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Multifunctional SnO_(2) QDs/MXene Heterostructures as Laminar Interlayers for Improved Polysulfide Conversion and Lithium Plating Behavior

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nano-Micro Letters 2024年第11期16卷 156-169页

作者： Shungui Deng Weiwei Sun Jiawei Tang Mohammad Jafarpour Frank nüesch Jakob Heier Chuanfang zhang College of Materials Science and Engineering Sichuan UniversityChengdu 610065People’s Republic of China Laboratory for Functional Polymers Swiss Federal Laboratories for Materials Science and Technology(EMPA)Überlandstrasse 1298600 DübendorfSwitzerland Institute of Materials Science and Engineering Ecole Polytechnique Fédérale de Lausanne(EPFL)Station 121015 LausanneSwitzerland Key Laboratory of Quantum Materials and Devices of Ministry of Education School of PhysicsSoutheast UniversityNanjing 211189People’s Republic of China SEU‑FEI nano‑Pico Center Key Laboratory of MEMS of Ministry of EducationSoutheast UniversityNanjing 210096People’s Republic of China

Poor cycling stability in lithium–sulfur(Li–S)batteries necessitates advanced electrode/electrolyte design and innovative interlayer *** catalysis has emerged as a promising approach,leveraging the adsorption and catalytic performance on lithium polysulfides(LiPSs)to inhibit LiPSs shuttling and improve redox *** this study,we report an ultrathin and laminar SnO_(2)@MXene heterostructure interlayer(SnO_(2)@MX),where SnO_(2) quantum dots(QDs)are uniformly distributed across the MXene *** combined structure of SnO_(2) QDs and MXene,along with the creation of numerous active boundary sites with coordination electron environments,plays a critical role in manipulating the catalytic kinetics of sulfur *** Li–S cell with the SnO_(2)@MX-modified separator not only demonstrates superior electrochemical performance compared to cells with a bare separator but also induces homogeneous Li deposition during *** a result,an areal capacity of 7.6 mAh cm^(-2) under a sulfur loading of 7.5 mg cm^(-2) and a high stability over 500 cycles are *** work demonstrates a feasible strategy of utilizing a laminar separator interlayer for advanced Li–S batteries awaiting commercialization and may shed light on the understanding of heterostructure catalysis with enhanced reaction kinetics.

关键词： Lithium-sulfur battery Heterogeneous catalysis Heterostructure Redox kinetics Lithium dendrites

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Physics-informed deep-learning parameterization of ocean vertical mixing improves climate simulations

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national Science Review 2022年第8期9卷 167-174页

作者： Yuchao Zhu Rong-Hua zhang James n.Moum Fan Wang Xiaofeng Li Delei Li CAS Key Laboratory of Ocean Circulation and Waves Institute of Oceanology and Center for Ocean Mega-Science Chinese Academy of Sciences Pilot national Laboratory for Marine Science and Technology (Qingdao) University of Chinese Academy of Sciences Center for Excellence in Quaternary Science and Global Change Chinese Academy of Sciences College of Earth Ocean and Atmospheric Sciences Oregon State University

Uncertainties in ocean-mixing parameterizations are primary sources for ocean and climate modeling biases. Due to lack of process understanding, traditional physics-driven parameterizations perform unsatisfactorily in the tropics. Recent advances in the deep-learning method and the new availability of long-term turbulence measurements provide an opportunity to explore data-driven approaches to parameterizing oceanic vertical-mixing processes. Here, we describe a novel parameterization based on an artificial neural network trained using a decadal-long time record of hydrographic and turbulence observations in the tropical Pacific. This data-driven parameterization achieves higher accuracy than current parameterizations, demonstrating good generalization ability under physical constraints. When integrated into an ocean model, our parameterization facilitates improved simulations in both ocean-only and coupled modeling. As a novel application of machine learning to the geophysical fluid, these results show the feasibility of using limited observations and well-understood physical constraints to construct a physics-informed deep-learning parameterization for improved climate simulations.

关键词： physics-informed deep learning climate model biases ocean vertical-mixing parameterizations long-term turbulence data artificial neural networks under physics constraint

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大学生负性情绪的隐喻接纳2周在线干预研究

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中国心理卫生杂志 2025年第1期39卷 75-80页

作者：李若楠于婉蓉张建新张文彩中国科学院心理健康重点实验室中国科学院心理研究所北京100101 中国科学院大学心理学系北京100049

目的:探讨隐喻接纳干预改善大学生负性情绪的效果。方法:112名大学生被分配至隐喻组(n=40)、非隐喻组(n=36)和空白对照组(n=36)。2个干预组接受2周在线团体干预,空白对照组不接受干预。在基线、2周干预后、1周随访和3周随访时施测广泛... 详细信息

目的:探讨隐喻接纳干预改善大学生负性情绪的效果。方法:112名大学生被分配至隐喻组(n=40)、非隐喻组(n=36)和空白对照组(n=36)。2个干预组接受2周在线团体干预,空白对照组不接受干预。在基线、2周干预后、1周随访和3周随访时施测广泛性焦虑量表-7 (GAD-7)、患者健康问卷-9 (PHQ-9)、接纳与行动问卷第二版(AAQ-Ⅱ)和自评接纳条目。结果:2周干预后,隐喻组的GAD-7、PHQ-9和AAQ-Ⅱ得分均低于基线,自评接纳得分均高于基线(均P<0.01);非隐喻组1周随访时的GAD-7得分,2周干预后和1周随访时的PHQ-9得分及2周干预后、1周随访和3周随访时的AAQ-Ⅱ得分均低于基线(均P <0.05),而2周干预后、1周随访和3周随访时的自评接纳得分均高于基线(均P<0.001)。AAQ-Ⅱ得分的减少仅对隐喻接纳干预造成的GAD-7和PHQ-9得分的减少存在中介作用(95%CI=-2.39~-0.38、-2.65~-0.44)。结论:隐喻接纳在线干预持续改善焦虑情绪的效果更优,经验性回避的减少是隐喻接纳干预改善焦虑和抑郁情绪的重要因素。

关键词：治疗性隐喻接纳干预经验性回避负性情绪大学生

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Sulfuric acid leaching kinetics of South African chromite

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International Journal of Minerals,Metallurgy and Materials 2015年第3期22卷 233-240页

作者： Qing Zhao Cheng-jun Liu Pei-yang Shi Bo zhang Mao-fa Jiang Qing-song zhang Ron Zevenhoven Henrik Saxén Key Laboratory for Ecological Metallurgy of Multimetallic Ores (Ministry of Education) Northeastern University Thermal and Flow Engineering Laboratory bo Akademi University

The sulfuric acid leaching kinetics of South African chromite was investigated. The negative influence of a solid product layer constituted of a silicon-rich phase and chromium-rich sulfate was eliminated by crushing the chromite and by selecting proper leaching con- ditions. The dimensionless change in specific surface area and the conversion rate of the chromite were observed to exhibit a proportional re- lationship. A modified shrinking particle model was developed to account for the change in reactive surface area, and the model was fitted to experimental data. The resulting model was observed to describe experimental findings very well. Kinetics analysis revealed that the leach- ing process is controlled by a chemical reaction under the employed experimental conditions and the activation energy of the reaction is 48 ***-1.

关键词： chromite ore treatment sulfuric acid leaching kinetics physical models

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Syntheses of DL-threo-Thiamphenicol via Green Oxidation

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Chemical Research in Chinese Universities 2006年第5期22卷 602-605页

作者： LIU Kai Robert Franzén YU Xiao-jing zhang Jun XU You-jun School of Pharmaceutical Engineering Shenyang Pharmaceutical University Shenyang 110016 P. R. China Institute of Materials Chemistry Tampere University of Technology Korkeakoulunkatu 8 FIN-33720 Tampere Finland

Four methyl aryl thioethers related to thiamphenicol syntheses and methyl phenyl sulfide were cleanly oxidized into methyl sulfones in high to excellent yields via catalytic green oxidation with aqueous hydrogen peroxide in combination with sodium tungstate. When the same reactions were similarly performed in the absence of the catalyst, the corresponding sulfoxides could be obtained. This viable synthetic approach for the synthesis of DL-threo-thiamphenicol is a simple procedure, which has an economic advantage in view of its application for the large-scale synthesis because it can be carried out under mild conditions.

关键词： Green oxidation Hydrogen peroxide Sodium tungstate Thiamphenicol

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Phase recovery and holographic image reconstruction using deep learning in neural networks

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Light(Science & Applications) 2017年第1期6卷 192-200页

作者： Yair Rivenson Yibo zhang Harun Günaydın Da Teng Aydogan Ozcan Electrical and Computer Engineering Department University of CaliforniaLos AngelesCA 90095USA Bioengineering Department University of CaliforniaLos AngelesCA 90095USA California nanoSystems Institute(CnSI) University of CaliforniaLos AngelesCA 90095USA Computer Science Department University of CaliforniaLos AngelesCA 90095USA Department of Surgery David Geffen School of MedicineUniversity of CaliforniaLos AngelesCA 90095USA

Phase recovery from intensity-only measurements forms the heart of coherent imaging techniques and *** this study,we demonstrate that a neural network can learn to perform phase recovery and holographic image reconstruction after appropriate *** deep learning-based approach provides an entirely new framework to conduct holographic imaging by rapidly eliminating twin-image and self-interference-related spatial *** neural network-based method is fast to compute and reconstructs phase and amplitude images of the objects using only one hologram,requiring fewer measurements in addition to being computationally *** validated this method by reconstructing the phase and amplitude images of various samples,including blood and Pap smears and tissue *** results highlight that challenging problems in imaging science can be overcome through machine learning,providing new avenues to design powerful computational imaging systems.

关键词： deep learning holography machine learning neural networks phase recovery

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Finite Element Analysis of Push-Out Test of SiC Fiber Reinforced Titanium Matrix Composites

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稀有金属材料与工程 2009年第A03期38卷 50-53页

作者： Yuan M n Yang Y Q Huang B zhang R J School of Materials Northwestern Polytechnical University Xi＇an 710072 China

Based on the interphase layer model and the spring layer model, an improved interface model was developed to evaluate the interfacial shear strength of Titanium matrix composites(TMCs) and to analyze the effects of various parameters on the interfacial properties. The results showed that the improved interface model is more suitable for calculating the interfacial properties of SiC fiber reinforced titanium matrix composites. The interfacial shear strength of SiC/Timetal-834 predicted is 500 MPa. In addition, in order to better understand the interfacial properties of composites, some push out phenomenon were analyzed.

关键词：复合材料剪切强度碳化硅纤维物理性能

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主动式气膜冷却对高超声速飞行器等离子体鞘套的影响

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中山大学学报（自然科学版）（中英文） 2025年第1期64卷 250-256页

作者：徐春光张源耕中山大学航空航天学院广东深圳518107

以钝锥模型为研究对象,采用热化学非平衡计算方法并结合可压缩n-S方程、SST k-ω湍流模型,对钝锥模型肩部台阶喷流和头部逆向喷流流场进行了数值模拟。在考虑不同喷流压强、喷口位置和数量等因素的基础上,分析了主动式气膜冷却对等离子... 详细信息

以钝锥模型为研究对象,采用热化学非平衡计算方法并结合可压缩n-S方程、SST k-ω湍流模型,对钝锥模型肩部台阶喷流和头部逆向喷流流场进行了数值模拟。在考虑不同喷流压强、喷口位置和数量等因素的基础上,分析了主动式气膜冷却对等离子体鞘套的影响。结果表明:高超声速飞行器采用主动式气膜冷却技术时,喷口的数量、位置及喷流压强对等离子体密度均具有显著的影响。肩部的切向喷流可有效抑制模型壁面附近的等离子体密度,进而可能对高频电磁波的传输和目标雷达散射截面(RCS)产生影响。头部逆向喷流可显著改变等离子体的分布情况,不同的逆向喷流参数配置会导致明显的差异。

关键词：高超声速飞行器等离子体鞘套主动式气膜冷却热化学非平衡双温模型

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A Study of Propagation in Shenzhen City

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Wuhan University Journal of natural Sciences 1999年第4期4卷 449-453页

作者： zhang Yuan-qiao zhang Li-xing Chen.zhang-you n. Alick Lu Shu Wuhan University College of Electronic Information Wuhan China (GRID:grid.49470.3e) (ISNI:***) Shenzhen Radio Manage Office Shenzhen China (GRID:grid.49470.3e)

Surveying the propagation path loss behavior of Shenzhen city and from the data recorded we can obtain the city’s path loss slopes, which can be comparatively regarded as the reliable bases of system design.

关键词： mobile radio communication multipath propagation path loss statistical model

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Delayed Bleeding of Coronary Artery after Thoracoscopic Intradiaphragmatic Bronchogenic Cyst Resection

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中国肺癌杂志 2018年第8期21卷 649-651页

作者： Yuanda CHEnG Yang GAO Abdillah n.JUMA Chunfang zhang Department of Thoracic Surgery Xiangya Hospital Central South University Changsha China Department of Surgery Kilosa Clinical Officer Training College Morogoro Tanzania

Bronchogenic cyst occurring in the diaphragm is rare and thoracoscopic cyst resection is mainly effective treatment. The coronary artery bleeding after video-assisted thoracoscopic surgery(VATS) has never been described; here we report a case of left coronary artery injury after thoracoscopic itradiaphragmatic bronchogenic cyst resection, which may be caused by metallic troca or chest tube.

关键词：肺癌患者临床治疗放射学治疗

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