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Mechanistic insight into the synergy between nickel single atoms and nanoparticles on N-doped carbon for electroreduction of CO2

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Journal of Energy Chemistry 2025年第1期100卷 327-336页

作者： Mingdong Sun Wenwen Guan Cailing Chen Chao wu Xiaoling Liu Biao Meng tao Chen yu Han Jun Wang shibo Xi yu Zhou State Key Laboratory of Materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Advanced Membranes and Porous Materials Center Physical Sciences and Engineering Division King Abdullah University of Science and Technology Institute of Sustainability for Chemicals Energy and Environment A*STAR (Agency for Science Technology and Research) College of Materials Science and Engineering Sichuan University

The synergy of single atoms （SAs） and nanoparticles （NPs） has demonstrated great potential in promoting the electrocatalytic carbon dioxide reduction reaction （CO2RR）;however,the rationalization of the SAs/NPs proportion remains one challenge for the catalyst ***,a Ni2+-loaded porous poly（ionic liquids）(PIL) precursor synthesized through the free radical self-polymerization of the ionic liquid monomer,1-allyl-3-vinylimidazolium chloride,was pyrolyzed to prepare the Ni,N co-doped carbon materials,in which the proportion of Ni SAs and NPs could be facilely modulated by controlling the annealing *** catalyst Ni-NC-1000 with a moderate proportion of Ni SAs and NPs exhibited high efficiency in the electrocatalytic conversion of CO2into *** Ni K-edge X-ray absorption near-edge structure （XANES） spectra and theoretical calculations were conducted to gain insight into the synergy of Ni SAs and *** charge transfer from Ni NPs to the surrounding carbon layer and then to the Ni SAs resulted in the electron-enriched Ni SAs active *** the electroreduction of CO2,the coexistence of Ni SAs and NPs strengthened the CO2activation and the affinity towards the key intermediate of*COOH,lowering the free energy for the potential-determining*CO2→*COOH step,and therefore promoted the catalysis efficiency.

关键词： Single atom catalyst Synergy effect Carbon catalyst Electrocatalysis

Algebraic Properties of Dual Toeplitz Operators on the Orthogonal Complement of the Dirichlet Space

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Acta Mathematica Sinica,English Series 2008年第11期24卷 1843-1852页

作者： tao yu shi yue wu Department of Mathematics Zhejiang Normal University Jinhua 321004 P. R. China Department of Mathematics Jilin University Changchun 130024 P. R. China

In this paper we investigate some algebra properties of dual Toeplitz operators on the orthogonal complement of the Dirichlet space in the Sobolev space. We completely characterize commuting dual Toeplitz operators with harmonic symbols, and show that a dual Toeplitz operator commutes with a nonconstant analytic dual Toeplitz operator if and only if its symbol is analytic. We also obtain the sufficient and necessary conditions on the harmonic symbols for SφSφψ= Sφψ.

关键词： Sobolev space Dirichlet space dual Toeplitz operator

Sine oculis homeobox homolog family function in gastrointestinal cancer:Progression and comprehensive analysis

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World Journal of Clinical Oncology 2025年第1期16卷 10-24页

作者： Yang-Zheng Lan Zheng wu Wen-Jia Chen Xin-Ning yu Hua-tao wu Jing Liu Department of The Breast Center Cancer Hospital of Shantou University Medical CollegeShantou 515041Guangdong ProvinceChina Department of General Surgery First Affiliated Hospital of Shantou University Medical CollegeShantou 515041Guangdong ProvinceChina

The sine oculis homeobox homolog(SIX)family,a group of transcription factors characterized by a conserved DNA-binding homology domain,plays a critical role in orchestrating embryonic development and organogenesis across various organisms,including *** six distinct members,from SIX1 to SIX6,each member contributes uniquely to the development and differentiation of diverse tissues and organs,underscoring the versatility of the SIX *** or mutations in SIX genes have been implicated in a spectrum of developmental disorders,as well as in tumor initiation and progression,highlighting their pivotal role in maintaining normal developmental trajectories and cellular *** to target the transcriptional complex of the SIX gene family have emerged as a promising strategy to inhibit tumor *** the development of inhibitors targeting this gene family is still in its early stages,the significant potential of such interventions holds promise for future therapeutic ***,this review aimed to comprehensively explore the advancements in understanding the SIX family within gastrointestinal cancers,focusing on its critical role in normal organ development and its implications in gastrointestinal cancers,including gastric,pancreatic,colorectal cancer,and hepatocellular *** conclusion,this review deepened the understanding of the functional roles of the SIX family and explored the potential of utilizing this gene family for the diagnosis,prognosis,and treatment of gastrointestinal cancers.

关键词： Sine oculis homeobox homolog Gastrointestinal cancer Transcription factor Development Regulation Diagnosis Therapeutics

miRNA-21-5p is an important contributor to the promotion of injured peripheral nerve regeneration using hypoxia-pretreated bone marrow-derived neural crest cells

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Neural Regeneration Research 2025年第1期20卷 277-290页

作者： Meng Cong Jing-Jing Hu Yan yu Xiao-Li Li Xiao-Ting Sun Li-Ting Wang Xia wu Ling-Jie Zhu Xiao-Jia Yang Qian-Ru He Fei Ding Hai-Yan shi School of Medicine Nantong UniversityNantongJiangsu ProvinceChina Key Laboratory of Neuroregeneration of Jiangsu and Ministry of Education and Coinnovation Center of Neuroregeneration Nantong UniversityNantongJiangsu ProvinceChina Department of Physiology Jiangsu Health Vocational CollegeNanjingJiangsu ProvinceChina Department of Pathology Affiliated Hospital of Nantong UniversityNantongJiangsu ProvinceChina Jiangsu Clinical Medicine Center of Tissue Engineering and Nerve Injury Repair Affiliated Hospital of Nantong UniversityNantongJiangsu ProvinceChina

Our previous study found that rat bone marrow–derived neural crest cells(acting as Schwann cell progenitors)have the potential to promote long-distance nerve ***-based therapy can enhance peripheral nerve repair and regeneration through paracrine bioactive factors and intercellular ***,the complex contributions of various types of soluble cytokines and extracellular vesicle cargos to the secretome remain *** investigate the role of the secretome and extracellular vesicles in repairing damaged peripheral nerves,we collected conditioned culture medium from hypoxia-pretreated neural crest cells,and found that it significantly promoted the repair of sensory neurons damaged by oxygen-glucose *** mRNA expression of trophic factors was highly expressed in hypoxia-pretreated neural crest *** performed RNA sequencing and bioinformatics analysis and found that miR-21-5p was enriched in hypoxia-pretreated extracellular vesicles of neural crest ***,to further clarify the role of hypoxia-pretreated neural crest cell extracellular vesicles rich in miR-21-5p in axonal growth and regeneration of sensory neurons,we used a microfluidic axonal dissociation model of sensory neurons in vitro,and found that hypoxia-pretreated neural crest cell extracellular vesicles promoted axonal growth and regeneration of sensory neurons,which was greatly dependent on loaded ***,we constructed a miR-21-5p-loaded neural conduit to repair the sciatic nerve defect in rats and found that the motor and sensory functions of injured rat hind limb,as well as muscle tissue morphology of the hind limbs,were obviously *** findings suggest that hypoxia-pretreated neural crest extracellular vesicles are natural nanoparticles rich in ***-21-5p is one of the main contributors to promoting nerve regeneration by the neural crest cell *** helps to explain the mechanism of action of the secretome and e

关键词： axotomy cell-free therapy conditioned medium extracellular vesicles hypoxic preconditioning microRNA oxygen-glucose deprivation peripheral nerve injury Schwann cell precursors

Tunable band structures of polycrystalline graphene by external and mismatch strains

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Acta Mechanica Sinica 2012年第6期28卷 1539-1544页

作者： Jiang-tao wu Xing-Hua shi yu-Jie Wei LNM Institute of Mechanics Chinese Academy of Sciences

Lacking a band gap largely limits the application of graphene in electronic devices. Previous study shows that grain boundaries （GBs） in polycrystalline graphene can dra- matically alter the electrical properties of graphene. Here, we investigate the band structure of polycrystalline graphene tuned by externally imposed strains and intrinsic mismatch strains at the GB by density functional theory （DFT） calcu- lations. We found that graphene with symmetrical GBs typ- ically has zero band gap even with large uniaxial and biax- ial strain. However, some particular asymmetrical GBs can open a band gap in graphene and their band structures can be substantially tuned by external strains. A maximum band gap about 0.19 eV was observed in matched-armchair GB （5, 5） I （3, 7） with a misorientation of θ = 13° when the applied uniaxial strain increases to 9%. Although mismatch strain is inevitable in asymmetrical GBs, it has a small influence on the band gap of polycrystalline graphene.

关键词： Graphene Grain boundary Defects Strain and gap

Effects of La addition on the microstructure and tensile properties of Al-Si-Cu-Mg casting alloys

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International Journal of Minerals,Metallurgy and Materials 2015年第4期22卷 405-410页

作者： tao Lu Ye Pan Ji-li wu shi-wen tao yu Chen School of Materials Science and Engineering Southeast University Jiangsu Key Laboratory of Advanced Metallic Materials Southeast University

The effects of La addition on the microstructure and tensile properties of B-refmed and Sr-modified A1-1 1Si-1.5Cu-0.3Mg cast- ing alloys were investigated. With a trace addition of La （0.05wt%-0. lwt%）, the mutual poisoning effect between B and Sr can be neutral- ized by the formation of LaB6 rather than SrB6. By employing a La/B weight ratio of 2：1, uniform microstructures, which are characterized by well refined ct-A1 grains and adequately modified eutectic Si particles as well as the incorporation of precipitated strengthening intermetal- lics, are obtained and lead to appreciable tensile properties with an ultimate tensile strength of 270 MPa and elongation of 5.8%.

关键词： aluminum silicon alloys rare earth addition lanthanum microstructure tensile properties precipitates

Resistin might not be a risk factor for carotid artery atherosclerosis in elderly Chinese males

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Journal of Geriatric Cardiology 2014年第3期11卷 222-228页

作者： Hao WANG yu-Tang WANG Li FAN yu-tao GUO Yang shi tao tao yue-Xiang ZHAO First Geriatric Cardiology Division Chinese PLA General Hospital 28 Fuxing Rd. Beijing 100853 China

Objective To investigate the correlation between the serum resistin level and carotid artery atherosclerosis in elderly Chinese males. Methods The study enrolled 235 elderly Chinese males [median age 76 （range 60-97） years] scheduled for ultrasound examination of carotid artery plaque and determination of carotid artery intima-media thickness （CIMT）. They were divided into carotid atherosclerotic plaque （CAP） and carotid atherosclerotic plaque-free （CAP-free） groups according to the ultrasound results. Their clinical profiles were col-lected, and the serum resistin and other blood biochemistry levels were *** The CAP group was older and had a thicker mean CIMT than the CAP-free group. However, there was no difference in the serum resistin level between the groups. CIMT was positively correlated with age （r = 0.299,P〈 0.001）. The serum resistin level was not correlated with CIMT, even after controlling for age. Multiple linear regression analysis revealed that age （β = 0.001,P〈 0.001） and body mass index （β = 0.002,P= 0.015） were significantly and posi-tively correlated with the mean CIMT. Only age [odds ratio （OR）： 1.159; 95% confidence interval （CI）： 1.078-1.183,P〈 0.001] was associ-ated with the presence of carotid artery atherosclerotic plaque. The serum resistin level was not correlated with the mean CIMT or associated with the presence of carotid artery atherosclerotic *** The results suggest that resistin might not be a risk factor for atherosclerosis in elderly Chinese males.

关键词： Resistin Intima-media thickness Atherosclerosis The elderly

A 2-D mesoscopic model for the evaluation of creep damage induced by void growth in polycrystalline metals

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Acta Metallurgica Sinica(English Letters) 2011年第3期24卷 213-219页

作者： tao yu Kimiaki YOshiDA Huiji shi Key Laboratory of Applied Mechanics Department of Engineering Mechanics Tsinghua University Beijing 100084 China v Research Laboratory Ishikawajima-Harima Heary Industries Co. Ltd. Tokyo Japan

At elevated temperature, creep failures of polycrystalline metals after long-term constant loading are often caused by the nucleation, growth and coalescence of creep voids on the grain boundaries. Void h＇action is an important parameter for the evaluation of creep damage level of structural materials operating at high temperature. In this paper, a 2-D numerical simulation method was developed for analyzing the void fraction evolution during the process of creep, based on some hypothesis from experiments. The model was implemented and then was used to predict the evolution of void fraction in the 2.25Cr-1Mo steel of uniaxial creep experiment at 570 ℃, in which the simulation results showed good agreement with the experimental results.

关键词： Creep damage Grain boundary Void fraction Voronoi tessellation

A Multi-model,Large-range Flexible Strain Sensor Based on Carbonized Silk Habotai for Human Health Monitoring

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Chinese Journal of Polymer Science 2023年第8期41卷 1238-1249,I0008页

作者： shi-Dong Ma yu-Ting wu Jian Tang yu-Min Zhang tao Yan Zhi-Juan Pan College of Textile and Clothing Engineering Soochow UniversitySuzhou 215123China National Engineering Laboratory for Modern Silk Suzhou 215123China

In recent years,flexible strain sensors have received considerable attention owing to their excellent flexibility and ***,it is still a great challenge for them to accurately monitor multi-model deformations with high sensitivity and *** this study,the industrial insulating silk habotai was successfully converted into carbonized silk habotai(CSH)for use in strain sensors.A strain sensor created using CSH exhibited excellent sensing performance under multi-model deformations,including stretching,twist and *** maximum tensile strain was 434%.The gauge factors were 14.6 in the wide tensile range of 0%–400%with a high linearity of *** addition,the CSH strain sensor exhibited an extremely fast response time(110 ms)and could accurately detect bending(0°–180°)and torsional(0°–180°)*** durability and repeatability were observed for the multi-model ***,a new type of smart pillow was developed to accurately record head movement and breathing during *** sensor may also be used for auxiliary training in table *** proposed CSH strain sensor has shown great potential for applications in smart devices and human-machine interactions.

关键词： Carbonized silk habotai Strain sensor Smart pillow Human motions