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Nanoforming of transferred metal contacts for enhanced twodimensional field effect transistors

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Nano Research 2024年第4期17卷 3210-3216页

作者： Shuoheng Xu Zheng Huang Jie guan Yaowu Hu The Institute of Technological Sciences Wuhan UniversityWuhan 430072China School of Power and Mechanical Engineering Wuhan UniversityWuhan 430072China School of Physics Southeast UniversityNanjing 211189China

Two-dimensional transition metal chalcogenides(2D-TMDs)have attracted much attention because of their unique layered structure and physical properties for transistor *** transferred metal contacts on these low-dimensional materials or their homogeneous and heterogeneous multilayers have generated huge interest to avoid deposition *** this paper,we show that there are large physical gaps at both the edge contact and surface contact between the transferred electrodes and the 2D materials.A method called laser shock induced superplastic deformation(LSISD)is proposed to tackle this issue and enhance the performance of the *** enhancement mechanism was investigated by molecular dynamics(MD)simulations of the nanoforming process,atomic force microscopy(AFM),scanning electron microscopy(SEM),transmission electron microscopy(TEM)characterizations of the interfaces,and density functional theory(DFT)*** force effect of laser shock can reduce the contact gap between metals and *** electrical performances of the transistors before and after LSISD,along with MD simulations,are used to find the optimal process *** addition,this paper applies the LSISD method to the short-channel MoS_(2)/graphene vertical transistors to show potential improvement in interface contact and electrical *** paper demonstrates the first report on using mechanical force induced by laser shock to enhance metal–semiconductor interfaces and transistor performances.

关键词： laser shock nanoforming metal-semiconductor contact electronics two-dimensional transistors

Evaluation of Auto-Ignition Characteristics of Diesel Surrogate Fuels with the Same Derived Cetane Numbers at Changed Thermodynamic Environments

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Journal of Thermal Science 2024年第4期33卷 1590-1606页

作者： ZHANG Cong guan Yuanhang HUANG Zhen HAN Dong Key Laboratory for Power Machinery and Engineering Ministry of EducationShanghai Jiao Tong UniversityShanghai200240China College of Smart Energy Shanghai Jiao Tong UniversityShanghai200240China Shanghai Non-carbon Energy Conversion and Utilization Institute Shanghai200240China

The ignition tendency of diesel fuels is highly sensitive to ambient conditions and fuel *** this study,the ignition characteristics of different diesel surrogate fuels with the same derived cetane numbers(DCN)were measured and compared in varied thermodynamic and oxidizing *** combustion pressures,heat release rates,ignition delays,and combustion delays of the test fuels were *** experimental results showed that the diesel surrogate fuels with the same DCNs exhibit similar ignition propensity at standard DCN test ***,for the test conditions of high cetane fuels,high ambient temperatures,and suficient oxygen concentrations,surrogate fuels with the same DCN have similar ignition behaviors,and using the DCN to evaluate fuel ignition tendency is ***,for the test conditions of low cetane fuels,low ambient temperatures,and reduced oxygen concentrations,different ignition behaviors are observed for the surrogate fuels with the same DCN,so at these conditions using DCN as the evaluation index for fuel ignition tendency may lead to higher uncertainty.

关键词： diesel fuels surrogate fuels derived cetane numbers constant volume combustion chamber

High-current pulsed electron beam modification on microstructure and performance of Cu/CuW diffusion bonding joints

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Rare Metals 2024年第6期43卷 2819-2831页

作者： Na-Na Tian Cong-Lin Zhang Peng Lyu Jin-Tong guan Jie Cai qing-Feng guan Shun Guo School of Materials Science and Engineering Jiangsu UniversityZhenjiang 212013China School of Material Science and Engineering Yancheng Institute of TechnologyYancheng 221051China Engineering Institute of Advanced Manufacturing and Modern Equipment Technology Jiangsu UniversityZhenjiang 212013China

This study investigates the influence of high-current pulsed electron beam(HCPEB)modification on the microstructure and shear strength of Cu/CuW *** solid-state diffusion bonding of modified-Cu(MCu)and modified-CuW(M-CuW)was achieved by HCPEB modification pretreatment at a temperature of 800-900℃and a pressure of 5 MPa for 10-50 *** demonstrate that HCPEB modification facilitates the dissolution of W and Cu,resulting in the formation of a Cu_(0.4)W_(0.6)solid solution and thus enhancing the uniform distribution of ***,HCPEB-induced defects play a beneficial role in promoting the diffusion process by providing fast diffusion paths for *** optimal joints with the maximum shear strength of 213.7 MPa were obtained through bonding M-Cu and M-CuW at 900℃and 5 MPa for 30 min,which attributes to the combined effects of fine-grained strengthening and solid solution ***,the application of HCPEB modification showcases its effectiveness in promoting element diffusion and enhancing the mechanical performance of the joints.

关键词： HCPEB Element diffusion Shear strength Crystal defects Surface modification

Flexibility potential of Cs_(2)BX_(6)(B=Hf,Sn,Pt,Zr,Ti;X=I,Br,Cl)with application in photovoltaic devices and radiation detectors

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Journal of Energy Chemistry 2024年第8期95卷 271-287,I0006页

作者： Songya Wang Changcheng Chen Shaohang Shi Ziyi Zhang Yan Cai Shuli Gao wen Chen Shuangna Guo Elyas Abduryim Chao Dong Xiaoning guan Ying Liu Gang Liu Pengfei Lu School of Science Xi’an University of Architecture and TechnologyXi’an 710055ShaanxiChina Key Laboratory of Eco Planning&Green Building Ministry of EducationTsinghua UniversityBeijing 100080China State Key Laboratory of Information Photonics and Optical Communications Beijing University of Posts and TelecommunicationsBeijing 100876China School of Physics and Optoelectronic Engineering Ludong UniversityYantai 264025ShandongChina

As interest in double perovskites is growing,especially in applications like photovoltaic devices,understanding their mechanical properties is vital for device *** extensive exploration of structure and optical properties,research on mechanical aspects is *** article builds a vacancyordered double perovskite model,employing first-principles calculations to analyze mechanical,bonding,electronic,and optical *** show Cs_(2)Hfl_(6),Cs_(2)SnBr_(6),Cs_(2)SnI_(6),and Cs_(2)PtBr_(6)have Young's moduli below 13 GPa,indicating *** parameters explain flexibility variations with the changes of B and X site *** characteristic exploration reveals the influence of B and X site electronegativity on mechanical ***_(2)SnBr_(6)and Cs_(2)PtBr_(6)are suitable for solar cells,while Cs_(2)HfI_(6)and Cs_(2)TiCl_(6)show potential for semi-transparent solar *** property calculations highlight the high light absorption coefficients of up to 3.5×10^(5) cm^(-1)for Cs_(2)HfI_(6)and Cs_(2)TiCl_(6).Solar cell simulation shows Cs_(2)PtBr_(6)achieves 22.4%of conversion ***_(2)ZrCl_(6)holds promise for ionizing radiation detection with its 3.68 eV bandgap and high absorption ***-ordered double perovskites offer superior flexibility,providing valuable insights for designing stable and flexible *** understanding enhances the development of functional devices based on these perovskites,especially for applications requiring high stability and flexibility.

关键词： Double perovskite Mechanical properties Flexible Photovoltaic Radiation detectors

Examination of two-phase behaviors in porous media during pool boiling

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Science China(Technological Sciences) 2024年第6期67卷 1695-1713页

作者： ZHANG ZhiHao guan ShuYa WU Rui ZHAO ChangYing School of Mechanical Engineering Shanghai Jiao Tong University

The enhancement of pool boiling heat transfer using porous media has been extensively *** the two-phase distribution and evolution in porous media are crucial to the heat transfer performance,including the critical heat flux(CHF)and heat transfer coefficient(HTC),direct observation of the two-phase flow inside the media is limited owing to the blockage of the direct view from the porous *** this study,pool boiling visualization experiments were conducted on porous samples with different throat widths in deionized *** results showed that the HTC increased with the throat ***,the growth-contraction cycle of the vapor region and the formation and drying of the wall liquid film inside the porous media were *** vapor region,including the maximum and minimum areas in the boiling cycle,was quantitatively ***,the relationship between the minimum gas-phase area and HTC peak was identified.A one-dimensional transient model was developed considering solid skeleton heat conduction,liquid film evaporation,and vapor region growth to quantitatively study the influence of heat flux on the internal two-phase *** model successfully captured the maximum gas-phase area,duration of boiling cycles,and HTC trends at specific heat *** results of this quantitative study provide insights into the internal two-phase distribution and evolution induced by pool boiling.

关键词： porous media two-phase behaviors pool boiling

Quasi-two-dimensional strong liquid-like dynamics of surface atoms in metallic glasses

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Science China(Physics,Mechanics & Astronomy) 2024年第3期67卷 102-109页

作者： Bing Wang Xuanqiao Gao Rui Su Pengfei guan School of Physical Science and Technology Northwestern Polytechnical UniversityXi'an 710072China Innovation Center NPU Chongqing Northwestern Polytechnical UniversityChongqing 401135China School of Mechanics Civil Engineering and ArchitectureNorthwestern Polytechnical UniversityXi'an 710072China Northwest Institute for Nonferrous Metal Research Xi'an 710016China Institute of Advanced Magnetic Materials College of Materials and Environmental EngineeringHangzhou Dianzi University Hangzhou 310018China Beijing Computational Science Research Center Beijing 100093China

The fast dynamic properties of the surface of metallic glasses(MGs) play a critical role in determining their potential applications. However, due to the significant difference in thermal history between atomic simulation models and laboratory-made samples, the atomic-scale behaviors of the fast surface dynamics of MGs in experiments remain uncertain. Herein, we prepared model MG films with notable variations in thermal stability using a recently developed efficient annealing protocol, and investigated their atomic-scale dynamics systematically. We found that the dynamics of surface atoms remain invariant, whereas the difference in dynamical heterogeneity between surface and interior regions increases with the improvement of thermal stability. This can be associated with the more pronounced correlation between atomic activation energy spectra and depth from the surface in samples with higher thermal stability. In addition, dynamic anisotropy appears for surface atoms, and their transverse dynamics are faster than normal components, which can also be interpreted by activation energy spectra. Our results reveal the presence of strong liquid-like atomic dynamics confined to the surface of laboratory-made MGs, illuminating the underlying mechanisms for surface engineering design, such as cold joining by ultrasonic vibrations and superlattice growth.

关键词： metallic glasses thermal stability invariant surface dynamics potential energy landscape dynamic anisotropy and heterogeneity

Black holes as the source of dark energy:A stringent test with high-redshift JWST AGNs

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Science China(Physics,Mechanics & Astronomy) 2024年第2期67卷 181-188页

作者： Lei Lei Lei Zu guan-wen Yuan Zhao-qiang Shen Yi-Ying Wang Yuan-Zhu Wang Zhen-Bo Su wen-Ke Ren Shao-Peng Tang Hao Zhou Chi Zhang Zhi-Ping Jin Lei Feng Yi-Zhong Fan Da-Ming Wei Key Laboratory of Dark Matter and Space Astronomy Purple Mountain ObservatoryChinese Academy of SciencesNanjing 210023China School of Astronomy and Space Science University of Science and Technology of ChinaHefei 230026China CAS Key Laboratory for Research in Galaxies and Cosmology Department of AstronomyUniversity of Science and Technology of ChinaHefei 230026China

Studies have proposed that there is evidence for cosmological coupling of black holes(BHs)with an index of k≈3;hence,BHs serve as the astrophysical source of dark ***,the data sample is limited for the redshifts of≤*** recent years,the James Webb Space Telescope(JWST)has detected many high-redshift active galactic nuclei(AGNs)and *** the JWST NIRSpec-/NIRCam-resolved AGNs,three are determined to be in early-type host galaxies with a redshift of z~***,their M_(*)and MBH are in tension with the predicted cosmological coupling of black holes with k=3 at a confidence level of~2σ,which challenges the hypothesis that BHs serve as the origin of dark *** work on high-redshift AGNs using the JWST will further assess such a hypothesis by identifying more early-type host galaxies in the higher mass range.

关键词： dark energy supermassive black hole active galactic nuclei James Webb Space Telescope

Tumor-targeted self-assembled micelles reducing PD-L1 expression combined with ICIs to enhance chemo-immunotherapy of TNBC

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Chinese Chemical Letters 2024年第2期35卷 305-310页

作者： Hongda Zhu Kai Ma Rui Ruan Chaobo Yang Aqin Yan Jing Li qi Yu Hongmei Sun Mingxing Liu Hongmei Zheng Jing Gao Xiaofang guan Zhu Dai Yao Sun Cooperative Innovation Center of Industrial Fermentation (Ministry of Education & Hubei Province) Key Laboratory of Fermentation Engineering (Ministry of Education)National “111” Center for Cellular Regulation and Molecular PharmaceuticsSchool of Food and Biological EngineeringHubei University of TechnologyWuhan 430068China Hubei Cancer Hospital Tongji Medical CollegeHuazhong University of Science and TechnologyWuhan 430079China National Key Laboratory of Green Pesticide College of ChemistryCentral China Normal UniversityWuhan 430079China Key Laboratory of Medical Optics Suzhou Institute of Biomedical Engineering and TechnologyChinese Academy of SciencesSuzhou 215163China Key Laboratory of Optic-electric Sensing and Analytical Chemistry for Life Science Ministry of EducationQingdao University of Science and TechnologyQingdao 266000China

Immune checkpoint inhibitors(ICIs)therapy targeting programmed cell death ligand 1(PD-L1)and programmed death protein 1(PD-1)had exhibited significant clinical benefits for cancer treatment such as triple negative breast cancer(TNBC).However,the relatively low anti-tumor immune response rate and ICIs drug resistance highlight the necessity of developing ICIs combination therapy strategies to improve the anti-tumor effect of ***,the immunomodulator epigallocatechin gallate palmitate(PEGCG)and the immunoadjuvant metformin(MET)self-assembled into tumor-targeted micelles via hydrogen bond and electrostatic interaction,which encapsulated the therapeutic agents doxorubicin(DOX)-loaded PEGCG-MET micelles(PMD)and combined with ICIs(anti-PD-1 antibody)as therapeutic strategy to reduce the endogenous expression of PD-L1 and improve the tumor immunosuppressive *** results presented that PMD integrated chemotherapy and immunotherapy to enhance antitumor efficacy in vitro and in vivo,compared with DOX or anti-PD-1 antibody for the therapy of *** micelles might be a potential candidate,which could remedy the shortcomings of antibody-based ICIs and provide synergistic effect to enhance the antitumor effects of ICIs in tumor therapy.

关键词： Immunotherapy Tumor-targeted Self-assembled micelles Metformin Reducing PD-L1 expression TNBC

Photothermal catalysts for efficient and clean fuel production at atmospheric pressure

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Science China Chemistry 2024年第6期67卷 1762-1764页

作者： Xinwei guan Yang Chen Tianyi Ma School of Science RMIT UniversityMelbourneVIC3000Australia Institute of Clean Energy Chemistry Key Laboratory for Green Synthesis and Preparative Chemistry of Advanced Materials of Liaoning ProvinceCollege of ChemistryLiaoning UniversityShenyang110036China

The use of waste carbon resources to produce valuable chemicals and hydrocarbon fuels has attracted great interest in recent *** a transformation not only maximises the utilisation of carbon resources but also plays a... 详细信息

关键词： thermal transformation clean