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Construction of 2D/2D Ti_(3)C_(2)T_(x)MXene/Cds heterojunction with photothermal effect for efficient photocatalytic hydrogen production

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journal of Materials science & Technology 2024年第4期171卷 1-9页

作者： T.Y.huang Z.Yang s.Y.Yang Z.H.Dai Y.j.Liu j.H.Liao G.Y.Zhong Z.j.Xie Y.P.Fang s.s.Zhang Key Laboratory for Biobased Materials and Energy of Ministry of Education Guangdong Laboratory for Lingnan Modern AgricultureCollege of Materials and EnergySouth China Agricultural UniversityGuangzhou 510643China school of Physics and Optoelectronics South China University of TechnologyGuangzhou 510640China school of Chemical Engineering and Energy Technology Guangdong Provincial Key Laboratory of Distributed Energy SystemsDongguan University of TechnologyDongguan 523808China

The insensitivity of semiconductors to visible and infrared light is a key constraint on the utilization of light energy in photocatalytic *** photocatalysts with full-spectrum absorption through surface engineering is an effective approach to fully harnessing light energy in semiconductor ***,a novel stable Ti_(3)C_(2)T_(x)MXene/Cds heterojunction catalyst is obtained by in-situ epitaxial growth of two-dimensional(2D)Cds nanosheets on 2D MXene interface via a solvothermal *** exceptional light absorption properties of MXene confer outstanding full-spectrum driven photocat-alytic hydrogen evolution capability upon the heterogeneous *** unique 2D/2D structure effectively mitigated the recombination of photogenerated carriers,enhancing the photocatalytic performance of the ***,the composite catalyst exhibits a significantly higher surface temperature of 80.4℃under visible light irradiation at an intensity of 0.1 W/cm^(2),which is 1.84 times higher than that of *** irradiation of visible and near infrared light,the composite catalyst with photothermal ef-fect demonstrates a remarkable hydrogen evolution rate of 65.4 mmol g^(-1)h^(-1),which is 7.2 times higher than that of Cds *** study introduces a novel approach for constructing full-spectrum absorption catalysts and expands the application of the photothermal effect in photocatalytic hydrogen evolution research.

关键词： Two-dimensional structure Heterostructure Photothermal effect Photocatalyst Hydrogen evolution

A thermodynamic perspective on electrode poisoning in solid oxide fuel cells

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International journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1449-1455页

作者： Kevin huang Department of Mechanical Engineering University of South CarolinaColumbiaUSA

A critical challenge to the commercialization of clean and high-efficiency solid oxide fuel cell(sOFC)technology is the insuf-ficient stack lifespan caused by a variety of degradation mechanisms,which are associated with cell components and chemical *** components related degradation refers to thermal/chemical/electrochemical deterioration of cell materials under operating conditions,whereas the latter regards impurities in feedstocks of oxidant(air)and reductant(fuel).This article provides a thermodynamic perspective on the understanding of the impurities-induced degradation mechanisms in *** discussion focuses on using thermodynamic ana-lysis to elucidate poisoning mechanisms in cathodes by impurity species such as Cr,CO_(2),H_(2)O,and sO_(2) and in the anode by species such as s(or H_(2)s),siO_(2),and P_(2)(or PH_(3)).The author hopes the presented fundamental insights can provide a theoretical foundation for search-ing for better technical solutions to address the critical degradation challenges.

关键词： impurities air fuel reaction activity

Emerging high-entropy strategy: A booster to the development of cathode materials for power batteries

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journal of Advanced Ceramics 2024年第8期13卷 1093-1118页

作者： Liping huang jinging Zhu j-Xuan Liu Houzheng Wu Guo-jun Zhang state Key Laboratory for Modification of Chemical Fibers and Polymer Materials Institute of Functional MaterialsCollege of Materials Science and EngineeringDonghua UniversityShanghai 201620China sIAMC Advanced Materials Cooperation Huzhou 313100China

The coordinated development of new energy vehicles and the energy storage industry has become essential for reducing carbon *** cathode material is the key material that determines the energy density and cost of a power battery,but currently developed and applied cathode materials cannot meet the requirements for high specific capacity,low cost,safety,and good ***-entropy materials(HEMs)are a new type of single-phase material composed of multiple principal elements in equimolar or near-equimolar *** interaction between multiple elements can play an important role in improving the comprehensive properties of the material,which is expected to solve the limitations of battery materials in practical ***,this review provides a comprehensive overview of the current development status and modification strategies of power batteries(lithium-ion batteries(LiBs)and sodium-ion batteries(sIBs)),proposes a high-entropy design strategy,and analyses the structure-activity relationship between the high-entropy effects and battery ***,future research topics related to high-entropy cathode materials,including computational guide design,specific synthesis methods,high-entropy electrochemistry,and high-throughput databases,are *** review aims to provide practical guidance for the development of high-entropy cathode materials for next-generation power batteries.

关键词： cathode materials lithium-ion battery(LIB) sodium-ion battery(sIB) high-entropy strategy

Distributed secondary Control Based on Dynamic Diffusion Algorithm for Current sharing and Average Voltage Regulation in DC Microgrids

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journal of Modern Power systems and Clean Energy 2024年第2期12卷 597-607页

作者： Dawei Liao Fei Gao Daniel j.Rogers Wentao huang Dong Liu Houjun Tang Department of Electrical Engineering Shanghai Jiao Tong UniversityShanghaiChina Department of Engineering science University of OxfordOxford OX12JDU.K. IEEE

This paper introduces a distributed secondary control scheme for achieving current sharing and average voltage regulation objectives in a DC *** proposed scheme employs a dynamic diffusion algorithm(DDA)instead of the consensus algorithm to enable distributed communication among *** help understand DDA,the relation of DDA and other diffusion algorithms is discussed in detail and its superiority is shown by comparison with diffusion and consensus ***,considering the discrete nature and different sampling time of the digital controller and communication network,a z-domain model of the entire DC microgrid is *** influence of communication and secondary control parameters on the system stability is *** on the established model,the tolerable communication rates are ***-time simulations conducted on the OPAL-RT platform validate the effectiveness of the proposed scheme,showcasing its advantages in terms of convergence speed and stability.

关键词： Cooperative control DC microgrid diffusion algorithm discrete-time modeling distributed secondary control

Granger causal representation learning for groups of time series

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science China(Information sciences) 2024年第5期67卷 56-68页

作者： Ruichu CAI Yunjin WU Xiaokai huang Wei CHEN Tom Z.j.FU Zhifeng HAO school of Computer science Guangdong University of Technology Peng Cheng Laboratory College of science Shantou University

Discovering causality from multivariate time series is an important but challenging *** existing methods focus on estimating the Granger causal structures among multivariate time series,while ignoring the prior knowledge of these time series, e.g., the group of the time series. Focusing on discovering the Granger causal structures among groups of time series, we propose a Granger causal representation learning method to solve this problem. First, we use the multiset canonical correlation analysis method to learn the Granger causal representation of each group of time series. Then, we model the Granger causal relationships among the learned Granger causal representations using a recurrent neural network with temporal information. Finally, we formulate the above two stages into one unified optimization problem, which is efficiently solved using the augmented Lagrangian method. We conduct extensive experiments on synthetic and real-world datasets to validate the correctness and effectiveness of the proposed method.

关键词： Granger causal discovery Granger causal representation learning time series data recurrent neural network multiset canonical correlation analysis

Hierarchical model updating for high-speed maglev vehicle/guideway coupled system based on multiobjective optimization

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Frontiers of structural and Civil Engineering 2024年第5期18卷 788-804页

作者： Dexiang Li jingyu huang College of Civil Engineering Tongji UniversityShanghai 200092China National Maglev Transportation Engineering R&D Center Tongji UniversityShanghai 201804China

The high-speed maglev vehicle/guideway coupled model is an essential simulation tool for investigating vehicle dynamics and mitigating coupled *** improve its accuracy efficiently,this study investigated a hierarchical model updating method integrated with field ***,a high-speed maglev vehicle/guideway coupled model,taking into account the real effect of guideway material properties and elastic restraint of bearings,was developed by integrating the finite element method,multi-body dynamics,and electromagnetic levitation ***,simultaneous in-site measurements of the vehicle/guideway were conducted on a high-speed maglev test line to analyze the system response and structural modal *** the hierarchical updating,an Elman neural network with the optimal Latin hypercube sampling method was used to substitute the FE guideway model,thus improving the computational *** multi-objective particle swarm optimization algorithm with the gray relational projection method was applied to hierarchically update the parameters of the guideway layer and magnetic force layer based on the measured modal parameters and the electromagnet vibration,***,the updated coupled model was compared with the field measurements,and the results demonstrated the model’s accuracy in simulating the actual dynamic response,validating the effectiveness of the updating method.

关键词： high-speed maglev vehicle/guideway coupled model field measurement model updating neural network multi-objective optimization

Revisiting the Mg isotopic systematics of siliciclastic components of sediments and sedimentary rocks:A new geochemical proxy of continental weathering in Earth's history

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science China Earth sciences 2024年第2期67卷 620-633页

作者： Tianzheng huang Bing sHEN Kangjun huang Meng NING Chao LI jinzhuang XUE Yuanlin sUN Baoqi huang Key Laboratory of Orogenic Belt and Crustal Evolution MOESchool of Earth and Space SciencesPeking UniversityBeijing100871China state Key Laboratory of Continental Dynamics Shaanxi Key Laboratory of Early Life and EnvironmentsDepartment of GeologyNorthwest UniversityXi’an710069China Institute of sedimentary Geology Chengdu University of TechnologyChengdu610059China Key Laboratory of Rhenium-Osmium Isotopic Geochemistry Chinese Academy of Geological SciencesBeijing100037China

The Mg isotopic compositions of siliciclastic components(δ^(26)Mg_(sili))of sediments and sedimentary rocks have been commonly used to constrain the intensity of continental weathering,based on observations of,(1)an upward enrichment of26Mg in modern weathering profiles,(2)preferential uptake of26Mg in soil clays,and(3)general positive correlations between weathering intensities andδ^(26)Mg_(sili)***,not all weathering profiles display an upward increase ofδ^(26)Mg_(sili),and not all soil clays enrich in26Mg,complicating the interpretations ofδ^(26)Mg_(sili)data of sediments and sedimentary *** further explore the controls ofδ^(26)Mg_(sili)of sediments and sedimentary rocks,here we measuredδ^(26)Mg_(sili),mineralogical compositions and major element compositions of deep sea sediments from south China sea(sCs)and carbonate rock samples from two late Paleozoic sections in south *** samples show decreasing trends of both normalized Mg concentration(Mgnorm)andδ^(26)Mg_(sili)values with the increase of weathering intensity,while sCs sediments samples do not show any correlation between Mgnormorδ^(26)Mg_(sili)values and weathering intensity.A three-stages weathering model is developed to explain the observed Mgnorm andδ^(26)Mg_(sili)*** the new model,weathering can be divided into three stages,(1)the preliminary weathering stage characterized by dissolution of primary minerals and formation of secondary clay minerals in saprolite,(2)the transitional stage with massive vermiculite and chlorite formation on the bottom of soil,and(3)the advanced stage showing dissolution of vermiculite and chlorite in the top of *** new model explains anδ^(26)Mg_(sili)increase and Mgnormdecrease with an increase weathering intensity in preliminary weathering stage and decrease of Mgnormandδ^(26)Mg_(sili)with increase weathering intensity in advanced weathering *** revised weathering model warrants the application of Mg isotope in the study of contin

关键词： Clay mineral Chemical weathering CIA soil Weathering model

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Tsinghua science and Technology 2024年第4期29卷 971-984页

作者： Yuze Peng shengjun Xu Qingkun Chen Wenjin huang Yihua huang school of Electronics and Information Technology Sun Yat-sen UniversityGuangzhou 510006China Guangdong Provincial Key Laboratory of Optoelectronic Information Processing Chips and systems Sun Yat-sen UniversityGuangzhou 510006Chinaand Southern Marine Science and Engineering Guangdong LaboratoryZhuhai 519080China

Popularity plays a significant role in the recommendation system. Traditional popularity is only defined as a static ratio or metric (e.g., a ratio of users who have rated the item and the box office of a movie) regardless of the previous trends of this ratio or metric and the attribute diversity of items. To solve this problem and reach accurate popularity, we creatively propose to extract the popularity of an item according to the Proportional Integral Differential (PID) idea. specifically, Integral (I) integrates a physical quantity over a time window, which agrees with the fact that determining the attributes of items also requires a long-term observation. The Differential (D) emphasizes an incremental change of a physical quantity over time, which coincidentally caters to a trend. Moreover, in the session-Based Recommendation (sBR) community, many methods extract session interests without considering the impact of popularity on interest, leading to suboptimal recommendation results. To further improve recommendation performance, we propose a novel strategy that leverages popularity to enhance the session interest (popularity-aware interest). The proposed popularity by PID is further used to construct the popularity-aware interest, which consistently improves the recommendation performance of the main models in the sBR community. For sTAMP, sRGNN, GCsAN, and TAGNN, on Yoochoose1/64, the metric P@20 is relatively improved by 0.93%, 1.84%, 2.02%, and 2.53%, respectively, and MRR@20 is relatively improved by 3.74%, 1.23%, 2.72%, and 3.48%, respectively. On Movieslen-1m, the relative improvements of P@20 are 7.41%, 15.52%, 8.20%, and 20.12%, respectively, and that of MRR@20 are 2.34%, 12.41%, 20.34%, and 19.21%, respectively.

关键词： popularity Proportional Integral Differential(PID) algorithm session-based recommendation user’s interests

Laminar Flame structure-Dependent Exergy Destruction Behavior at Auto-Ignition Time scale:A Case study of Dimethyl Ether(DME)

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journal of Thermal science 2024年第4期33卷 1257-1271页

作者： WU Honghuan huang Wenlin ZHAO Hao sUN Wuchuan huang Zuohua ZHANG Yingjia state Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an710049China

Hybrid deflagration/auto-ignition flame structures coexist in the combustion of advanced *** exergy destruction caused by different irreversible processes under varied flame regimes is thus important for understanding engine *** this study,the flame propagation modes for the premixed DME/air mixtures are numerically investigated under engine-relevant *** entropy generation and exergy destruction characteristics are compared under different flame *** reveal that as the typical premixed flame transition towards auto-ignition front,the exergy destruction from heat conduction and species mass diffusion gradually vanish and are dominated by chemical *** distributions of temperature and species mole fraction in the flame domain are analyzed to clarify the exergy destruction behaviors caused by heat conduction and mass ***,by dividing the DME oxidation process into four stages,the main reaction channels that contribute to the increase in exergy destruction from chemical reaction have been *** is found that the production and consumption of CH_(2)O and HO_(2) radical dominate the exergy destruction behavior during DME *** this basis,the kinetic mechanism of low-temperature chemistry causing greater exergy destruction is ***,low-temperature chemistry leads to significant exergy destruction due to(a)the large irreversibility of itself and(b)(mainly)the enhancement of H_(2)O_(2)loop reactions by low-temperature reaction *** the reduction of combustion irreversibility is promising to be achieved by reasonably regulating the fuel oxidation path.

关键词： exergy destruction flame structures entropy generation low-temperature chemistry DME