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plasma-etching on monolithic MOFs-based MIM filter boosted chemical sensing

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Nano Research 2024年第4期17卷 2800-2807页

作者： Jianxi Liu Li Feng Zhihuan Li Yang Wu Feng Zhou Yadong xu Research&Development institute Northwestern Polytechnical University in ShenzhenShenzhen 518057China State Key Laboratory of Solidification processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi’an 710072China Yantai Zhongke Research institute of Advanced Materials and Green Chemical Engineering Shandong Laboratory of Advanced Materials and Green Manufacturing at YantaiYantai 264006China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

Metal-insulator-metal(MIM)cavity as a lithography-free structure to control light transmission and reflection has great potential in the field of optical ***,the dense top metal layer of the MIM prohibits any external medium from entering the dielectric insulation layer,which limits the application of the cavity in the sensing ***,we demonstrate a series of monolithic metal-organic frameworks(MOFs)based MIM cavities,which are treated by plasma etching to provide channels for chemical diffusion and to advance *** modulate the bandwidth of the MIM filters by controlling the MOF thickness as insulator *** plasma-etching is applied to build channels on the top metal layer without altering their saturation and brightness for chemical sensing *** etching time regulates the number and size of channels on the top metal *** behavior is demonstrated on the plasma-etched MOFs-based MIM cavity when external chemicals diffuse in the *** addition,we generate patterned structure of the MOFs-based MIM cavity via plasma-mask method,which can transfer to different substrates and produce a controllable structure color change for chemical *** MIM cavity may promote the advancement and applications of structural color in security imaging,color display,information anticounterfeiting,and color printing.

关键词： metal-organic frameworks(MOFs) spin-coating metal-insulator-metal filter patterns sensing

Dendrite and fractal growth of C_(60) crystals from solution

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Chinese Science Bulletin 1997年第2期42卷 112-115页

作者： YANG Guowei, XIONG Shu and HU GuobinCentre Laboratory, institute of modern physics, Xiangtan University, Xiangtan 411105, China Centre Laboratory Institute of Modem Physics Xiangtan University Xiangtan China

IN recent years, C60 molecules and fullerence as new functional material have aroused many researchers’ attention. In the full investigation of the structures, properties and potential applications of C60, the growth of large, high-quality C60 single crystals is of importance. So far,two kinds of methods have been used to grow C60 crystals: one is the growth from solution, i.e. the C60 powder is dissolved in benzene, toluene and hexane, and thus C60 crystals can be grown

关键词： C60 crystals dendrite fractal.

Microstructures and micromechanical behaviors of high -entropy alloys investigated by synchrotron X-ray and neutron diffraction techniques: A review

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International Journal of Minerals,Metallurgy and Materials 2024年第6期31卷 1333-1349页

作者： Yubo Huang Ning xu Huaile Lu Yang Ren Shilei Li Yandong Wang Beijing Advanced Innovation Center of Materials Genome Engineering State Key Laboratory for Advanced Metals and MaterialsUniversity of Science and Technology BeijingBeijing 100083China AnSteel Beijing Research institute Co.Ltd. Beijing 102200China Spallation Neutron Source Science Center Dongguan 523803China Department of physics City University of Hong KongHong Kong 999077China institute for Materials Intelligent Technology Liaoning Academy of MaterialsShenyang 110004China

High-entropy alloys(HEAs)possess outstanding features such as corrosion resistance,irradiation resistance,and good mechan-ical properties.A few HEAs have found applications in the fields of aerospace and *** studies on the deformation mech-anisms of HEAs can guide microstructure control and toughness design,which is vital for understanding and studying state-of-the-art structural *** X-ray and neutron diffraction are necessary techniques for materials science research,especially for in situ coupling of physical/chemical fields and for resolving macro/microcrystallographic information on ***,several re-searchers have applied synchrotron X-ray and neutron diffraction methods to study the deformation mechanisms,phase transformations,stress behaviors,and in situ processes of HEAs,such as variable-temperature,high-pressure,and hydrogenation *** this review,the principles and development of synchrotron X-ray and neutron diffraction are presented,and their applications in the deformation mechanisms of HEAs are *** factors that influence the deformation mechanisms of HEAs are also *** review fo-cuses on the microstructures and micromechanical behaviors during tension/compression or creep/fatigue deformation and the application of synchrotron X-ray and neutron diffraction methods to the characterization of dislocations,stacking faults,twins,phases,and intergrain/interphase stress *** on future developments of synchrotron X-ray and neutron diffraction and on research directions on the deformation mechanisms of novel metals are discussed.

关键词： high-entropy alloys microstructures micromechanical behaviors synchrotron X-ray diffraction neutron diffraction

Vulnerability assessment of UAV engine to laser based on improved shotline method

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Defence Technology（防务技术） 2024年第3期33卷 588-600页

作者： Le Liu Chengyang xu Changbin Zheng Sheng Cai Chunrui Wang Jin Guo Changchun institute of Optics Fine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China University of Chinese Academy of Sciences Beijing 100049China

Laser anti-drone technology is entering the sequence of actual combat,and it is necessary to consider the vulnerability of typical functional parts of *** the concept of"vulnerability"was proposed,a variety of analysis programs for battlefield targets to traditional weapons have been developed,but a comprehensive assessment methodology for targets'vulnerability to laser is still *** on the shotline method,this paper proposes a method that equates laser beam to shotline array,an efficient vulnerability analysis program of target to laser is established by this method,and the program includes the circuit board and the wire into the vulnerability analysis category,which improves the precision of the vulnerability *** the UAV engine part as the target of vulnerability analysis,combine with the"life-death unit method"to calculate the laser penetration rate of various materials of the UAV,and the influence of laser weapon system parameters and striking orientation on the killing probability is quantified after introducing the penetration rate into the vulnerability analysis *** quantitative analysis method proposed in this paper has certain general expansibility,which can provide a fresh idea for the vulnerability analysis of other targets to laser.

关键词： Laser weapon Laser damage Vulnerability UAV Engine Killing probability

Building stabilized Cu_(0.17)Mn_(0.03)V_(2)O_(5−□)·2.16H_(2)O cathode enables an outstanding room‐/low‐temperature aqueous Zn‐ion batteries

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Carbon Energy 2024年第8期6卷 25-35页

作者： Ao Wang Dai‐Huo Liu Lin Yang Fang xu Dan Luo Haozhen Dou Mengqin Song Chunyan xu Beinuo Zhang Jialin Zheng Zhongwei Chen Zhengyu Bai Key Laboratory of Green Chemical Media and Reactions Ministry of EducationCollaborative Innovation Center of Henan Province for Green Manufacturing of Fine ChemicalsSchool of Chemistry and Chemical EngineeringHenan Normal UniversityXinxiangHenanChina The State Key Laboratory of Catalysis(SKLC) Power Battery and System Research CenterDalian Institute of Chemical PhysicsChinese Academy of SciencesDalianChina

Vanadium oxide cathode materials with stable crystal structure and fast Zn^(2+)storage capabilities are extremely important to achieving outstanding electrochemical performance in aqueous zinc‐ion *** this work,a one‐step hydrothermal method was used to manipulate the bimetallic ion intercalation into the interlayer of vanadium *** pre‐intercalated Cu ions act as pillars to pin the vanadium oxide(V‐O)layers,establishing stabilized two‐dimensional channels for fast Zn^(2+)*** occupation of Mn ions between V‐O interlayer further expands the layer spacing and increases the concentration of oxygen defects(Od),which boosts the Zn^(2+)diffusion *** a result,as‐prepared Cu_(0.17)Mn_(0.03)V_(2)O_(5−□)·2.16H_(2)O cathode shows outstanding Zn‐storage capabilities under room‐and lowtemperature environments(e.g.,440.3 mAh g^(−1)at room temperature and 294.3 mAh g^(−1)at−60°C).Importantly,it shows a long cycling life and high capacity retention of 93.4%over 2500 cycles at 2 A g^(−1)at−60°***,the reversible intercalation chemistry mechanisms during discharging/charging processes were revealed via operando X‐ray powder diffraction and ex situ Raman *** strategy of a couple of 3d transition metal doping provides a solution for the development of superior room‐/lowtemperature vanadium‐based cathode materials.

关键词： aqueous zinc‐ion batteries Cu_(0.17)Mn_(0.03)V_(2)O_(5−□)·2.16H_(2)O oxygen defects room‐/lowtemperature performance stabilized nanostructure

pairwise entanglement and local polarization of Heisenberg model

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Science China(physics,Mechanics & Astronomy) 2008年第10期51卷 1515-1522页

作者： XI XiaoQiang1,2, ZHANG Tao3, YUE RuiHong3,4 & LIU WuMing2 1 Department of Applied Mathematics and physics, Xi’an institute of post and Telecommunications, Xi’an 710061, China 2 Beijing National Laboratory for Condensed Matter physics, institute of physics, Chinese Academy of Sciences, Beijing 100080, China 3 institute of modern physics, Northwest University, Xi’an 710069, China 4 Department of physics, Ningbo University, Ningbo 315211, China Department of Applied Mathematics and physics Xi’an Institute of Post and Telecommunications Xi’an China Beijing National Laboratory for Condensed Matter physics Institute of Physics Chinese Academy of Sciences Beijing China institute of modern physics Northwest University Xi’an China Department of physics Ningbo University Ningbo China

The characteristics of pairwise entanglement and local polarization (Lp) are dis-cussed by studying the ground state (states) of the Heisenberg XX model. The re-sults show that: the ground state (states) is (are) composed of the micro states with the minimal polarization (0 for even qubit and 1/2 for odd qubit); Lp and the prob-ability of the micro state have an intimate relation, i.e. the stronger the Lp, the smaller the probability, and the same Lp corresponds to the same probability; the pairwise entanglement of the ground state is the biggest in all eigenvectors. It is found that the pairwise entanglement is decreased by the state degeneracy and the system size. The concurrence approaches a fixed value of about 0.3412 (for odd-qubit chain) or 0.3491 (for even-qubit chain) if the qubit number is large enough.

关键词： Heisenberg XX model local polarization pairwise entanglement

Analysis of products of thymine irradiated by ^(18)O^(8+) ion beam in N_2O saturated aqueous solution

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Nuclear Science and Techniques 1999年第3期10卷 180-183页

作者： CAI Xichen WEI Zengquan LI Wenjian LIANG Jianping LI Qiang (institute of modern physics, the Chinese Academy of Sciences, Lanzhou 730000) institute of modern physics Chinese Academy of sciences Lanzhou 730000 China

Some methods of capillary gas chromatography, such as GC, GC-MS,GC-FT-IR, are used to analyze the products of thymine irradiated by 18O8+ ion beam in N2O saturated aqueous solution. From the results of GC-MS the molecular weight of products can be determined, and from the results of GC-FT-IR some molecular structure information of products can be obtained. By this way the products,5,6-Dihydrothyndne, 5-Hydroxyl-5-Methylhydantoin, 5-Hydroxyl-6-Hydrothymine, 5-Hydro-6-Hydroxylthymine, 5-Hydroxymethyluracil, Trans-Thymine glycol, Cis-Thymine glycol and dimers are determined without separation of them from samples. Though these products are as same as those products of thymine irradiated by γ rays in N2O saturated aqueous solution, the mechanism of thymine irradiated by heavy ion beam in aqueous solution is different from that by γ rays. The main products of thymine irradiated by 18O8+ ion beam in N2O saturated aqueous solution are hydroxyl adducts at 5-6 band of thymine, while the main products of thymine irradiated by γ ray in N2O saturated aqueous solution are dimers of thymine.

关键词： ^18O^8+离子束辐照胸腺碱 N2O饱和水溶液

Understanding the Interfacial Energy Structure and Electron Extraction process in Inverted Organic Solar Cells with phosphine-Doped Cathode Interlayers

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Chinese Journal of Chemistry 2024年第12期42卷 1347-1354页

作者： Yi Yang Jingwen Wang Yang Xiao Bowei xu Jianhui Hou State Key Laboratory of polymer physics and Chemistry Beijing National Laboratory for Molecular SciencesInstitute of ChemistryChinese Academy of SciencesBeijing 100190China State Key Laboratory of Chemical Resource Engineering College of Materials Science and EngineeringBeijing University of Chemical TechnologyBejing 100029China University of Chinese Academy of Sciences Beijing 100049China

Comprehensive Summary Cathode interlayers(CILs)play an essential role in achieving efficient organic solar cells(OSCs).However,the electronic structure at the electrode/CIL/active layer interfaces and the underlying mechanisms for electron collection remain unclear,which becomes a major obstacle to develop high-performance ***,we investigate the relationship of the electron collection abilities of four cross-linked and n-doped CILs(c-NDI:p0,c-NDI:p1,c-NDI:p2,c-NDI:p3)with their electronic structure of space charge region at heterojunction *** accurately calculating the depletion region width according to the barrier height,doping density and permittivity,we put forward that the optimal thickness of CIL should be consistent with the depletion region width to realize the minimum energy *** a result,the depletion region width is largely reduced from 13 nm to 0.8 nm at the indium tin oxide(ITO)/c-NDI:p0 interface,resulting in a decent pCE of 17.7%for the corresponding inverted OSCs.

关键词： Organic solar cells Cathode interlayer Depletion region width Electric conductivity Electron transport Electron transfer Electron extraction process

Towards growth of pure AB-stacked bilayer graphene single crystals

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Nano Research 2024年第5期17卷 4616-4621页

作者： Xiaowen Zhang Tao Zhou Yunlong Ren Zuo Feng Ruixi Qiao Qinghe Wang Bin Wang Jinxia Bai Muhong Wu Zhilie Tang xu Zhou Kaihui Liu Xiaozhi xu Guangdong Basic Research Center of Excellence for Structure and Fundamental Interactions of Matter Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum MaterialsSchool of PhysicsSouth China Normal UniversityGuangzhou 510006China Guangdong-Hong Kong Joint Laboratory of Quantum Matter School of PhysicsSouth China Normal UniversityGuangzhou 510006China physical Science and Engineering Division King Abdullah University of Science and TechnologyThuwal 23955–6900Saudi Arabia State Key Laboratory for Mesoscopic physics Frontiers Science Center for Nano-optoelectronicsSchool of PhysicsPeking UniversityBeijing 100871China institute for Frontier Science Nanjing University of Aeronautics and AstronauticsNanjing 210094China International Centre for Quantum Materials Collaborative Innovation Centre of Quantum MatterPeking UniversityBeijing 100871China Songshan Lake Materials Laboratory Institute of PhysicsChinese Academy of SciencesDongguan 523808China

Given its intriguing band structure and unique tunable bandgap,AB-stacked bilayer graphene has great potentials in the applications of high-end electronics,optoelectronics and *** epitaxial growth of AB-stacked single-crystal bilayer graphene films requires a strict AB-stacked lattice,identical orientations and seamless stitching of bilayer graphene ***,the particles inevitably present on the metal surface that produced during high temperature growth would induce random orientations,twisted stacking islands,and uncontrollable multilayers,which is a great challenge to ***,we propose a heat-resisting-box assisted strategy to produce nearly pure AB-stacked bilayer graphene single-crystal films on Cu/Ni(111)*** our technique,the particles on the Cu/Ni(111)surface are effectively eliminated,which greatly minimizes the occurrence of randomly twisted islands and uncontrollable *** as-grown AB-stacked bilayer graphene films show>99%alignment and>99%AB stacking *** work provides a promising method towards the growth of pure AB-stacked bilayer graphene single crystals and would accelerate its device applications.

关键词： bilayer graphene AB stacking uniform growth heat-resisting box