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Hybrid 2D/3D Graphitic Carbon Nitride-Based High-Temperature Position-Sensitive Detector

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Energy & Environmental Materials 2024年第1期7卷 275-283页

作者： Xuexia Chen Dongwen yang Xun yang qing Lou Zhiyu Liu Yancheng Chen Chaofan Lv Lin Dong Chongxin Shan Henan Key Laboratory of Diamond Optoelectronic Materials and Devices Key Laboratory of Material PhysicsMinistry of EducationSchool of Physics and MicroelectronicsZhengzhou UniversityZhengzhou 450052China

Ultraviolet position-sensitive detectors(PSDs)are expected to undergo harsh environments,such as high temperatures,for a wide variety of applications in military,civilian,and ***,no report on relevant PSDs operating at high temperatures can be found up to ***,we design a new 2D/3D graphitic carbon nitride(g-C_(3)N_(4))/gallium nitride(GaN)hybrid heterojunction to construct the ultraviolet high-temperature-resistant *** g-C_(3)N_(4)/GaN PSD exhibits a high position sensitivity of 355 mV mm^(-1),a rise/fall response time of 1.7/2.3 ms,and a nonlinearity of 0.5%at room *** ultralow formation energy of-0.917 eV atom^(-1)has been obtained via the thermodynamic phase stability calculations,which endows g-C_(3)N_(4)with robust stability against *** merits of the strong built-in electric field of the 2D/3D hybrid heterojunction and robust thermo-stability of g-C_(3)N_(4),the g-C_(3)N_(4)/GaN PSD delivers an excellent position sensitivity and angle detection nonlinearity of 315 mV mm^(-1)and 1.4%,respectively,with high repeatability at a high temperature up to 700 K,outperforming most of the other counterparts and even commercial silicon-based *** work unveils the high-temperature PSD,and pioneers a new path to constructing g-C_(3)N_(4)-based harsh-environment-tolerant optoelectronic devices.

关键词： graphitic carbon nitride high-temperature stability lateral photovoltaic effect position-sensitive detectors two-dimensional materials

Prediction of the potential distribution and analysis of the freezing injury risk of winter wheat on the Loess Plateau under climate change

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Journal of Integrative Agriculture 2024年第9期23卷 2941-2954页

作者： qing Liang Xujing yang Yuheng Huang Zhenwei yang Meichen Feng Mingxing qing Chao Wang Wude yang Zhigang Wang Meijun Zhang Lujie Xiao Xiaoyan Song College of Agriculture Shanxi Agricultural UniversityTaigu 030801China Smart Agriculture College Shanxi Agricultural UniversityTaigu 030801China College of Resources and Environment Shanxi Agricultural UniversityTaigu 030801China

Determining the suitable areas for winter wheat under climate change and assessing the risk of freezing injury are crucial for the cultivation of winter *** used an optimized Maximum Entropy(MaxEnt)Model to predict the potential distribution of winter wheat in the current period(1970-2020)and the future period(2021-2100)under four shared socioeconomic pathway scenarios(SSPs).We applied statistical downscaling methods to downscale future climate data,established a scientific and practical freezing injury index(FII)by considering the growth period of winter wheat,and analyzed the characteristics of abrupt changes in winter wheat freezing injury by using the Mann-Kendall(M-K)*** results showed that the prediction accuracy AUC value of the MaxEnt Model reached *** minimum temperature in the coldest month,precipitation in the wettest season and annual precipitation were the main factors affecting the spatial distribution of winter *** total suitable area of winter wheat was approximately 4.40×10^(7)ha in the current *** the 2070s,the moderately suitable areas had the greatest increase by 9.02×10^(5)ha under SSP245 and the least increase by 6.53×10^(5)ha under *** centroid coordinates of the total suitable areas tended to move *** potential risks of freezing injury in the high-latitude and-altitude areas of the Loess Plateau,China increased *** northern areas of Xinzhou in Shanxi Province,China suffered the most serious freezing injury,and the southern areas of the Loess Plateau suffered the *** factors such as temperature,precipitation and geographical location had important impacts on the suitable area distribution and freezing injury risk of winter *** the future,greater attention should be paid to the northward boundaries of both the winter wheat planting areas and the areas of freezing injury risk to provide the early warning of freezing injury and implement corresponding management strat

关键词： climate change scenarios winter wheat freezing injury risk downscaling MaxEnt

Gastric metastasis of small cell lung carcinoma:Three case reports and review of literature

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World Journal of Gastroenterology 2024年第31期30卷 3717-3725页

作者： Shan yang qing-Yun He qing-Jing Zhao Han-Tao yang Zheng-Yi yang Wen-Yi Che Hua-Mei Li Hui-Chao Wu Department of Gastroenterology The Affiliated Hospital of Zunyi Medical UniversityZunyi 563000Guizhou ProvinceChina Department of Gastroenterology Guizhou Hospital of The First Affiliated HospitalSun Yat-sen UniversityGuiyang 550000Guizhou ProvinceChina Department of Gastroenterology Zhejiang Provincial People's Hospital Bijie HospitalBijie 551700Guizhou ProvinceChina Department of Gastroenterology Zunyi Medical UniversityZunyi 563000Guizhou ProvinceChina

BACKGROUND Small cell lung carcinoma(SCLC)is highly susceptible to metastasis in the early stages of the ***,the stomach is an uncommon site of metastasis in SCLC,and only a few cases of this type of metastasis have been ***,SCLC gastric metastases have not been systematically characterized and are easily missed and *** SUMMARY We report three cases of gastric metastasis from SCLC in this *** first patient presented primarily with cough,hemoptysis,and epigastric *** other two patients presented primarily with abdominal discomfort,epigastric distension,and *** patients underwent gastroscopy and imaging ***,the immunohistochemical results of the lesions in three patients were suggestive of small cell ***,the three patients were diagnosed with gastric metastasis of SCLC through a comprehensive *** three patients did not receive appropriate treatment and died within a short *** Here,we focused on summarizing the characteristics of gastric metastasis of SCLC to enhance clinicians'understanding of this disease.

关键词： Small cell lung cancer Gastric neoplasms Neoplasm metastasis Diagnosis Case report

Catalyst-free and Reprocessable Aromatic Polydithiourethanes

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Chinese Journal of Polymer Science 2024年第10期42卷 1435-1441,I0007页

作者： Bo yang Hai-Jun Feng Tian-Tian Ni Xiao-Rui Zhou Tao Xie ning Zheng State Key Laboratory of Chemical Engineering College of Chemical and Biological EngineeringZhejiang UniversityHangzhou310058China Department of Colorectal Surgery and Oncology Key Laboratory of Cancer Prevention and InterventionMinistry of EducationThe Second Affiliated HospitalZhejiang University School of MedicineHangzhou310009China

The incorporation of dynamic covalent bonds into thermosets facilitates the reprocessing of polymer networks,thereby meeting the sustainable requirements for polymer ***,the mechanical properties of many materials often decline significantly upon reprocessing due to side reactions caused by harsh processing *** this work,we find that the aromatic dithiocarbamate bond can undergo dissociation under mild conditions without the need for a catalyst,enabling the efficient reprocessing of the corresponding *** a consequence,the mechanical properties of the polydithiourethane can be largely preserved after *** discovery of this dynamic chemistry is anticipated to broaden the potential for material design in dynamic covalent polymer networks.

关键词： Reprocessing Polydithiourethane Dynamic covalent bond

Additive manufactured osseointegrated screws with hierarchical design

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Bio-Design and Manufacturing 2024年第2期7卷 206-235页

作者： Wenbo yang Hao Chen Haotian Bai Yifu Sun Aobo Zhang yang Liu Yuchao Song qing Han Jincheng Wang Department of Orthopedics Second Hospital of Jilin UniversityChangchun 130022China College of Biological and Agricultural Engineering Jilin UniversityChangchun 130022China School of Materials Science and Engineering Jilin UniversityChangchun 130022China

Bone screws are devices used to fix implants or bones to ***,conventional screws are mechanically fixed with thread and often face long-term failure due to poor *** improve osseointegration,screws are evolving from solid and smooth to porous and *** manufacturing(AM)offers a high degree of manufacturing freedom,enabling the preparation of predesigned screws that are porous and *** paper provides an overview of the problems currently faced by bone screws:long-term loosening and screw ***,advances in osseointegrated screws are summarized hierarchically(sub-micro,micro,and macro).At the sub-microscale level,we describe surface-modification techniques for enhancing *** the micro level,we summarize the micro-design parameters that affect the mechanical and biological properties of porous osseointegrated screws,including porosity,pore size,and pore *** addition,we highlight three promising pore shapes:triply periodic minimal surface,auxetic structure with negative Poisson ratio,and the Voronoi *** the macro level,we outline the strategies of graded design,gradient design,and topology optimization design to improve the mechanical strength of porous osseointegrated ***,this paper outlines advances in AM technology for enhancing the mechanical properties of porous osseointegrated *** osseointegrated screws with hierarchical design are expected to provide excellent long-term fixation and the required mechanical strength.

关键词： Bone screws Additive manufacturing Architecture design Surface modification

Enhanced electrical properties and Vickers hardness of calcium bismuth niobate ceramics by W/Co substituted at B-site

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Journal of Advanced Dielectrics 2024年第4期14卷 92-103页

作者： Fei Wang Jia yang qing yang ning Chen Xinji yang Mingyue Mo Jie Xing Zhi Tan Zhongqing Tian Fancheng Meng Yuheng Guo Huixing Lin Jianguo Zhu College of Materials Science and Engineering Chongqing University of TechnologyChongqing 400054P.R.China College of Materials Science and Engineering Sichuan UniversityChengdu 610064P.R.China School of Electronic Engineering Chengdu Technological UniversityChengdu 611730P.R.China Key Laboratory of Inorganic Functional Material and Device Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 201899P.R.China

Calcium bismuth niobate(CBN)ceramic,as a core element of high-temperature piezoelectric sensors,has attracted widespread attention due to its high Curie temperature within the class of Aurivillius ***,CBN usually faces two *** piezoelectric constant and low *** this work,CBN-based ceramics with donor–acceptor ions(W/Co)co-substituted at B-site were prepared by solid-state reaction method,and structure–property relationship of ceramics was studied in ***-substitution of W/Co ions effectively improved the electrical property and hardness of CBN ***_(2)Nb_(1.91)(W_(2/3)Co_(1/3)T_(0.09)O_(9))exhibits enhanced electrical and mechanical properties including high resistivity of-10^(7)Ω·cm at 500℃,piezoelectric constant of-15.3 pC/N and hardness value of-3.57 *** values are two orders of magnitude,over two times,and 1.36 times higher than those of pure CBN ceramic,*** work provides a reference for exploring other bismuth-layered structural ceramics.

关键词： Calcium bismuth niobate ceramics donor and acceptor ions B-site electrical properties Vickers hardness

Photocatalytic in situ H_(2)O_(2) production and activation for enhanced ciprofloxacin degradation over CeO_(2)-Co_(3)O_(4)/g-C_(3)N_(4):key role of CeO_(2)

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Rare Metals 2024年第6期43卷 2695-2707页

作者： Hong-Jie Zhu Yi-Kai yang Ming-Hui Li Lu-ning Zou Hai-Tao Zhao Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology School of Chemistry and Chemical Engin College of Ecology and Environment Anhui Normal UniversityWuhu241002China Liaocheng YiLu Advanced Materials Co. LtdLiaocheng 252000China

The abused ciprofloxacin antibiotics have caused significant environmental *** oxidative degradation of ciprofloxacin exhibits promising efficacy,it often entails excessive energy ***,it is necessary to explore an effective and ecologically sustainable degradation ***,we demonstrated that g-C_(3)N_(4) decorated with the coordinated CeO_(2)and Co_(3)O_(4)(CeO_(2)-Co_(3)O_(4)/CN)exhibited effective ciprofloxacin photodegradation via in situ H_(2)O_(2) production and activation *** indicate that the introduced CeO_(2) enhances the transference of photogenerated electrons to O_(2) by adjusting the oxygen vacancy of photocatalyst,thereby increasing the generation of superoxide radicals,which in turn generate H_(2)O_(2),resulting in a 22.4-fold increase in H_(2)O_(2) generation over g-C_(3)N_(4).Moreover,the in situ H_(2)O_(2)generation facilitated by CeO_(2) is confirmed to be essential for ciprofloxacin degradation via CeO_(2)-Co_(3)O_(4)/CN,as it provides enough oxidant for Co_(3)O_(4) to activate into hydroxyl radicals for the pollutants ***,CeO_(2)-Co_(3)O_(4)/CN achieves a ciprofloxacin degradation ratio of 97.7%within 80 *** study introduces a novel approach that combines H_(2)O_(2) generation and activation,offering an innovative perspective for achieving clean and efficient purification of antibiotic-contaminated water.

关键词： CeO_(2) In situ H_(2)O_(2)generation Ciprofloxacin degradation Photocatalyst

Enhancement of heavy metals desorption from the soil by eddy deep leaching in hydrocyclone

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Journal of Environmental Sciences 2024年第1期135卷 242-251页

作者： ning Wang Hao Lu Bo Liu Tai Xiong Jianping Li Hualin Wang Qiang yang School of Mechanical and Power Engineering East China University of Science and TechnologyShanghai 200237China National Engineering Laboratory for High Concentration Refractory Organic Wastewater Treatment Technology East China University of Science and TechnologyShanghai 200237China

An eddy deep leaching technology was developed in this paper to address the challenge of treating heavy metal contaminants in industrial mining *** desorption effect of As,Cd,Sb and Pb was investigated utilizing chemical leaching and physical eddy *** was found that the heavy metals concentration increased with decreasing particle *** highest proportion of Cd in the form distribution of soil was in the bound to iron and manganese oxides,while the maximum proportion of As,Sb and Pb were in the *** optimal solid-liquid ratio of the hydrocyclone was 1:20,and the corresponding separation efficiency and flow rate were 84.7%and 1.76 m^(3)/hr,*** grade efficiency of soil particle separation increases with particle size and exceeds 99%for particles above 1,000μ*** experiments have revealed that oxalic acid(OA)and a combination of oxalic acid and EDTA(OAPE)were more efficient than citric acid(CA)and a combination of citric acid and EDTA(CAPE)for the desorption of heavy metals,*** comparison of OAPE and eddy leaching found that the latter improved the desorption efficiency by 9.4%,7.5%,7.2%and 7.8%for As,Cd,Sb and Pb compared to the former,*** results demonstrated that the eddy leaching technique could further enhance the desorption efficiency of heavy *** is expected to provide technical support for soil remediation with reduced usage of leaching agents.

关键词： Heavy metals Soil remediation Oxalic acid Eddy leaching Hydrocyclone

Ordovician reservoirs in Fuxian area:Gas accumulation patterns and their implications for the exploration of lower Paleozoic carbonates in the southern Ordos Basin

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Energy Geoscience 2024年第1期5卷 63-71页

作者： ning Gu Juntao Zhang Xiaohui Jin Fei yang Lu Liu Petroleum Exploration and Production Research Institute SINOPECBeijing102206China Huabei Oil&Gas Branch SINOPECZhengzhouHenan450000China

In recent years,the Fuxian area in the southeastern Ordos Basin has undergone significant exploration,with industrial gas flow tested in wells drilled into the Ordovician marine *** this,the gas accumulation patterns of this area are not fully understood,posing challenges for further *** analysis of geological conditions indicates that the Ordovician Majiagou Formation in this area hosts two gas plays:one found in weathering crusts and the other found in interior of the *** investigated various typical gas reservoirs in the area,focusing on differentiating the geological conditions and factors controlling gas accumulation in the weathering-crust and interior gas *** results suggest three primary gas accumulation patterns in the Majiagou Formation in the Fuxian area:(1)upper gas accumulation in weathering crusts,present in the high parts of landforms such as residual paleo-hills or buried paleo-platform(Pattern I);(2)the stereoscopic pattern with gas accumulation in both weathering crusts and strata interior,arising in high parts of landforms such as residual paleo-hills or buried paleo-platforms(Pattern II);(3)lower gas accumulation in strata interior,occurring in the upper reaches and on both sides of paleo-trenches(Pattern III).This study will serve as a geological basis for future exploration deployment in the Fuxian area.

关键词： Gas accumulation Ordovician Weathering crust play Interior play Fuxian area The ordos basin