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Hydration lubrication modulated by water structure at TiO2–aqueous interfaces

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Friction 2024年第4期12卷 591-605页

作者： Pingsu ma yuan LIU Ke HAN Yu tian Liran ma State Key Laboratory of Tribology in Advanced Equipment Department of Mechanical EngineeringTsinghua UniversityBeijing 100084China

The nature of solid-liquid interfaces is of great significance in *** advances have been made in lubrication based on hydration ***,a detailed molecular-level understanding is still ***,we investigated water molecule behaviors at the TiO2-aqueous interfaces by the sum-frequency generation vibrational spectroscopy(SFG-VS)and atomic force microscope(AFM)to elucidate the fundamental role of solid-liquid interfaces in *** contributions of water structures and hydration effects were revealed,where water structures played the dominant role in lubrication for TiO2 surfaces of varying hydrophilicity,while hydration effects dominated with the increasing of ion *** lubrication is observed on the initial TiO2 surfaces with strongly H-bonded water molecules compared to the hydrophilic TiO2 surfaces with more disordered *** stable ordered water arrangement with strong hydrogen bonds and the shear plane occurring between the ordered water layer and subsequent water layer may play a significant role in achieving lower *** adsorbed hydrated molecules with the increasing ionic concentration perturb ordered water but lead to the enhancement of hydration effects,which is the main reason for the improved lubrication for both *** work provides more insights into the detailed molecular-level understanding of the mechanism of hydration lubrication.

关键词： hydration lubrication interfacial water structures hydration effects titanium dioxide(TiO2)

Additives strategies to improving cycling stability of Li metal batteries by modifying electrode electrolyte interphases

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Progress in Natural Science:materials International 2024年第2期34卷 338-344页

作者： yuan Li Pengfei Huang Chunyu Cui Xiaoyuan ma Li Chen Zekun Li Linhai Li Yuhong tian School of Biological and Chemical Engineering Guangxi University of Science and Technology School of College of Chemistry and Chemical Engineering Hunan University Isky Future energy institute

Li metal batteries（LMBs） have attracted much attention due to the ultra-high theoretical capacity of the Li metal anode（Lma）.However,the uncontrollable dendrites growth and low coulombic efficiency hinder their practical ***,we explore 3,5-difluoropyridine（2F-BD） as a novel electrolyte additive to enable highperformance *** 2F-BD additive participates in and modifies the solvation structure of Li ions by reducing the coordinated number of PF6-at the electrode surface,leading to the formation of a LiF and Li3N-rich solid electrolyte interphase（SEI）.The LiF component increases the robustness of SEI and suppresses the formation of Li dendrites,while the Li3N component facilitates the transportation and reaction kinetics of Li *** a result,the Li‖Li symmetric cell presents a stable cycling performance of up to 500 h at a current density of 1 ma *** coupling with LiFePO4cathode,the obtained full cell achieves high specific capacities of 106.06 ma h g-1and 84.98 ma h g-1at 2.55 ma cm-2and 5.10 ma cm-2,respectively,and maintains a high capacity retention of84.0% after 1000 cycles at 0.13 ma cm-2,with an average cycling CE of 99.58%.

关键词： Li metal batteries Li dendrites Electrolyte additive LiF and Li3N-Rich electrode-electrolyte interphase LiFePO4 cathode

Advance and Application of Single‑cell Transcriptomics in Auditory Research

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Neuroscience Bulletin 2024年第7期40卷 963-980页

作者： Xiangyu ma Jiamin Guo Mengyao tian Yaoyang Fu Pei Jiang yuan Zhang Renjie Chai State Key Laboratory of Digital Medical Engineering Department of Otolaryngology Head and Neck SurgeryZhongda HospitalSchool of Life Sciences and TechnologyAdvanced Institute for Life and HealthJiangsu Province High‑Tech Key Laboratory for Bio‑Medical ResearchSoutheast UniversityNanjing 210096China Department of Psychiatry Affiliated Hangzhou First People’s HospitalZhejiang University school of MedicineHangzhou 310030China Department of Otolaryngology Head and Neck Surgery Affiliated Drum Tower Hospital of Nanjing University Medical SchoolJiangsu Provincial Key Medical Discipline(Laboratory)NanjingChina Research institute of Otolaryngology Nanjing 210008China Department of Otolaryngology Head and Neck Surgery Sichuan Provincial People’s HospitalUniversity of Electronic Science and Technology of ChinaChengdu 610072China Co‑Innovation Center of Neuroregeneration Nantong UniversityNantong 226001China institute for Stem Cell and Regeneration Chinese Academy of ScienceBeijing 101408China beijing Key Laboratory of Neural Regeneration and Repair Capital Medical UniversityBeijing 100069China

Hearing loss and deafness,as a worldwide disability disease,have been troubling human ***,the auditory organ of the inner ear is highly heterogeneous and has a very limited number of cells,which are largely uncharacterized in ***,with the development and utilization of single-cell RNA sequencing(scRNA-seq),researchers have been able to unveil the complex and sophisticated biological mechanisms of various types of cells in the auditory organ at the single-cell level and address the challenges of cellular heterogeneity that are not resolved through by conventional bulk RNA sequencing(bulk RNAseq).Herein,we reviewed the application of scRNA-seq technology in auditory research,with the aim of providing a reference for the development of auditory organs,the pathogenesis of hearing loss,and regenerative *** about spatial transcriptomic scRNA-seq,single-cell based genome,and Live-seq technology will also be discussed.

关键词： Single-cell RNA sequencing Inner ear Cochlear Auditory sensory epithelium Spiral ganglion neuron

Artemordins A-S, Cadinane-Type Sesquiterpenoid Dimers from Artemisia ordosica and Their Antihepatoma Activities

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Chinese Journal of Chemistry 2024年第13期42卷 1493-1508页

作者： yuan Wang tian-Ze Li Yun-Bao ma Chang-An Geng Yong-Cui Wang Ji-Jun Chen State Key Laboratory of Phytochemistry and Plant Resources in West china Kunming Institute of BotanyChinese Academy of SciencesKunmingYunnan 650201China University of Chinese Academy of Sciences Beijing 100049China

Nineteen new cadinane-involving sesquiterpenoid dimers,artemordins A-S(1-—19),together with 13 known SDs(20-32)were isolated from Artemisia *** structures and absolute configurations were established by comprehensive spectral analyses,X-ray single crystal diffraction,theoretical ECD,and NMR ***,artemordins A-F(1—6)were the first examples of two cadinane units constructed by unprecedented C-3−C-15′or C-3−C-13′single bond with an oxido-rearranged 6/5/6/6 fused ring system;artemordins G-K(7-11)were biogenetically connected by[4+2]cycloaddition reaction and artemordins G-J(7-10)possessed a novel 5/6/6/6/6/6/5-heptacyclic fused ring *** L-S(12-19)were formed by esterification,which involved three different types of *** assay suggested that the most active compounds,artemordins B and H(2 and 8),exhibited inhibitory activities on three hepatoma cell lines with IC50 values of 26.9 and 25.1μmol/L(HepG2),29.5 and 18.3μmol/L(Huh7),19.7 and 15.7μmol/L(SK-Hep-1).

关键词： Artemisia ordosica Artemordins A-s Cadinane-type sesquiterpenoid dimers Antihepatoma activities Terpenoids Natural products Cytotoxicity

Random Phase Approximation in Relativistic Approach

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原子核物理评论 2009年第S1期26卷 49-54页

作者： ma Zhong-yu1,2,YANG Ding1,tian yuan1,CAO Li-gang2,3(1 china institute of atomic energy,beijing 102413.china 2 Center of Theoretical Nuclear Physics,National Laboratory of Heavy Ion Research Facility in Lanzhou,Lanzhou 730000,china 3 institute of Modern Physics,Chinese Academy of Sciences,Lanzhou 730000,china) china institute of atomic energy Beijing 102413China Center of Theoretical Nuclear Physics National Laboratory of Heavy Ion Research Facility in LanzhouLanzhou 730000China china institute of atomic energy Beijing 102413China Center of Theoretical Nuclear Physics National Laboratory of Heavy Ion Research Facility in LanzhouLanzhou 730000China institute of Modern Physics Chinese Academy of SciencesLanzhou 730000China

Some special issues of the random phase approximation(RPA) in the relativistic approach are reviewed. A full consistency and proper treatment of coupling to the continuum are responsible for the successful application of the RPA in the description of dynamical properties of finite nuclei. The fully consistent relativistic RPA(RRPA) requires that the relativistic mean filed (RMF) wave function of the nucleus and the RRPA correlations are calculated in a same effective Lagrangian and the consistent treatment of the Dirac sea of negative energy states. The proper treatment of the single particle continuum with scattering asymptotic conditions in the RMF and RRPA is discussed. The full continuum spectrum can be described by the single particle Green's function and the relativistic continuum RPA is established. A separable form of the paring force is introduced in the relativistic quasi-particle RPA.

关键词： fully consistent RRPA coupling to the continuum pairing correlation

Short-term displacement prediction for newly established monitoring slopes based on transfer learning

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china Geology 2024年第2期7卷 351-364页

作者： yuan tian Yang-landuo Deng Ming-zhi Zhang Xiao Pang Rui-ping ma Jian-xue Zhang institute of Remote Sensing and Geographical Information Systems Peking UniversityBeijing 100871China beijing Key Laboratory of Spatial Information Integration and Its Applications Beijing 100871China institute of Public Safety Research Department of Engineering PhysicsTsinghua UniversityBeijing 100084China china institute of Geo-Environment Monitoring Beijing 100081China Technology Innovation Center for Geohazard Monitoring and Risk Early Warning Ministry of Natural ResourcesBeijing 100081China

This study makes a significant progress in addressing the challenges of short-term slope displacement prediction in the Universal Landslide Monitoring Program,an unprecedented disaster mitigation program in china,where lots of newly established monitoring slopes lack sufficient historical deformation data,making it difficult to extract deformation patterns and provide effective predictions which plays a crucial role in the early warning and forecasting of landslide hazards.A slope displacement prediction method based on transfer learning is therefore ***,the method transfers the deformation patterns learned from slopes with relatively rich deformation data by a pre-trained model based on a multi-slope integrated dataset to newly established monitoring slopes with limited or even no useful data,thus enabling rapid and efficient predictions for these ***,as time goes on and monitoring data accumulates,fine-tuning of the pre-trained model for individual slopes can further improve prediction accuracy,enabling continuous optimization of prediction results.A case study indicates that,after being trained on a multi-slope integrated dataset,the TCN-Transformer model can efficiently serve as a pretrained model for displacement prediction at newly established monitoring *** three-day average RMSE is significantly reduced by 34.6%compared to models trained only on individual slope data,and it also successfully predicts the majority of deformation *** fine-tuned model based on accumulated data on the target newly established monitoring slope further reduced the three-day RMSE by 37.2%,demonstrating a considerable predictive *** conclusion,taking advantage of transfer learning,the proposed slope displacement prediction method effectively utilizes the available data,which enables the rapid deployment and continual refinement of displacement predictions on newly established monitoring slopes.

关键词： Landslide Slope displacement prediction Transfer learning Integrated dataset Transformer Pre-trained model Universal Landslide Monitoring Program(ULMP) Geological hazards survey engineering

Study of proton resonances in ^(18)Ne via resonant elastic scattering of ^(17)F+p and its astrophysical implication

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Science china(Physics,Mechanics & Astronomy) 2011年第S1期54卷 32-36页

作者： HE JianJun1, HU Jun1,2, XU ShiWei1, CHEN ZhiQiang1, ZHANG XueYing1, WANG JianSong1, YU XiangQing1, ZHANG LiYong1,2, LI Long1,2, YANG YanYun1,2, ma Peng1,2, ZHANG XueHeng1, HU ZhengGuo1, GUO ZhongYan1, XU Xing1,2, yuan XiaoHua1, LU Wan1,2, YU YuHong1, ZANG YongDong1,2, TANG ShuWen1,2, YE RuiPing1,2, CHEN JinDa1,2, JIN ShiLun1,2, DU ChengMing1,2, WANG ShiTao1,2, ma JunBing1,2, LIU LongXiang1,2, BAI Zhen1,2, LEI XiangGuo1, SUN ZhiYu1, ZHANG YuHu1, ZHOU XiaoHong1, XU HuShan1, SU Jun3, LI ErTao3, WANG HongWei4, tian WenDong4 & LI XiangQing5 1 institute of Modern Physics (IMP), Chinese Academy of Sciences, Lanzhou 730000, china 2 Graduate University of Chinese Academy of Sciences, beijing 100049, china 3 china institute of atomic energy (CIAE), beijing 102413. china 4 Shanghai institute of Applied Physics (SINAP), Chinese Academy of Sciences, Shanghai 201800, china 5 School of Physics and State Key Laboratory of Nuclear Physics and Technology, Peking University, beijing 100871, china 1. institute of Modern Physics (IMP) Chinese Academy of Sciences Lanzhou 730000 China2. Graduate University of Chinese Academy of Sciences Beijing 100049 China3. China Institute of Atomic Energy (CIAE) Beijing 102413 China4. Shanghai Institute of Applied Physics (SINAP) Chinese Academy of Sciences Shanghai 201800 China5. School of Physics and State Key Laboratory of Nuclear Physics and Technology Peking University Beijing 100871 China

The proton resonant properties in 18Ne, which determine the reaction rate of the key stellar 14O(α,p)17F reaction, have been studied by using a technique of proton resonant elastic scattering of 17F+p. A 4.22 MeV/nucleon 17F radioactive ion (RI) beam was produced via a projectile-fragmentation reaction, and separated by a Radioactive Ion Beam Line in Lanzhou (RIBLL). By bombarding a thick (CH2)n target, the energy spectra of the recoiled protons were measured by two ΔE-E silicon telescopes at the center-of-mass scattering angles of θc.m.≈175°±5°, θc.m.≈152°±8°, respectively. Several proton resonances in 18Ne were ob served clearly. A further R-matrix analysis of the experimental data is under way to determine the resonant parameters. The present work reports the preliminary results briefly.

关键词： resonant reaction reaction rate explosive burning accreting binary systems

Whole-genome resequencing of Hu sheep identifies candidate genes associated with agronomic traits

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Journal of Genetics and Genomics 2024年第8期51卷 866-876页

作者： Liming Zhao Lvfeng yuan Fadi Li Xiaoxue Zhang Huibin tian Zongwu ma Deyin Zhang Yukun Zhang yuan Zhao Kai Huang Xiaolong Li Jiangbo Cheng Dan Xu Xiaobin Yang Kunchao Han Xiuxiu Weng Weimin Wang State Key Laboratory of Herbage Improvement and Grassland Agro-Ecosystems Key Laboratory of Grassland Livestock Industry InnovationMinistry of Agriculture and Rural AffairsEngineering Research Center of Grassland IndustryMinistry of EducationCollege of Pastoral Agriculture Science and TechnologyLanzhou UniversityLanzhouGansu 730020China Lanzhou Veterinary Research institute Chinese Academy of Agricultural SciencesLanzhouGansu 730046China College of Animal Science and Technology Gansu Agricultural UniversityLanzhouGansu 730070China

The phenotypic diversity resulting from artificial or natural selection of sheep has made a significant contribution to human *** sheep are a local sheep breed unique to china with high reproductive rates and rapid *** selection signatures have been widely used to investigate the genetic mechanisms underlying phenotypic variation in ***,we conduct whole-genome sequencing of 207 Hu sheep and compare them with the wild ancestors of domestic sheep(Asiatic mouflon)to investigate the genetic characteristics and selection signatures of Hu *** on six signatures of selection approaches,we detect genomic regions containing genes related to reproduction(BMPR1B,BMP2,PGFS,CYP19,CAMK4,GGT5,and GNAQ),vision(ALDH1A2,SAG,and PDE6B),nervous system(NAV1),and immune response(GPR35,SH2B2,PIK3R3,and HRAS).Association analysis with a population of 1299 Hu sheep reveals that those missense mutations in the GPR35(GPR35 g.952651 A>G;GPR35 g.952496 C>T)and NAV1(NAV1 g.84216190 C>T;NAV1 g.84227412 G>A)genes are significantly associated(P<0.05)with immune and growth traits in Hu sheep,*** research offers unique insights into the selection characteristics of Hu sheep and facilitates further genetic improvement and molecular investigations.

关键词： Hu sheep Whole-genome resequencing Selection signature GPR35 NAV1 Single nucleotide polymorphism

Experimental study of the influencing factors and mechanisms of the pressure-reduction and augmented injection effect by nanoparticles in ultra-low permeability reservoirs

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Petroleum Science 2024年第3期21卷 1915-1927页

作者： Pan Wang Yu-Hang Hu Liao-yuan Zhang Yong Meng Zhen-Fu ma tian-Ru Wang Zi-Lin Zhang Ji-Chao Fang Xiao-Qiang Liu Qing You Yan Zhang beijing Key Laboratory of Unconventional Natural Gas Geological Evaluation and Development Engineering China University of Geosciences(Beijing)Beijing100083China School of energy Resources China University of Geosciences(Beijing)Beijing100083China Petroleum Engineering Technology Research institute Sinopec Shengli Oilfield CompanyDongying257000ShandongChina Hekou Oil Production Plant Sinopec Shengli Oilfield CompanyDongying257200ShandongChina Petroleum Exploration and Production Research institute SINOPECBeijing102206China CNPC Engineering Technology R&D Company Limited Beijing102206China

Nanoparticles(NPs)have gained significant attention as a functional material due to their ability to effectively enhance pressure reduction in injection processes in ultra-low permeability *** are typically studied in controlled laboratory conditions,and their behavior in real-world,complex environments such as ultra-low permeability reservoirs,is not well understood due to the limited scope of their *** study investigates the efficacy and underlying mechanisms of NPs in decreasing injection pressure under various injection conditions(25—85℃,10—25 MPa).The results reveal that under optimal injection conditions,NPs effectively reduce injection pressure by a maximum of 22.77%in core *** pressure reduction rate is found to be positively correlated with oil saturation and permeability,and negatively correlated with temperature and ***,particle image velocimetry(PIV)experiments(25℃,atmospheric pressure)indicate that the pressure reduction is achieved by NPs through the reduction of wall shear resistance and wettability *** work has important implications for the design of water injection strategies in ultra-low permeability reservoirs.

关键词： Nanoparticle Pressure reduction Augmented injection Ultra-low permeability reservoir