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Electrophoretic deposition of a supercapacitor electrode of activated carbon onto an indium-tin-oxide substrate using ethyl cellulose as a binder

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Journal of Materials Science & Technology 2020年第23期58卷 188-196页

作者： Taeuk Kim Seong-Hoon Yi sang-eun chun School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea

A transparent energy storage device is an essential component for transparent *** increasing demand for high-power devices stimulates the development of transparent supercapacitors with high power density.A transparent electrode for such supercapacitors can be assembled via the electrophoretic deposition of an active material powder with a binder onto a transparent *** properties of the binder critically influence the electrochemical behavior and performance of the resulting *** cellulose(EC)is known as an eco-friendly,transparent,flexible,and inexpensive ***,we fabricated an electrode film with EC binder via electrophoretic deposition on an indium tin oxide(ITO)substrate instead of using the conventional polytetrafluoroethylene(PTFE)*** assembled electrodes with EC and PTFE were compared to investigate the feasibility of EC as a binder from different perspectives,including homogeneity,wettability,electrochemical behavior,and mechanical *** EC enabled the formation of a homogeneous film composed of smaller particles and with a higher specific capacitance compared with films prepared with *** annealing improved the adhesion strength of the EC because of its glass transition;however,its hydrophobic nature limited utilization of the active material for charge *** electrochemical activation improved the wettability of the electrode,resulting in an increased capacitance of 60 F g^(-1).Furthermore,even with the lower wettability of EC compared with that of PTFE,better rate performance was possible with the EC *** increased mechanical stability after the annealing process ensured an excellent cycle life of 95%capacitance retention for 15,000 cycles.

关键词： Electrophoretic deposition Transparent electrode Activated carbon Ethyl cellulose Indium tin oxide

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Enhanced stability and rate performance of zinc-doped cobalt hexacyanoferrate (CoZnHCF) by the limited crystal growth and reduced distortion

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Journal of Energy Chemistry 2022年第6期31卷 649-658,I0018页

作者： Jihwan Kim Seong-Hoon Yi Li Li sang-eun chun School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea State Key Laboratory of Rolling and Automation Northeastern UniversityShenyang 110819LiaoningChina School of Metallurgy Northeastern UniversityShenyang 110819LiaoningChina School of Industrial Technology Advances Kyungpook National UniversityDaegu 41566Republic of Korea

Cobalt hexacyanoferrate (CoHCF) is a potential cathode for aqueous Na-ion batteries due to its high theoretical specific capacity (170 m Ah g^(-1));however,its lower rate capability and cyclability limit its *** distortion at a weak N-coordinated crystal field during cycling disintegrates Co,yielding an irreversible *** Zn amounts ranging 0–1 were added to the Co site to suppress the structural irreversibility of CoHCF,yielding Co_(1-x)Zn_(x)HCF powder;this Zn (x≤0.09) addition reduced the powder’s dimension because the lower four coordination of Zn–N,not the six coordination of Co–N,limits the powder ***,a small lattice parameter and interaxial angle (~90°) are obtained,implying that a narrower Co_(1-x)Zn_(x)HCF inner structure is formed to accommodate Na ***,the electronic conductivity of Co_(1-x)Zn_(x)HCF gradually increased within 0–0.09 range.A smaller particle size with a high surface area leads to a near-surface-limited redox process,similar to a capacitive *** the surface-limited reaction and electronic conductivity enhances the reversibility due to the smaller charge transfer resistance at the electrode/electrolyte interface caused by Zn *** redox-active Co with non-active Zn amount of 0.07 (Co_(1-x)Zn_(x)HCF) slightly reduces the specific capacity from 127 to 119 mAh g^(-1)at 0.1 A g^(-1)due to the shrunken Co charging *** performance is enhanced by compromising the capacity and reduced distortion,resulting in 81%retention at a 20-times-faster charging ***,the Co_(1-x)Zn_(x)HCF sample exhibited the good stability while preserving 74%of the initial capacity at 0.5 A g^(-1)after 200 cycles.

关键词： Cobalt hexacyanoferrate Rate capability Stability Growth limitation Structural distortion Near-surface-limited redox process

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Synthesis of crystalline g-C_(3)N_(4) with rock/molten salts for efficient photocatalysis and piezocatalysis

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Green Energy & Environment 2024年第5期9卷 890-898页

作者： Tingting Xu Jung Hur Ping Niu Shulan Wang sangwook Lee sang-eun chun Li Li Department of Chemistry College of ScienceNortheastern UniversityShenyang110819China State Key Laboratory of Rolling and Automation Northeastern UniversityShenyang110819China School of Metallurgy Northeastern UniversityShenyang110819China School of Materials Science and Engineering Kyungpook National UniversityDaegu41566Republic of Korea School of Industrial Technology Advances Kyungpook National UniversityDaegu41566Republic of Korea

Graphitic carbon nitride(g-C_(3)N_(4))is emerging as a promising visible-light photocatalyst while the low crystallinity with sluggish charge separation/migration dynamics signiﬁcantly restricts its practical ***,synthesizing highly crystalline g-C_(3)N_(4) with sufﬁcient surface activities still remains ***,different from using alkali molten salts which is commonly reported,we propose an approach for synthesis of highly crystalline g-C_(3)N_(4) with FeCl3/KCl rock/molten mixed *** rock salt can serve as the structure-directing template while molten salt provides the required liquid medium for ***,the synthesized photocatalyst showed further enhanced crystallinity and improved surface area along with high p/p*excitation compared with crystalline C_(3)N_(4) prepared from conventional molten-salt *** catalytically advantageous features lead to its superior photocatalytic and piezocatalytic activities with a high reactivity for overall water splitting that is not commonly reported for C_(3)N_(4).This work provides an effective strategy for structural optimization of organic semiconductor based materials and may inspire new ideas for the design of advanced photocatalysts.

关键词： High crystallinity Carbon nitride Photocatalysis Piezocatalysis Overall water splitting

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Enhanced thermoelectric composite performance from mesoporous carbon additives in a commercial Bi_(0.5)Sb_(1.5)Te_(3) matrix

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Journal of Materials Science & Technology 2021年第35期94卷 175-182页

作者： Seong-Tae Kim Jong Min Park Kwi-Il Park sang-eun chun Ho Seong Lee Pyuck-Pa Choi Seonghoon Yi School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea Department of Materials Science and Engineering Korea Advanced Institute of Science and Technology(KAIST)291 Daehak-roYuseong-guDaejeon 34141Republic of Korea

Composites were prepared,through hot pressing,using carbon materials with different pore size distributions as additives for commercial Bi_(0.5)Sb_(1.5)Te_(3) thermoelectric material(BST,p-type).Thermoelectric properties of the composites were measured in a temperature range of 298-473 *** conductivity of the composites,especially lattice thermal conductivity,was effectively decreased due to the mesoporous properties of the incorporated carbon *** electrical conductivity of the composites slightly decreased due to the electron scattering at the interface between the carbon material and the commercial BST *** composite with 0.2 vol.%mesoporous carbon powder(36%mesoporosity)exhibited a figure of merit value approximately 10.7%higher than that of commercial BST without *** behavior resulted in 116%improved output power in the composite block-based single element compared with a bare BST thermoelectric *** enhanced figure of merit was attributed to the effective reduction of lattice thermal conductivity by acoustic phonons scattering at the interface between the BST matrix and the mesoporous carbon as well as at the pore surfaces within the mesoporous *** utilizing mesoporous carbon materials used in this study,the shortcomings and economic difficulties of the composite process with low dimensional carbon additives(carbon nanotubes,graphene,and nanodiamond)can be overcome for extensive practical *** carbon powder with a tailored porosity distribution revealed the validity of bulk-type carbon additives to enhance the figure of merit of commercial thermoelectric materials.

关键词： Thermoelectric material Bi_(0.5)Sb_(1.5)Te_(3) Mesoporous carbon Lattice thermal conductivity Figure of merit

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Transfer RNA-derived small RNA serves as potential non-invasive diagnostic marker and a novel therapeutic target for acute pancreatitis

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World Journal of Gastroenterology 2025年第1期31卷 152-156页

作者： Jing Zhang chun-Lin Ou Department of Immunology School of Basic MedicineCentral South UniversityChangsha 410000Hunan ProvinceChina Department of Pathology Xiangya HospitalCentral South UniversityChangsha 410008Hunan ProvinceChina

Transfer RNA(tRNA)-derived fragments,a new type of tRNA-derived small RNA(tsRNA),can be cleaved from tRNA by enzymes to regulate target gene expression at the transcriptional and translational *** are not only degradation fragments but also have biological functions,including those in immune inflammation,metabolic disorders,and cell *** dysregulation is closely associated with multiple diseases,including various cancers and acute pancreatitis(AP).AP is a common gastrointestinal disease,and its incidence increases *** development is associated with tsRNAs,which regulate cell injury and induce inflammation,especially pyroptosis and ***,serum tRF36 has the potential to serve as a non-invasive diagnostic biomarker and leads to pancreatic acinar cell ferroptosis causing inflammation to promote *** show the characteristics of tsRNAs and their diagnostic value and function in AP,and discuss the potential opportunities and challenges of using tsRNAs in clinical applications and research.

关键词： Transfer RNA derived small RNAs Acute pancreatitis Liquid biopsy Biomarker Cell pyroptosis Ferroptosis

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Analysis of the current density characteristics in through-mask electrochemical micromachining(TMEMM) for fabrication of micro-hole arrays on invar alloy film

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Chinese Journal of Aeronautics 2017年第3期30卷 1231-1241页

作者： Da-som JIN Kwang-ho chun eun-sang LEE School of Mechanical Engineering Inha University Incheon 22212 Republic of Kore Department of Mechanical Engineering Inha University Incheon 22212 Republic of Korea

Invar alloy consisting of 64% iron and 36% nickel has been widely used for the production of shadow masks for organic light emitting diodes（OLEDs） because of its low thermal expansion coefficient（1.86 × 10^-6cm/°C）.To fabricate micro-hole arrays on 30 lm invar alloy film,through-mask electrochemical micromachining（TMEMM） was developed and combined with a portion of the photolithography etching *** precise hole shapes,patterned photoresist（PR） film was applied as an insulating *** investigate the relationship between the current density and the material removal rate,the principle of the electrochemical machining was studied with a focus on the *** finite element method（FEM） was used to verify the influence of each parameter on the current density on the invar alloy film *** parameters considered were the thickness of the PR mask,inter-electrode gap（IEG）,and electrolyte *** of experiments（DOE） was used to figure out the contribution of each parameter.A simulation was conducted with varying parameters to figure out their relationships with the current *** was conducted to select the suitable *** experiment was carried out to verify the simulation *** was possible to fabricate micro-hole arrays on invar alloy film using TMEMM,which is a promising method that can be applied to fabrications of OLEDs shadow masks.

关键词： Electrochemical Invar alloy film Micromachining OLED shadow mask Photoresist film mask(PR film mask) Through-mask electrochemical micromachining(TMEMM)

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Fanlian Huazhuo formula:A promising therapeutic approach for metabolic associated steatotic liver disease

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World Journal of Gastroenterology 2025年第1期31卷 167-171页

作者： chun-Han Cheng Wen-Rui Hao Tzu-Hurng Cheng Department of Medical Education Linkou Chang Gung Memorial HospitalTaoyuan 33305Taiwan Division of Cardiology Department of Internal MedicineShuang Ho HospitalMinistry of Health and WelfareTaipei Medical UniversityNew Taipei 23561Taiwan Division of Cardiology Department of Internal MedicineSchool of MedicineCollege of MedicineTaipei Medical UniversityTaipei 11002Taiwan Department of Biochemistry School of MedicineCollege of MedicineChina Medical UniversityTaichung 404328Taiwan

This article reviews the study,“Fanlian huazhuo formula alleviates high-fat-dietinduced nonalcoholic fatty liver disease by modulating autophagy and lipid synthesis signaling pathway”published in the World Journal of *** study explores the therapeutic potential of Fanlian Huazhuo formula(FLHZF)in treating metabolic-associated steatotic liver disease(MASLD),demonstrating that FLHZF reduces lipid accumulation,oxidative stress,and liver injury in MASLD models by modulating key signaling pathways involved in lipid metabolism and *** editorial emphasizes the potential of FLHZF as a treatment for MASLD and calls for further research to verify its clinical efficacy.

关键词： Fanlian Huazhuo formula Metabolic associated steatotic liver disease Autophagy Lipid metabolism Oxidative stress

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Surface embedded binary Co-Cu hydroxy phosphate over surface of oxy/hydroxides for efficient nitrate reduction to ammonia

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Nano Research 2025年第1期18卷 195-207页

作者： chun Zhu Yifei Yang Yike Jing Zhen Zeng Xuesong Yi Wei Sun Fei Yang Key Laboratory of Agro-Forestry Environmental Processes and Ecological Regulation of Hainan Province School of Environmental Science and EngineeringHainan UniversityHaikou 570228China

Electrochemical nitrate reduction reaction(NO3RR)to ammonia is a promising approach to address excess Ncontamination in aqueous environment but suffers from a limited ammonia yield and selectivity due to the low concentration and sluggish *** work reports a three-dimensional porous electrode with binary Co_(2)Cu_(1)hydroxy phosphate embedded into the surface of Ni_(3)Co_(1)oxy/hydroxides(CoCu-PH@NiCo/Ni,“PH”means phosphate-hydroxide),which delivers a yield of 4.13 mg·h^(-1)·cm^(-2)with a high Faraday efficiency of 92.6%under a low nitrate concentration of 40 mM and provide an impressive *** embedded structure of the as-prepared catalyst exhibits unique metal coordination ligands and valence states different from the unitary *** electrochemical in situ infrared spectra and theoretical calculations revealed that the Co sites with the ability to dissociate water molecular to form adsorbed OH*can effectively provide the required protons for the deoxygenation and hydrogenation steps during NO3-conversion,thereby,effectively reducing the energy barrier of the key transition states in the NO3RR process to improve the intrinsic *** demonstrate that the rational design of binary components with the appropriate ability to activate water molecules as well as the threedimensional porous skeletal structure are expected to promote effectively the low-concentration nitrates conversion to ammonia.

关键词： nitrate reduction hydroxy phosphate surface embedded water dissociation active hydroxy adsorbed

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CHEBYSHEV WEIGHTED NORM LEAST-SQUARES SPECTRAL METHODS FOR THE ELLIPTIC PROBLEM

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Journal of Computational Mathematics 2006年第4期24卷 451-462页

作者： sang Dong Kim Byeong chun Shin Department of Mathematics Kyungpook National University Taegu 702-701 Korea Department of Mathematics Chonnam National University Kwangju 500-757 Korea

We develop and analyze a first-order system least-squares spectral method for the second-order elhptic boundary value problem with variable coefficients. We first analyze the Chebyshev weighted norm least-squares functional defined by the sum of the Lw^2- and Hw^-1- norm of the residual equations and then we eplace the negative norm by the discrete negative norm and analyze the discrete Chebyshev weighted least-squares method. The spectral convergence is derived for the proposed method. We also present various numerical experiments. The Legendre weighted least-squares method can be easily developed by following this paper.

关键词： Least-squares methods Spectral method Negative norm.

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EXPLICIT BOUNDS OF EIGENVALUES FOR STIFFNESS MATRICES BY QUADRATIC HIERARCHICAL BASIS METHOD)

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Journal of Computational Mathematics 2003年第2期21卷 113-124页

作者： sang Dong KIM Byeong chun SHIN Department of Mathematics Kyungpook National UniversityTaegu 702-701KoreaDepartment of MathematicsChonnam National UniversityGwangju 500-757Korea

The bounds for the eigenvalues of the stiffness matrices in the finite element discretization corresponding to Lu := - u' with zero boundary conditions by quadratic hierarchical basis are shown explicitly. The condition number of the resulting system behaves like O(1/h) where h is the mesh size. We also analyze a main diagonal preconditioner of the stiffness matrix which reduces the condition number of the preconditioned system to O(1).

关键词： hierarchical basis multilevel

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