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道路沥青紫外老化及抗老化材料研究综述

材料导报 2024年第1期38卷 44-56页

作者：孔令云席晗重庆交通大学土木工程学院重庆400074 重庆交通大学交通土建工程材料国家地方联合工程实验室重庆400074

道路沥青材料在使用过程中由于长期受到太阳光紫外辐射作用会产生紫外老化现象,并且这种现象在紫外辐射强度高的地区更明显。紫外老化会使沥青的物理特性和化学组成发生改变,从而导致沥青黏塑性上升、低温和疲劳性能下降、使用裂缝增加... 详细信息

道路沥青材料在使用过程中由于长期受到太阳光紫外辐射作用会产生紫外老化现象,并且这种现象在紫外辐射强度高的地区更明显。紫外老化会使沥青的物理特性和化学组成发生改变,从而导致沥青黏塑性上升、低温和疲劳性能下降、使用裂缝增加,进而劣化路面的耐久性、影响沥青路面的运营品质和服役寿命。为了防止和延缓紫外老化的产生和发展,可在道路沥青中添加抗老化材料以增强其抵御紫外老化能力,同时延长沥青路面的使用寿命并降低其性能的衰变速率。本文阐述了基于自由基和胶体理论的紫外老化机理;从处理方式、光源与辐射强度选择等方面介绍了室内模拟老化试验条件;总结了紫外老化对沥青物理和流变性能、组分构成、微观形貌、特征峰和官能团等宏微观特性的影响;归纳了现行抗老化材料的优缺点和使用情况。分析表明后期可在老化机理深度、试验方法标准化、室外老化监测、微观数值模拟、抗紫外老化剂针对性和抑制紫外老化措施等方面开展进一步研究。

关键词：道路沥青紫外老化老化机理室内模拟老化沥青特性影响抗紫外老化材料

Emerging two-dimensional Mo-based materials for rechargeable metal-ion batteries:Advances and perspectives

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Journal of Energy Chemistry 2024年第2期89卷 487-518,I0012页

作者： Qingqing Ruan Yuehua Qian Mengda Xue lingyun Chen Qichun Zhang Department of Applied Chemistry School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 401331China Department of Materials Science and Engineering City University of Hong Kong999077Hong KongChina

With the rapid development of rechargeable metal-ion batteries(MIBs)with safety,stability and high energy density,significant efforts have been devoted to exploring high-performance electrode materials.In recent years,two-dimensional(2D)molybdenum-based(Mo-based)materials have drawn considerable attention due to their exceptional characteristics,including low cost,unique crystal structure,high theoretical capacity and controllable chemical compositions.However,like other transition metal compounds,Mo-based materials are facing thorny challenges to overcome,such as slow electron/ion transfer kinetics and substantial volume changes during the charge and discharge processes.In this review,we summarize the recent progress in developing emerging 2D Mo-based electrode materials for MIBs,encompassing oxides,sulfides,selenides,carbides.After introducing the crystal structure and common synthesis methods,this review sheds light on the charge storage mechanism of several 2D Mo-based materials by various advanced characterization techniques.The latest achievements in utilizing 2D Mo-based materials as electrode materials for various MIBs(including lithium-ion batteries(LIBs),sodium-ion batteries(SIBs)and zinc-ion batteries(ZIBs))are discussed in detail.Afterwards,the modulation strategies for enhancing the electrochemical performance of 2D Mo-based materials are highlighted,focusing on heteroatom doping,vacancies creation,composite coupling engineering and nanostructure design.Finally,we present the existing challenges and future research directions for 2D Mo-based materials to realize high-performance energy storage systems.

关键词： Molybdenum-based materials Two-dimensional materials Lithium-ion batteries Sodium-ion batteries Zinc-ion batteries

Environmentally persistent free radicals in PM_(2.5)from a typical Chinese industrial city during COVID-19 lockdown:The unexpected contamination level variation

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Journal of Environmental Sciences 2024年第1期135卷 424-432页

作者： lingyun Wang Wuduo Zhao Peiru Luo Qingyun He Wenfen Zhang Chuan Dong Yanhao Zhang College of Chemistry Zhengzhou UniversityZhengzhou 450001China Center of Advanced Analysis and Gene Sequencing Key Laboratory of Molecular Sensing and Harmful Substances Detection TechnologyZhengzhou UniversityZhengzhou 450001China State Key Laboratory of Environmental and Biological Analysis Department of ChemistryHong Kong Baptist UniversityHong Kong 999077China Institute of Environmental Science Shanxi UniversityTaiyuan 030006China

The outbreak of COVID-19 has caused concerns globally.To reduce the rapid transmission of the virus,strict city lockdown measures were conducted in different regions.China is the country that takes the earliest home-based quarantine for people.Although normal industrial and social activities were suspended,the spread of virus was efficiently controlled.Simultaneously,another merit of the city lockdown measure was noticed,which is the improvement of the air quality.Contamination levels of multiple atmospheric pollutants were decreased.However,in this work,24 and 14 air fine particulate matter(PM_(2.5))samples were continuously collected before and during COVID-19 city lockdown in Linfen(a typical heavy industrial city in China),and intriguingly,the unreduced concentration was found for environmentally persistent free radicals(EPFRs)in PM_(2.5)after normal life suspension.The primary non-stopped coal combustion source and secondary Cu-related atmospheric reaction may have impacts on this phenomenon.The cigarette-based assessment model also indicated possible exposure risks of PM_(2.5)-bound EPFRs during lockdown of Linfen.This study revealed not all the contaminants in the atmosphere had an apparent concentration decrease during city lockdown,suggesting the pollutants with complicated sources and formation mechanisms,like EPFRs in PM_(2.5),still should not be ignored.

关键词： PM_(2.5) EPFRs COVID-19 City lockdown Health risks

The interaction between KIF21A and KANK1 regulates dendritic morphology and synapse plasticity in neurons

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Neural Regeneration Research 2025年第1期20卷 209-223页

作者： Shi-Yan Sun lingyun Nie Jing Zhang Xue Fang Hongmei Luo Chuanhai Fu Zhiyi Wei Ai-Hui Tang Hefei National Research Center for Physical Sciences at the Microscale CAS Key Laboratory of Brain Function and DiseaseMinistry of Education Key Laboratory for Membrane-less Organelles and Cellular DynamicsDivision of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefeiAnhui ProvinceChina Institute of Artificial Intelligence Hefei Comprehensive National Science CenterHefeiAnhui ProvinceChina CAS Center for Excellence in Molecular Cell Sciences Division of Life Sciences and MedicineUniversity of Science and Technology of ChinaHefeiAnhui ProvinceChina Department of Neurobiology School of Life SciencesSouthern University of Science and TechnologyShenzhenGuangdong ProvinceChina Brain Research Center Southern University of Science and TechnologyShenzhenGuangdong ProvinceChina

Morphological alterations in dendritic spines have been linked to changes in functional communication between neurons that affect learning and memory.Kinesin-4 KIF21A helps organize the microtubule-actin network at the cell cortex by interacting with KANK1;however,whether KIF21A modulates dendritic structure and function in neurons remains unknown.In this study,we found that KIF21A was distributed in a subset of dendritic spines,and that these KIF21A-positive spines were larger and more structurally plastic than KIF21A-negative spines.Furthermore,the interaction between KIF21A and KANK1 was found to be critical for dendritic spine morphogenesis and synaptic plasticity.Knockdown of either KIF21A or KANK1 inhibited dendritic spine morphogenesis and dendritic branching,and these deficits were fully rescued by coexpressing full-length KIF21A or KANK1,but not by proteins with mutations disrupting direct binding between KIF21A and KANK1 or binding between KANK1 and talin1.Knocking down KIF21A in the hippocampus of rats inhibited the amplitudes of long-term potentiation induced by high-frequency stimulation and negatively impacted the animals’cognitive abilities.Taken together,our findings demonstrate the function of KIF21A in modulating spine morphology and provide insight into its role in synaptic function.

关键词： actin cytoskeleton dendrite KANK1 KIF21A microtubule spine morphology spine synaptic plasticity talin1

基于集料力学特征与级配分形的沥青混合料抗滑衰变预测

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Journal of Southeast University(English Edition) 2024年第1期40卷 58-67页

作者：孔令云曾启岚张政奇彭毅王大为余苗战友重庆交通大学交通土建工程材料国家地方联合工程实验室重庆400074 重庆交通大学土木工程学院重庆400074 重庆交通大学交通运输学院重庆400074 哈尔滨工业大学交通科学与工程学院哈尔滨150090 西南交通大学土木工程学院成都610031

以粗集料的力学指标、分形维数以及BPN作为研究对象进行数据采集,基于前馈神经网络算法与支持向量机算法,提出了一种新型路面抗滑性能预测模型.采用加速加载试验,记录沥青混合料在轮载作用下表面抗滑性能的衰减过程,并利用指数模型对轮... 详细信息

以粗集料的力学指标、分形维数以及BPN作为研究对象进行数据采集,基于前馈神经网络算法与支持向量机算法,提出了一种新型路面抗滑性能预测模型.采用加速加载试验,记录沥青混合料在轮载作用下表面抗滑性能的衰减过程,并利用指数模型对轮载次数与BPN的数值关系进行拟合.通过灰色关联度分析和相关性分析,评估各项因素对沥青路面抗滑性的影响程度.基于主成分分析结果,设计了6种方案,用于前馈神经网络算法和支持向量机算法的训练、验证和测试.结果表明,不同类型集料呈现出不同的抗滑性能,石英砂岩最佳,玄武岩次之,石灰岩较差.磨光值与沥青抗滑性能衰减模型的关联性最高.前馈神经网络算法构建的模型表现更为稳定,R 2值约为0.8,展现出良好的预测能力.

关键词：加速加载抗滑性能指数模型前馈神经网络支持向量机

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新型高强度钛合金切削刀具技术研究

工具技术 2024年第1期58卷 106-109页

作者：姜怡君孔繁锦王伟赵凌云中航西安飞机工业集团股份有限公司

针对TB18航空结构件在实际加工过程中加工效率低、刀具寿命短等问题,开展TB18材料与通用钛合金材料的切削过程对比试验,分析影响刀具切削性能的关键因素,并结合具体的加工需求,通过典型刀具选型改进、新型刀具研制和切削参数优化,提高T... 详细信息

针对TB18航空结构件在实际加工过程中加工效率低、刀具寿命短等问题,开展TB18材料与通用钛合金材料的切削过程对比试验,分析影响刀具切削性能的关键因素,并结合具体的加工需求,通过典型刀具选型改进、新型刀具研制和切削参数优化,提高TB18材料加工效率,延长刀具使用寿命。

关键词： TB18钛合金刀具选型刀具寿命加工效率参数优化

Comparing 11 early warning scores and three shock indices in early sepsis prediction in the emergency department

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World Journal of Emergency Medicine 2024年第4期15卷 273-282页

作者： Rex Pui Kin Lam Zonglin Dai Eric Ho Yin Lau Carrie Yuen Ting Ip Ho Ching Chan lingyun Zhao Tat ChiTsang Matthew Sik Hon Tsui Timothy Hudson Rainer Department of Emergency Medicine School of Clinical MedicineLi Ka Shing Faculty of Medicinethe University of Hong KongHong KongChina School of Public Health Li Ka Shing Faculty of Medicinethe University of Hong KongHong KongChina Accident and Emergency Department Queen Mary HospitalHong KongChina

BACKGROUND:This study aimed to evaluate the discriminatory performance of 11 vital sign-based early warning scores(EWSs)and three shock indices in early sepsis prediction in the emergency department(ED).METHODS:We performed a retrospective study on consecutive adult patients with an infection over 3 months in a public ED in Hong kong.The primary outcome was sepsis(Sepsis-3 definition)within 48 h of ED presentation.Using c-statistics and the DeLong test,we compared 11 EWSs,including the National Early Warning Score 2(NEWS2),Modified Early Warning Score,and Worthing Physiological Scoring System(WPS),etc.,and three shock indices(the shock index[SI],modified shock index[MSI],and diastolic shock index[DSI]),with Systemic Inflammatory Response Syndrome(SIRS)and quick Sequential Organ Failure Assessment(qSOFA)in predicting the primary outcome,intensive care unit admission,and mortality at different time points.RESULTS:We analyzed 601 patients,of whom 166(27.6%)developed sepsis.NEWS2 had the highest point estimate(area under the receiver operating characteristic curve[AUROC]0.75,95%CI 0.70-0.79)and was significantly better than SIRS,qSOFA,other EWSs and shock indices,except WPS,at predicting the primary outcome.However,the pooled sensitivity and specificity of NEWS2≥5 for the prediction of sepsis were 0.45(95%CI 0.37-0.52)and 0.88(95%CI 0.85-0.91),respectively.The discriminatory performance of all EWSs and shock indices declined when used to predict mortality at a more remote time point.CONCLUSION:NEWS2 compared favorably with other EWSs and shock indices in early sepsis prediction but its low sensitivity at the usual cut-off point requires further modification for sepsis screening.

关键词： Sepsis Emergency department Clinical prediction rule Early warning score Shock index

MSCs-laden injectable self-healing hydrogel for systemic sclerosis treatment

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Bioactive Materials 2022年第11期7卷 369-378页

作者： Min Nie Bin kong Guopu Chen Ying Xie Yuanjin Zhao lingyun Sun Department of Rheumatology and Immunology Institute of Translational MedicineThe Affiliated Drum Tower Hospital of Nanjing University Medical SchoolNanjing210002China Department of Neurosurgery Health Science CenterThe First Affiliated Hospital of Shenzhen UniversityShenzhen Second People’s HospitalShenzhen518035China State Key Laboratory of Quality Research in Chinese Medicines Macao University of Science and TechnologyTaipaMacao(SAR)China State Key Laboratory of Bioelectronics School of Biological Science and Medical EngineeringSoutheast UniversityNanjing210096China

As a novel cellular therapy, the anti-inflammatory and immunomodulatory virtues of mesenchymal stem cells (MSCs) make them promising candidates for systemic sclerosis (SSc) treatment. However, the clinical efficacy of this stratagem is limited because of the short persistence time, poor survival, and engraftment of MSCs after injection in vivo. Herein, we develop a novel MSCs-laden injectable self-healing hydrogel for SSc treatment. The hydrogel is prepared using N, O-carboxymethyl chitosan (CS-CM) and 4-armed benzaldehyde-terminated poly-ethylene glycol (PEG-BA) as the main components, imparting with self-healing capacity via the reversible Schiff-base connection between the amino and benzaldehyde groups. We demonstrate that the hydrogel laden with MSCs not only promoted the proliferation of MSCs and increased the cellular half-life in vivo, but also improve their immune-modulating functions. The tube formation assay indicates that the MSCs could significantly pro-mote angiopoiesis. Moreover, the MSCs-laden hydrogel could inhibit fibrosis by modulating the synthesis of collagen and ameliorate disease progression in SSc disease model mice after subcutaneous injection of bleo-mycin. All these results highlight this novel MSCs-laden hydrogel and its distinctive functions in treatment of chronic SSc, indicating the additional potential to be used widely in the clinic.

关键词： Mesenchymal Stem cell Injectable Self-healing Hydrogel Systemic sclerosis

Modeling turbulent transport effects on kernel formation and ?ame propagation in an ignition process

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Chinese Journal of Aeronautics 2019年第4期32卷 895-905页

作者： Linghan kong Zhuyin REN lingyun HOU School of Aerospace Engineering Tsinghua University

Reliable relighting is crucial for advanced low-emission aero-engine combustors. For forced ignition under highly-turbulent conditions, eddies of sizes being smaller than the flame kernel can affect its formation through penetrating and modifying the kernel structure. In this study, a one-dimensional model for small-scale turbulence on kernel formation is developed through the incorporation of turbulence-induced diffusion in governing equations. With given flow conditions,the spatial and time-dependent turbulent diffusivity is modeled using the idea of residual eddy viscosity. One-dimensional spherical flames of premixed pre-vaporized n-dodecane/air mixtures under high-altitude conditions are simulated to investigate the effects of turbulence. It is revealed that the range of the equivalence ratio for successful turbulent ignition is much narrower than that for laminar ignition. The range decreases with an increased turbulent intensity, and this effect is more pronounced for a low spark energy. In addition, turbulent transport has more pronounced effects on rich mixtures. An analysis on energy budget and species profiles shows that turbulence-induced diffusion enhances the heat loss at the very beginning of the kernel formation process that could lead to ignition failure. After the flame kernel is established, turbulent transport broadens the flame front, enhances the heat release rate, and thereafter increases the flame propagation speed.

关键词： Flame kernel Flame propagation High-altitude ignition Kernel formation probability Turbulence-induced diffusion