits outstanding fast-charging capabilities,achieving an 80%state of charge in just 8.1 *** assembled VPS-1//SbSn/NPC full cell demonstrated stable cycling over 200 cycles at a high 5 C current,maintaining an average coulombic efficiency of 95.35%.

关键词： Anionic group modulation Polarization behavior Fast-charging Sodium-ion battery Fluorophosphate Cathode

EZH2-dependent myelination following sciatic nerve injury

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Neural Regeneration Research 2025年第8期20卷 2382-2394页

作者： Hui Zhu Li Mu Xi Xu Tianyi Huang Ying wang Siyuan Xu Yiting wang Wencong wang Zhiping wang Hongkui wang Chengbin Xue Research Center of Clinical Medicine Affiliated Hospital of Nantong UniversityKey Laboratory of Neuroregeneration of Jiangsu and Ministry of EducationCo-innovation Center of NeuroregenerationNMPA Key Laboratory for Research and Evaluation of Tissue Engineering Technology ProductsNantong UniversityNantongJiangsu ProvinceChina Medical School of Nantong University NantongJiangsu ProvinceChina Department of Neurology Affiliated Hospital of Nantong UniversityNantongJiangsu ProvinceChina Department of Rehabilitation Medicine Affiliated Hospital of Nantong UniversityNantongJiangsu ProvinceChina Department of Critical Care Medicine Nantong Fourth People’s HospitalNantongJiangsu ProvinceChina

Demyelination and remyelination have been major focal points in the study of peripheral nerve regeneration following peripheral nerve ***,the gene regulatory network of regenerated myelin differs from that of native *** of enhancer of zeste homolog 2(EZH2)hinders the differentiation,maturation,and myelination of Schwann cells in *** further determine the role of EZH2 in myelination and recovery post-peripheral nerve injury,conditional knockout mice lacking Ezh2 in Schwann cells(Ezh2^(fl/fl);Dhh-Cre and Ezh2^(fl/fl);Mpz-Cre)were *** results show that a significant proportion of axons in the sciatic nerve of Ezh2-depleted mice remain *** highlights the crucial role of Ezh2 in initiating Schwann cell ***,we observed that 21 days after inducing a sciatic nerve crush injury in these mice,most axons had remyelinated at the injury site in the control nerve,while Ezh2^(fl/fl);Mpz-Cre mice had significantly fewer remyelinated axons compared with their wild-type *** suggests that the absence of Ezh2 in Schwann cells impairs myelin formation and *** conclusion,EZH2 has emerged as a pivotal regulatory factor in the process of demyelination and myelin regeneration following peripheral nerve *** EZH2 activity during these processes may offer a promising therapeutic target for the treatment of peripheral nerve injuries.

关键词： demyelination EZH2 myelination peripheral nerve injury PRC2 remyelination Schwann cells sciatic nerve crush sciatic nerve transection

RF Optimizer Model for Predicting Compressive Strength of Recycled Concrete

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Journal of Wuhan University of Technology(Materials Science) 2025年第1期40卷 215-223页

作者： LIU Lin wang Liuyan wang Hui SUN Huayue School of Civil Engineering and Architecture Shenyang UniversityShenyang 110000China

Traditional machine learning(ML)encounters the challenge of parameter adjustment when predicting the compressive strength of reclaimed *** address this issue,we introduce two optimized hybrid models:the Bayesian optimization model(B-RF)and the optimal model(Stacking model).These models are applied to a data set comprising 438 observations with five input variables,with the aim of predicting the compressive strength of reclaimed ***,we evaluate the performance of the optimized models in comparison to traditional machine learning models,such as support vector regression(SVR),decision tree(DT),and random forest(RF).The results reveal that the Stacking model exhibits superior predictive performance,with evaluation indices including R2=0.825,MAE=2.818 and MSE=14.265,surpassing the traditional ***,we also performed a characteristic importance analysis on the input variables,and we concluded that cement had the greatest influence on the compressive strength of reclaimed concrete,followed by ***,the Stacking model can be recommended as a compressive strength prediction tool to partially replace laboratory compressive strength testing,resulting in time and cost savings.

关键词： machine learning recycled concrete compressive strength

Intermolecular reductive coupling of aliphatic ketones with alkynes and alkenes by BCN photocatalysts

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Science China Chemistry 2025年第1期68卷 181-185页

作者： Yanping Xia Luyang Sun Jiajia Cheng Sibo wang Meifang Zheng Xinchen wang State Key Laboratory of Photocatalysis on Energy and Environment College of Chemistry Fuzhou University

A photocatalytic process was developed for intermolecular reductive coupling of aliphatic ketones with alkynes/alkenes to furnish tertiary alcohols. Mechanistic studies support that boron carbonitrides(BCN) promote the single electron reduction of unactivated aliphatic ketones to generate ketyl radicals with visible light irradiation, which then react with alkynes and alkenes to afford the allylic and aliphatic alcohols, respectively. The heterogeneous photocatalytic system is compatible with diverse substrates including pharmaceutical-related molecules(43 examples) with reusability and scale-up experiments, verifying the complementary synthetic utility of this method to the homogeneous catalysts.

关键词： aliphatic ketones ketyl radical intermolecular cross-coupling tertiary alcohols

Achieving ultralow leakage current in Schottky-MIS cascode anode lateral field-effect diode based on AlGaN/GaN HEMT

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Science China(Information Sciences) 2025年第1期68卷 379-385页

作者： Fangzhou wang Changhong GAO Guojian DING Cheng YU Zhuocheng wang Xiaohui wang Qi FENG Ping YU Peng ZUO Wanjun CHEN Yang wang Haiqiang JIA Hong CHEN Bo ZHANG Zeheng wang Songshan Lake Materials Laboratory School of Microelectronics Southern University of Science and Technology State Key Laboratory of Electronic Thin Films and Integrated Devices University of Electronic Science and Technology of China Manufacturing Commonwealth Scientific and Industrial Research Organisation

In this paper,we design and fabricate a Schottky-metal-insulator-semiconductor（MIS） cascode anode GaN lateral field-effect diode（CA-LFED） to achieve ultralow reverse leakage current(ILEAK).The device based on AlGaN/GaN highelectron-mobility-transistor（HEMT） includes a normally-off MIS-controlled channel that is cascoded with a high barrier height Schottky *** reverse bias,the high electric-field is effectively prevented by the normally-off MIS-controlled channel *** with the high barrier height Schottky contact,this feature significantly suppresses the *** by the device fabrication,the CA-LFED with high breakdown voltage（BV）>600 V shows an ultralow ILEAKof 3.6×10-9A/mm as well as a low forward voltage drop（VF） of 2.2 *** performance suggests that the CA-LFED can be a promising candidate for ultralow ILEAKand better VF-ILEAKtrade-off GaN power diode applications.

关键词： Schottky-MIS cascode anode lateral field-effect diode (LFED) ultralow reverse leakage current ($I_{\rm{LEAK}}$) forward drop and reverse leakage trade-off AlGaN/GaN HEMTs

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锂离子动力电池中等荷电状态下热失控产物喷发过程

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储能科学与技术 2019年第6期8卷 1076-1081页

作者：王贺武张亚军李成李伟峰欧阳明高清华大学汽车安全与节能国家重点实验室

以电动汽车用方壳型镍钴锰(NCM)锂离子动力电池为研究对象,以氮气为惰性保护,采用高速摄影的方法,在密闭容器内开展了电池热失控产物喷发过程的试验研究。检测压力突变表明,中等荷电状态下的电池热失控后的喷发过程出现了2次剧烈喷射,... 详细信息

以电动汽车用方壳型镍钴锰(NCM)锂离子动力电池为研究对象,以氮气为惰性保护,采用高速摄影的方法,在密闭容器内开展了电池热失控产物喷发过程的试验研究。检测压力突变表明,中等荷电状态下的电池热失控后的喷发过程出现了2次剧烈喷射,分别导致了喷发物射流区温度的突然降低和快速升高。借助辅助光源,捕捉到了热失控产物首次喷发演变过程的高速影像,进一步分析发现,首次喷发经历了初期的带状和锥形喷发,然后进入较长时间的无定形喷发和后期的倒锥形喷发;同时,在影像中还观察到了气-液-固三相共存的特征。

关键词：锂离子电池热失控喷发高速摄影