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Multi-electron reaction and fast Al ion diffusion of δ-MnO_(2) cathode materials in rechargeable aluminum batteries via first-principle calculations

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Chinese Chemical Letters 2024年第4期35卷 248-254页

作者： Lumin Zheng Ying bai Chuan Wu School of Materials Science&Engineering Beijing Institute of TechnologyBeijing 100081China Yangtze Delta Region Academy of Beijing Institute of Technology Jiaxing 314019China

Rechargeable aluminum batteries with multi-electron reaction have a high theoretical capacity for next generation of energy storage devices. However, the diffusion mechanism and intrinsic property of Al insertion into MnO_(2) are not clear. Hence, based on the first-principles calculations, key influencing factors of slow Al-ions diffusion are narrow pathways, unstable Al-O bonds and Mn^(3+) type polaron have been identified by investigating four types of δ-MnO_(2)(O3, O'3, P2 and T1). Although Al insert into δ-MnO_(2) leads to a decrease in the spacing of the Mn-Mn layer, P2 type MnO_(2) keeps the long(spacious pathways)and stable(2.007–2.030 A) Al-O bonds resulting in the lower energy barrier of Al diffusion of 0.56 e V. By eliminated the influence of Mn^(3+)(low concentration of Al insertion), the energy barrier of Al migration achieves 0.19 e V in P2 type, confirming the obviously effect of Mn^(3+) polaron. On the contrary, although the T1 type MnO_(2) has the sluggish of Al-ions diffusion, the larger interlayer spacing of Mn-Mn layer,causing by H_(2)O could assist Al-ions diffusion. Furthermore, it is worth to notice that the multilayer δ-MnO_(2) achieves multi-electron reaction of 3|e|. Considering the requirement of high energy density, the average voltage of P2(1.76 V) is not an obstacle for application as cathode in RABs. These discover suggest that layered MnO_(2) should keep more P2-type structure in the synthesis of materials and increase the interlayer spacing of Mn-Mn layer for providing technical support of RABs in large-scale energy storage.

关键词： Rechargeable aluminum batteries δ-MnO_(2) First-principles calculations Multi-electron reaction Diffusion mechanism

Periodontitis exacerbates pulmonary hypertension by promoting IFNγ+T cell infiltration in mice

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International Journal of Oral Science 2024年第2期16卷 359-369页

作者： Xiaoqian meng Linjuan Du Shuo Xu Lujun Zhou Boyan Chen Yulin Li Chumao Chen Huilin Ye Jun Zhang Guocai Tian Xuebing bai Ting Dong Wenzhen Lin mengjun Sun Kecong Zhou Yan Liu Wuchang Zhang Shengzhong Duan Department of Endodontics Shanghai Ninth People’s HospitalCollege of StomatologyShanghai Jiao Tong University School of MedicineShanghaiChina Laboratory of Oral Microbiota and Systemic Diseases Shanghai Ninth People’s HospitalCollege of StomatologyShanghai Jiao Tong University School of MedicineNational Center for StomatologyNational Clinical Research Center for Oral DiseasesShanghai Key Laboratory of StomatologyShanghaiChina Hongqiao International Institute of Medicine Shanghai Tongren Hospital/Faculty of Basic MedicineKey Laboratory of Cell Differentiation and Apoptosis of Chinese Ministry of EducationShanghai Jiao Tong University School of MedicineShanghaiChina Department of Orthodontics Shanghai Ninth People’s HospitalCollege of StomatologyShanghai Jiao Tong University School of MedicineShanghaiChina Department of Periodontology Shanghai Ninth People’s HospitalCollege of StomatologyShanghai Jiao Tong University School of MedicineShanghaiChina Stomatology Hospital School of StomatologyZhejiang University School of MedicineHangzhouChina

Uncovering the risk factors of pulmonary hypertension and its mechanisms is crucial for the prevention and treatment of the *** the current study,we showed that experimental periodontitis,which was established by ligation of molars followed by orally smearing subgingival plaques from patients with periodontitis,exacerbated hypoxia-induced pulmonary hypertension in ***,periodontitis dysregulated the pulmonary microbiota by promoting ectopic colonization and enrichment of oral bacteria in the lungs,contributing to pulmonary infiltration of interferon gamma positive(IFNγ^(+))T cells and aggravating the progression of pulmonary *** addition,we identified Prevotella zoogleoformans as the critical periodontitis-associated bacterium driving the exacerbation of pulmonary hypertension by periodontitis,and the exacerbation was potently ameliorated by both cervical lymph node excision and IFNγneutralizing *** study suggests a proof of concept that the combined prevention and treatment of periodontitis and pulmonary hypertension are necessary.

关键词： hypertension prevention interferon

On Linear Homogeneous Biwave Equations

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Journal of Partial Differential Equations 2024年第1期37卷 59-87页

作者： bai Yaqian Department of Mathematics Zhejiang Sci-Tech UniversityHangzhou 310018China.

The biwave maps are a class of fourth order hyperbolic *** this paper,we are interested in the solution formulas of the linear homogeneous biwave *** on the solution formulas and the weighted energy estimate,we can obtain the L∞(R^(n))−WN,1(R^(n))and L∞(R^(n))−WN,2(R^(n))estimates,*** our results,we find that the biwave maps enjoy some different properties compared with the standard wave equations.

关键词： Biwave maps Duhamel’s principle Fourier transform Cauchy peoblem deacy estimate.

Infrared radiation characteristics of dagger-type hypersonic missile

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Chinese Journal of Aeronautics 2024年第4期37卷 137-150页

作者： Xubo DU Qingzhen YANG Haoqi YANG Jin bai Yongqiang SHI School of Power and Energy Northwestern Polytechnical UniversityXi’an 710129China

Hypersonic vehicles emit strong infrared radiation from their high-temperature exhaust plume and body, which is critical for infrared early warning, tracking, and guidance. In this work, a comprehensive analysis is conducted on the factors involved in air dissociation reaction within the shock layer of hypersonic missile heads, as well as the multi-component afterburning effect of the exhaust plume. A novel Reverse Monte Carlo Method(RMCM) is proposed for infrared radiation calculation, which utilizes two-dimensional Low-Discrepancy Sequences(LDS) to improve computational accuracy. The numerical calculations for a dagger-type missile show that afterburning reactions increase the temperature on the centerline of the outlet exhaust plume by about 1000 K. The total infrared radiation intensity of the missile is the highest in the 1–3 μm band, with the hightemperature wall of the nozzle being the primary source of solid radiation, and gas radiation primarily coming from H_(2)O. The radiation intensity of the missile exhaust plume in the 3–5 μm band is the highest, with radiation sources primarily coming from CO_(2), CO, and HCl. Afterburning reactions of the exhaust plume increase the total infrared radiation intensity of the missile by about 0.7times. These results can provide reference for the detection and guidance of hypersonic missiles.

关键词： Hypersonic vehicles Infrared radiation Monte Carlo methods Low-discrepancy sequences Exhaust plume Afterburning

A cloud-edge-device collaborative offloading scheme with heterogeneous tasks and its performance evaluation

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Frontiers of Information Technology & Electronic Engineering 2024年第5期25卷 664-684页

作者： Xiaojun bai Yang ZHANG Haixing WU Yuting WANG Shunfu JIN School of Information Science and Engineering Yanshan UniversityQinhuangdao 066004China Key Laboratory for Computer Virtual Technology and System Integration of Hebei Province Yanshan UniversityQinhuangdao 066004China

How to collaboratively offload tasks between user devices,edge networks(ENs),and cloud data centers is an interesting and challenging research *** this paper,we investigate the offoading decision,analytical modeling,and system parameter optimization problem in a collaborative cloud-edge device environment,aiming to trade off different performance *** to the differentiated delay requirements of tasks,we classify the tasks into delay-sensitive and delay-tolerant *** meet the delay requirements of delay-sensitive tasks and process as many delay-tolerant tasks as possible,we propose a cloud-edge device collaborative task offoading scheme,in which delay-sensitive and delay-tolerant tasks follow the access threshold policy and the loss policy,*** establish a four-dimensional continuous-time Markov chain as the system *** using the Gauss-Seidel method,we derive the stationary probability distribution of the system ***,we present the blocking rate of delay-sensitive tasks and the average delay of these two types of *** experiments are conducted and analyzed to evaluate the system performance,and numerical simulations are presented to evaluate and validate the effectiveness of the proposed task offloading ***,we optimize the access threshold in the EN buffer to obtain the minimum system cost with different proportions of delay-sensitive tasks.

关键词： Edge computing Ofloading scheme Cloud-edge device collaboration Markov chain Cost function

Advances in sodium-ion batteries at low-temperature: Challenges and strategies

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Journal of Energy Chemistry 2024年第3期90卷 518-539,I0012页

作者： Haoran bai Xiaohui Zhu Huaisheng Ao Guangyu He Hai Xiao Yinjuan Chen Key Laboratory of Advanced Catalytic Materials and Technology Advanced Catalysis and Green Manufacturing Collaborative Innovation CenterChangzhou UniversityChangzhou 213164JiangsuChina Department of Chemistry Tsinghua UniversityBeijing 100084China

With the continuing boost in the demand for energy storage,there is an increasing requirement for batteries to be capable of operation in extreme environmental ***-ion batteries(SIBs) have emerged as a highly promising energy storage solution due to their promising performance over a wide range of temperatures and the abundance of sodium resources in the earth's *** to lithiumion batteries(LIBs),although sodium ions possess a larger ionic radius,they are more easily desolvated than lithium *** rthermore,SIBs have a smaller Stokes radius than lithium ions,resulting in improved sodium-ion mobility in the ***,SIBs demonstrate a significant decrease in performance at low temperatures(LT),which constrains their operation in harsh weather *** the increasing interest in SIBs,there is a notable scarcity of research focusing specifically on their mechanism under LT *** review explores recent research that considers the thermal tolerance of SIBs from an inner chemistry process perspective,spanning a wide temperature spectrum(-70 to100℃),particularly at LT *** addition,the enhancement of electrochemical performance in LT SIBs is based on improvements in reaction kinetics and cycling stability achieved through the utilization of effective electrode materials and electrolyte ***,the safety concerns associated with SIBs are addressed and effective strategies are proposed for mitigating these ***,prospects conducted to extend the environmental frontiers of commercial SIBs are discussed mainly from three viewpoints including innovations in materials,development and research of relevant theoretical mechanisms,and intelligent safety management system establishment for larger-scale energy storage SIBs.

关键词： Low-temperature Sodium-ion batteries Reaction kinetics Cycle stability Safety concerns of Sodium-ion batteries

Observing eddy dye patches induced by shear instabilities in the surf zone on a plane beach

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Acta Oceanologica Sinica 2024年第3期43卷 15-29页

作者： Chunping Ren Nannan Fu Chong Yu Yuchuan bai Kezhao Fang State Key Laboratory of Hydraulic Engineering Simulation and Safety Tianjin UniversityTianjin 300072China College of Water Resource Science and Engineering Taiyuan University of TechnologyTaiyuan 030024China State Key Laboratory of Coastal and Offshore Engineering Dalian University of TechnologyDalian 116024China

The effects of surf zone eddy generated by alongshore currents on the deformation and transport of dye are still poorly understood,and related tracer release experiments are ***,a tracer release laboratory experiment was conducted under monochromatic,unidirectional incident waves with a large incident angle(30°)on a plane beach with a 1:100 slope in a large wave basin.A charge-coupled device suspended above the basin recorded the dye patch *** evolution of eddy dye patch was observed and the transport and diffusion were analyzed based on the collected ***,a linear instability numerical model was adopted to calculate the perturbation velocity field at the initial *** observation and image processing results show that surf zone eddy patches occurred and were separated from the original dye *** numerical analysis results demonstrate that the structure of the perturbation velocity field is consistent with the experimental observations,and that the ejection of eddy patches shoreward or offshore may be ascribed to the double vortex.

关键词： surf zone tracer release experiment evolution of eddy patch shear instability of alongshore currents

Unbound^(28)O,the heaviest oxygen isotope observed:a cutting-edge probe for testing nuclear models

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Nuclear Science and Techniques 2024年第2期35卷 1-2页

作者： Jian-Guo Li bai-Shan Hu Shuang Zhang Fu-Rong Xu School of Physics and State Key Laboratory of Nuclear Physics and TechnologyPeking UniversityBeijing 100871China Institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China Southern Center for Nuclear-Science Theory(SCNT) Institute of Modern PhysicsChinese Academy of SciencesHuizhou 516000China

The beyond-dripline oxygen isotopes^(27,28)O were recently observed at RIKEN,and were found to be unbound decaying into^(24)O by emitting *** unbound feature of the heaviest oxygen isotope,^(28)O,provides an excellent test for stateof-the-art nuclear *** atomic nucleus is a self-organized quantum manybody system comprising specific numbers of protons Z and neutrons N.

关键词： testing quantum system

On the electric behaviour of conductive grease inside the contact zone

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Friction 2024年第4期12卷 683-697页

作者： Yuxin ZHOU Jinjie LIU Xinming LI He CHONG Bo HAN Qinghua bai SKF(Shanghai)Automotive Technologies Co. Ltd.Shanghai 201814China School of Mechanical and Automotive Engineering Qingdao University of TechnologyQingdao 266250China

Conductive grease has been considered as a potential solution in addressing electric erosion issue inside motor *** the conductive grease performance,especially the electric and tribological behaviour is crucial for its *** paper combines bulk grease characterization and contact film study considering both electrical and tribological loading *** results show that the electric performance for the selected conductive grease sample is electric field dependent,including both frequency and voltage *** film impedance inside the contact area is closely related to the external electric field,running condition,and lubrication *** following film impedance calculation tells that not only bulk grease electric parameters,but the contact parameter,lubricant film contour and lubrication condition should be considered when performing the overall bearing electrical modelling.

关键词： Electric erosion lubricant conductivity grease film impedance