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High Na-ion conductivity andmechanical integrity of anion-exchanged polymeric hydrogel electrolytes for flexible sodium ion hybrid energy storage

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SusMat 2024年第1期4卷 140-153页

作者： JungWoo Hong Harpalsinh H.Rana Jeong Hee Park Jun Su Kim sang joon lee Gun Jang Tae Hoon Kang Kang Ho Shin sang Ha Baek Wooseok Yang Kwang Ho Kim Ju-Hyuk lee Ho Seok Park School of Chemical Engineering Sungkyunkwan UniversitySuwonRepublic of Korea Clean Energy Research Center Korea Institute of Science and Technology(KIST)SeoulRepublic of Korea KIST-SKKU Carbon-Neutral Research Center Sungkyunkwan University(SKKU)SuwonRepublic of Korea SKKU Institute of Energy Science and Technology(SIEST) Sungkyunkwan UniversitySuwonRepublic of Korea COSMOS LAB/92 Jomaru-ro 385beon-gilBucheon-siRepublic of Korea SKKU Advanced Institute of Nano Technology(SAINT) Sungkyunkwan UniversitySuwonRepublic of Korea Department of Health Sciences and Technology Samsung Advanced Institute for Health Sciences and Technology(SAIHST)Sungkyunkwan UniversitySuwonRepublic of Korea

The polymeric gel electrolytes are attractive owing to their higher ionic conductivities than those of dry polymer electrolytes and lowered water activity for enlarged potential window.However,the ionic conductivity and mechanical strength of the Na-ion conducting polymeric gel electrolytes are limited by below 20 mS cm−1 and 2.2 MPa.Herein,we demonstrate Na-ion conducting and flexible polymeric hydrogel electrolytes of the chemically coupled poly(diallyldimethylammonium chloride)-dextrin-N,N′-methylene-bisacrylamide film immersed in NaClO_(4) solution(ex-DDA-Dex+NaClO_(4))for flexible sodium-ion hybrid capacitors(f-NIHC).In particular,the anion exchange reaction and synergistic interaction of ex-DDA-Dex with the optimum ClO_(4)−enable to greatly improve the ionic conductivity up to 27.63 mS cm−1 at 25◦C and electrochemical stability window up to 2.6 V,whereas the double networking structure leads to achieve both the mechanical strength(7.48 MPa)and softness of hydrogel electrolytes.Therefore,the f-NIHCs with the ex-DDA-Dex+NaClO_(4) achieved high specific and high-rate capacities of 192.04 F g^(−1)at 500 mA g^(−1)and 116.06 F g^(−1)at 10000 mA g^(−1),respectively,delivering a large energy density of 120.03Wh kg^(−1)at 906Wkg^(−1)and long cyclability of 70%over 500 cycles as well as demonstrating functional operation under mechanical stresses.

关键词： anion exchange chemistry flexible energy storage hybrid energy storage hydrogel electrolytes renewable electrolytes sodium storage

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Thermoresponsive Al^(3+)-crosslinked poly(N-isopropylacrylamide)/alginate composite for green recovery of lithium from Li-spiked seawater

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Green Energy & Environment 2022年第2期7卷 334-344页

作者： Sung Ho Park sang joon lee Department of Mechanical Engineering Pohang University of Science and Technology(POSTECH)Pohang790-784South Korea

With the rapid increase in the demand for lithium as an energy-critical element,the recovery of Li+ions from seawater is a worldwide challenging issue.Herein,we propose a new facile and fast selective recovery approach of Li+using an Al^(3+)-crosslinked poly(N-isopropylacrylamide)(PNIPAAm)/alginate(Alg)(PNP/Alg(Al)) adsorbent.The in situ TEM images indicate that Alg-Al^(3+)coordination is reorganized via the rearrangement of PNIPAAm and Alg networks,as the temperature increases.The reorganization eventually leads to the formation of polycrystalline structure.The in situ FTIR results exhibit that PNP/Alg(Al) composite has peculiar phase transitions,which includes a retrogressive phase change from hydrophobic to hydrophilic.The synergetic effect of the strong repulsion force of Al^(3+) ions and the attractive force of negatively charged polymeric chains enables the efficient adsorption of Li+ions with a low affinity from Li-spiked seawater.7.3% of Li+ions are recovered from Li-spiked seawater although the concentration of Li-spiked seawater is very high.In addition,Li+ions can be extracted from PNP/Alg(Al) composite with the use of a small thermal energy.The proposed thermoresponsive IPN gel provides a strong potential in practical applications for Li+recovery as an innovative energy-material strategy.

关键词： structure seawater lithium

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Callus proliferation-induced hypoxic microenvironment decreases shoot regeneration competence in Arabidopsis

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Molecular Plant 2024年第3期17卷 395-408页

作者： Dohee Koo Hong Gil lee Soon Hyung Bae Kyounghee lee Pil joon Seo Department of Chemistry Seoul National UniversitySeoul 08826Korea Plant Genomics and Breeding Institute Seoul National UniversitySeoul 08826Korea Research Institute of Basic Sciences Seoul National UniversitySeoul 08826Korea

Plants are aerobic organisms that rely on molecular oxygen for respiratory energy production.Hypoxic conditions,with oxygen levels ranging between 1%and 5%,usually limit aerobic respiration and affect plant growth and development.Here,we demonstrate that the hypoxic microenvironment induced by active cell proliferation during the two-step plant regeneration process intrinsically represses the regener-ation competence of the callus in Arabidopsis thaliana.We showed that hypoxia-repressed plant regener-ation is mediated by the RELATED TO APETALA2.12(RAP2.12)protein,a memberof the Ethylene Response Factor VIl(ERF-Vll)family.We found that the hypoxia-activated RAP2.12 protein promotes salicylic acid(SA)biosynthesis and defense responses,thereby inhibiting pluripotency acquisition and de novo shoot regeneration in calli.Molecular and genetic analyses revealed that RAP2.12 could bind directly to the SALICYLIC ACID INDUCTION DEFICIENT 2(SID2)gene promoter and activate SA biosynthesis,repressing plant regeneration possibly via a PLETHORA(PLT)-dependent pathway.Consistently,the rap2.12 mutant calli exhibits enhanced shoot regeneration,which is impaired by SA treatment.Taken together,these find-ings uncover that the cell proliferation-dependent hypoxic microenvironment reduces cellular pluripotency and plant regeneration through the RAP2.12-SID2 module.

关键词： callus cell proliferation-induced hypoxia SID2 plant regeneration salicylic acid RAP2.12

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Prediction of NFT Sale Price Fluctuations on OpenSea Using Machine Learning Approaches

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Computers, Materials & Continua 2023年第5期75卷 2443-2459页

作者： Zixiong Wang Qiuying Chen sang-joon lee Interdisciplinary Program of Digital Future Convergence Service Chonnam National UniversityGwangju61186Korea

The rapid expansion of the non-fungible token(NFT)market has attracted many investors.However,studies on the NFT price fluctuations have been relatively limited.To date,the machine learning approach has not been used to demonstrate a specific error in NFT sale price fluctuation prediction.The aim of this study was to develop a prediction model for NFT price fluctuations using the NFT trading information obtained from OpenSea,the world’s largest NFT marketplace.We used Python programs to collect data and summarized them as:NFT information,collection information,and related account information.AdaBoost and Random Forest(RF)algorithms were employed to predict the sale price and price fluctuation of NFTs using regression and classification models,respectively.We found that the NFT related account information,especially the number of favorites and activity status of creators,confer a good predictive power to both the models.AdaBoost in the regression model had more accurate predictions,the root mean square error(RMSE)in predicting NFT sale price was 0.047.In predicting NFT sale price fluctuations,RF performed better,which the area under the curve(AUC)reached 0.956.We suggest that investors should pay more attention to the information of NFT creators.We anticipate that these prediction models will reduce the number of investment failures for the investors.

关键词： NFT sale price fluctuation OpenSea AdaBoost Random forest

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Tailoring local structures of atomically dispersed copper sites for highly selective CO2 electroreduction

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Carbon Energy 2024年第4期6卷 79-90页

作者： Kyung‐Jong Noh Byoung joon Park Ying Wang Yejung Choi sang‐Hoon You Yong‐Tae Kim Kug‐Seung lee Jeong Woo Han Department of Chemical Engineering Pohang University of Science and Technology(POSTECH)PohangGyeongbukRepublic of Korea Department of Materials Science and Engineering Pohang University of Science and Technology(POSTECH)PohangGyeongbukRepublic of Korea Pohang Accelerator Laboratory(PAL) Beamline DivisionPohangGyeongbukRepublic of Korea

Atomically‐dispersed copper sites coordinated with nitrogen‐doped carbon(Cu–N–C)can provide novel possibilities to enable highly selective and active electrochemical CO_(2) reduction reactions.However,the construction of optimal local electronic structures for nitrogen‐coordinated Cu sites(Cu–N_(4))on carbon remains challenging.Here,we synthesized the Cu–N–C catalysts with atomically‐dispersed edge‐hosted Cu–N_(4) sites(Cu–N_(4)C_(8))located in a micropore between two graphitic sheets via a facile method to control the concentration of metal precursor.Edge‐hosted Cu–N_(4)C_(8) catalysts outperformed the previously reported M–N–C catalysts for CO_(2)‐to‐CO conversion,achieving a maximum CO Faradaic efficiency(FECO)of 96%,a CO current density of–8.97 mA cm–2 at–0.8 V versus reversible hydrogen electrode(RHE),and over FECO of 90%from–0.6 to–1.0 V versus RHE.Computational studies revealed that the micropore of the graphitic layer in edge‐hosted Cu–N_(4)C_(8) sites causes the d‐orbital energy level of the Cu atom to shift upward,which in return decreases the occupancy of antibonding states in the*COOH binding.This research suggests new insights into tailoring the locally coordinated structure of the electrocatalyst at the atomic scale to achieve highly selective electrocatalytic reactions.

关键词： atomic local structure density functional theory electrochemical CO_(2)reduction metal nitrogen‐doped carbon single‐atom catalyst

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Delayed-onset endophthalmitis associated with Achromobacter species developed in acute form several months after cataract surgery:Three case reports

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World Journal of Clinical Cases 2022年第19期10卷 6496-6500页

作者： Tae-Hoon Kim sang-joon lee Ki-Yup Nam Department of Ophthalmology Kosin University HospitalBusan 49267South Korea Department of Ophthalmology Kosin UniversityCollege of MedicineBusan 49267South Korea Department of Ophthalmology Chungnam National UniveristyCollege of MedicineDaejeon 35015South Korea Department of Ophthalmology Chungnam National University Sejong HospitalSejong 30099South Korea

BACKGROUND Achromobacter species-associated endophthalmitis is rare and may present as either acute or chronic postoperative endophthalmitis.Delayed-onset Achromobacter species endophthalmitis appearing in acute presentation that develops more than several months after cataract surgery is very rare.Intraocular lens(IOL)removal is commonly recommended to treat Achromobacter species endophthalmitis,which is based on previous studies.Here,we report the results of surgery without IOL removal when treating patients with delayed-onset postoperative Achromobacter species endophthalmitis that developed in an acute form.CASE SUMMARY Three patients visited our ophthalmology clinic due to visual impairment that began 2-3 d earlier.They had undergone cataract surgery 5-18 mo prior.Bestcorrected visual acuity of the diseased eye was between counting fingers at 30 cm to non-light perception.They showed conjunctival injection,inflammation in the anterior chamber(cell reaction 4+)and hypopyon formation.The patients were diagnosed with infectious endophthalmitis and immediately underwent pars plana vitrectomy,anterior chamber irrigation and intravitreal injection of ceftazidime and vancomycin.Before fluid infusion,a vitreous specimen was obtained. In all cases, the IOLs were not removed. Achromobacter species was detected on vitreousspecimen culture. After surgery, the vitreous opacity decreased gradually and there was littleretinal damage. At 1 mo after treatment, the best-corrected visual acuity had improved to 20/50and 20/40.CONCLUSIONDelayed onset postoperative endophthalmitis caused by Achromobacter species can appear in anacute form. All patients responded well to early vitrectomy and administration of empiricalantibiotics including ceftazidime. There was no need for IOL removal during surgery.

关键词： Achromobacter species Chronic endophthalmitis Postoperative endophthalmitis Case report

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View Types and Visual Communication Cues for Remote Collaboration

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Computers, Materials & Continua 2023年第2期74卷 4363-4379页

作者： Seungwon Kim Weidong Huang Chi-Min Oh Gun lee Mark Billinghurst sang-joon lee AI Convergence College Chonnam National UniversityGwangju61186Korea University of Technology Sydney Sydney2007Australia SafeMotion Gwangju61011Korea School of ITMS University of South AustraliaAdelaide5001Australia Interdisciplinary Program of Digital Future Convergence Service Chonnam National UniversityGwangju61186Korea

Over the last several years,remote collaboration has been getting more attention in the research community because of the COVID-19 pandemic.In previous studies,researchers have investigated the effect of adding visual communication cues or shared views in collaboration,but there has not been any previous study exploring the influence between them.In this paper,we investigate the influence of view types on the use of visual communication cues.We compared the use of the three visual cues(hand gesture,a pointer with hand gesture,and sketches with hand gesture)across two view types(dependent and independent views),respectively.We conducted a user study,and the results showed that hand gesture and sketches with the hand gesture cueswerewell matchedwith the dependent viewcondition,and using a pointer with the hand gesture cue was suited to the independent view condition.With the dependent view,the hand gesture and sketch cues required less mental effort for collaborative communication,had better usability,provided better message understanding,and increased feeling of co-presence compared to the independent view.Since the dependent view supported the same viewpoint between the remote expert and a local worker,the local worker could easily understand the remote expert’s hand gestures.In contrast,in the independent view case,when they had different viewpoints,it was not easy for the local worker to understand the remote expert’s hand gestures.The sketch cue had a benefit of showing the final position and orientation of the manipulating objects with the dependent view,but this benefit was less obvious in the independent view case(which provided a further view compared to the dependent view)because precise drawing in the sketches was difficult from a distance.On the contrary,a pointer with the hand gesture cue required less mental effort to collaborate,had better usability,provided better message understanding,and an increased feeling of co-presence in the independent view condition than in the dependent view condition.The

关键词： Mixed reality remote collaboration

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GRU-based Buzzer Ensemble for Abnormal Detection in Industrial Control Systems

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Computers, Materials & Continua 2023年第1期74卷 1749-1763页

作者： Hyo-Seok Kim Chang-Gyoon Lim sang-joon lee Yong-Min Kim Interdisciplinary Program of Information Security Chonnam National UniversityGwangju61186Korea Major in Computer Engineering Chonnam National UniversityYeosu59626Korea School of Business Administration Chonnam National UniversityGwangju61186Korea Department of Electronic Commerce Chonnam National UniversityYeosu59626Korea

Recently,Industrial Control Systems(ICSs)have been changing from a closed environment to an open environment because of the expansion of digital transformation,smart factories,and Industrial Internet of Things(IIoT).Since security accidents that occur in ICSs can cause national confusion and human casualties,research on detecting abnormalities by using normal operation data learning is being actively conducted.The single technique proposed by existing studies does not detect abnormalities well or provide satisfactory results.In this paper,we propose a GRU-based Buzzer Ensemble for AbnormalDetection(GBE-AD)model for detecting anomalies in industrial control systems to ensure rapid response and process availability.The newly proposed ensemble model of the buzzer method resolves False Negatives(FNs)by complementing the limited range that can be detected in a single model because of the internal models composing GBE-AD.Because the internal models remain suppressed for False Positives(FPs),GBE-AD provides better generalization.In addition,we generated mean prediction error data in GBE-AD and inferred abnormal processes using soft and hard clustering.We confirmed that the detection model’s Time-series Aware Precision(TaP)suppressed FPs at 97.67%.The final performance was 94.04%in an experiment using anHIL-basedAugmented ICS(HAI)Security Dataset(ver.21.03)among public datasets.

关键词： Industrial control system abnormal detection ensemble learning HAI dataset

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Vertical plane depth-resolved surface potential and carrier separation characteristics in flexible CZTSSe solar cells with over 12% efficiency

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Carbon Energy 2024年第3期6卷 36-52页

作者： Dae-Ho Son Ha Kyung Park Dae-Hwan Kim Jin-Kyu Kang Shi-joon Sung Dae-Kue Hwang Jaebaek lee Dong-Hwan Jeon Yunae Cho William Jo Taeseon lee JunHo Kim sang-Hoon Nam Kee-Jeong Yang Division of Energy Technology DGISTDaeguRepublic of Korea Research Center for Thin Film Solar Cells DGISTDaeguRepublic of Korea Department of Physics Ewha Womans UniversitySeoulRepublic of Korea Department of Physics Incheon National UniversityIncheonRepublic of Korea Department of Mechanical Engineering Massachusetts Institute of TechnologyCambridgeMassachusettsUSA

Cu2ZnSn(S,Se)4(CZTSSe)solar cells have resource distribution and economic advantages.The main cause of their low efficiency is carrier loss resulting from recombination of photo-generated electron and hole.To overcome this,it is important to understand their electron-hole behavior characteristics.To determine the carrier separation characteristics,we measured the surface potential and the local current in terms of the absorber depth.The elemental variation in the intragrains(IGs)and at the grain boundaries(GBs)caused a band edge shift and bandgap(Eg)change.At the absorber surface and subsurface,an upward Ec and Ev band bending structure was observed at the GBs,and the carrier separation was improved.At the absorber center,both upward Ec and Ev and downward Ec-upward Ev band bending structures were observed at the GBs,and the carrier separation was degraded.To improve the carrier separation and suppress carrier recombination,an upward Ec and Ev band bending structure at the GBs is desirable.

关键词： carrier separation CZTSSe flexible solar cell local current surface potential

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Two distinct subpopulations of marginal zone B cells exhibit differential antibody-producing capacities and radioresistance

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Cellular & Molecular Immunology 2024年第4期21卷 393-408页

作者： Sujin lee Yeunjung Ko Hyun Woo lee Won joon Oh Hun Gi Hong Dinuka Ariyaratne Se Jin Im Tae Jin Kim Department of Immunology Graduate School of Basic Medical ScienceSungkyunkwan University School of MedicineSuwon16419Republic of Korea Department of Immunology and Molecular Medicine Faculty of Medical SciencesUniversity of Sri JayewardenepuraNugegodaSri Lanka Present address:Immunology and Microbiology Graduate Program Baylor College of MedicineHoustonTX77030USA

Marginal zone(MZ)B cells,which are splenic innate-like B cells that rapidly secrete antibodies(Abs)against blood-borne pathogens,are composed of heterogeneous subpopulations.Here,we showed that MZ B cells can be divided into two distinct subpopulations according to their CD80 expression levels.CD80^(high)MZ B cells exhibited greater Ab-producing,proliferative,and IL-10-secreting capacities than did CD80^(low)MZ B cells.Notably,CD80^(high)MZ B cells survived 2-Gy whole-body irradiation,whereas CD80^(low)MZ B cells were depleted by irradiation and then repleted with one month after irradiation.Depletion of CD80^(low)MZ B cells led to accelerated development of type II collagen(CII)-induced arthritis upon immunization with bovine CII.CD80^(high)MZ B cells exhibited higher expression of genes involved in proliferation,plasma cell differentiation,and the antioxidant response.CD80^(high)MZ B cells expressed more autoreactive B cell receptors(BCRs)that recognized double-stranded DNA or CII,expressed more immunoglobulin heavy chain sequences with shorter complementarity-determining region 3 sequences,and included more clonotypes with no N-nucleotides or with B-1a BCR sequences than CD80^(low)MZ B cells.Adoptive transfer experiments showed that CD21^(+)CD23^(+)transitional 2 MZ precursors preferentially generated CD80^(low)MZ B cells and that a proportion of CD80^(low)MZ B cells were converted into CD80^(high)MZ B cells;in contrast,CD80^(high)MZ B cells stably remained CD80^(high)MZ B cells.In summary,MZ B cells can be divided into two subpopulations according to their CD80 expression levels,Ab-producing capacity,radioresistance,and autoreactivity,and these findings may suggest a hierarchical composition of MZ B cells with differential stability and BCR specificity.

关键词： Marginal Zone B Cell CD80 Autoreactivity Radioresistance

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