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Transparent, stretchable, and rapid-response humidity sensor for body-attachable wearable electronics

Nano Research 2017年第6期10卷 2021-2033页

作者： Tran Quang Trung Le Thai Duy Subramanian Ramasundaram nae-eung lee School of Advanced Materials Science & Engineering Sungkyunkwan University (SKKU) Suwon Kyunggi-do 16419 Republic of Korea Center for Water Resource Cycle Research Korea Institute of Science and Technology Hwarang-ro 14 gil Seongbuk-gu Seoul 02793 Republic of Korea SKKU Advanced Institute of Nanotechnology (SAINT) SKKU Suwon Kyunggi-do 16419 Republic of Korea Samsung Advanced Institute for Health Sciences & Technology (SAIHST) SKKU Suwon Kyunggi-do 16419 Republic of Korea

Stretchable and conformal humidity sensors that can be attached to the human body for continuously monitoring the humidity of the environment around the human body or the moisture level of the human skin can play an important role in electronic skin and personal healthcare applications. However, most stretchable humidity sensors are based on the geometric engineering of non-stretchable components and only a few detailed studies are available on stretchable humidity sensors under applied mechanical deformations. In this paper, we propose a transparent, stretchable humidity sensor with a simple fabrication process, having intrinsically stretchable components that provide high stretchability, sensitivity, and stability along with fast response and relaxation time. Composed of reduced graphene oxide-polyurethane composites and an elastomeric conductive electrode, this device exhibits impressive response and relaxation time as fast as 3.5 and 7 s, respectively. The responsivity and the response and relaxation time of the device in the presence of humidity remain almost unchanged under stretching up to a strain of 60% and after 10,000 stretching cycles at a 40% strain. Further, these stretchable humidity sensors can be easily and conformally attached to a finger for monitoring the humidity levels of the environment around the human body, wet objects, or human skin.

关键词： transparent stretchablehumidity sensor reduced graphene oxide wearable electronics body-attachable intrinsically stretchable components

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Ultra-thin vertical tft photosensor and photosynapse based on au-doped-graphene under transition metal selenide reaction

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Journal of Materials Science & Technology 2024年第16期183卷 215-222页

作者： Ting Kang Adila Rani Wanqi Ren M Junaid Sultan nae-eung lee Tae Geun Kim School of Electrical Engineering Korea UniversitySeoul 02841South Korea School of Advanced Materials Science&Engineering Sungkyunkwan UniversityGyeonggi-do 16419South Korea

The development of artificial photosensitive synapses with high sensitivity and biomimetic properties that combine innovative concepts and neuromorphic architectures is crucial to achieving highly integrated and flexible intelligent visual ***,graphene heterostructure-based photosensitive synaptic transistors have been extensively studied for this ***,compared to traditional transistors,vertical structure thin film transistors(VTFTs)with ultra-short channels and advantages,such as high integration,have yet to be investigated in photosensitive ***,we report an ultra-thin VTFT featuring a graphene/W_(x)Se_(x-1)van der Waals heterostructure that combines photonic and neuromorphic *** demonstrate a VTFT in which the channel layer is formed by covalently bonded W_(x)Se_(x-1)nanomaterials produced by introducing Se atoms on the surface of a tungsten metal thin film deposited via radio-frequency *** structure successfully simulated the main synaptic function,exhib-ited photosensitive synaptic responses to ultraviolet(λ=365 nm)light,and demonstrated highly reliable electrical ***,the incorporation of gold nanoparticles changed the photosensitive synaptic response properties of the graphene/W_(x)Se_(x-1)heterostructure from excitatory to inhibitory,show-ing a responsivity of about∼14 A W-1,which was attributed to the heterojunction interface resonant effects and efficient charge transfer induced by localized surface *** further enabled optical artificial synaptic applications while operating with low voltage spikes and low light *** work provides a novel strategy for integrating and developing biological and nano-electronic systems.

关键词： Ultra-thin Vertical TFT Au nanoparticles Photo sensor Photo responsivity Photo synapse

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A flexible magnetoelectric field-effect transistor with magnetically responsive nanohybrid gate dielectric layer

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Nano Research 2015年第10期8卷 3421-3429页

作者： Nguyen Minh Triet Tran Quang Trung Nguyen Thi Dieu Hien Saqib Siddiqui Do-ll Kim Jai Chan lee nae-eung lee SchoolofAdvancedMaterialsScienceandEngineering SungkyunkwanUniversitySuwonKyunggi-do440-746RepublicofKorea SungkyunkwanUniversity(SKKU)AdvancedInstituteofNanotechnology(SAINT) 5ungkyunkwanUniversitySuwonKyunggi-do440-746RepublicofKorea SamsungAdvancedInstituteforHealthSciencesandTechnology(SAIHST) SungkyunkwanUniversitySuwonKyunggi-do440-746RepublicofKorea

Flexible magnetoelectric （ME） materials have been studied for new applications such as memory, energy harvesters, and magnetic field sensors. Herein, with the widely studied and progressive advantages of ME phenomena in the multiferroic field, we demonstrate a new approach for utilizing flexible ME materials as gate dielectric layers in ME organic field-effect transistors （ME-OFET） that can be used for sensing a magnetic field and extracting the ME properties of the gate dielectric itself. The magnetoelectric nanohybrid gate dielectric layer comprises sandwiched stacks of magnetostrictive CoFe2O4 nanoparticles and a highly piezoelectric poly（vinylidene fluoride-co-trifluoroethylene） layer. While varying the magnetic field applied to the ME gate dielectric, the ME effect in the functional gate dielectric modulates the channel conductance of the ME-OFET owing to a change in the effective gate field. The clear separation of the ME responses in the gate dielectric layer of ME-OFET from those of the other parameters was demonstrated using the AC gate biasing method and enabled the extraction of the ME coefficient of ME materials. Additionally, the device shows high stability after cyclic bending of 10,000 cycles at a banding radius of 1.2 cm. The device has significant potential for not only the extraction of the intrinsic characterization of ME materials but also the sensing of a magnetic field in integrated flexible electronic systems.

关键词： magnetoelectric magnetostriction CoFe2O4 nanoparticles P(VDF-TrFE) organic field-effecttransistor magnetic sensor

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Field-effect transistor with a chemically synthesized MoS2 sensing channel for label-free and highly sensitive electrical detection of DNA hybridization

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Nano Research 2015年第7期8卷 2340-2350页

作者： Doo-Won lee Jinhwan lee II Yung Sohn Bo-Yeong Kim Young Min Son Hunyoung Bark JaehyuckJung Minseok Choi Tae Hyeong Kim Changgu lee nae-eung lee Department of Advanced Materials Science & Engineering Sungkyunkwan University Suwon Gyunggi-do 440-746 Republic of Korea Department of Mechanical Engineering Sungkyunkwan University Suwon Gyunggi-do 440-746 Republic of Korea SKKU Advanced Institute of Nanotechnology (SAINT) Sungkyunkwan University Suwon Gyunggi-do 440-746 Republic of Korea Samsung Advanced Institute for Health Sciences & Technology (SAIHST) Sungkyunkwan University Suwon Gyeonggi-do 440-746 Republic of Korea New Materials Team Future Device R&D Department LG Electronics Advanced Research Institute Seou1137-724 Republic of Korea These authors contributed equally to this work.

A field-effect transistor （FET） with two-dimensional （2D） few-layer MoS2 as a sensing-channel material was investigated for label-free electrical detection of the hybridization of deoxyribonucleic acid （DNA） molecules. The high-quality MoS2-channel pattern was selectively formedthrough the chemical reaction of the Mo layer with H2S gas. The MoS2 FET was very stable in an electrolyte and inert to pH changes due to the lack of oxygen-containing functionalities on the MoS2 surface. Hybridization of single-stranded target DNA molecules with single-stranded probe DNA molecules physically adsorbed on the MoS2 channel resulted in a shift of the threshold voltage （Vt,） in the negative direction and an increase in the drain current. The negative shift in Vth is attributed to electrostatic gating effects induced by the detachment of negatively charged probe DNA molecules from the channel surface after hybridization. A detection limit of 10 fM, high sensitivity of 17 mWdec, and high dynamic range of 106 were achieved. The results showed that a bio-FET with an ultrathin 2D MoS2 channel can be used to detect very small concentrations of target DNA molecules specifically hybridized with the probe DNA molecules.

关键词： two-dimensional(2D)materials, MoS2,field-effect transistor, biosensor,deoxyribonucleic acid (DNA) hybridization

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PGLYRP1 protein as a novel mediator of cellular dialogue in neuroinflammation

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Neural Regeneration Research 2025年第7期20卷 1993-1994页

作者： Anup Bhusal Won-Ha lee Kyoungho Suk Department of Pharmacology School of MedicineKyungpook National UniversityDaeguRepublic of Korea BK21 Plus KNU Biomedical Convergence Program Department of Biomedical ScienceSchool of MedicineKyungpook National UniversityDaeguRepublic of Korea School of Life Sciences BK21 plus KNU Creative BioResearch GroupKyungpook National UniversityDaeguRepublic of Korea Brain Science and Engineering Institute Kyungpook National UniversityDaeguRepublic of Korea

Neuroinflammation has been identified as a crucial element in several neurological disorders. Glial cells play a critical role in directing neuroinflammation, both in deleterious and beneficial ways.

关键词： inflammation considerably

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Single-cell and spatial omics:exploring hypothalamic heterogeneity

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Neural Regeneration Research 2025年第6期20卷 1525-1540页

作者： Muhammad Junaid Eun Jeong lee Su Bin Lim Department of Biochemistry&Molecular Biology Ajou University School of MedicineSuwonSouth Korea Department of Biomedical Sciences Graduate School of Ajou UniversitySuwonSouth Korea Department of Brain Science Ajou University School of MedicineSuwonSouth Korea

Elucidating the complex dynamic cellular organization in the hypothalamus is critical for understanding its role in coordinating fundamental body functions. Over the past decade, single-cell and spatial omics technologies have significantly evolved, overcoming initial technical challenges in capturing and analyzing individual cells. These high-throughput omics technologies now offer a remarkable opportunity to comprehend the complex spatiotemporal patterns of transcriptional diversity and cell-type characteristics across the entire hypothalamus. Current single-cell and single-nucleus RNA sequencing methods comprehensively quantify gene expression by exploring distinct phenotypes across various subregions of the hypothalamus. However, single-cell/single-nucleus RNA sequencing requires isolating the cell/nuclei from the tissue, potentially resulting in the loss of spatial information concerning neuronal networks. Spatial transcriptomics methods, by bypassing the cell dissociation, can elucidate the intricate spatial organization of neural networks through their imaging and sequencing technologies. In this review, we highlight the applicative value of single-cell and spatial transcriptomics in exploring the complex molecular-genetic diversity of hypothalamic cell types, driven by recent high-throughput achievements.

关键词： cellular diversity hypothalamus multi-omics single-cell transcriptomics spatial transcriptomics

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Landscape pattern and its effect on ecosystem functions in Seoul Metropolitan area:Urban ecology on distribution of the naturalized plant species

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Journal of Environmental Sciences 2003年第2期15卷 199-204页

作者： Sun-Kee Hong In-Ju Song Hyun-Ok Kim eung-Kyong lee Environmental Planning Institute Seoul National UniversitySeoul Development InstituteTechnical University BerlinEnvironmental Planning Institute Seoul National University Seoul 151-742 Korea Seoul 100-250 KoreaGermanySeoul 151-742 Korea

During land transformation process in the human history, naturalized plants were introduced to several land use patterns by the different ways of plant itself. Including some naturalized plants that had been contribute to land restoration, many naturalized plants have been invaded to original habitat or landscape for native plants. Once the plants were colonized, they extend their area and population size. Urban developed areas often give an important role of source habitat for naturalized plants and expanding their population size. In recent, this situation is appearing as one of environmental problems about the urban landscape management controlling the naturalized plants that invaded in the developed area and conserving the native vegetation. This paper is focusing on relationships between distribution of habitat of naturalized plants and landscape patch in urban area in Seoul. Gangdong-Gu, one of the administrative areas in Seoul was selected for this study. We examined the recent land use change using LANDSAT TM data and spreading of the representative naturalized plants (Robinia pseudoacacia and Eupatorium rugosum) by Seoul Biotope Mapping Project and field survey in 1999. As a result, these two species were often occurred in the same habitat and distributed in forest edge disturbed by man. Their distribution patterns were related to landscape indices (patch size and shape) in the forest edge.

关键词： biotope mapping ecosystem management human impact landscape pattern naturalized plants urban ecology

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Generation of brain vascular heterogeneity:recent advances from the perspective of angiogenesis

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Neural Regeneration Research 2025年第7期20卷 2013-2014页

作者： Nathanael J.lee Ryota L.Matsuoka Department of Neurosciences Lerner Research InstituteCleveland ClinicClevelandOHUSA Department of Molecular Medicine Cleveland Clinic Lerner College of MedicineCase Western Reserve UniversityClevelandOHUSA

Heterogeneous proper t i es of vascular endothelial cells in the brain:The brain displays large energy dynamics and consumption,and this high level of metabolic demands is fulfilled by a continuous supply of glucose and oxygen through its vascular *** vasculature consists of highly divergent blood vessel branches,giving rise to a dense network of capillaries that supply blood to all cells across the *** elaborated vascular network is thought to develop via angiogenesis,a process in which new blood vessels grow from pre-existing *** capillaries exhibit organotypic features distinct from other tissues and are formed primarily by two major endothelial cell(EC)types:those that form the semi-permeable blood-brain barrier(BBB)and those that develop highly permeable pores known as fenestrae(Matsuoka et al.,2022).The structural and functional differences between BBB and fenestrated vascular ECs represent a fundamental feature of brain vasculature and form the foundation for both brain function and homeostasis.

关键词： angiogenesis homeostasis network

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Development of a Powder Extruder System for Dual-pore Tissue-engineering Scaffold Fabrication

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Journal of Bionic Engineering 2019年第4期16卷 686-695页

作者： nae-Un Kang Myoung Wha Hong Young Yul Kim Young-Sam Cho Seung-Jae lee Department of Mechanical Design Engineering College of EngineeringWonkwang University460 Iksandae-roIks an Jeonbuk570-749Republic of Korea Department of Orthopedics Daejeon StMary's HospitalCatholic University of Korea64Daeheung-i Jung-guDaejeon301-723Republic of Korea

In this study,we developed a powder extruder system that can extrude and deposit powder mixtures to overcome the reported limitations of conventional dualpore scaffold manufacturing *** evaluate the extrusion and deposition capability of the powder extruder system,3D tissue-engineering scaffolds with dual-pore characteristics were fabricated with a PCL/PEO/NaCl(polycaprolactone/polyethylene oxide/sodium chloride)powder *** addition,to evaluate the fabricated scaffolds,their compressive modulus,morphology,and in-vitro cell activity were ***,it was confirmed that the proposed powder extruder system can fabricate dual-pore scaffolds with well-interconnected pores as well as arbitrary 3D shapes shown by the fabrication of a 3D femur-shape scaffold similar to the femur *** results of the cell proliferation and Cell Counting Kit-8(CCK-8)assays,DNA content analysis and viability assays confirm that the dual-pore scaffold fabricated by the powder extruder system improves cell attachment,proliferation,and viability.

关键词： dual-pore scaffold powder extruder system polycaprolactone 3D tissue-engineering scaffold

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Tailoring Light–Matter Interactions in Overcoupled Resonator for Biomolecule Recognition and Detection

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Nano-Micro Letters 2025年第1期17卷 262-280页

作者： Dongxiao Li Hong Zhou Zhihao Ren Cheng Xu Chengkuo lee Department of Electrical and Computer Engineering National University of SingaporeSingapore 117583Singapore Center for Intelligent Sensors and MEMS(CISM) National University of SingaporeSingapore 117608Singapore

Plasmonic nanoantennas provide unique opportunities for precise control of light–matter coupling in surface-enhanced infrared absorption(SEIRA)spectroscopy,but most of the resonant systems realized so far suffer from the obstacles of low sensitivity,narrow bandwidth,and asymmetric Fano resonance ***,we demonstrated an overcoupled resonator with a high plasmon-molecule coupling coefficient(μ)(OC-Hμresonator)by precisely controlling the radiation loss channel,the resonator-oscillator coupling channel,and the frequency detuning *** observed a strong dependence of the sensing performance on the coupling state,and demonstrated that OC-Hμresonator has excellent sensing properties of ultra-sensitive(7.25%nm^(−1)),ultra-broadband(3–10μm),and immune asymmetric Fano *** characteristics represent a breakthrough in SEIRA technology and lay the foundation for specific recognition of biomolecules,trace detection,and protein secondary structure analysis using a single array(array size is 100×100μm^(2)).In addition,with the assistance of machine learning,mixture classification,concentration prediction and spectral reconstruction were achieved with the highest accuracy of 100%.Finally,we demonstrated the potential of OC-Hμresonator for SARS-CoV-2 *** findings will promote the wider application of SEIRA technology,while providing new ideas for other enhanced spectroscopy technologies,quantum photonics and studying light–matter interactions.

关键词： Plasmonic nanoantennas Light-matter interaction Surface-enhanced infrared absorption Overcoupled Biosensing

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