检索结果-南通市图书馆

green Chemical Engineering 2024年第2期5卷 236-244页

作者： Chi ma Lihong Zhao Zhengxin mao Hao Su Qingfen Liu CAS Key Laboratory of green Process and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing100190China School of Chemical Engineering University of Chinese Academy of SciencesBeijing100049China

Industrial pharmaceutical wastewater usually contains butyl acetate(BA)with a concentration of 1 wt%-7 wt%,and the traditional method for BA recovery is distillation with high energy *** method is developed to recover BA with low concentration for the high efficiency and low energy *** polar polyacrylate resins with macroporous structure of 233.1 nm and average particle size of about 526.5μm are successfully synthesized by suspension polymerization and used for the BA adsorption and *** maximum adsorption capacity reaches 171.1 mg g^(-1)with relative standard deviation(RSD)value of 0.2%,which is more than twice the results in the *** BA desorption rate is 97.0%at 100℃with RSD value of 0.4%,and the resins are beneficial to the reuse in the adsorption-desorption *** adsorption thermodynamics and kinetics are investigated,and the BA adsorption is a spontaneous and endothermic process with the increase of disorder *** process is mainly contributed by physical absorption and agree well with Freundlich model and pseudo-first-order adsorption kinetic *** adsorption method avoids boiling a large amount of wastewater and hopefully provides a novel alternative technology for the BA recovery.

关键词： Butyl acetate recovery Resin adsorption Desorption Thermodynamics Kinetics

维普期刊数据库

A self-centering and stiffness-controlled MEMS accelerometer

在线全文

学校读者我要写书评

暂无评论

Microsystems & Nanoengineering 2024年第1期10卷 27-40页

作者： Yiming Jin Zhipeng ma Ziyi Ye Mingkang Li Xudong Zheng Zhonghe Jin School of Aeronautics and Astronautics Zhejiang UniversityHangzhou 310013China Key Laboratory of Micro/Nano-Satellite Research of Zhejiang Province Hangzhou 310007PR China

This paper presents a high-performance MEMS accelerometer with a DC/AC electrostatic stiffness tuning capability based on double-sided parallel plates(DSPPs).DC and AC electrostatic tuning enable the adjustment of the effective stiffness and the calibration of the geometric offset of the proof mass,respectively.A dynamical model of the proposed accelerometer was developed considering both DC/AC electrostatic tuning and the temperature *** on the dynamical model,a self-centering closed loop is proposed for pulling the reference position of the forceto-rebalance(FTR)to the geometric center of *** self-centering accelerometer operates at the optimal reference position by eliminating the temperature drift of the readout circuit and nulling the net electrostatic tuning *** stiffness closed-loop is also incorporated to prevent the pull-in instability of the tuned low-stiffness accelerometer under a dramatic temperature ***-time adjustments of the reference position and the DC tuning voltage are utilized to compensate for the residue temperature drift of the proposed *** a result,a novel controlling approach composed of a self-centering closed loop,stiffness-closed loop,and temperature drift compensation is achieved for the accelerometer,realizing a temperature drift coefficient(TDC)of approximately 7μg/℃ and an Allan bias instability of less than 1μg.

关键词： stiffness electrostatic centering

Overcoming the Na-ion conductivity bottleneck for the cost-competitive chloride solid electrolytes

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2024年第8期95卷 1-8,I0001页

作者： Lv Hu Hui Li Fang Chen Yating Liu Jinzhu Wang Cheng ma Hefei National Research Center for Physical Sciences at the Microscale CAS Key Laboratory of Materials for Energy ConversionDepartment of Materials Science and EngineeringUniversity of Science and Technology of ChinaHefei 230026AnhuiChina National Synchrotron Radiation Laboratory Hefei 230026AnhuiChina

Chloride solid electrolytes possess multiple advantages for the construction of safe,energy-dense allsolid-state sodium batteries,but presently the chlorides with sufficiently high cost-competitiveness for commercialization almost all exhibit low Na-ion conductivities of around 10^(-5)S cm^(-1)or ***,we report a chloride solid electrolyte,Na_(2.7)ZFCl_(5.3)O_(0.7),which reaches a Na-ion conductivity of 2.29×10^(-4)S cm^(-1)at 25℃without involving overly expensive raw materials such as rare-earth chlorides or Na_(2)*** addition to the efficient ion transport,Na_(2.7)ZrCl_(5.3)O_(0.7)also shows an excellent deformability surpassing that of the widely studied Na_(3)PS_(4),Na_(3)SbS_(4),and Na_(2)ZrCl_(6)solid *** combination of these advantages allows the all-solid-state cell based on Na_(2.7)ZrCl_(5.3)O_(0.7)and NaCrO_(2)to realize stable room-temperature cycling at a much higher specific current than those based on other non-viscoelastic chloride solid electrolytes in literature(120 ma g^(-1)vs.12-55 ma g^(-1));after 100 cycles at such a high rate,the Na_(2.7)ZFCl_(5.3)O_(0.7)-based cell can still deliver a discharge capacity of 80 mah g^(-1)at25℃.

关键词： All-solid-state sodium batteries Ionic conductivities Solid electrolytes Chlorides High voltage stability

维普期刊数据库

Rational design of new in situ reduction of Ni(II)catalytic system for low-cost and large-scale preparation of porous aromatic frameworks

在线全文

学校读者我要写书评

暂无评论

Carbon Energy 2024年第5期6卷 105-113页

作者： Shanshan Wang Yue Wu Wenxiang Zhang Hao Ren guangshan Zhu Heping ma School of Chemical Engineering and Technology Xi'an Jiaotong UniversityXi'anChina State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of ChemistryJilin UniversityChangchunChina College of Chemistry Northeast Normal UniversityChangchunChina

Porous aromatic framework 1(PAF-1)is an extremely representative nanoporous organic framework owing to its high stability and exceptionally high surface ***,the synthesis of PAF-1 is catalyzed by the Ni(COD)2/COD/bpy system,suffering from great instability and high ***,we developed an in situ reduction of the Ni(II)catalytic system to synthesize PAF-1 in low cost and high *** active Ni(0)species produced from the NiCl_(2)/bpy/NaI/Mg catalyst system can effectively catalyze homocoupling of tetrakis(4-bromophenyl)methane at the room temperature to form PAF-1 with high Brunauer-Emmett-Teller(BET)-specific surface area up to 4948 m^(2) g^(−1)(Langmuir surface area,6785 m2 g−1).The possible halogen exchange and dehalogenation coupling mechanisms for this new catalytic process in PAF's synthesis are discussed in *** efficiency and universality of this innovative catalyst system have also been demonstrated in other PAFs'*** work provides a cheap,facile,and efficient method for scalable synthesis of PAFs and explores their application for high-pressure storage of Xe and Kr.

关键词： adsorption carbon material nickel catalysis porous aromatic framework porous organic polymer

Design of Differential Multi-Point Feeding Dual-Polarized SISL Antenna Based on CM Analysis

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Journal of Electronics 2024年第5期33卷 1245-1252页

作者： Bin TANg Kaixue ma Eric Newton MORO Yu LUO Tianjin Key Laboratory of Imaging and Sensing Microelectronics Technology School of MicroelectronicsTianjin University

Dual-polarized antennas are required in the current mobile communication to increase the channel capacity and reducing multi-path effects. Utilizing characteristic mode(CM) analysis, this paper presents a five-patch substrate integrated suspended line(SISL) antenna with suppressed unwanted higher-order modes, and achieves an enhanced bandwidth by using differential multi-point feeding(MPF) systems. Compared to single-point feeding systems, the proposed dual-polarized SISL antenna with the MPF system demonstrates a bandwidth 1.87 times wider. The novel SISL feeding system incorporates two pairs of differentially-fed branch line feed structures. A prototype of the proposed differential-fed antenna is fabricated and measured, showing good agreement between simulated and measured results. The dual-polarization SISL antenna can achieve realized gain from 8.1 dBi to 10.8 dBi within a working frequency from 3.17 gHz to 3.61 gHz(12.98%). Moreover, utilizing low-cost substrates, the proposed SISL antenna has the potential for 5g applications.

关键词： Dual polarized Characteristic mode analysis Feeding system Broadband 5g Substrate integrated suspended line antenna Bandwidth enhanced Suppressed higher-order modes Characteristic mode analysis Feeding system Broadband 5g Substrate integrated suspended line antenna Bandwidth enhanced Suppressed higher-order modes MICROSTRIP PATCH ANTENNA LEAKY-WAVE ANTENNA LOW-PROFILE BANDWIDTH ENHANCEMENT ORDER MODES RADIATION REDUCTION OPERATION TM10

Virus-Host Interactions Drive Contrasting Bacterial Diel Dynamics in the Ocean

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Research 2024年第2期6卷 389-399页

作者： Xiaowei Chen Chen Hu Wei Wei Yunlan Yang markus g.Weinbauer Hongbo Li Shiying Ren Ruije ma YVibin Huang Tingwei Luo Nianzhi Jiao Rui Zhang State Key Laboratory of marine Environmental Science College of Ocean and Earth SciencesFujian Key Laboratory of Marine Carbon SequestrationXiamen UniversityXiamen 361102PR China College of the Environment and Ecology Xiamen UniversityXiamen 361102PR China Research Center for Environmental Ecology and Engineering School of Environmental Ecology and Biological EngineeringWuhan Institute of TechnologyWuhan 430205PR China Sorbonne Universités UPMCUniversitéParis 06CNRSLaboratoire d'Oceanographie de Villefranche(LOV)Villefranche-sur-Mer 06230France National marine Environmental Monitoring Center Ministry of Ecological EnvironmentDalian 116023PR China Department of Ocean Sciences University of CaliforniaSanta CruzCAUSA NOAA/OAR Pacific marine Environmental Laboratory SeattleWAUSA Institute for Advanced Study Shenzhen UniversityShenzhen 518055PR China

marine organisms perform a sea of diel *** diel dynamics have been shown to be driven by light,energy resources,circadian rhythms,and the coordinated coupling of photoautotrophs and heterotrophic ***,we explore the diel fluctuation of viral production and decay and their impact on the total and active bacterial community in the coastal and open seawaters of the South China *** results showed that the night-production diel pattern of lytic viral production was concurrent with the lower viral decay at night,contributing to the accumulation of the viral population size during the night for surface *** diel variations in bacterial activity,community composition,and diversity were found highly affected by viral *** was revealed by the finding that bacterial community diversity was positively correlated to lytic viral production in the euphotic zone of the open ocean but was negatively related to lysogenic viral production in the coastal *** distinct but contrasting correlations suggest that viral life strategies can not only contribute to diversifying bacterial community but also potentially piggyback their host to dominate bacterial community,suggesting the tightly synchronized depth-dependent and habitat-specific diel patterns of virus-host *** further implies that viruses serve as an ecologically important driver of bacterial diel dynamics across the ocean,highlighting the viral roles in bacterial ecological and biogeochemical processes in the ocean.

关键词： coastal ocean marine

Special Unipotent Representations of Simple Linear Lie groups of Type A

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Acta mathematica Sinica,English Series 2024年第3期40卷 707-716页

作者： Dan BARBASCH Jia Jun ma Bin Yong SUN Chen Bo ZHU Department of mathematics Cornell UniversityIthacaNY 14853USA School of mathematical Sciences Xiamen UniversityXiamen 361005P.R.China Department of mathematics Xiamen University Malaysia CampusSepangSelangor Darul Ehsan43900Malaysia Institute for Advanced Study in mathematics&New Cornerstone Science Laboratory Zhejiang UniversityHangzhou 310058P.R.China Department of mathematics National University of Singapore10 Lower Kent Ridge RoadSingapore 119076

Let g be a special linear group over the real,the complex or the quaternion,or a special unitary *** this note,we determine all special unipotent representations of g in the sense of Arthur and Barbasch-Vogan,and show... 详细信息

关键词： Special unipotent representations unitary representations coherent continuation Weyl group representations

维普期刊数据库

Micelle-directed self-assembly of single-crystal-like mesoporous stoichiometric oxides for high-performance lithium storage

在线全文

学校读者我要写书评

暂无评论

National Science Review 2024年第4期11卷 195-205页

作者： Yanhua Wan Changyao Wang Xingmiao Zhang Yang Yin Mengmeng Liu Bing ma Linlin Duan Yuzhu ma Wei Zhang Changlin Zheng Dongliang Chao Fei Wang Yongyao Xia Wei Li Department of Chemistry Laboratory of Advanced Materials Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials State Key Laboratory of Molecular Engineering of Polymers College of Chemistry and Materials ScienceFudan University State Key Laboratory of Surface Physics and Department of Physics Fudan University

Due to their uncontrollable assembly and crystallization process,the synthesis of mesoporous metal oxide single crystals remains a formidable ***,we report the synthesis of single-crystal-like mesoporous Li2TiSiO5by using soft micelles as *** key lies in the atomic-scale self-assembly and step-crystallization processes,which ensure the formation of single-crystal-like mesoporous Li2TiSiO5microparticles via an oriented attachment growth mechanism under the confinement of an in-situ formed carbon *** mesoporous Li2TiSiO5anode achieves a superior rate capability(148 mah g-1at5.0 A g-1) and outstanding long-term cycling stability(138 mah g-1after 3000 cycles at 2.0 A g-1) for lithium storage as a result of the ultrafast Li+diffusion caused by penetrating mesochannels and nanosized crystal frameworks（5-10 nm）.In comparison,bulk Li2TiSiO5exhibits poor rate capability and cycle performance due to micron-scale diffusion *** method is very simple and reproducible,heralding a new way of designing and synthesizing mesoporous single crystals with controllable frameworks and chemical functionalities.

关键词： mesoporous materials micelles single-crystal-like Li2TiSiO5 lithium-ion batteries

The on-chip thermoelectric cooler:advances,applications and challenges

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Chip 2024年第2期3卷 96-108页

作者： Chengjun Li Yubo Luo Wang Li Boyu Yang Chengwei Sun Wenyuan ma Zheng ma Yingchao Wei Xin Li Junyou Yang State Key Laboratory of materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China

With the development of 5g technology and increasing chip integration,traditional active cooling methods struggle to meet the growing thermal demands of *** coolers(TECs)have garnered great attention due to their rapid response,significant cooling differentials,strong compatibility,high stability and controllable device *** this review,starting from the fundamental principles of thermoelectric cooling and device design,high-performance thermoelectric cooling materials are summarized,and the progress of advanced on-chip TECs is comprehensively ***,the paper outlines the challenges and opportunities in TEC design,performance and applications,laying great emphasis on the critical role of thermoelectric cooling in addressing the evolving thermal management requirements in the era of emerging chip technologies.

关键词： Chip Thermal management Thermoelectric materials Thermoelectric cooler Cooling performance

Cobalt-doped TiO_(2)@C hierarchical nanocomposites derived from Ti_(3)C_(2) MXene as cathodes for hybrid magnesium-lithium batteries

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nano Research 2024年第1期17卷 253-261页

作者： Xiaohui Li Yakun Tang Lang Liu Yue Zhang Yang gao mao Qian Wenjie ma State Key Laboratory of Chemistry and Utilization of Carbon Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830017China

TiO_(2)has been explored in hybrid magnesium-lithium batteries(HMLBs)due to the advantages of low self-discharge and small volume expansion during ion ***,how to improve the inherently low ionic and electrical conductivity of TiO_(2)is the problem that needs to be *** this work,a smart strategy is adopted to prepare cobalt-doped TiO_(2)@C(Co^(4+)-TiO_(2)@C)hierarchical nanocomposite derived from Co(II)(OH)n@*** with TiO_(2)@C(without cobalt doping),Co^(4+)-TiO_(2)@C shows the highest specific capacity(154.7 mah·g^(-1)at 0.1 A·g^(-1)after 200 cycles)and extraordinary rate performance in *** excellent electrochemical performance of Co4+-TiO_(2)@C is ascribed to the synergistic effect of the hierarchical structure and *** experimental results and density functional theory(DFT)calculation reveal that the cobalt-doping has effectively improved the electronic conductivity and reduced the Li+migration *** work provides a new insight to design TiO_(2)-based cathode materials with high-performance in HMLBs.

关键词： Ti_(3)C_(2)MXene TiO_(2) hybrid magnesium-lithium batteries hierarchical structure cobalt-doping