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Rare Metals 2024年第5期43卷 1965-1976页

作者： Jin Long Kai-Wen zhuang wei Liao Yan An Bin wang Chen-Zhong Wu Jian-Xin Cao qing wang Jun-Song Chen qing-Mei wang Guizhou University Key Laboratory of Green Chemical and Clean Energy technology School of Chemistry and Chemical EngineeringGuizhou UniversityGuiyang 550025China Guizhou University engineering Research Center of Effcient Utilization for Industrial Waste Guizhou UniversityGuiyang 550025China institute of Dual-Carbon and New Energy technology Innovation and Development of Guizhou Province Guiyang 550025China Department of Dermatology West China HospitalSichuan UniversityChengdu610041China institute for Catalysis Hokkaido UniversitySapporo 001-0021Japan school of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731China Interdisciplinary Materials Research Center Institute for Advanced StudyChengdu UniversityChengdu 610106China

Opportunity to harmonize aspects of oxygen reduction reaction(ORR)performance and structure,and morphology,as well as composition,is urgent for the commercialization of proton exchange membrane fuel ***,we demonstrate the design and synthesis of a functionalized-supported-Pt catalyst(Pt@HNC)featuring a hollow nitrogen-modified dodecahedral carbon substrate obtained by a stress-induced-shrink tailoring *** as-obtained Pt@HNC catalyst possesses enhanced ORR per-formance,in particular with half-wave potential,mass activity(MA)and specific activity,which greatly exceed the commercial Pt/*** density functional theory(DFT)calculations further confirmed that the charge redistribution induced by the electronegativity differences improved the electron interaction between Pt and HNC *** optimized electronic structure of Pt weakens the reaction energy barrier on the Pt@HNC surface and adsorption of^(*)OH species,thus cooperatively improving the intrinsic activity toward ***,our work indeed provides a guide for the future design of functional nanomaterials in the field of catalysts and clean energy.

关键词： Proton exchange membrane fuel cell(PEMFC) Oxygen reduction catalysis Supported Pt-based catalyst Stability

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Wearable and interactive multicolored photochromic fiber display

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Light(Science & Applications) 2024年第3期13卷 454-465页

作者： Pan Li Yuwei wang Xiaoxian He Yuyang Cui Jingyu Ouyang Ju Ouyang Zicheng He Jiayu Hu Xiaojuan Liu Hang wei Yu wang Xiaoling lu Qian Ji Xinyuan Cai Li Liu Chong Hou ning Zhou Shaowu Pan Xiangru wang Huamin Zhou Cheng-wei Qiu Yan-qing lu Guangming Tao State Key Laboratory of Material Processing and Die&Mould technology School of Materials Science and Engineering and Wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhan 430074China Key Laboratory of Vascular Aging(HUST) Ministry of EducationWuhan 430030China school of Optoelectronic Science and engineering University of Electronic Science and Technology of ChinaChengdu 611731China Department of electrical and Computer engineering National University of SingaporeSingapore 117583Singapore National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and ManipulationCollege of Engineering and Applied Sciencesand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210023China school of Performing Arts Wuhan Conservatory of MusicWuhan 430060China school of Mechanical Science and engineering Huazhong University of Science and TechnologyWuhan 430074China school of Architecture and Urban Planning Huazhong University of Science and TechnologyWuhan 430074China school of Fashion Beijing Institute of Fashion TechnologyBeijing 100029China school of Optical and electronic Information Huazhong University of Science and TechnologyWuhan 430074China Tongji Medical College Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China

Endowing flexible and adaptable fiber devices with light-emitting capabilities has the potential to revolutionize the current design philosophy of intelligent,wearable interactive ***,significant challenges remain in developing fiber devices when it comes to achieving uniform and customizable light effects while utilizing lightweight ***,we introduce a mass-produced,wearable,and interactive photochromic fiber that provides uniform multicolored light *** designed independent waveguides inside the fiber to maintain total internal reflection of light as it traverses the *** impact of excessive light leakage on the overall illuminance can be reduced by utilizing the saturable absorption effect of fluorescent materials to ensure light emission uniformity along the transmission *** addition,we coupled various fluorescent composite materials inside the fiber to achieve artificially controllable spectral radiation of multiple color systems in a single *** prepared fibers on mass-produced kilometer-long using the thermal drawing *** fibers can be directly integrated into daily wearable devices or clothing in various patterns and combined with other signal input components to control and display patterns as *** work provides a new perspective and inspiration to the existing field of fiber display interaction,paving the way for future human–machine integration.

关键词： fiber interactive colored

A lithium–tin fluoride anode enabled by ionic/electronic conductive paths for garnet-based solid-state lithium metal batteries

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Rare Metals 2024年第2期43卷 575-587页

作者： Lei Zhang Qian-Kun Meng Xiang-Ping Feng Ming Shen Yu-qing Zhang Quan-Chao zhuang Run-Guo Zheng Zhi-Yuan wang Yan-Hua Cui Hong-Yu Sun Yan-Guo Liu school of Materials Science and engineering Northeastern UniversityShenyang110819China school of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao066004China school of Materials and Physics China University of Mining&TechnologyXuzhou221116China institute of electronic engineering China Academy of Engineering PhysicsMianyang621900China

The high energy density and stability of solid-state lithium metal batteries(SSLMBs)have garnered great ***-type oxides,especially Li_(6.4)La_(3)Zr_(1.4)Ta_(0.6)O_(12)(LLZTO),with high ionic conductivity,wide electrochemical window,and stability to Li metal anode,are promising solid-state electrolyte(SSEs)materials for ***,Li/LLZTO interface issues including high interface resistance,inhomogeneous Li deposition,and Li dendrite growth have hindered the practical application of ***,a multi-functional Li–SnF_(2) composite anode with Li,LiF,and Li-Sn alloy was specifically designed and *** composite anode improves the wettability to LLZTO,constructing an intimate contact interface between it and ***,ionic/electronic conductive paths in situ formed at the interface can effectively uniform Li deposition and suppress Li *** solid-state symmetric cell exhibits low interface resistance(11Ω·cm^(2)) and high critical current density(1.3 mA·cm^(−2))at 25℃.The full SSLMB based on LiFePO_(4) or Lini_(0.5)Co_(0.2)Mn_(0.3)O_(2) cathode also shows stable cycling performance and high rate *** work provides a new composite anode strategy for achieving high-energy density and high-safety SSLMBs.

关键词： Solid-state lithium metal batteries(SSLMBs) Lithium-tin fluoride anode Ionic/electronic conductive Interface resistance Lithium dendrite

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Wear-resistant Ag-MAX phase 3D interpenetrating-phase composites:Processing,structure,and properties

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Nano Research 2024年第2期17卷 806-819页

作者： Yu Guo Xi Xie Zengqian Liu Longchao Zhuo Jian Zhang Shaogang wang Qiqiang Duan qing Jia Dake Xu weihai Xue Deli Duan Filippo Berto Zhefeng Zhang Rui Yang Shi-Changxu Innovation Center for Advanced Materials Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China school of Materials Science and engineering University of Science and Technology of ChinaHefei 230026China school of Materials Science and engineering Xi’an University of TechnologyXi’an 710048China Electrobiomaterials institute Key Laboratory for Anisotropy and Texture of Materials(Ministry of Education)Northeastern UniversityShenyang 110819China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Department of Chemical engineering Materials and EnvironmentSapienza University of RomeRoma 00185Italy

electrical contact materials are generally Ag-or Cu-based composites and play a critical role in ensuring the reliability and efficiency of electrical equipments and electronic *** MAX(M is an early transition metal,A is an element from III or IV main groups,and X is carbon or/and nitrogen)phase ceramics display a unique combination of properties and may serve as an ideal reinforcement phase for electrical contact *** biological materials evolved in nature generally exhibit three-dimensional(3D)interpenetrating-phase architectures,which may offer useful inspiration for the architectural design of electrical contact ***,a series of bi-continuous Ag-Ti_(3)SiC_(2) MAX phase composites with high ceramic contents exceeding 50 vol.%and having micron-and ultrafine-scaled 3D interpenetrating-phase architectures,wherein both constituents were continuous and mutually interspersed,were exploited by pressureless infiltration of Ag melt into partially sintered Ti_(3)SiC_(2) *** mechanical and electrical properties as well as the friction and wear performance of the composites were investigated and revealed to be closely dependent on the ceramic contents and characteristic structural *** composites exhibited a good combination of properties with high hardness over 2.3 GPa,high flexural strength exceeding 530 MPa,decent fracture toughness over 10 MPa·m^(1/2),and good wear resistance with low wear rate at an order of 10^(-5)mm^(3)/(N·m),which were much superior compared to the counterparts made by powder metallurgy *** particular,the hardness,electrical conductivity,strength,and fracture toughness of the composites demonstrated a simultaneous improvement as the structure was refined from micron-to ultrafine-scales at equivalent ceramic *** good combination of properties along with the facile processing route makes the Ag-Ti_(3)SiC_(2)3D interpenetrating-phase composites appealing for electrical contact applicatio

关键词： three-dimensional(3D)interpenetrating-phase architecture Ag-MAX(M=early transition metal A=element from III or IV main groups and X=carbon or/and nitrogen)phase composites melt infiltration electrical contact materials mechanical

Analyses on an electronic voltage transformer's failure by its resonance with very fast transient overvoltage and suppression

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High Voltage 2024年第1期9卷 150-162页

作者： Ruoyu Han Houda Zhu qing Chen Hongbin Li Yue Tong Linshan Han Yang Jiao school of electrical and electronic engineering Huazhong University of Science and TechnologyWuhanChina china Electric Power Research institute WuhanChina school of Artificial Intelligence and Automation Huazhong University of Science and TechnologyWuhanChina

As voltage measuring devices are widely used in the high voltage power system with a primary-secondary-fusion structure,electronic voltage transformers are directly connected to the primary conductor and would face much more serious electromagnetic environments than general secondary *** a result,they would still experience failures even when general protection measures are adopted to suppress overvoltages'*** address this issue,an innovative method is proposed after analyses are conducted on the resonance between a transformer and an *** this method,an air-cored coil is installed in a transformer to artificially shift its natural frequency and to dodge the high-frequency dominant component of a transient overvoltage,avoiding the aforementioned resonance and suppressing the secondary *** addition,simulations and laboratory tests are conducted to prove this method's validity.

关键词： transient resonance mentioned

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构网型直驱风电机组间控制相互作用研究

电力自动化设备 2024年第3期44卷 82-90页

作者：王玉坤张慕婕李壮穆清王东泽孙海顺潘晓杰邵德军国家电网公司华中分部湖北武汉430070 中国电力科学研究院有限公司北京100192 华中科技大学电气与电子工程学院电力安全与高效湖北省重点实验室湖北武汉430074

构网型风电控制技术具有很好的弱电网适应性,可以有效避免风电并网次超同步振荡问题。但是虚拟同步控制引入固有的低频特征模式,接入强电网时会发生低频振荡,同时多台构网型风电机组并联运行时存在控制器相互作用。针对此问题,采用特征... 详细信息

构网型风电控制技术具有很好的弱电网适应性,可以有效避免风电并网次超同步振荡问题。但是虚拟同步控制引入固有的低频特征模式,接入强电网时会发生低频振荡,同时多台构网型风电机组并联运行时存在控制器相互作用。针对此问题,采用特征模式分析方法,研究了基于虚拟同步控制方法的构网型直驱风电机组并联运行时的控制相互作用及主导低频特征模式稳定性。揭示了虚拟惯量控制参数及系统运行方式对构网型风电机组并联运行低频振荡特性的影响。通过详细时域仿真验证了分析结果的正确性。

关键词：构网型直驱风电机组次同步振荡弱电网特征模式分析

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Quasi-two dimensional Ruddlesden−Popper halide perovskites for laser applications

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Frontiers of physics 2024年第2期19卷 53-71页

作者： Kun Chen Qianpeng Zhang Yin Liang Jiepeng Song Chun Li Shi Chen Fang Li qing Zhang school of Mechanical and electrical engineering Wuhan Institute of TechnologyWuhan 430205China school of Materials Science and engineering Peking UniversityBeijing 100871China institute of Applied Physics and Materials engineering Macao UniversityMacao 999078China

Quasi-two-dimensional(2D)Ruddlesden‒Popper(RP)halide perovskites,as a kind of emerged two-dimensional layered materials,have recently achieved great attentions in lasing materials field owing to their large exciton binding energy,high emission yield,large optical gain,and wide-range tuning of optical *** review will introduce research progresses of RP halide perovskites for lasing applications in aspects of materials,photophysics,and devices with emphasis on emission and lasing properties tailored by the molecular composition and *** materials,structures and fabrications are introduced in the first ***,the optical transitions and amplified spontaneous emission properties are discussed from the aspects of electronic structure,exciton,gain dynamics,and interface ***,the research progresses on lasing devices are summarized and several types of lasers including VCSEL,DFB lasers,microlasers,random lasers,plasmonic lasers,and polariton lasers are *** last,the challenges and perspectives would be provided.

关键词： two-dimensional materials metal halide perovskite Ruddlesden−Popper halide perovskites lasing emission

Emerging interactively stretchable electronics with optical and electrical dual-signal feedbacks based on structural color materials

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Nano Research 2024年第3期17卷 1837-1855页

作者： Jialin wang Kai Zhao Changqing Ye Yanlin Song school of Materials Science and engineering Suzhou University of Science and TechnologySuzhou 215009China Key Laboratory of Green Printing Institute of ChemistryChinese Academy of SciencesBeijing 100190China

The booming development of wearable devices has aroused increasing interests in flexible and stretchable *** mechanosensory functionality,these devices are highly desirable on account of their wide range of applications in electronic skin,personal healthcare,human–machine interfaces and ***,they are mostly limited by single electrical signal feedback,restricting their diverse applications in visualized mechanical *** by the mechanochromism of structural color materials,interactively stretchable electronics with optical and electrical dual-signal feedbacks are recently emerged as novel sensory platforms,by combining both of their sensing mechanisms and ***,recent studies on interactively stretchable electronics based on structural color materials are *** a brief introduction of their basic components(i.e.,stretchable electronics and mechanochromic structural color materials),two types of interactively stretchable electronics with respect to the nanostructures of mechanochromic materials are outlined,focusing primarily on their design considerations and fabrication ***,the main challenges and future perspectives of these emerging devices are discussed.

关键词： stretchable electronics structural color materials interactive sensing mechanochromism dual-signal feedbacks

助溶剂法生长的AgNbO_(3)晶体相转变特征、电学和光学性能

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物理学报 2024年第3期73卷 291-298页

作者：牛佳林董思远魏永星靳长清南瑞华杨斌西安工业大学材料与化工学院陕西省光电功能材料与器件重点实验室西安710021 陕西煤业化工技术研究院有限责任公司西安710070 科学技术部高技术研究发展中心北京100044

AgNbO_(3)具有反铁电性及高的极化强度,在智能器件领域有着重要的应用前景.本文采用助溶剂法合成了高质量的AgNbO_(3)单晶(最大尺寸5 mm×4 mm×4 mm),系统研究了其相转变特征、光学和电学性能.当AgNbO_(3)晶体处于正交M相时,保持着相... 详细信息

AgNbO_(3)具有反铁电性及高的极化强度,在智能器件领域有着重要的应用前景.本文采用助溶剂法合成了高质量的AgNbO_(3)单晶(最大尺寸5 mm×4 mm×4 mm),系统研究了其相转变特征、光学和电学性能.当AgNbO_(3)晶体处于正交M相时,保持着相同的畴结构;由M_(2)相转变至地相时,偏光显微镜(PLM)照片衬度变暗,同时电导率和介电损耗明显上升.当AgNbO_(3)单晶由M_(3)相到顺电O相时,畴结构消失;同时,表现出明显的热滞后现象,属于第一类相变.室温下,AgNbO_(3)单晶的直接带隙拟合禁带宽度为2.73 eV,略窄于AgNbO_(3)陶瓷.在临界电场以下,AgNbO_(3)单晶表现出更高的电致应变(0.076%,E_(m)=130 kV/cm).在绿色激光照射下,介电常数由70增至73,表现出明显的光致介电效应.

关键词： AgNbO_(3)单晶助溶剂法相转变特征

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