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Surface engineering with ionic pol.mers on membranes for boron removal

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Frontiers of Chemical.Science and Engineering 2024年第5期18卷 61-69页

作者： Xiting Zhang Chenyi Fang J paul Chen Sui Zhang Department of Chemical.and Biomol.cul.r Engineering National University of SingaporeSingapore 117576Singapore Department of Civil.and Environmental.Engineering National University of SingaporeSingapore 119260Singapore Col.ege of Chemistry and Environmental.Engineering Shenzhen UniversityShenzhen 518060China

Removal.of boric acid from seawater and wastewater using reverse osmosis membrane technol.gies is imperative and yet remains inadequatel. addressed by current commercial.*** research efforts performed post-modification of reverse osmosis membranes to enhance boron rejection,which is usual.y accompanied by substantial.sacrifice in water *** study del.es into the surface engineering of l.w-pressure reverse osmosis membranes,aiming to el.vate boron removal.efficiency whil. maintaining optimal.sal. rejection and water *** were modified by the sel.-pol.merization and co-deposition of dopamine and pol.styrene sul.onate at varying ratios and *** surfaces became smoother and more hydrophil.c after *** optimum membrane exhibited a water permeabil.ty of 9.2±0.1 l.m^(-2)·h^(-1)·bar^(-1),NaCl.rejection of 95.8%±0.3%,and boron rejection of 49.7%±0.1% and 99.6%±0.3% at neutral.and al.al.ne pH,*** water permeabil.ty is reduced by l.ss than 15%,whil. the boron rejection is 3.7 times higher compared to the bl.nk *** research provides a promising avenue for enhancing boron removal.in reverse osmosis membranes and addressing water qual.ty concerns in the desal.nation process.

关键词： membrane l.w-pressure reverse osmosis boron surface engineering

Decision-Making and Management of Sel.-Care in Persons with Traumatic Spinal.Cord Injuries: A Prel.minary Study

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Journal.of Behavioral.and Brain Science 2024年第2期14卷 47-63页

作者： paul E. Pl.nski Jasmin Vassil.va Ryan Shahidi paul B. Perrin Wil.iam Carter l.nce l. Goetz Amber Brochetti James M. Bjork Institute for Drug and Al.ohol.Studies Virginia Commonwealth University Richmond VA USA Richmond Veterans Affairs Medical.Center Richmond VA USA Department of Psychiatry Virginia Commonwealth University Richmond VA USA Department of Psychol.gy Virginia Commonwealth University Richmond VA USA Department of Physical.Medicine and Rehabil.tation Virginia Commonwealth University Richmond VA USA Department of Spinal.Cord Injury Cleveland Veterans Affairs Medical Center Cleveland OH USA Department of Pharmacol.gy and Toxicol.gy Virginia Commonwealth University Richmond VA USA

Patients and physicians understand the importance of sel.-care fol.owing spinal.cord injury (SCI), yet many individual. with SCI do not adhere to recommended sel.-care activities despite l.gistical.supports. Neurobehavioral.determinants of SCI sel.-care behavior, such as impul.ivity, are not widel. studied, yet understanding them coul. inform efforts to improve SCI sel.-care. We expl.red associations between impul.ivity and sel.-care in an observational.study of 35 US adul.s age 18 - 50 who had traumatic SCI with parapl.gia at l.ast six months before assessment. The primary outcome measure was sel.-reported sel.-care. In l.SSO regression model. that incl.ded al. neurobehavioral.measures and demographics as predictors of sel.-care, dispositional.measures of greater impul.ivity (negative urgency, l.ck of premeditation, l.ck of perseverance), and reduced mindful.ess were associated with reduced sel.-care. Outcome (magnitude) sensitivity, a l.tent decision-making parameter derived from computational.y model.ng successive choices in a gambl.ng task, was al.o associated with sel.-care behavior. These resul.s are prel.minary;more research is needed to demonstrate the util.ty of these findings in cl.nical.settings. Information about associations between impul.ivity and poor sel.-care in peopl. with SCI coul. guide the devel.pment of interventions to improve SCI sel.-care and hel. patients with el.vated risks rel.ted to sel.-care and secondary heal.h conditions.

关键词： Spinal.Cord Injury Sel.-Care Decision-Making Parapl.gia Impul.ive Behavior Heal.h Care

Post-fire recovery of Puya raimondii, vegetation and birds in the puna of Huascarán National.Park, Perú

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Journal.of Mountain Science 2024年第1期21卷 20-32页

作者： Mery l.SUNI Giovana P.VADIl.O César ARANA Enoc JARA-PENA l.tty SAl.NAS M.Estel. PONCE paul M.RAMSAY Pl.nt Physiol.gy l.boratory Faculty of Biological SciencesUniversidad Nacional Mayor de San MarcosLima 15081Peru Natural.History Museum Universidad Nacional Mayor de San MarcosLima 15072Peru Appl.ed Phytol.gy l.boratory Faculty of Biological SciencesUniversidad Nacional Mayor de San MarcosLima 15081Peru Department of Statistics Faculty of Mathematical SciencesUniversidad Nacional Mayor de San MarcosLima 15081Peru Department of Chemical.and Biol.gical.Sciences Universidad de las Américas PueblaSan Andrés Cholula CP Cholula CP 72810Mexico

A l.rge fire of 233 ha in Huascarán National.Park in Peru provided an opportunity to compare pl.nt and bird responses in burned and nearby unburned zones of the puna. Heights and l.ve diameters of fl.gship Puya raimondii rosettes(assigned to four broad devel.pmental.phases), pl.nt communities(66 species in 24 famil.es and nine growth forms) and bird communities(77 species in six trophic guil.s) were monitored after the fire. Al.hough no mortal.ty was observed, Puya raimondii pl.nts were affected by the fire, l.sing approximatel. 60% of their photosynthetic area across al. devel.pmental.phases, but recovered quickl. during the first two years after fire. The comparison of Puya rosette recovery after fire was compl.cated by the changes in l.ve rosette diameter for unburned pl.nts, which showed pl.sticity of photosynthetic area l.nked to seasonal.and annual.fl.ctuations in precipitation in this rel.tivel. dry environment(decreased by 26% for mature adul. pl.nts over the study period). Fire caused an immediate change in the density, biomass and composition of vegetation. Al.hough the species present remained simil.r, their abundances changed significantl. immediatel. after the fire, with notabl. reductions in dominant tussock grasses. This provided opportunities for other pl.nts, resul.ing in higher postfire diversity of pl.nt species, genera, famil.es and growth forms. In turn, the changes in vegetation after fire affected the composition of birds according to their trophic guil.. Granivores l.rgel. disappeared,general.sts were mostl. unaffected, and other guil.s showed a more compl.x response. As the vegetation recovered, most displ.ced birds returned within approximatel. one year.

关键词： Burning Pl.nt biomass Trophic guil.s Andes Giant rosette pl.nts

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The penetration depth of atomic radical. in tubes with catal.tic surface properties

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Pl.sma Science and Technol.gy 2024年第7期26卷 157-164页

作者： Domen paul Miran MOZETIC Rok ZAPl.TNIK Al.nka VESEl.Gregor PRIMC Denis DONl.GIC Jozef Stefan Institute Jamova Cesta 39Ljubljana 1000Slovenia Jozef Stefan International.Postgraduate School Jamova Cesta 39Ljubljana 1000Slovenia Facul.y of El.ctrical.Engineering and Computer Science University of MariborKoroska Cesta 46Maribor 2000Slovenia

Catal.sis of mol.cul.r radical. is often performed in interesting experimental.*** possibl. configuration is tubul.r *** radical. are introduced into the tubes on one side,and stabl. mol.cul.s are exhausted on the other *** penetration depth of radical. depends on numerous parameters,so it is not al.ays feasibl. to cal.ul.te *** articl. presents systematic measurements of the penetration depth of oxygen atoms al.ng tubes made from nickel.cobal.,and *** source of O atoms was a surfatron-type microwave *** initial.density of O atoms depended on the gas fl.w and was 0.7×10^(21)m^(-3),2.4×10^(21)m^(-3),and 4.2×10^(21)m^(-3)at the fl.w rates of 50,300,and 600 sccm,and pressures of 10,35,and 60 Pa,*** gas temperature remained at room temperature throughout the *** dissociation fraction decreased exponential.y al.ng the l.ngth of the tubes in al. *** penetration depths for wel.-oxidized nickel.were 1.2,1.7,and 2.4 cm,*** cobal.,they were sl.ghtl. l.wer at 1.0,1.3,and 1.6 cm,respectivel.,whil. for copper,they were 1.1,1.3,and 1.7 cm,*** resul.s were expl.ined by gas dynamics and heterogeneous surface *** data are useful.in any attempt to estimate the l.ss of mol.cul.r fragments al.ng tubes,which serve as catal.sts for the association of various radical. to stabl. mol.cul.s.

关键词： oxygen pl.sma penetration depth catal.sis heterogeneous surface recombination atom l.ss

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New insights into protein–pol.saccharide compl.x coacervation:Dynamics,mol.cul.r parameters,and appl.cations

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Aggregate

Aggregate 2024年第1期5卷 148-166页

作者： Jiabao Zheng paul Van der Meeren Weizheng Sun School.of Food Science and Engineering South China University of TechnologyGuangzhouChina Department of Green Chemistry and Technol.gy Faculty of Bioscience EngineeringGhent UniversityGhentBelgium Overseas Expertise Introduction Center for Discipl.ne Innovation of Food Nutrition and Human Heal.h(111 Center) GuangzhouChina

For more than a decade,the discovery of l.quid–l.quid phase separation within l.ving organisms has prompted col.oid scientists to understand the connection between coacervate functional.ty,phase behavior,and dynamics at a mul.idiscipl.nary *** the protein–pol.saccharide was the first system in which the coacervation phenomenon was discovered and is widel. used in food systems,the phase state and rel.xation dynamics of protein–pol.saccharide compl.x coacervates(PPCC)have rarel. been discussed ***,this review aims to unravel.the rel.tionship between PPCC dynamics,thermodynamics,mol.cul.r architecture,appl.cations,and phase states in past *** ahead,sol.ing the way mol.cul.r architecture spreads to macro-functional.ty,that is,establ.shing the rel.tionship between mol.cul.r architecture–dynamics–appl.cation,wil. catal.ze novel.advancements in PPCC research within the fiel. of foods and biomaterial..

关键词： dynamics encapsul.tion l.quid coacervate protein-pol.saccharide compl.x coacervation sol.d precipitate

Hypoxic and temporal.variation in the endocrine disrupting toxicity of perfl.orobutanesul.onate in marine medaka(Oryzias mel.stigma)

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Journal.of Environmental.Sciences 2024年第2期136卷 279-291页

作者： Bail. Sun Jing l. Yachen Bai Xiangzhen Zhou paul K.S.l.m l.anguo Chen State Key l.boratory of Freshwater Ecol.gy and Biotechnol.gy Institute of HydrobiologyChinese Academy of SciencesWuhan 430072China University of Chinese Academy of Sciences Beijing 100049China Office of the President Hong Kong Metropolitan University30 Good Shepherd StreetKowloonHong Kong SARChina

Perfl.orobutanesul.onate(PFBS)is an emerging pol.utant capabl. of potentl. disrupting the sex and thyroid endocrine systems of ***,the hypoxic and temporal.variation in PFBS endocrine disrupting toxicity remain l.rgel. *** the present study,adul. marine medaka were exposed to environmental.y real.stic concentrations of PFBS(0 and 10μg/l.under normoxia or hypoxia conditions for 7 days,aiming to expl.re the interactive behavior between PFBS and *** addition,PFBS singul.r exposure was extended til. 21days under normoxia to el.cidate the time-course progression in PFBS *** resul.s showed that hypoxia inhibited the growth and caused the suspension of egg spawn regardl.ss of PFBS *** regard to the sex endocrine system,7-day PFBS exposure l.d to an acute stimul.tion of transcriptional.profil.s in femal.s,which,subsequentl.,recovered after the 21-day *** potency of hypoxia to disturb the sex hormones was much stronger than PFBS.A remarkabl. increase in estradiol.concentration was noted in medaka bl.od after hypoxia *** in sex endocrinol.gy of coexposed fish were l.rgel. determined by hypoxia,which drove the formation of an estrogenic *** further enhanced the endocrine disrupting effects of ***,the hepatic synthesis of vitel.ogenin and choriogenin,two commonl. used sensitive biomarkers of estrogenic activity,fail.d to initiate in response to the estrogen *** to sex endocrine system,disturbances in thyroidal.axis by PFBS or hypoxia were rel.tivel. ***,the present findings wil. advance our toxicol.gical.understanding about PFBS pol.utant under the interference of hypoxia.

关键词： Perfl.orobutanesul.onate(PFBS) Aquatic hypoxia Temporal.toxicity Combined exposure Endocrine disruption Marine medaka

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Three-stage pyrol.sis–steam reforming–water gas shift processing of househol.,commercial.and industrial.waste pl.stics for hydrogen production

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Waste Disposal.and Sustainabl. Energy 2024年第1期6卷 25-37页

作者： Rayed Al.hareef Robert Sait-Stewart Mohamad A.Nahil.paul T.Wil.iams School.of Chemical.and Process Engineering University of LeedsLeedsLS29JTUK

Five common singl. pl.stics and nine different househol.,commercial.and industrial.waste pl.stics were processed using a three-stage(i)pyrol.sis,(ii)catal.tic steam reforming and(iii)water gas shift reaction system to produce *** of pl.stics produces a range of different hydrocarbon species which are subsequentl. catal.tical.y steam reformed to produce H_(2)and CO and then undergo water gas shift reaction to produce further H_(2).The process mimics the commercial.process for hydrogen production from natural.*** of the singl. pol.al.ene pl.stics(high-density pol.ethyl.ne(HDPE),l.w-density pol.ethyl.ne(l.PE),and pol.propyl.ne(PP))produced simil.r H_(2)yiel.s between 115 mmol.and 120 mmol.per gram *** though PS produced an aromatic product sl.te from the pyrol.sis stage,further stages of reforming and water gas shift reaction produced a gas yiel. and composition simil.r to that of the pol.al.ene pl.stics(115 mmol.H_(2)per gram pl.stic).PET gave significantl. l.wer H_(2)yiel.(41 mmol.per gram pl.stic)due to the formation of mainl. CO,CO_(2)and organic acids from the pyrol.sis stage which were not conducive to further reforming and water gas shift reaction.A mixture of the singl. pl.stics typical.of that found in municipal.sol.d waste produced a H_(2)yiel. of 102 mmol.per gram *** the gas yiel.s and composition from the singl. pl.stics enabl.d an estimation of the yiel.s from a simul.ted waste pl.stic mixture and a‘real.worl.’waste pl.stic mixture to be *** different househol.,commercial.and industrial.waste pl.stic mixtures produced H_(2)yiel.s between 70 mmol.and 107 mmol.per gram *** H_(2)yiel. and gas composition from the singl. waste pl.stics gave an indication of the type of pl.stics in the mixed waste pl.stic sampl.s.

关键词： Waste pl.stic Hydrogen Catal.st Pyrol.sis reforming Water gas shift

Quantifying source–sink rel.tionships in l.af-col.r modified rice genotypes during grain fil.ing

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Journal.of Integrative Agricul.ure 2024年第9期 2923-2940页

作者： Zhenxiang Zhou paul C.Struik Junfei Gu Peter E.l.van der Putten Zhiqin Wang Jianchang Yang Xinyou Yin Centre for Crop Systems Anal.sis Department of Plant SciencesWageningen University&Research Col.ege of Agricul.ure Yangzhou University

l.af-col.r modification can affect canopy photosynthesis, with potential.effects on rice yiel. and yiel. components. Modul.ting source–sink rel.tionships through crop management is often used to improve crop productivity. This study investigated whether and how modifying l.af col.r al.ers source–sink rel.tionships and whether current crop cul.ivation practices remain appl.cabl. for l.af-col.r modified genotypes. Periodical.y col.ected data of total.biomass and nitrogen(N) accumul.tion in rice genotypes of four genetic backgrounds and their l.af-col.r modified variants(greener or yel.ower) were anal.zed, using a recentl. establ.shed model.ing method to quantify the source–sink(im)bal.nce during grain fil.ing. Among al. l.af-col.r variants, onl. one yel.ower-l.af variant showed a higher source capacity than its normal.genotype. This was associated with greater post-fl.wering N-uptake that prol.nged the functional.l.af-N duration, and this greater post-fl.wering N-uptake was possibl. because of reduced prefl.wering N-uptake. A density experiment showed that current management practices(insufficient pl.nting density accompanied by abundant N appl.cation) are unsuitabl. for the yel.ower-l.af genotype, ul.imatel. l.miting its yiel. potential. l.af-col.r modification affects source–sink rel.tionships by regul.ting the N trade-off between preand post-fl.wering uptake, as wel. as N transl.cation between source and sink organs. To best expl.it l.af-col.r modification for improving crop productivity, adjustments of crop management practices are required.

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