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Microwave excited hyperthermy and catalysis of heterostructured Au/Cu–BTA for effective bacteria killing by accelerating charge separation

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Rare Metals 2024年第10期43卷 5186-5201页

作者： Wen-Jing Zhang li-Guo Jin Shui-lin Wu Chao-Feng Wang Yu-Feng Zheng Zhao-Yang li Zhen-Duo Cui Hui Jiang sheng-li zhu Xiang-Mei liu School of Materials Science and Engineering the Key Laboratory of Advanced Ceramics and Machining Technology by the Ministry of Education of ChinaTianjin University Biomedical Materials Engineering Research Center Hubei Key Laboratory of Polymer MaterialsMinistry-of-Education Key Laboratory for the Green Preparation and Application of Functional MaterialsSchool of Materials Science&EngineeringHubei University School of Materials Science and Engineering Peking University School of Health Science and Biomedical Engineering Hebei University of Technology

Deep tissue infections caused by pathogenic bacteria seriously threat the lives of *** this study a smart heterostructured Au/Cu-BTA （BTA=1,2,4,5-benzenetetramine） with microwave （MW） response is synthesized via NaBH4reduction of HAuCl4on the ***/Cu-BTA exhibits excellent hyperthermy and dynamics under MW *** MW thermal mechanism of Au/Cu-BTA is attributed to the excellen dielectric loss and polarization of the heterogeneous ***,the surface energy levels of the Cu-BTA interface alleviate the difficulty of electron hopping through multistage ***,MW can excite Cu-BTA to produce free ***,Au nanoparticles rapidly increase electron transfer and inhibit electron-hole ***,the yields of reactive oxygen species can be enhanced for MW dynamic therapy Consequently,under 10 min of MW irradiation,Au/Cu-BTA killed 99.998%±0.001% of Gram-positive Staphylococcus aureus,99.966%±0.014% of methicillin-resistant Staphylococcus aureus,and 96.871%±0.831% of Gram-negative Pseudomonas *** effective MW bacteria-killing strategy designed in this study shows significant potential for application in the MW-responsive treatment of deep tissue infections without antibiotics.

关键词： Anti-infection Antibacterial Microwave therapy

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Low-cost 0D and 2D carbon material co-decorated titanium dioxide ternary heterojunction for rapid and efficient bacteria killing under visible light

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cMat 2024年第2期1卷 20-29页

作者： Yuan li Peng-Feng Yuan Chao-Feng Wang Xiang-Mei liu sheng-li zhu Zhao-Yang li Zhen-Duo Cui Hui Jiang Paul KChu Shui-lin Wu Biomedical Materials Engineering Research Center Hubei Key Laboratory of Polymer MaterialsMinistry-of-Education Key Laboratory for the Green Preparation and Application of Functional MaterialsSchool of Materials Science&EngineeringHubei UniversityWuhanChina School of Materials Science&Engineering Peking UniversityBeijingChina School of Materials Science&Engineering The Key Laboratory of Advanced Ceramics and Machining Technology by the Ministry of Education of ChinaTianjin UniversityTianjinChina School of Health Science&Biomedical Engineering Hebei University of TechnologyTianjinChina Department of Physics City University of Hong KongHong KongChina Department of Materials Science and Engineering City University of Hong KongHong KongChina Department of Biomedical Engineering City University of Hong KongHong KongChina

Recently,the issue of bacterial resistance has gotten worse because of the overuse of *** newborn superbacteria,such as vancomycin-resistant bacteria,were hard to kill,inspiring researchers to find new ways to kill the bacteria ***_(2) was used as an efficient photocatalyst for water split-ting and pollutant ***,the weak efficiency limited the application to solve the drug-resistance ***,the incorpora-tion of low-cost 0D carbon quantum dots(CQDs)and 2D graphene oxide(GO)was pursued to amplify the visible light absorption capabilities of TiO_(2) and thereby elevate its photocatalytic *** forming the heterogeneous interface of CQDs and TiO_(2),CQDs converted part of visible light into wave-length less than 400 nm using the up-conversion *** modification of CQDs enabled electrons to be easily transferred from the conduction band of CQDs to the conduction band of TiO_(2).Meanwhile,GO can act as an electron acceptor,reduce the recombination efficiency of holes and electrons,and transfer the photogenerated electrons in the redox reaction in the heterogeneous *** of the excellent absorption of GO,TiO_(2)/CQDs/GO reached 57.8℃after 20 min irradiation under 1.5 times sunlight,which provided a prerequisite for photodynamic antibacterial therapy/photothermal antibacterial therapy synergistic antibacterial ***_(2)/CQDs/GO possessed an anti-bacterial efficiency as high as 99.3%toward Staphylococcus aureus which has a bright future in disinfection in vivo and medical devices as well as water sterilization.

关键词： anitbacterial carbon quantum dots graphene oxide heterojunction TiO_(2)

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Incorporating contextual evidence to improve implicit discourse relation recognition in Chinese

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Frontiers of Computer Science 2024年第3期18卷 91-104页

作者： sheng XU Peifeng li Qiaoming zhu School of Computer Science and Technology Soochow UniversitySuzhou 215000China

The discourse analysis task,which focuses on understanding the semantics of long text spans,has received increasing attention in recent *** a critical component of discourse analysis,discourse relation recognition aims to identify the rhetorical relations between adjacent discourse units(e.g.,clauses,sentences,and sentence groups),called arguments,in a *** works focused on capturing the semantic interactions between arguments to recognize their discourse relations,ignoring important textual information in the surrounding ***,in many cases,more than capturing semantic interactions from the texts of the two arguments are needed to identify their rhetorical relations,requiring mining more contextual *** this paper,we propose a method to convert the RST-style discourse trees in the training set into dependency-based trees and train a contextual evidence selector on these transformed *** this way,the selector can learn the ability to automatically pick critical textual information from the context(i.e.,as evidence)for arguments to assist in discriminating their *** we encode the arguments concatenated with corresponding evidence to obtain the enhanced argument ***,we combine original and enhanced argument representations to recognize their *** addition,we introduce auxiliary tasks to guide the training of the evidence selector to strengthen its selection *** experimental results on the Chinese CDTB dataset show that our method outperforms several state-of-the-art baselines in both micro and macro F1 scores.

关键词： discourse parsing discourse relation recognition contextual evidence selection

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Flower-like CuS/graphene oxide with photothermal and enhanced photocatalytic effect for rapid bacteria-killing using visible light

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Rare Metals 2022年第2期41卷 639-649页

作者： Rui Lv Yan-Qin liang Zhao-Yang li sheng-li zhu Zhen-Duo Cui Shui-linWu School of Materials Science&Engineering the Key Laboratory of Advanced Ceramics and Machining Technology by the Ministry of Education of ChinaTianjin UniversityTianjin 300072China The Key Laboratory of Advanced Ceramics and Machining Technology by the Ministry of Education of China Tianjin UniversityTianjin 300072China

Pathogenic bacteria have been threatening the daily life of human *** effective methods without causing drug-resistance of bacteria need to be developed to fight against these ***,flower-like CuS/-graphene oxide(GO)hybrids have been successfully synthesized via simple one-pot hydrothermal *** worked as an excellent electron acceptor to transport the photogenerated electrons from CuS,which can suppress the recombination of hole–electron pairs efficiently,thus enhancing the photocatalytic *** addition,the morphology of CuS and GO with high specific surface area and the increased defect in GO also improved photocatalytic performance of the *** to the synergy of photothermal,enhanced photocatalytic effect and released Cu ions,CuS/GO exhibited outstanding antibacterial efficacy under visible light irradiation for 15 ***,the hybrid showed great biocompatibility to L929 ***,the synthesized CuS/GO would be a promising antibacterial material for daily life including rapid water disinfection and wounds sterilization.

关键词： Antibacterial Photocatalytic CuS Graphene oxide Photoresponsive

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Preparation of hydroxyapatite layer on Ti-based bulk metallic glasses by acid and alkali pre-treatment

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Rare Metals 2015年第1期34卷 22-27页

作者： Hao Hu Zhen-Duo Cui sheng-li zhu Zhao-Yang li Yan-Qin liang Xian-Jin Yang School of Materials Science and Engineering Tianjin University Tianjin Key Laboratory of Composite and Functional Materials

In this paper, a thin calcium phosphate layer was prepared on the surface of Ti4oZr10Cu36Pd14 bulk metallic glasses （BMGs）. All samples were dipped in HNO3 aqueous solution and boiled in 1.2 mol-L-I NaOH aqueous solution. After the two preliminary treatment steps, they were soaked in simulated body fluid （SBF） to form an apatite layer on the surface. After immersion for 12 days, a coating composed mainly of Ca-P particles was rapidly deposited on the surface of Ti40Zr10Cu36Pd14 bulk metallic glasses. The surfaces of chemically treated sam- ples and the samples after immersion in SBF were char- acterized by X-ray diffraction （XRD）, X-ray photoemission spectroscopy （XPS）, field emission scanning electron microscopy （FESEM）, and energy dispersive spectroscopy （EDS）. Analysis results indicate that this apatite coating consists of Ca-P particles with different diameters. In addition, the Ca/P ratio of the apatite coatings immersed for 14 days is 1.62, which is close to that of hydroxyapatite （HA）.

关键词： Metallic glass Titanium alloy Hydroxyapatite Thin film

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Zr_(55)Al_(10)Ni_(5)Cu_(30)amorphous alloy film prepared by magnetron sputtering method

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Rare Metals 2021年第8期40卷 2237-2243页

作者： Dong-Mei Mi sheng-li zhu Yan-Qin liang Zhao-Yang li Zhen-Duo Cui Xian-Jin Yang Akihisa Inoue School of Materials Science and Engineering Tianjin UniversityTianjin300072China Tianjin Key Laboratory of Composite and Functional Materials Tianjin300072China Key Laboratory of Advanced Ceramics and Machining Technology Ministry of EducationTianjin300072China Department of Physics Kings Abudulaziz UniversityJeddah22254Saudi Arabia

In this work,amorphous Zr_(55)Al_(10)Ni_(5)Cu_(30)alloy thin film was prepared on D36 steel substrate by magnetron sputtering *** film was characterized by scanning electron microscopy(SEM),X-ray diffraction(XRD),atomic force microscopy(AFM),hardness tester and nano *** behavior of the film was investigated in 3.5%NaCl aqueous solutions by an electrochemical *** room temperature,the amorphous alloy film was formed completely after sputtering for 5 *** surface morphology of the amorphous alloy film was uniform and *** of the amorphous alloy film improved the microhardness and corrosion resistance of the D36 *** amorphous alloy film(prepared at room temperature for 5 h)exhibited good adhesion strength with the *** as-sputtered sample exhibited a crevice corrosion trend when the sputtering time was too short(1 h)or too long(10 h).

关键词： Magnetron sputtering Amorphous alloy Thin film Corrosion resistance Zr_(55)Al_(10)Ni_(5)Cu_(30)

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Microstructure and mechanical properties of TC4 joints brazed with Ti-Zr-Cu-Sn amorphous filler alloy

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Rare Metals 2021年第7期40卷 1881-1889页

作者： Hui-Hui Zhang Zhen-Duo Cui sheng-li zhu Shi-Wei Guo Xian-Jin Yang Akihisa Inoue School of Materials Science and Engineering Tianjin UniversityTianjin 30007China Key Laboratory of Advanced Ceramics and Machining Technology Ministry of EducationTianjin 300072China Tianjin Key Laboratory of Composite and Functional Materials Tianjin 300072China Department of Physics King Abdulaziz UniversityJeddah 22254Saudi Arabia

The Ti_(51.44)Zr_(16.26)Cu_(30)Sn_(2.3)(at%)amorphous filler alloy in a ribbon form was prepared by melt *** Ti-6 Al-4 V alloy was brazed in vacuum furnace by using the Ti_(51.44)Zr_(16.26)Cu_(30)Sn_(2.3)amorphous filler *** effects of brazing temperature and holding time on the interfacial microstructure and mechanical properties of the Ti-6 Al-4 V brazed joints were *** brazed joints are composed ofα-Ti,β-Ti,and(Ti,Zr)_(2)Cu *** shear strength of the joints increases with brazing temperature increasing from 1153 to 1193 K and holding time from 10 to 15 min,while decreases with brazing temperature and time further *** temperature brazing results in the formation of microcracks and voids in the seams,which are harmful for the shear strength of the *** the joint brazed at 1193 K for 15 min,a fineα+βWidmansta¨tten structure beneficial to the mechanical property is formed,and the joint exhibits relatively high joint strength of 180 MPa.

关键词： Amorphous alloy Brazing Titanium alloy Microstructure Mechanical property

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Electrodeposition of self-supported NiMo amorphous coating as an efficient and stable catalyst for hydrogen evolution reaction

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Rare Metals 2022年第8期41卷 2624-2632页

作者： Fu-Hang Yuan Mohammad-Reza Mohammadi li-li Ma Zhen-Duo Cui sheng-li zhu Zhao-Yang li Shui-lin Wu Hui Jiang Yan-Qin liang School of Materials Science and Engineering Tianjin UniversityTianjin300072China Department of Physics University of Sistan and BaluchestanZahedan98167-45845Iran

NiMo-based materials have been identified as potential candidates of Pt/C electrocatalysts for hydrogen evolution reaction(HER)due to appropriate binding energy to hydrogen,and good resistance to corrosive ***,little work has been carried out to enhance the catalytic performance in large-scale water-alkali *** NoMo amorphous coating,as a highefficient and cost-effective catalyst toward HER,was synthesized by a facile electrodeposition strategy in this *** effects of the pH value of electrolyte on the structure and HER activity of NiMo coating were *** as-prepared NiMo_((pH10))exhibited the highest HER activity with overpotentials of 63.9 and 157.1 mV(***,with 80%potential drop due to electrical resistance(iR)compensation)at the current density of-10 mA·cm^(-2)and-100 mA·cm^(-2).This NiMo_((pH10))coating also had excellent long-term durability of up to100 h stable operation under the constant current density of-100 mA·cm^(-2).The rapid HER kinetics and outstanding endurance can be ascribed to the NiMo compact coating with amorphous structures as well as good contact between NiMo coating and Ni foam substrate,endowing it grand feasibility in practical industrial applications.

关键词： Electrodeposition NiMo coating Hydrogen evolution reaction(HER) Alkaline water electrolysis

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Solvent-free carbon sphere nanofluids towards intelligent lubrication regulation

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Friction 2024年第1期12卷 95-109页

作者： sheng ZHANG Wen li Xiaoliang MA Xiaoqiang FAN Minhao zhu Tribology Research Institute School of Mechanical EngineeringSouthwest Jiaotong UniversityChengdu 610031China Key Laboratory of Advanced Technologies of Materials Ministry of EducationSchool of Materials Science and EngineeringSouthwest Jiaotong UniversityChengdu 610031China

By simply switching the electrical circuit installed on steel/steel contact,the tribological behaviors of nanofluids(NFs)can be regulated in real time,thereby achieving the desired performance of friction reduction and wear ***,solvent-free carbon spherical nanofluids(C-NFs)were successfully prepared for intelligent lubrication regulation.C-NFs with excellent lubrication performance can immediately reduce the coefficient of friction(COF)despite applying a weak electric potential(1.5 V).Moreover,polyethylene glycol 400(PEG400)containing 5.0 wt%C-NFs remained responsive to electrical stimulation under the intermittent voltage application with an average coefficient of friction(ACOF)reduction of 20.8%over *** intelligent lubrication regulation of C-NFs under an external electric field(EEF)mainly depends on the orderly arranged double-electric adsorption film of ion canopy-adsorbed carbon spheres(CSs).The intermittent electrical application can continuously reinforce the adsorption film and its durability for real-time controlling the sliding ***-stimulation-responsive intelligent lubricants provide a new technical support for realizing intelligent stepless control of devices.

关键词： solvent-free carbon spherical nanofluids(C-NFs) intelligent lubrication regulation lubrication performance adsorption film

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Highly efficient nanoporous CoBP electrocatalyst for hydrogen evolution reaction

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Rare Metals 2021年第5期40卷 1031-1039页

作者： Hui-Lan Guang sheng-li zhu Yan-Qin liang Shui-lin Wu Zhao-Yang li Shui-Yuan Luo Zhen-Duo Cui Akihisa Inoue School of Materials Science and Engineering Tianjin UniversityTianjin 300350China School of Materials Science and Engineering Lanzhou Jiaotong UniversityLanzhou 730070China College of Chemistry Engineering and Materials Science Quanzhou Normal UniversityQuanzhou 362000China International Institute of Green Materials Josai International UniversityTogane 283-8555Japan Department of Physics King Abdulaziz UniversityJeddah 22254Saudi Arabia

Water splitting is an environment friendly and efficient way to produce *** efficient and low-cost non-noble metal catalysts play an important role in hydrogen evolution reaction(HER).Dealloying is a simple method to prepare three-dimensional self-supporting nanoporous materials without conductive supports and *** this work,we prepared self-supporting nanoporous CoBP electrocatalyst by dealloying *** influence of the synergistic effect of nonmetallic elements on catalytic activity was *** synergistic electronic effect of Co,B and P atoms on the surface optimizes the H atoms desorption and results in superior HER *** bi-continuous structure of nanoporous CoBP provides more active area and favors of electron and electrolyte *** nanoporous CoBP with the B/P atomic ratio of 1/3 exhibits low overpotential of 42 mV at 10 mA·cm^(-2),small Tafel slope of 39.8 mV·dec-1 and good long-term stability with no performance decrease for 20 h in alkaline solution.

关键词： Hydrogen evolution reaction Nanoporous Self-supporting electrocatalyst Co-B-P alloy Dealloying

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