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Effect of Dye Structure on the Photodegradation Kinetic Using TiO<sub>2</sub>Nanoparticles

Journal of Materials Science and Chemical Engineering 2017年第6期5卷 31-45页

作者： Hawraa Ayoub Mounir Kassir mohammad raad Houssein Bazzi Akram Hijazi Laboratory of Materials Catalysis Environment and Analytical Methods Faculty of Sciences I Lebanese University Beirut Lebanon Platform for Research and Analysis in Environmental Sciences (PRASE) Doctoral School of Science and Technology (EDST) Lebanese University Beirut Lebanon

In this study the effect of pH, adsorption behavior and the chemical struc-tures of two dyes (Methyl Orange and Bromothymol Blue) on the photo-degradation rate constant, was investigated. Adsorption isotherm shows that the adsorption amount of dyes on TiO2 surface is highly related to the pH of the solution and to the pKa of each dye. In acidic medium the adsorption percentage of Methyl Orange on TiO2 surface was 76% facing 5% for Bromothymol Blue. The kinetic study shows compatibility between the degradation rate constant and the adsorption percentage on the surface. In basic medium the adsorption percentage of Methyl orange and Bromothymol Blue is similar while the degradation rate of Methyl orange is two times faster than that of Bromothymol Blue which reveals the role of chemical structure in the photodegradation rate.

关键词： Photocatalysis Titanium Dioxide Adsorption Dyes Depollution

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Impact of climate change on hydropower generation in Rio Jubones Basin, Ecuador

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Water Science and Engineering 2018年第2期11卷 157-166页

作者： mohammad Mehedi Hasan Guido Wyseure Hydraulic Research Directorate River Research Institute Department of Earth and Environmental Sciences KU Leuven

This study attempted to use the soil and water assessment tool(SWAT), integrated with geographic information systems(GIS), for assessment of climate change impacts on hydropower generation. This methodology of climate change impact modeling was developed and demonstrated through application to a hydropower plant in the Rio Jubones Basin in Ecuador. ArcSWAT 2012 was used to develop a model for simulating the river flow. The model parameters were calibrated and validated on a monthly scale with respect to the hydro-meteorological inputs observed from 1985 to 1991 and from 1992 to 1998, respectively. Statistical analyses produced Nash-Sutcliffe efficiencies(NSEs) of 0.66 and 0.61 for model calibration and validation, respectively, which were considered acceptable. Numerical simulation with the model indicated that climate change could alter the seasonal flow regime of the basin, and the hydropower potential could change due to the changing climate in the *** analysis indicates that, though the hydropower generation will increase in the wet season, the plant will face a significant power shortage during the dry season, up to 13.14% from the reference scenario, as a consequence of a 17% reduction of streamflow under an assumption of a 2.9℃ increase in temperature and a 15% decrease in rainfall. Overall, this study showed that hydrological processes are realistically modeled with SWAT and the model can be a useful tool for predicting the impact of climate change.

关键词： SWAT Hydropower generation Climate change Sensitivity analysis Nash-Sutcliffe efficiency(NSE)

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