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Tunable nitrogen crafted 2D-graphene nano-hybrid from industrial expansive and ecological approach as robust cathode microporous layer to improve performance of a direct methanol fuel cell

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中国科学:技术科学英文版 2023年第9期66卷 2669-2680页

作者： BALAKRISHNAN Prabhuraj GUAN Li LIU HuiYuan LEUNG PuiKi SHAH Akeel XING Lei su huaneng XU Qian Institute for Energy Research Jiangsu UniversityZhenjiang 212013China School of Energy and Power Engineering Chongqing UniversityChongqing 400030China Department of Chemical Process Engineering University of SurreyGuildford GU27XHUK

In this work, the excess water-stagnation issue in the high current region in direct methanol fuel cells(DMFCs) is resolved by using atomic precision modulated nitrogen-crafted graphene(NG) in the cathode microporous layer by utilizing simplistic,industrial-expansive and ecological strategy. Few-layer 2D-graphene(~2–5 nm thickness) is prepared by bath sonication approach from abundant feedstock-graphite and is treated with nitric acid to yield 1.8 wt.% uniformly dispersed nitrogen containing NG. Specifically, 1:4 weight ratio NG:carbon-black(CB) hybrid architecture, displays 0.252 V in 370 mA cm^(-2) with the peak power density of 93.4 mW cm^(-2), improving cell power density by 45.6% compared with standard one at 60℃ and 1 mol/L methanol/oxygen conditions at ultra-low catalyst loadings and displaying exceptional stability. Atomic insights into NG reveal that interplay between bonding configurations, altered hydrophobic/hydrophilic porosity of graphene(10.6% less wettability from contact angle and 13.1% high electrode porosity measurements) contribute to the better mass-transport-porogenic effect(16.3% high oxygen-permeability), mildly affecting the electron pathway(6.5% reduced in-plane electrical conductivity),overall significantly improving cell performance. Altogether, this work delivers multiple advantages, i.e., the usage of material from facile, sustainable and cost-effective routes, while improving DMFC performance with potential industrial promise.

关键词： direct methanol fuel cells(DMFCs) membrane electrode assembly(MEA) 2D materials liquid phase exfoliation nitrogen doping

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Enhanced electro-oxidation of formic acid by a PdPt bimetallic catalyst on a CeO_2-modified carbon support

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Science China Chemistry 2012年第3期55卷 391-397页

作者： YANG LiJun su huaneng SHU Ting LIAO ShiJun School of Chemistry and Chemical Engineering South China University of TechnologyGuangzhou 510641China

PdPt bimetallic catalysts that employ CeO2-modified carbon black as a support have been prepared using an organic colloidal ***/CeO2-C shows excellent performance toward the anodic oxidation of formic *** effects of varying both Pd to Pt ratio and CeO2 content have been *** optimal Pd to Pt atomic ratio is 15,indicating that addition of small amounts of Pt can significantly enhance the activity of the *** the CeO2 content in the catalyst reaches as high as ～15 wt.%,the catalyst shows the maximum *** CeO2 not only enhances the catalytic activity of the material,but may also change the mechanism of its catalysis of the anodic oxidation of formic ***15Pt1/15CeO2-C exhibited 60% higher activity than Pd/C,and had a negative shift in onset potential of more than 0.1 *** on characterization by X-ray diffraction,X-ray photoelectron spectroscopy,thermogravimetric analysis and transmission electron microscopy,the interactions between the components are revealed and discussed in detail.

关键词：双金属催化剂氧化铈甲酸修饰电氧化 X射线光电子能谱催化活性 X射线衍射仪

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Hollow cobalt oxide nanoparticles embedded in nitrogen-doped carbon nanosheets as an efficient bifunctional catalyst for Zn–air battery

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Journal of Energy Chemistry 2019年第6期28卷 59-66页

作者： Yuhui Tian Li Xu Jian Bao Junchao Qian huaneng su Huaming Li Haidong Gu Cheng Yan Henan Li School of Chemistry and Chemical Engineering Institute for Energy ResearchJiangsu UniversityZhenjiang 212013JiangsuChina Jiangsu Key Laboratory for Environment Functional Materials School of Environmental Science and EngineeringSuzhou University of Science and TechnologySuzhou 215009JiangsuChina School of Chemistry Physics and Mechanical EngineeringQueensland University of TechnologyBrisbaneQLD 4001Australia

Rational design of low-cost, highly electrocatalytic activity, and stable bifunctional electrocatalysts for oxygen reduction reaction(ORR) and oxygen evolution reaction(OER) has been a great significant for metal–air batteries. Herein, an efficient bifunctional electrocatalyst based on hollow cobalt oxide nanoparticles embedded in nitrogen-doped carbon nanosheets(Co/N-Pg) is fabricated for Zn–air batteries. A lowcost biomass peach gum, consisting of carbon, oxygen, and hydrogen without other heteroatoms, was used as carbon source to form carbon matrix hosting hollow cobalt oxide nanoparticles. Meanwhile, the melamine was applied as nitrogen source and template precursor, which can convert to carbon-based template graphitic carbon nitride by polycondensation process. Owing to the unique structure and synergistic effect between hollow cobalt oxide nanoparticles and Co-N-C species, the proposal Co/N-Pg catalyst displays not only prominent bifunctional electrocatalytic activities for ORR and OER, but also excellent durability. Remarkably, the assembled Zn–air battery with Co/N-Pg air electrode exhibited a low discharge-charge voltage gap(0.81 V at 50 mA cm^-2) and high peak power density(119 mW cm^-2) with long-term cycling stability. This work presents an effective approach for engineering transition metal oxides and nitrogen modified carbon nanosheets to boost the performance of bifunctional electrocatalysts for Zn–air battery.

关键词： Zn-air batteries Oxygen reduction reaction Oxygen evolution reaction Nitrogen-doped carbon nanosheets Cobalt oxides

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Shock Formation for 2D Isentropic Euler Equations with Self-similar Variables

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Chinese Annals of Mathematics,Series B 2024年第3期45卷 349-412页

作者： Wenze su School of Mathematical Sciences Fudan UniversityShanghai 200433China

The author studies the 2D isentropic Euler equations with the ideal gas *** exhibits a set of smooth initial data that give rise to shock formation at a single point near the planar *** solutions to the 2D isentropic Euler equations are associated with non-zero vorticity at the shock and have uniform-in-time-1/3-Holder ***,these point shocks are of self-similar type and share the same profile,which is a solution to the 2D self-similar Burgers *** proof of the solutions,following the 3D construction of Buckmaster,Shkoller and Vicol(in 2023),is based on the stable 2D self-similar Burgers profile and the modulation method.

关键词： 2D isentropic Euler equations Shock formation Self-similar solution

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Design and pricing of maintenance service contract based on Nash non-cooperative game approach

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Journal of Systems Engineering and Electronics 2024年第1期35卷 118-129页

作者： su Chun HUANG Kui School of Mechanical Engineering Southeast UniversityNanjing 211189China

Nowadays manufacturers are facing fierce *** from the products,providing customers with multiple maintenance options in the service contract becomes more popular,since it can help to improve customer satisfaction,and ultimately promote sales and maximize profit for the *** considering the combinations of corrective maintenance and preventive maintenance,totally three types of maintenance service contracts are ***,attractive incentive and penalty mechanisms are adopted in the *** this basis,Nash non-cooperative game is applied to analyze the revenue for both the manufacturer and customers,and so as to optimize the pricing mechanism of maintenance service contract and achieve a win-win *** experiments are *** results show that by taking into account the incentive and penalty mechanisms,the revenue can be improved for both the customers and ***,with the increase of repair rate and improvement factor in the preventive maintenance,the revenue will increase gradually for both the parties.

关键词： maintenance service contract Nash game incentive and penalty mechanism corrective maintenance preventive maintenance

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Performance Investigation of Membrane Electrode Assemblies for High Temperature Proton Exchange Membrane Fuel Cell

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Journal of Power and Energy Engineering 2013年第5期1卷 95-100页

作者： huaneng su Sivakumar Pasupathi Bernard Bladergroen Vladimir Linkov Bruno G. Pollet HySA Systems Competence Centre South African Institute for Advanced Materials Chemistry University of the Western Cape Private Bag X17 Bellville 7535 South Africa

Different types of ABPBI (poly(2,5-benzimidazole)) membranes and polymer binders were evaluated to investigate the performance of MEAs for high temperature proton exchange membrane fuel cell (HT-PEMFC). The properties of the prepared MEAs were evaluated and analyzed by polarization curve, electrochemistry impedance spectroscopy (EIS), cyclic voltammetry (CV) and durability test. The results showed that MEA with modified ABPBI membrane (AM) has satisfactory performance and durability for fuel cell application. Compare to conventional PBI or Nafion binders, polytetrafluoroethylene (PTFE) and polyvinylidene difluoride (PVDF) are more attractive as binders in the catalyst layer (CL) of gas diffusion electrode (GDE) for HT-PEMFC.

关键词： High Temperature Proton Exchange Membrane Fuel Cell ABPBI (Poly(2 5-Benzimidazole)) Polymer Binders Gas Diffusion Electrode Membrane Electrode Assembly

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A Time-Domain Numerical Simulation for Free Motion Responses of Two Ships Advancing in Head Waves

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China Ocean Engineering 2024年第3期38卷 519-530页

作者： PAN su-yong CHENG Yong School of Naval Architecture and Ocean Engineering Jiangsu University of Science and TechnologyZhenjiang 212003China

The constant panel method within the framework of potential flow theory in the time domain is developed for solving the hydrodynamic interactions between two parallel ships with forward *** solving problems within a time domain framework,the free water surface needs to simultaneously satisfy both the kinematic and dynamic boundary conditions of the free water *** provides conditions for adding artificial damping *** the Runge−Kutta method to solve equations related to *** upwind differential scheme is used in the present method to deal with the convection terms on the free surface to prevent waves *** the comparison with the available experimental data and other numerical methods,the present method is proved to have good mesh convergence,and satisfactory results can be *** constant panel method is applied to calculate the hydrodynamic interaction responses of two parallel ships advancing in head *** simulations are conducted on the effects of forward speed,different longitudinal and lateral distances on the motion response of two modified Wigley ships in head *** further investigations are conducted on the effects of different ship types on the motion response.

关键词： ship motions time domain simulation forward speed different distances wave loads

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Stochastic and Distributed Optimal Energy Management of Active Distribution Networks Within Integrated Office Buildings

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CSEE Journal of Power and Energy Systems 2024年第2期10卷 504-517页

作者： Zening Li su su Xiaolong Jin Mingchao Xia Qifang Chen Koji Yamashita National Active Distribution Network Technology Research Center Beijing Jiaotong UniversityBeijing 100044China Key Laboratory of Smart Grid of Ministry of Education Tianjin UniversityTianjin 300072China Electrical and Computer Engineering University of California RiversideCA92521USA.

This paper proposes a stochastic and distributed optimal energy management approach for active distribution networks(ADNs)within office *** proposed approach aims at scheduling office buildings fitted with heating ventilation and air conditioning(HVAC)systems,and electric vehicle(EV)charging piles,to participate in the ADN ***,an energy management approach for the ADN with aggregated office buildings is *** the ADN optimization model is formulated considering the detailed building thermal dynamics and the mobile behaviors of ***,to consider un-certainties of photovoltaic(PV)power,scenario-based stochastic programming is integrated into the ADN optimization *** further realize the stochastic energy management of the ADN within office buildings in a distributed manner,the alternating direction method of multipliers(ADMM)is used to solve the ADN optimization *** original ADN optimization problem is divided into the network-side and the building-side sub-problems to effectively protect the privacy of the ADN and the office ***,the ADN optimization model incorporating office buildings is validated in the winter by numerical *** addition,the impacts of comfort temperature range and expected state of charge(SOC)at departure are *** Terms—ADN,EV,HVAC system,Office building,Stochastic and distributed energy management.

关键词： ADN EV HVAC system Office building Stochastic and distributed energy management

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Numerical simulation of microwave-induced cracking and melting of granite based on mineral microscopic models

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International Journal of Minerals,Metallurgy and Materials 2024年第7期31卷 1512-1524页

作者： Xiaoli su Diyuan Li Junjie Zhao Mimi Wang Xing su Aohui Zhou School of Resources and Safety Engineering Central South UniversityChangsha 410083China

This study introduces a coupled electromagnetic–thermal–mechanical model to reveal the mechanisms of microcracking and mineral melting of polymineralic rocks under microwave *** tests validate the rationality of the proposed *** microscopic mineral sections into the granite model for simulation shows that uneven temperature gradients create distinct molten,porous,and nonmolten zones on the fracture ***,the varying thermal expansion coefficients and Young's moduli among the minerals induce significant thermal stress at the mineral *** and biotite with higher thermal expansion coefficients are subjected to compression,whereas plagioclase with smaller coefficients experiences tensile *** the molten zone,quartz undergoes transgranular cracking due to theα–βphase *** local high temperatures also induce melting phase transitions in biotite and *** numerical study provides new insights into the distribution of thermal stress and mineral phase changes in rocks under microwave irradiation.

关键词： microwave numerical modeling microcracking phase change granite

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UNIFORM ERROR BOUNDS OF A CONSERVATIVE COMPACT FINITE DIFFERENCE METHOD FOR THE QUANTUM ZAKHAROV SYSTEM IN THE suBSONIC LIMIT REGIME

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Journal of Computational Mathematics 2024年第1期42卷 289-312页

作者： Gengen Zhang Chunmei su School of Mathematics and Statistics Yunnan UniversityKunming 650504China Yau Mathematical Sciences Center Tsinghua UniversityBeijing 100084China

In this paper,we consider a uniformly accurate compact finite difference method to solve the quantum Zakharov system(QZS)with a dimensionless parameter 0<ε≤1,which is inversely proportional to the acoustic *** the s... 详细信息

In this paper,we consider a uniformly accurate compact finite difference method to solve the quantum Zakharov system(QZS)with a dimensionless parameter 0subsonic limit regime,i.e.,when 0sults are reported to verify the error behavior.

关键词： Quantum Zakharov system subsonic limit Compact finite difference method Uniformly accurate Error estimate

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