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Theoretical and Experimental Studies of Schottky Diodes that Use Aligned Arrays of Single-Walled Carbon Nanotubes

Nano Research 2010年第6期3卷 444-451页

作者： Xinning Ho Lina Ye slava v.rotkin Xu Xie Frank Du Simon Dunham Jana Zaumseil John A.Rogers Department of Materials Science and Engineering Beckman Instituteand Frederick Seitz Materials Research LaboratoryUniversity of Illinois at Urbana-Champaign1304 West Green StreetUrbanaIllinois 61801USA Department of Chemistry University of Science and Technology of ChinaHefei 230026China Department of Physics Lehigh UniversityBethlehemPennsylvania 18015 and Centre for Advanced Materials and NanotechnologyLehigh UniversityBethlehemPennsylvania 18015USA Center for Nanoscale Materials Argonne National LaboratoryArgonneIllinois 60439USA Department of Chemistry University of Illinois at Urbana-ChampaignUrbanaIllinois 61801USA Department of Electrical and Computer Engineering Mechanical Science and EngineeringUniversity of Illinois at Urbana-ChampaignUrbanaIllinois 61801USA

We present theoretical and experimental studies of Schottky diodes that use aligned arrays of single-walled carbon nanotubes. A simple physical model, taking into account the basic physics of current rectification, can adequately describe the single-tube and array devices. We show that for as-grown array diodes, the rectification ratio, defined by the maximum-to-minimum-current-ratio, is low due to the presence of metallic-single-walled nanotube (SWNT) shunts. These tubes can be eliminated in a single voltage sweep resulting in a high rectification array device. Further analysis also shows that the channel resistance, and not the intrinsic nanotube diode properties, limits the rectification in devices with channel length up to 10 μm.

关键词： Schottky diodes aligned arrays single-walled carbon nanotubes

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Two-color spectroscopy of Uv excited ssDNA complex with a single-wall nanotube photoluminescence probe： Fast relaxation by nucleobase autoionization mechanism

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Nano Research 2016年第2期9卷 571-583页

作者： Tetyana Ignatova Alexander Balaeff Michael Blades Ming Zheng: Peter Stoeckl slava v. rotkin Physics Department Lehigh University 16 Memorial Dr. E. Bethlehem PA 1801S USA NanoScience Technology Center University of Central Florida 12424 Research Parkway Suite 400 Orlando FL 32826 USA National Institute of Standards and Technology 100 Bureau Drive Gaithersburg MD 20899 USA Department of Physics & Astronomy University of Rochester 206 Bausch & Lomb Hall Rochester NY 14627 USA Physics Department Center for Advanced Materials & Nanotechnology and Center for Photonics & Nanoelectronics Lehigh University16 Memorial Dr. E. Bethlehem PA 18015 USA

DNA autoionization is a fundamental process wherein ultraviolet （Uv）- photoexcited nucleobases dissipate energy by charge transfer to the environment without undergoing chemical damage. Here, single-wall carbon nanotubes （SWNT） are explored as a photoluminescent reporter for the study of the mechanism and rates of DNA autoionization. Two-color photoluminescence spectroscopy allows separate photoexcitation of the DNA and the SWNTs in the Uv and visible range, respectively. A strong SWNT photoluminescence quenching is observed when the Uv pump is resonant with the DNA absorption, consistent with charge transfer from the excited states of the DNA to the SWNT. Semiempirical calculations of the DNA-SWNT electronic structure, combined with a Green＇s function theory for charge transfer, show a 20 fs autoionization rate, dominated by hole transfer. Rate-equation analysis of the spectroscopy data confirms that the quenching rate is limited by thermalization of the free charge carriers transferred to the nanotube reservoir. This approach has great potential for monitoring DNA excitation, autoionization, and chemical damage, both in vivo and in vitro.

关键词： single-wall nanotube optical spectroscopy two-color spectroscopy DNA autoionization DNA ultraviolet (Uv) excitation quantum-mechanical modeling

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