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Stable multi-electron reaction stimulated by W doping VS_(4)for enhancing magnesium storage performance

Journal of Energy Chemistry 2024年第2期89卷 89-98,I0004页

作者： Yuxin tian Jiankang Chen Guofeng wang Bing Sun Alan Meng Lei wang Guicun li Jianfeng Huang Shiqi Ding Zhenjiang li College of Materials Science and Engineering Qingdao University of Science and TechnologyQingdao 266042ShandongChina Key Laboratory of Optic-electric Sensing and Analytical Chemistry for life Science MOEShandong Key Laboratory of Biochemical AnalysisCollege of Chemistry and Molecular EngineeringQingdao University of Science and TechnologyQingdao 266042ShandongChina School of Material Science and Engineering International S&T Cooperation Foundation of Shaanxi ProvinceXi’an Key Laboratory of Green Manufacture of Ceramic MaterialsShaanxi University of Science and TechnologyXi’an 710021ShaanxiChina

Rechargeable magnesium batteries(RMBs)hold promise for offering higher volumetric energy density and safety features,attracting increasing research interest as the next post lithium-ion *** high performance cathode material by inducing multi-electron reaction process as well as maintaining structural stability is the key to the development and application of ***,multielectron reaction occurred in VS_(4)by simple W doping strategy.W doping induces valence of partial V as V^(2+)and V^(3+)in VS_(4)structure,and then stimulates electrochemical reaction involving multi-electrons in 0.5%*** flower-like microsphere morphology as well as rich S vacancies is also modulated by W doping to neutralize structure change in such multi-electron reaction *** fabricated 0.5%W-V-S delivers higher specific capacity(149.3 m A h g^(-1)at 50 m A g^(-1),which is 1.6 times higher than that of VS_(4)),superior rate capability(76 mA h g^(-1)at 1000 mA g^(-1)),and stable cycling performance(1500cycles with capacity retention ratio of 93.8%).Besides that,pesudocapaticance-like contribution analysis as well as galvanostatic intermittent titration technique(GITT)further confirms the enhanced Mg^(2+)storage kinetics during such multi-electron involved electrochemical reaction *** discovery provides new insights into the designing of multi-electron reaction process in cathode as well as neutralizing structural change during such reaction for realizing superior electrochemical performance in energy storage devices.

关键词： Multi-electron reaction W doping Stable structure Cathode Rechargeable magnesium batteries

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Research on denoising of joint detection signal of water quality with multi-parameter based on IEEMD

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Optoelectronics Letters 2024年第2期20卷 107-115页

作者： li Wen li Dejian MA Yongyue tian wang WEN Xin li Jie Institute of Mechanical and Electrical Engineering North China University of TechnologyBeijing 100144China1

An improved ensemble empirical mode decomposition(IEEMD) is suggested to process water quality spectral signals in order to address the issue that noise interference makes it difficult to extract and evaluate water quality spectral *** algorithm effectively solves the problems of modal mixing,poor reconstruction accuracy in the empirical mode decomposition(EMD),and a large amount of calculation in the ensemble empirical mode decomposition(EEMD).Based on EEMD,IEEMD firstly preprocesses the original water quality spectral signals,then performs Savitzky-Golay(S-G) smoothing on the decomposed effective intrinsic mode function(IMF) components,and finally reconstructs them to obtain the denoised *** sample data at different concentrations can be accurately analyzed based on the noise-reduced spectral *** this paper,three water quality parameters are used as research objects:benzene(C_(6)H_(6)),benzo(b)fluoranthene(C_(20)H_(12)),and chemical oxygen demand(COD).The original water quality multi-parameter(C_(6)H_(6),C_(20)H_(12),COD) spectral signals were subjected to denoising based on the IEEMD and the water quality multi-parameter joint detection *** signal-to-noise ratio(SNR) and the correlation coefficient(R^(2)) of the fitted curves obtained from the processing of the IEEMD were compared and analyzed with those obtained from the processing of the EMD and the *** experimental results show that the SNR of the spectral signals and the R^(2) of the fitting curve in three water quality parameters have been significantly ***,the IEEMD effectively improves the phenomenon of modal mixing,reduces the amount of calculation,improves the reconstruction accuracy,and provides an important guarantee for the effective extraction of multi-parameter spectral signals of water quality.

关键词： signal parameter noise

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RGB oralscan video-based orthodontic treatment monitoring

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Science China(Information Sciences) 2024年第1期67卷 124-139页

作者： Yan tian Hanshi FU Hao wang Yuqi liU Zhaocheng XU Hong CHEN Jianyuan li Ruili wang School of Computer Science and Technology Zhejiang Gongshang University Shining3D Tech Co. Ltd. School of Information and Technology Monash University School of Mathematical and Computational Sciences Massey University Department of Stomatology Zhejiang Provincial People's HospitalHangzhou Medical College School of Computer and Computing Science Zhejiang University City College

Orthodontic treatment monitoring involves using current images and previous 3D models to estimate the relative position of individual teeth before and after orthodontic *** process differs from image-based object 6D pose estimation due to the gingiva deformation and varying pose offsets for each tooth during *** by the fact that the poses of molars remain relatively fixed in implicit orthodontics,we design an approach that employs multiview pose evaluation and bidirectional temporal propagation for jaw pose estimation and then employs an iteration-based method for tooth *** handle changes in tooth appearance or location with weak texture across frames,we also introduce an instance propagation module that leverages positional and semantic information to explore instance relations in the temporal *** evaluated the performance of our approach using both the Shining3D tooth pose dataset and the Aoralscan3 tooth registration *** experimental results demonstrate remarkable accuracy improvements compared with existing methods.

关键词： digital dentistry object 6D pose estimation deep learning computer vision

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RAD-seq data reveals robust phylogeny and morphological evolutionary history of Rhododendron

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Horticultural Plant Journal 2024年第3期10卷 866-878页

作者： Yuanting Shen Gang Yao Yunfei li Xiaoling tian Shiming li Nian wang Chengjun Zhang Fei wang Yongpeng Ma Yunnan Key Laboratory for Integrative Conservation of Plant Species with Extremely Small Populations Kunming Institute of BotanyChinese Academy of SciencesKunmingYunnan 650201China Key Laboratory for Plant Diversity and Biogeography of East Asia Kunming Institute of BotanyChinese Academy of SciencesKunmingYunnan 650201China University of Chinese Academy of Sciences Beijing 100049China Beijing Genomics of Institute ShenzhenGuangdong 518120China Guiyang Institute of Humanities and Technology GuiyangGuizhou 550025China State Forestry and Grassland Administration Key Laboratory of Silviculture in Downstream Areas of the Yellow River College of ForestryShandong Agricultural UniversityTai'anShandong 271018China The Southwest China of Germplasm Bank of Wild Species Kunming Institute of BotanyChinese Academy of SciencesKunmingYunnan 650201China West China Subalpine Botanical Garden Institute of BotanyChinese Academy of SciencesChengduSichuan 611834China

Rhododendron is famous for its high ornamental ***,the genus is taxonomically difficult and the relationships within Rhododendron remain *** addition,the origin of key morphological characters with high horticulture value need to be *** problems largely hinder utilization of germplasm *** studies attempted to disentangle the phylogeny of Rhododendron,but only used a few genomic markers and lacked large-scale sampling,resulting in low clade support and contradictory phylogenetic ***,we used restriction-site associated DNA sequencing(RAD-seq)data and morphological traits for 144 species of Rhododendron,representing all subgenera and most sections and subsections of this species-rich genus,to decipher its intricate evolutionary history and reconstruct ancestral *** results revealed high resolutions at subgenera and section levels of Rhododendron based on RAD-seq *** optimal phylogenetic tree and split tree recovered five lineages among ***(cladeⅠ)formed the basal *** and Azaleastrum formed cladeⅡand had sister ***Ⅲincluded all scaly rhododendron ***(cladeⅣ)formed a sister group to ***(cladeⅤ).The results of ancestral state reconstruction showed that Rhododendron ancestor was a deciduous woody plant with terminal inflorescence,ten stamens,leaf blade without scales and broadly funnelform corolla with pink or purple *** study shows significant distinguishability to resolve the evolutionary history of Rhododendron based on high clade support of phylogenetic tree constructed by RAD-seq *** also provides an example to resolve discordant signals in phylogenetic trees and demonstrates the application feasibility of RAD-seq with large amounts of missing data in deciphering intricate evolutionary ***,the reconstructed ancestral state of six important characters provides insights into the inn

关键词： Rhododendron RAD-seq Missing data Quartet sampling(QS) Ancestral state reconstruction

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Improving the Forecasts of Coastal Wind Speeds in tianjin,China Based on the WRF Model with Machine Learning Algorithms

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Journal of Meteorological Research 2024年第3期38卷 570-585页

作者： Weihang ZHANG Meng tian Shangfei HAI Fei wang Xiadong AN Wanju li Xiaodong li lifang SHENG College of Oceanic and Atmospheric Sciences Ocean University of ChinaQingdao266100China tianjin Key Laboratory for Oceanic Meteorology Tianjin Institute of Meteorological ScienceTianjin300074China CMA Earth System Modeling and Prediction Centre China Meteorological Administration(CMA)Beijing100081China Qingdao Meteorological Bureau Qingdao266003China

Characterized by sudden changes in strength,complex influencing factors,and significant impacts,the wind speed in the circum-Bohai Sea area is relatively challenging to *** the western side of Bohai Bay,as the economic center of the circum-Bohai Sea,tianjin exhibits a high demand for accurate wind *** this study,three machine learning algorithms were employed and compared as post-processing methods to correct wind speed forecasts by the Weather Research and Forecast(WRF)model for *** results showed that the random forest(RF)achieved better performance in improving the forecasts because it substantially reduced the model bias at a lower computing cost,while the support vector machine(SVM)performed slightly worse(especially for stronger winds),but it required an approximately 15 times longer computing *** back propagation(BP)neural network produced an average forecast significantly closer to the observed forecast but insufficiently reduced the *** regard to wind speed frequency forecasting,the RF method commendably corrected the forecasts of the frequency of moderate(force 3)wind speeds,while the BP method showed a desirable capability for correcting the forecasts of stronger(force>6)*** addition,the 10-m u and v components of wind(u_(10)and v_(10)),2-m relative humidity(RH_(2))and temperature(T_(2)),925-hPa u(u925),sea level pressure(SLP),and 500-hPa temperature(T_(500))were identified as the main factors leading to bias in wind speed forecasting by the WRF model in tianjin,indicating the importance of local dynamical/thermodynamic processes in regulating the wind *** study demonstrates that the combination of numerical models and machine learning techniques has important implications for refined local wind forecasting.

关键词： machine learning Weather Research and Forecast(WRF)model wind speed forecasting coastal region

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Analysis on unit maximum capacity of orthogonal multiple watermarking for multimedia signals in B5G wireless communications

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Digital Communications and Networks 2024年第1期10卷 38-44页

作者： Mianjie li Senfeng Lai Jiao wang Zhihong tian Nadra Guizani Xiaojiang Du Chun Shan School of Electronics and Information Guangdong Polytechnic Normal UniversityGuangzhou510665China Cyberspace Institute of Advanced Technology Guangzhou UniversityGuangzhou510006China Schoolof Electrical Engineering and Computer Science Washington State UniversityPullmanWA99164USA Department of Computer and Information Science Temple UniversityPhiladelphiaPA19122USA

Beyond-5G(B5G)aims to meet the growing demands of mobile traffic and expand the communication *** that intelligent applications to B5G wireless communications will involve security issues regarding user data and operational data,this paper analyzes the maximum capacity of the multi-watermarking method for multimedia signal hiding as a means of alleviating the information security problem of *** multiwatermarking process employs spread transform dither *** the watermarking procedure,Gram-Schmidt orthogonalization is used to obtain the multiple spreading ***,multiple watermarks can be simultaneously embedded into the same position of a multimedia ***,the multiple watermarks can be extracted without affecting one another during the extraction *** analyze the effect of the size of the spreading vector on the unit maximum capacity,and consequently derive the theoretical relationship between the size of the spreading vector and the unit maximum capacity.A number of experiments are conducted to determine the optimal parameter values for maximum robustness on the premise of high capacity and good imperceptibility.

关键词： B5G Multimedia information security Spread transform dither modulation Spreading vector measurement Unit maximum capacity

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Identification of S-RNase genotype and analysis of its origin and evolutionary patterns in Malus plants

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Journal of Integrative Agriculture 2024年第4期23卷 1205-1221页

作者： Zhao liu Yuan Gao Kun wang Jianrong Feng Simiao Sun Xiang Lu lin wang Wen tian Guangyi wang Zichen li Qingshan li lianwen li Dajiang wang Research Institute of Pomology Chinese Academy of Agricultural Sciences/Key Laboratory of Horticultural Crops Germplasm Resources UtilizationMinistry of Agriculture and Rural AffairsXingcheng 125100China College of Agriculture Shihezi University/Key Laboratory of Special Fruits and Vegetables Cultivation Physiology and Germplasm Resources Utilization of Xinjiang Production and Construction CorpsShihezi 832000China

Identification of the S genotype of Malus plants will greatly promote the discovery of new genes,the cultivation and production of apple,the breeding of new varieties,and the origin and evolution of self-incompatibility in Malus *** this experiment,88 Malus germplasm resources,such as Aihuahong,Xishuhaitang,and Reguanzi,were used as *** gene-specific primer combinations were used in the genotype *** amplification using leaf DNA produced a single S-RNase gene fragment in all *** results revealed that 70 of the identified materials obtained a complete S-RNase genotype,while only one S-RNase gene was found in 18 of *** homology comparison and analysis,13 S-RNase genotypes were obtained:S_(1)S_(2)(Aihuahong,etc.),S_(1)S_(28)(Xixian Haitang,etc.),S_(1)S_(51)(Hebei Pingdinghaitang),S_(1)S_(3)(Xiangyangcun Daguo,etc.),S_(2)S_(3)(Zhaiyehaitang,etc.),S_(3)S_(51)(Xishan 1),S_(3)S_(28)(Huangselihaerde,etc.),S_(2)S_(28)(Honghaitang,etc.),S_(4)S_(28)(Bo 11),S_(7)S_(28)(Jiuquan Shaguo),S_(10)S_e(Dongchengguan 13),S_(10)S_(21)(Dongxiangjiao)and S_(3)S_(51)(Xiongyue Haitang).Simultaneously,the frequency of the S gene in the tested materials was *** findings revealed that different S genes had varying frequencies in Malus resources,as well as varying frequencies between intraspecific and interspecific.S_(3) had the highest frequency of 68.18%,followed by S_(1)(42.04%).In addition,the phylogenetic tree and origin evolution analysis revealed that the S gene differentiation was completed prior to the formation of various apple species,that cultivated species also evolved new S genes,and that the S_(50) gene is the oldest S allele in Malus *** S_(1),S_(29),and S_(33) genes in apple-cultivated species,on the other hand,may have originated in ***,***,and ***,*** addition to ***,*** and *** may have also played a role in the origin and evolution of some Chine

关键词： Malus S-RNase genotype self-incompatibility origin and evolution

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Recent advances in core-shell organic framework-based photocatalysts for energy conversion and environmental remediation

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Journal of Energy Chemistry 2024年第8期95卷 168-199,I0004页

作者： Qibing Dong Ximing li Yanyan Duan Qingyun tian Xinxin liang Yiyin Zhu lin tian Junjun wang Atif Sial Yongqian Cui Ke Zhao Chuanyi wang School of Environmental Science and Engineering Shaanxi University of Science and TechnologyXi’an 710021ShaanxiChina Guangdong Engineering Technology Research Center for Environmental Purification and Functional Materials Guangzhou Institute of Industrial IntelligenceGuangzhou 511400GuangdongChina Jiangxi Key Lab of Flexible Electronics Flexible Electronics Innovation InstituteJiangxi Science and Technology Normal UniversityNanchang 330013JiangxiChina Helmholtz-Zentrum Berlin für Materialien und Energie Kekuléstraße 512489 BerlinGermany

Direct conversion of solar energy into chemical energy in an environmentally friendly manner is one of the most promising strategies to deal with the environmental pollution and energy *** a variety of materials developed as photocatalysts,the core-shell metal/covalent-organic framework(MOF or COF)photocatalysts have garnered significant attention due to their highly porous structure and the adjustability in both structure and *** existing reviews on core-shell organic framework photocatalytic materials have mainly focused on core-shell MOF ***,there is still a lack of indepth reviews specifically addressing the photocatalytic performance of core-shell COFs and MOFs@***,there is an urgent need for a comprehensive review encompassing these three types of core-shell *** on this,this review aims to provide a comprehensive understanding and useful guidelines for the exploration of suitable core-shell organic framework photocatalysts towards appropriate photocatalytic energy conversion and environmental ***,the classification,synthesis,formation mechanisms,and reasonable regulation of core-shell organic framework were ***,the photocatalytic applications of these three kinds of core-shell structures in different areas,such as H_(2)evolution,CO_(2)reduction,and pollutants degradation are ***,the main challenges and development prospects of core-shell organic framework photocatalysts were *** review aims to provide insights into the development of a novel generation of efficient and stable core-shell organic framework materials for energy conversion and environmental remediation.

关键词： Organic framework Core-shell structure Photocatalysis Energy conversion Environmental remediation

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When Does Sora Show:The Beginning of TAO to Imaginative Intelligence and Scenarios Engineering

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IEEE/CAA Journal of Automatica Sinica 2024年第4期11卷 809-815页

作者： Fei-Yue wang Qinghai Miao lingxi li Qinghua Ni Xuan li Juanjuan li lili Fan Yonglin tian Qing-Long Han School of Artificial Intelligence University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory for Management and Control of Complex Systems Chinese Academy of SciencesBeijing 100190China Faculty of Innovation Engineering Macao University of Science and TechnologyMacao 999078China Department of Electrical and Computer Engineering Indiana University-Purdue University IndianapolisIndianapolisIN 46202USA Faculty of Innovation Engineering Macao University of Science and TechnologyMacao 999078China Virtual Reality Fundamental Research Laboratory Department of Mathematics and TheoriesPeng Cheng LaboratoryShenzhen 518000China State Key Laboratory of Multimodal Artificial Intelligence Systems Institute of AutomationChinese Academy of SciencesBeijing 100190China School of Information and Electronics Beijing Institute of TechnologyBeijing 100081China School of Science Computing and Engineering TechnologiesSwinburne University of TechnologyMelbourneVIC 3122Australia

DURING our discussion at workshops for writing“What Does ChatGPT Say:The DAO from Algorithmic Intelligence to linguistic Intelligence”[1],we had expected the next milestone for Artificial Intelligence(AI)would be in the direction of Imaginative Intelligence(II),i.e.,something similar to automatic wordsto-videos generation or intelligent digital movies/theater technology that could be used for conducting new“Artificiofactual Experiments”[2]to replace conventional“Counterfactual Experiments”in scientific research and technical development for both natural and social studies[2]-[6].Now we have OpenAI’s Sora,so soon,but this is not the final,actually far away,and it is just the beginning.

关键词： something Intelligence replace

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Hydrodechlorination of trifluoro-trichloroethane to chlorotrifluoroethylene:Revealing the deactivation mechanism and regeneration strategy of Pd-Cu/AC catalyst

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Chinese Journal of Chemical Engineering 2024年第6期70卷 261-268页

作者： Song tian Yicheng Chen Xiaoyu Wen Bingcheng li Jian Lu Zile li Feng Feng Qingtao wang Qunfeng Zhang Xiaonian li State Key Laboratory Breeding Base of Green Chemistry Synthesis Technology Institute of Industrial Catalysis of Zhejiang University of TechnologyHangzhou 310014China State Key Laboratory of Fluorine&Nitrogen Chemicals Xi'an Modern Chemistry Research InstituteXi'an 710065China

Chlorotrifluoroethylene(CTFE)is a vital fluorinated olefinic monomer produced through the catalytic hydrodechlorination of trichlorotrifluoroethane(CFC-113),an eco-friendly ***,hydrodechlorination catalysts for olefin production often suffer from poor *** Pd/AC catalyst and Pd-Cu/AC catalyst prepared by co-impregnation method exhibited poor stability,Pd-Cu/AC catalyst with CFC-113 conversion dropping to around 37%after 50 h of hydrodechlorination ***-Emmett-Teller,transmission electron microscopy,X-ray photoelectron spectroscopy,and X-ray diffraction of fresh and deactivated Pd/AC catalysts indicate that the deactivation of Pd/AC catalysts is due to high-temperature agglomeration of *** analysis of fresh and deactivated Pd-Cu/AC catalysts using Brunauer-Emmett-Teller,transmission electron microscopy,and thermogravimetric analysis techniques revealed decreased dispersion of active sites,reduced surface area,catalyst aggregation deactivation,and a significant decrease in Cu ***,the results of NH3-TPD revealed that the acid sites of the catalyst increased significantly.X-ray diffraction spectra indicated the formation of new species,basic copper chloride(Cu_(2)(OH)_(3)Cl),during the *** the reaction progressed,these new species agglomerated,leading to a gradual loss of catalyst ***,the deactivated catalyst was successfully reactivated using a simple alkaline washing method.

关键词： CFC-113 Hydrodechlorination Chlorotrifluoroethylene Catalyst deactivation

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