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Multifunctional Sodium Gluconate Electrolyte Additive Enabling Highly Reversible Zn Anodes

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Chemical Research in Chinese Universities 2024年第4期40卷 722-729页

作者： zhao Kang zhao Jianan YU meng LIU Fangming DONG yang WANG Shiwen CHENG Fangyi College of Chemistry Nankai UniversityTianjin300071P.R.China College of New Energy Zhengzhou University of Light IndustryZhengzhou450002P.R.China

Sodium gluconate(SG)is reported as an electrolyte additive for rechargeable aqueous zinc *** SG addition is proposed to modulate the nucleation overpotential and plating behaviors of Zn by forming a shielding buffer layer because of the adsorption priority and large steric hindrance effect,which contributes to limited rampant Zn^(2+)diffusion and mitigated hydrogen evolution and *** the introduction of 30 mmol/L SG in 2 mol/L ZnSO_(4)electrolyte,the Zn anode harvests a reversible cycling of 1200 h at 5 mA/cm^(2)and a high average Coulombic efficiency of Zn plating/stripping(99.6%).Full cells coupling Zn anode with V_(2)O_(5)·1.6H_(2)O or polyaniline cathode far surpass the SG additivefree batteries in terms of cycle stability and rate *** work provides an inspiration for design of a high-effective and low-cost electrolyte additive towards Zn-based energy storage devices.

关键词： Electrolyte additive Zn anode Sodium gluconate Adsorption Zn dendrite

Composite Braking Control Strategy for Electromechanical-Hydraulic Vehicles

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CSEE Journal of Power and Energy Systems 2024年第4期10卷 1722-1732页

作者： Zewen meng Jichao Hong Hongxin Zhang Tiezhu Zhang Xiaoming Xu Qinghai zhao Jian yang College of Mechanical and Electrical Engineering Qingdao UniversityQingdao 260071China Power Integration and Energy Storage Systems Engineering Technology Center(Qingdao) Qingdao 260071China School of Mechanical Engineering University of Science and Technology BeijingBeijing 100083China Shunde Graduate School of University of Science and Technology Beijing Foshan 528000China

Short driving ranges and low braking energy recovery efficiencies are two recognized technical bottlenecks to be overcome in electric vehicles. In this paper, a novel electromechanical-hydraulic coupling system is proposed and integrated as a powertrain for electric vehicles, which can assist the electric vehicle to fully utilize its braking energy. The hydraulic regenerative braking force and electric regenerative braking force can provide all the braking needs using the medium and small braking intensities. Furthermore, an improved compound brake control strategy based on the braking force distribution is proposed and simulated. The results show that under the premise of ensuring braking stability, the electromechanical-hydraulic coupling driving electric vehicle can adapt to various working conditions with excellent energy-saving results. The hydraulic accumulator recovery efficiency is above 99%, and the state of charge consumption rate of the battery pack can be reduced by more than 9%. More importantly, the proposed hybrid power system can significantly improve the driving range and energy efficiency, as well as reduce the consumers' mileage anxiety in electric vehicles.

关键词： Braking control strategy electric vehicle electromechanical-hydraulic coupling energy recovery state of charge

Mediated electron transfer process in α-MnO_(2)catalyzed Fenton-like reaction for oxytetracycline degradation

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Chinese Chemical Letters 2024年第8期35卷 367-372页

作者： Yiqian Jiang Zihan yang Xiuru Bi Nan Yao Peiqing zhao Xu meng State Key Laboratory for Oxo Synthesis and Selective Oxidation Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100049China

In Fenton-like oxidation,the catalyst directly influences the reaction mechanism for the degradation of pollutants from ***,a α-MnO_(2)catalyst(OAm-1)was synthesized via a self-assembly method with the assistance of a ***-1 possessed a large specific surface area of_(2)21 m2/g,abundant mesoporous structures and a large proportion of Mn(III).Further characterization exhibited that OAm-1 had abundant oxygen vacancies and excellent reducibility and *** adsorption and catalytic ability of OAm-1 were studied in the degradation of oxytetracycline(OTC)via the activation of hydrogen peroxide(H_(2)O_(2)).Through the radical quenching experiments,electron resonance spectroscopy(EPR),X-ray photoelectron spectroscopy(XPS)and Fourier-transform infrared spectroscopy(FT-IR)analysis,Mn(III)of OAm-1 was proved to be the active sites for the chemisorption of *** electrochemical ex-periments and analysis have shown that a process of electron transfer mediated by OAm-1 occurred be-tween the pollutant and H_(2)O_(2)during a Fenton-like *** work experimentally verifies the elec-tron transfer process dominated nonradical mechanism overα-MnO_(2),which is helpful for understanding the catalytic mechanism of the Fenton-like oxidation.

关键词： Mediated electron transfer Hydrogen peroxide Oxidative degradation Manganese oxide Fenton oxidation

Evolution of inclusions in vacuum induction melting of superalloys containing 70%return material

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Journal of Iron and Steel Research International 2024年第3期31卷 719-728页

作者： Jin-guo Gao Shu-lei yang Shu-feng yang Jing-she Li Wei Liu meng-jing zhao An-ren Wang School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083China State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Metallurgical and Building Materials Business Department China International Engineering Consulting CorporationBeijing 100048China

The variation law of inclusions type and size in the vacuum induction melting process and ingot of Ni-based superalloy containing 70%return material was studied by industrial test sampling,and the mechanism of inclusions formation was analyzed with thermodynamic *** results show that there are mainly two types of composite inclusions in the vacuum induction melting of Ni-based superalloys,which are nitride-and oxide-based composite inclusions,like Al_(2)O_(3)-SiO_(2)-Cr_(2)O_(3),TiN-(Mo,Nb)C,*** type and proportion of inclusions from the center to the edge of the vacuum induction ingot did not change *** number density of inclusions from the center to the edge of the ingot varied less,and the size of inclusions became smaller from the center to the *** addition,thermodynamic calculations show that oxides(M_(2)O_(3))are present in the liquid phase and mainly contain Al,Ti,Cr,Fe and O *** nitride consists mainly of Ti and N and contains small amounts of Cr,C,Nb,and Mo *** is consistent with the results of industrial *** the temperature decreases,the precipitation phases such as M_(2)O_(3),MN,γ,MC,δ,γ'andμphases are gradually precipitated,where oxides and nitrides are present in the liquid *** contents of O and N elements are the main influencing factors for the inclusions content and precipitation temperature;when the nitrogen content is reduced to below 0.0015%,it can make MN precipitate below the liquid-phase line.

关键词： Ni-based superalloy Vacuum induction melting Return material Inclusion Thermodynamic

Review of the application of in-situ sensing techniques to address the tea growth characteristics from leaf to field

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International Journal of Agricultural and Biological Engineering 2024年第1期17卷 1-11页

作者： Qiong Cao Chunjiang zhao Ze Xu Ping Jiang Haibin yang Xiangyu meng Guijun yang Information Technology Research Center Beijing Academy of Agriculture and Forestry SciencesBeijing 100097China College of Machnical and Electrical Engineering Hunan Agricultural UniversityChangsha 410125China Tea Research Institute of Chongqing Academy of Agricultural Sciences Chongqing 400000China

The tea plant is a valuable and evergreen crop that is extensively cultivated in China and many other ***,there is growing research interest in this *** the tea industry,it is crucial to develop rapid and non-invasive methods to evaluate tea plants in their natural *** article provides a comprehensive overview of non-invasive sensing techniques used for in-situ detection of tea *** topics covered include leaf,canopy,and field-level assessments,as well as statistical analysis techniques and characteristics specific to the ***-invasive testing technology is primarily used for monitoring and predicting tea pests and diseases,monitoring quality,and nutrients,determining tenderness and grade,identifying tea plant varieties,automatically detecting,and identifying tea buds,monitoring tea plant growth,and extracting tea garden areas through remote *** also helps to evaluate planting suitability,assess disasters,and estimate ***,the article examines the challenges and prospects of emerging techniques aimed at resolving the in-situ detection problem for tea *** can assist researchers and producers in comprehensively understanding the tea environment,quality characteristics,and growth process,thereby enhancing tea production quality,and fostering tea industry development.

关键词： non-destructive in-situ detection tea plants growth characteristics sensors

UNCONDITIONAL ERROR ANALYSIS OF VEMS FOR A GENERALIZED NONLINEAR SCHRODINGER EQUATION

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Journal of Computational Mathematics 2024年第2期42卷 500-543页

作者： meng Li Jikun zhao Shaochun Chen School of Mathematics and Statistics Zhengzhou UniversityZhengzhouHenan 450001China

In this work,we focus on the conforming and nonconforming leap-frog virtual element methods for the generalized nonlinear Schrodinger equation,and establish their unconditional stability and optimal error *** constructing a time-discrete system,the error between the solutions of the continuous model and the numerical scheme is separated into the temporal error and the spatial error,which makes the spatial error τ-*** inverse inequalities in the existing conforming and new constructed nonconforming virtual element spaces are utilized to derive the L^(∞)-norm uniform boundedness of numerical solutions without any restrictions on time-space step ratio,and then unconditionally optimal error estimates of the numerical schemes are obtained *** needs to be emphasized is that if we use the pre-existing nonconforming virtual elements,there is no way to derive the L^(∞)-norm uniform boundedness of the functions in the nonconforming virtual element spaces so as to be hard to get the corresponding inverse ***,several numerical examples are reported to confirm our theoretical results.

关键词： Conforming and nonconforming Virtual element methods Leap-frog scheme Generalized nonlinear Schrodinger system Unconditionally optimal error estimates

Attractor for the Extensible Beam Equation with Nonlocal Weak Damping on Time–Dependent Space

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Acta Mathematica Sinica,English Series 2024年第4期40卷 1115-1126页

作者： Chun Xiang zhao Feng Juan meng Institute of Applied System Analysis Jiangsu UniversityZhenjiang 212013P.R.China School of Mathematics and Physics Jiangsu University of TechnologyChangzhou 213001P.R.China

In this article,we consider the long-time behavior of extensible beams with nonlocal weak damping:ε(t)u_(tt)+Δ^(2)u-m(‖▽u‖^(2))Δu+‖u_(t)‖^(p_(u_(t)))+f(u)=h,whereε(t)is a decreasing function vanishing at *** the theory of process on time-dependent spaces,we investigate the existence of the time-dependent attractor by using the Condition(C_(t))method and more detailed *** results obtained essentially improve and complete some previous works.

关键词： Time-dependent attractor extensible beams equation nonlocal weak damping

Bioinspired design of integral molded Janus silk fibroin-MXene evaporator for efficient solar vapor generation

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Nano Research 2024年第4期17卷 2824-2835页

作者： Ling-Qing Kong Zhi-Cheng Zeng Guang-Zong Min zhao-Hui meng Guo-Qing meng Xiao-Xiao Guo Nai-Bo Lin Xiang-yang Liu The Higher Educational Key Laboratory for Biomedical Engineering of Fujian Province Research Center of Biomedical Engineering of XiamenDepartment of BiomaterialsCollege of MaterialsXiamen UniversityXiamen 361005China The State Key Laboratory of Marine Environmental Science(MEL) College of Ocean and Earth SciencesXiamen UniversityXiamen 361005China

Solar vapor generation is a promising sustainable technology that uses solar distillation to produce fresh water from seawater and wastewater,helping relieve global water resource ***,inspired by naturally grown integrally molded mulberry leaves with a Janus hydrophilic and hydrophobic structure,a novel,simple,and efficient integrated molding method is proposed to break through the limitations of the traditional split manufacturing strategy and realizes the integrated formation of Janus *** on the spontaneous sedimentation characteristics of MXene in silk fibroin solution and its regulation of mesoscopic structure and hydrophilicity of silk fibroin,layered structures with different compositions and hydrophilicities were obtained in one ***,ethanol and glutaraldehyde were added to construct a physical crystallization-chemical crosslinking dual stabilization structure in silk *** evaporator has the evaporation rate of 3.07 kg·m^(-2)·h^(-1) and the efficiency of 86.8%under 1 sun and maintains high evaporation performance under various extreme test conditions including vigorous washing,repeated compression,and high-intensity ultraviolet(UV)***,the evaporator performs well in practical application scenarios,its evaporation rate in the simulated Dead Sea seawater exceeds 2.13 kg·m^(-2)·h^(-1),and more than 99.9%of the salt,heavy metal ions,oil pollution,and dyes are purified.

关键词： silk fibroin MXene bioinspired integrated molding Janus structure solar vapor generation

Atmospheric chemistry of 2-nitrobenzaldehyde:Initiated by photo-excitation,OH-oxidation,and small TiO_(2) clusters adsorption catalysis

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Journal of Environmental Sciences 2024年第5期139卷 123-137页

作者： Feng-yang Bai Xiang-Huan Liu Ting-Ting meng Zhou Yu Yi-Chen Wang Shuang Ni Zhen zhao Institute of Catalysis for Energy and Environment College of Chemistry and Chemical EngineeringShenyang Normal UniversityShenyang 110034China

The fate of 2-nitrobenzaldehyde(2-NBA)is of interest in atmospheric chemistry as it is a semi-volatile organic compound with high *** study presents a quantum chemical study of the gas-phase reactions of 2-NBA photo-excitation and OH-oxidation in the absence and presence of small TiO_(2) *** further understand the unknown photolysis mechanism,the photo-reaction pathways of ground singlet state and the lying excited triplet state of 2-NBA were investigated including the initial and subsequent reactions of proton transfer,direct CO,NO_(2),and HCO elimination routes in the presence of O_(2) and ***,the OH-mediated degradation of 2-NBA proceeded via five H-extraction and six OH-addition channels by indirect mechanism,which follows a succession of reaction steps initiated by the formation of weakly stable intermediate *** H-extraction from the-CHO group was the dominant pathway with a negative activation energy of-1.22 kcal/*** calculated rate coefficients at 200–600 K were close to the experimental data in literature within 308-352 K,and the kinetic negative temperature independence was found in both experimental literature and computational ***,2-NBA was favored to be captured onto small TiO_(2) clusters via six adsorption configurations formed via various combination of three types of bonds of Ti…O,Ti…C,and O…H between the molecularly adsorbed 2-NBA and TiO_(2) *** indicted that the chemisorptions of aldehyde oxygen have largest *** results suggested adsorption conformations have a respectable impact on the catalysis *** study is significant for understanding the atmospheric chemistry of 2-nitrobenzaldehyde.

关键词： 2-nitrobenzaldehyde OH radical oxidation Rate coefficient Photolysis mechanism Adsorption catalysis