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Material conversion from paper sludge ash in NaOH solution to synthesize adsorbent for removal of Pb^(2+),NH_4^+and PO_4^(3-) from aqueous solution

氟化学与美好生活——中国化学会第十一届全国氟化学会议

作者： takaaki sonoda Institute for Materials Chemistry and Engineering Kyushu University

＜正＞Phenyl cations and benzyne are known as reactive intermediates in aromatic nucleophilic substitution *** effects of substituent groups on the stability and reactivity of these intermediates in some thermal and photochemical reactions of aryl triflates and halides as well as arene diazonium ions are comparativelyinvestigated by experimental and computational *** displacement of triflate group of aryl triflates with various nucleophiles is demonstrated as a novel aromatic nucleophilic substitution reaction.

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Journal of Environmental Sciences 2011年第5期23卷 718-724页

作者： takaaki Wajima Kenzo Munakata Faculty of Engineering and Resource Sciences Akita University

Material conversion from paper sludge ash （PSA） in NaOH solution was attempted to synthesize the adsorbent for removal of inorganic pollutants, such as Pb^2＋, NH^4＋ and PO4^3- from aqueous solution. PSA of 0.5 g was added into 10 mL of 3 mol/L NaOH solution, and then heated at 80, 120, and 160℃ for 6-48 hr to obtain the product. PSA mainly composed of two crystalline phases, gehlenite （Ca2Al2SiO7） and anorthite （CaAl2Si2O8）, and amorphous phase. Hydroxysodalite （Na6Al6Si6O24-8H2O） was formed at 80℃, and anorthite dissolved, whereas gehlenite remained unaffected. Katoite （Ca3Al2SiO4（OH）8） was formed over 120℃, and hydroxycancrinite （Nas（OH）2Al6Si6O24·2H2O） was formed at 160℃, due to the dissolution of both gehlenite and anorthite. Specific surface areas of the products were almost same and were higher than that of raw ash. Cation exchange capacities （CECs） of the products were also higher than that of raw ash, and CEC obtained at lower temperature was higher. Removal abilities of products for Pb^2＋, NH4＋, and PO4^3- were higher than that of raw ash. With increasing reaction temperature, the removal efficiencies of Pb^2＋ and NH4＋ decreased due to the decrease of CEC of the product, while removal efficiency for PO4^3- was almost same. The concentrations of Si and AI in the solution and the crystalline phases in the solid during the reaction explain the formation of the product phases at each temperature.

关键词： paper sludge ash hydrothermal synthesis gehlenite anorhite heavy metal ion ammonium ion phosphate ion

First molecular genetic evidenee for automictic parthenogenesis in cockroaches

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Insect Science 2019年第4期26卷 649-655页

作者： Masashi Tanaka takaaki Daimon Department of Applied Biosciences Graduate School of Agriculture Kyoto University Kitashirakawa Oiwakecho Sakyo-ku Kyoto Japan

Parthenogenesis is an asexual mode of reproduction that plays an important role in the evolution of sex, sociality, and reproduction strategies in insects. Some species of cockroach exhibit thelytoky, a type of parthenogenesis in which female offspring are produced without fertilization. However, the cytological and genetic mecha? nisms of parthenogenesis in cockroaches are not well understood. Here we provide the first molecular genetic evidence that cockroaches can reproduce through automixis. Using the American cockroach Periplaneta aniericana, we performed microsatellite analysis to investigate the genetic relationship between parthenogenetically produced nymphs and the parent virgin females, and found that all parthenogenetic offspring were homozygous for autosomal microsatellite markers, whereas the female parents were heterozygous. In addition, flow cytometry analysis revealed that the parthenogenetic offspring were diploid. Taken together, our results demonstrate that P. americana exhibits automixis-type thelytoky, in which diploidy is restored by gamete duplication or terminal fusion. These findings highlight the unique reproduction strategies of cockroaches, which are more varied than was previously recognized.

关键词： American cockroach automixis microsatellite Periplaneta thelytoky

Linear seesaw model with a modular S_(4)flavor symmetry

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Chinese Physics C 2022年第5期46卷 11-19页

作者： takaaki Nomura Hiroshi Okada College of Physics Sichuan UniversityChengdu 610065China Asia Pacific Center for Theoretical Physics(APCTP)-Headquarters San 31 Hyoja-dongNam-guPohang 790-784Korea Department of Physics Pohang University of Science and TechnologyPohang 37673Korea

We discuss a linear seesaw model with a field content as minimum as possible,introducing a modular S_(4)using gauged U(1)_(B−L) *** to the rank two neutrino mass matrix,we obtain a vanishing neutrino mass eigenvalue,and only the normal mass hierarchy of neutrinos is favored via the modular S_(4)*** our numericalΔχ^(2)analysis,we especially determine a relatively sharp prediction on the sum of neutrino masses to be approximately 60 meV,in addition to other predictions.

关键词： neutrino mass linear seesaw mechanism modular S_(4)flavor symmetry

Potentials of GHG reductions from wastewater treatment for the CDM

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Science China(Technological Sciences) 2011年第7期54卷 1649-1654页

作者： takaaki FURUBAYASHI Toshihiko NAKATA Department of Management Science & Technology Graduate school of Engineering Tohoku University

The study aims to evaluate the potential of GHG （greenhouse gas） reductions by installing an anaerobic digester in a wastewater treatment facility in Southeast Asia. Then the break-even point of additional investment to reduce GHG is obtained by exchanging carbon price as emissions credits. In the project scenario, the wastewater treatment system has the digester, where methane （biogas） is produced and recovered. Compared with the baseline scenario, the biogas has calorific value to produce heat and electricity, and can substitute fossil fuels for power generation. The objective of the study is to define the relationship between CERs （certified emission reductions） and investment costs, and the beak-even point, finding out the dominant pa- rameters in the system. Financial parameters such as capital costs and operating costs are considered to evaluate the investmerit costs. The result shows that the methane recovery reduces 54% of GHG emissions. Although the substitution of the biogas for the fossil fuels reduces only 6% of the GHG emissions, the electricity output can satisfy the electricity consumption. The results also show that the maximum CER credit is 73000 t-COEe/a, and the GHG reduction cost is 14 USD/t-CO2e.

关键词： wastewater treatment system anaerobic digestion GHG reductions developing countries CDM

Optical second-harmonic generation measurement for probing organic device operation

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Light(Science & Applications) 2015年第1期4卷 99-108页

作者： takaaki Manaka Mitsumasa Iwamoto Department of Physical Electronics Tokyo Institute of Technology2-12-1 O-okayamaMeguro-kuTokyo 152-8552Japan

We give a brief overview of the electric-field induced optical second-harmonic generation(EFISHG)technique that has been used to study the complex behaviors of organic-based *** analyzing EFISHG images of organic field-effect transistors,the in-plane two-dimensional distribution of the electric field in the channel can be *** susceptibility tensor of the organic semiconductor layer and the polarization of the incident light are considered to determine the electric field *** imaging can effectively evaluate the distribution of the vectorial electric field in organic films by selecting a light *** the time-resolved technique,measurement of the electric field originating from the injected carriers allows direct probing of the carrier motion under device operation,because the transient change of the electric field distribution reflects the carrier *** applications of the EFISHG technique to organic electronic devices are reviewed.

关键词： electric field optical second-harmonic generation semiconductor device

Numerical Simulation for Fan Broadband Noise Prediction

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Journal of Thermal Science 2011年第1期20卷 58-63页

作者： takaaki Hase Nobuhiko Yamasaki Tsutomu Ooishi Kyushu University Fukuoka819-0395Japan IHI Corporation Nishitama-gunTokyo190-1297Japan

In order to elucidate the broadband noise of fan,the numerical simulation of fan operating at two different rotational speeds is carried out using the three-dimensional unsteady Reynolds-averaged Navier-Stokes (URANS) *** computed results are compared to experiment to estimate its accuracy and are found to show good agreement with experiment.A method is proposed to evaluate the turbulent kinetic energy in the framework of the Spalart-Allmaras one equation turbulence *** the calculation results,the turbulent kinetic energy is visualized as the turbulence of the flow which leads to generate the broadband noise,and its noise sources are identified.

关键词： Broadband Noise Fan Noise Rotor-Stator Interaction URANS

A multi-charged particle model with local U(1)_(μ-τ) to explain muon g-2,flavor physics,and possible collider signature

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Chinese Physics C 2022年第4期46卷 57-69页

作者： Nilanjana Kumar takaaki Nomura Hiroshi Okada Department of Physics and Astrophysics University of DelhiDelhi 110007India School of Physics KIASSeoul 02455Korea Asia Pacific Center for Theoretical Physics(APCTP)-Headquarters San 31 Hyoja-dongNam-guPohang 790-784Korea Department of Physics Pohang University of Science and TechnologyPohang 37673Korea

We consider a model with multi-charged particles,including vector-like fermions,and a charged scalar under a local U(1)_(μ−τ) *** search for an allowed parameter region explaining muon anomalous magnetic moment(muon g−2)and b→sℓ^(+)ℓ^(−) anomalies,satisfying constraints from the lepton flavor violations,Z boson decays,meson anti-meson mixing,and collider *** numerical analysis,we explore the typical size of the muon g−2 and Wilson coefficients to explain the b→sℓ^(+)ℓ^(−) anomalies in our model when all other experimental constraints are ***,we discuss the collider physics of the multicharged vectorlike fermions,considering a number of benchmark points in the allowed parameter space.

关键词： new gauge boson new gauge symmetry muon anomalous magnetic moment B meson decay anomalies collider physics

Heavy metal removal from aqueous solution using carbonaceous K_2S-impregnated adsorbent

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Journal of Environmental Sciences 2009年第12期21卷 1730-1734页

作者： takaaki Wajima Kenji Murakami Takahiro Kato Katsuyasu Sugawara Faculty of Engineering and Resource Science Akita University

A novel carbonaceous adsorbent for heavy metal removal was prepared from raw coal by one-step simple sulfur impregnation using K2S. Raw coal was mixed with K2S powder and then heated at 800℃ for 30 min in nitrogen to produce K2S char. The sulfur content and form in K2S char were determined, and the ability of K2S char to adsorb Zn^2＋, Cd^2＋ and Pb^2＋ was examined. The K2S impregnation was effective at impregnating sulfur into coal, especially in the form of elemental, thiophenic and sulfatic sulfur. The sulfur content of K2S char was higher than those of raw coal and pyrolysis char. The Zn^2＋ removal in 2.4 mmol/L of Zn^2＋ solution by K2S char was higher than raw coal with the removal rate of 100%. K2S char adsorbed Pb^2＋ and Cd^2＋ in 24 mmol/L of Pb^2＋ and Cd^2＋ solution with the removal rate of 97% and 35%, respectively. The elution extents of adsorbed Pb^2＋ and Cd^2＋ were zero in distilled water and 27% in 0.1 mol/L HCl solution. These results indicated that an effective adsorbent for heavy metal ions was prepared from coal using K2S sulfur impregnation, and that the adsorbed metals were strongly retained in K2S char.

关键词： sulfur impregnation carbonaceous adsorbent K2S heavy metal adsorption

ZKP Protocols for Usowan,Herugolf,and Five Cells

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Tsinghua Science and Technology 2024年第6期29卷 1651-1666页

作者： Daiki Miyahara Léo Robert Pascal Lafourcade takaaki Mizuki Graduate School of Informatics and Engineering The University of Electro-CommunicationsTokyo 1828585Japan MIS Lab University of Picardy Jules VerneAmiens 80000France Laboratory of Computer Science Modelling and Systems OptimisationUniversity of Clermont AuvergneClermont-Ferrand 63178France Cyberscience Center Tohoku UniversitySendai 9808578Japan

A Zero-Knowledge Proof (ZKP) protocol allows a participant to prove the knowledge of some secret without revealing any information about it. While such protocols are typically executed by computers, there exists a line of research proposing physical instances of ZKP protocols. Up to now, many card-based ZKP protocols for pen-and-pencil puzzles, like Sudoku, have been designed. Those games, mostly edited by Nikoli, have simple rules, yet designing them in card-based ZKP protocols is non-trivial. In this work, we propose a card-based ZKP protocol for Usowan, a Nikoli game. In Usowan, for each room of a puzzle instance, there is exactly one piece of false information. The goal of the game is to detect this wrong data amongst the correct data and also to satisfy the other rules. Designing a card-based ZKP protocol to deal with the property of detecting a liar has never been done. In some sense, we propose a physical ZKP for hiding of a liar. This work extends a previous paper appearing in Ref. [1]. In this extension, we propose two other protocols, for Herugolf and Five Cells. The puzzles are specifically chosen because each of those three puzzles shares a common constraint, connectivity. However, showing the connected configuration cannot be done with generic approach and brings new construction to the existing connectivity ZKP protocol. Indeed, in Herugolf, the connectivity is handled with a given length of cell which is decremental (i.e., the length of each connected cell decreases by one at each step). For Five Cells, there is an additional step in the setup allowing to encode all the information needed to ensure a valid ZKP protocol.

关键词： Zero-Knowledge Proof(ZKP)protocol playing cards card-based cryptography physical assumptions Usowan Herugolf FiveCells