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Micro-strain regulation strategy to stabilize perovskite lattice based on the categories and impact of strain on perovskite solar cells

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Journal of Energy Chemistry 2025年第1期100卷 578-604页

作者： Caixia Li Wenwu Liu Shiji Da lingbin kong Fen Ran State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of Technology School of Materials Science and Engineering Lanzhou University of Technology

Photovoltaic metal halide perovskite solar cells(PSCs) convert light to electricity more efficiently than crystalline silicon cells, and the cost of materials used to make them is lower than that of silicon *** efficiency is not a core issue affecting the application of perovskite solar cells in special *** present, stability is the major technical encounters that hinders its further commercial development. Microstrain in PSCs is currently a significant factor responsible for the device's instability. Strain-induced ion migration is widely believed to accelerate perovskite degradation even when external stimuli are ***, it is imperative to study strain to enhance the stability of PSCs. This paper reviews recent developments to understand strain's origin and effect mechanisms on performance of PSCs, including ion migration,failure behavior, defect formation, and its effect on photoelectric properties, stability, and ***, several well-known strain management strategies are systematically introduced based on the strain effect mechanism and strain engineering on the film, providing more clues for further preparation with increased stability. The manipulation of external physical strain applied from films to entire devices has been extensively studied. Furthermore, recommendations for future research directions and chemical approaches have been provided. It is emphasized that strain engineering plays a crucial role in improving the efficiency and longevity of PSCs. Tensile strain causes rapid degradation, while moderate compressive strain and external strain control could improve properties and stability. Efforts should focus on controlling compressive strain to mitigate residual tensile strain and introducing it in a controlled manner. Future research endeavors may focus on exploring these pathways to improve the efficiency and lifespan of PSCs.

关键词： Halide perovskite solar cells Strain origins Strain effects Strain management

Biotransformation of 4-Hydroxybenzen Derivatives by Hairy Root Cultures of Polygonum multiflorum Thunb

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Journal of Integrative Plant Biology 2007年第2期49卷 207-212页

作者： Chun-Yan Yan rong-Min Yu Zhang Zhang ling-Yi kong Department of Natural Medicinal Chemistry College of Traditional Chinese Medicines China Pharmaceutical University Nanjing 210038 China Department of Natural Medicinal Chemistry and Pharmacognosy College of Pharmacy Jinan University Guangzhou 510632 China

The biotransformation of four 4-hydroxybenzen derivatives （1,4-benzenediol （compound 1）, 4-hydroxybenzaldehyde （compound 2）, 4-hydroxybenzyl alcohol （compound 3） and 4-hydroxybenzoic acid （compound 4）） by the hairy root cultures of Polygonum multiflorum Thunb. as a new biocatalyst was investigated. It was found that the substrates were transformed to their corresponding glucosides, 4-hydroxyphenyl β-D-glucopyranoside （arbutin, compound la）, 4-hydroxymethylphenyl β-D-glucopyranoside （gastrodin, compounds 2a, 3a） and 4-carboxyphenyl α-D- glucopyranoside （compound 4a）, respectively. In the meantime, the hairy roots of P. multiflorum were able to stereoselectively and regioselectively glucosylate phenolic hydroxyl groups of compounds 1-4, but the cultures could not glucosylate the aldehyde group of compound 2 or the benzyllc hydroxyl group of compound 3, and no glucosyl esterification of carboxyl groups of compound 4 was detected. On the other hand, the result also showed that the hairy roots of P. multiflorum were able to reduce the 4-hydroxybenzaldehyde to its corresponding alcohol. This is the first report that substrate 4 has been converted into its α-D-glucopyranoside by a plant biotransformα- tion system.

关键词： 4-hydroxybenzen derivatives arbutin biotransformation gastrodin hairy root cultures Polygonum multiflorum.

A low redox potential and long life organic anode material for sodium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 557-564页

作者： Zhi Li Yang Wei Kang Zhou Xin Huang Xing Zhou Jie Xu Taoyi kong Junwei Lucas Bao Xiaoli Dong Yonggang Wang Department of Chemistry and Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials Institute of New Energy Collaborative Innovation Center of Chemistry for Energy Materials (iChEM) Fudan University Department of Chemistry Boston College School of Materials Science and Engineering Anhui University of Technology

Sodium-ion batteries （SIBs） with organic electrodes are an emerging research direction due to the sustainability of organic materials based on elements like C,H,O,and sodium ***,organic electrode materials for SIBs are mainly used as cathodes because of their relatively high redox potentials（>1 V）.Organic electrodes with low redox potential that can be used as anode are ***,a novel organic anode material （tetrasodium 1,4,5,8-naphthalenetetracarboxylate,Na4TDC） has been developed with low redox potential （ling stability for 1200 cycles even with a high mass loading of up to 20 mg *** pairing with a thick Na3V2（PO4）3cathode (20.6 mg cm-2),the as-fabricated full cell exhibited high operating voltage （2.8 V）,excellent rate performance and cycling stability with a high capacity retention of 88.7% after 200 cycles,well highlighting the Na4TDC anode material for SIBs.

关键词： Organic anode material Low redox potential Composite anode Sodium-ion batteries

Subtropical urban turfs： Carbon and nitrogen pools and the role of enzyme activity

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Journal of Environmental Sciences 2018年第3期30卷 18-28页

作者： ling kong LM Chu School of Life Sciences The Chinese University of Hong Kong Shatin NT Hong Kong SAR China department of orthopaedics & traumatology faculty of medicine the chinese university of hong kong

Urban grasslands not only provide a recreational venue for urban residents, but also sequester organic carbon in vegetation and soils through photosynthesis, and release carbon dioxide through respiration, which largely contribute to carbon storage and fluxes at regional and global scales. We investigated organic carbon and nitrogen pools in subtropical turfs and found that dissolved organic carbon（DOC） and dissolved organic nitrogen（DON）were regulated by several factors including microbial activity which is indicated by soil enzymatic activity. We observed a vertical variation and different temporal patterns in both soil DOC, DON and enzyme activities, which decreased significantly with increasing soil depths. We further found that concentration of soil DON was linked with turf age. There were correlations between grass biomass and soil properties, and soil enzyme activities. In particular, soil bulk density was significantly correlated with soil moisture and soil organic carbon（SOC）. In addition, DOC correlated significantly with DON. Significant negative correlations were also observed between soil total dissolved nitrogen（TDN） and grass biomass of Axonopus compressus and Zoysia matrella. Specifically, grass biomass was significantly correlated with the soil activity of urease and β-glucosidase. Soil NO3-N concentration also showed negative correlations with the activity of both β-glucosidase and protease but there were no significant correlations between cellulase and soil properties or grass biomass. Our study demonstrated a relationship between soil C and N dynamics and soil enzymes that could be modulated to enhance SOC pools through management and maintenance practices.

关键词： Dissolved organic carbon (DOC)lDissolved organic nitrogen (DON)lSoil enzymelTurfgrass

On the Integrality of Characteristic Elements in Nonabelian Iwasawa Theory

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Acta Mathematica Sinica,English Series 2008年第1期24卷 43-58页

作者： ling Quan kong School of Mathematical Sciences Beijing Normal University Beijing 100875 P. R. China

This paper is concerned with a conjecture formulated by Coates et al in [4] which describes the relation between the integrality of the characteristic elements and their evaluations in the noncommutative Iwasawa theor... 详细信息

关键词： p-adic Lie group K group characteristic element Iwasawa theory

Precision measurement and compensation of kinematic errors for industrial robots using artifact and machine learning

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Advances in Manufacturing 2022年第3期10卷 397-410页

作者： ling-Bao kong Yi Yu Shanghai Engineering Research Center of Ultra-precision Optical Manufacturing Department of Optical Science and EngineeringFudan UniversityShanghai 200438People's Republic of China

Industrial robots are widely used in various areas owing to their greater degrees of freedom(DOFs)and larger operation space compared with traditional frame movement systems involving sliding and rotational ***,the geometrical transfer of joint kinematic errors and the relatively weak rigidity of industrial robots compared with frame movement systems decrease their absolute kinematic accuracy,thereby limiting their further application in ultraprecision *** imposes a stringent requirement for improving the absolute kinematic accuracy of industrial robots in terms of the position and orientation of the robot arm *** measurement and compensation methods for industrial robots either require expensive measuring systems,producing positioning or orientation errors,or offer low measurement ***,a kinematic calibration method for an industrial robot using an artifact with a hybrid spherical and ellipsoid surface is proposed.A system with submicrometric precision for measuring the position and orientation of the robot arm end is developed using laser displacement ***,a novel kinematic error compensating method involving both a residual learning algorithm and a neural network is proposed to compensate for nonlinear errors.A six-layer recurrent neural network(RNN)is designed to compensate for the kinematic nonlinear errors of a six-DOF industrial *** results validate the feasibility of the proposed method for measuring the kinematic errors of industrial robots,and the compensation method based on the RNN improves the accuracy via parameter *** studies show that the measuring system and compensation method can reduce motion errors by more than 30%.The present study provides a feasible and economic approach for measuring and improving the motion accuracy of an industrial robot at the submicrometric measurement level.

关键词： Industrial robot Kinematic error Calibration Machine learning Recurrent neural network(RNN)

Mesoscopic measurement of damage and shear bands of granite residual soil using Micro-CT and digital volume correlation

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Journal of Mountain Science 2023年第11期20卷 3423-3436页

作者： LI Cheng-sheng ZHANG Bing-xin LIU Zhi-jun kong ling-wei SHU rong-jun Department of Civil and Environmental Engineering Shantou UniversityShantou 515000China State Key Laboratory of Geomechanics and Geotechnical Engineering Institute of Rock and Soil MechanicsChineseAcademy of SciencesWuhan 430000China College of Civil and Architecture Engineering Chuzhou UniversityChuzhou 239000China

The mesomechanics of geotechnical materials are closely related to the macromechanical properties,especially the mesoscale evolution of shear bands,which is helpful for understanding the failure mechanism of geotechnical ***,there is lack of effective quantitative analysis method for the complex evolution mechanism of threedimensional shear *** this work,we used X-ray computed tomography(CT)to reconstruct volume images and used the digital volume correlation(DVC)method to calculate the three-dimensional strain fields of granite residual soil samples at different loading *** trend of the failure surface of the shear bands was obtained by the planar fitting method,and the connectivity index was constructed according to the projection characteristics of the shear bands on the failure trend *** results support the following findings:the connectivity index of the shear band increases rapidly and then slowly with increasing axial strain,which is characterized by a near'S'*** the stress reaches the peak value,the connectivity index of the shear bands almost exceeds *** contribution of the new shear band volume to the connectivity of the shear bands becomes increasingly small with increasing axial *** by quartz grains and stress at the initial stage,the dip angle gradually and finally approaches the included angle of the maximum shear stress from the discrete state with increasing axial *** tendency and dip angle of the resulting shear bands are dynamic,and the tendency slightly deflects with increasing loading.

关键词： Damage Shear band Digital volume correlation Micro-CT Granite residual soil

Labdane Diterpenoids from Coleus forskohlii （Willd.） Briq.

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Journal of Integrative Plant Biology 2006年第4期48卷 478-481页

作者： ling-ling Xu ling-Yi kong Department of Natural Medicinal Chemistry China Pharmaceutical University Nanjing 210009 China

in order to investigate the active substances of Coleus forskohlii（Wiiid.） Brlq., a new labdane dlterpenold, 12- hydroxy-8,*** acid, together with two 8,13-epoxylabd-14-ene-11-one dlterpenolds, 6-acetyl-1- deoxyforskolln and 6-acetyl-1,9-dldeoxyforskolln, was Isolated on the basis of various chromatographic technlques and spectroscopic methods.

关键词： 6-acetyl-1-deoxyforskolin 6-acetyl-1 ,9-dideoxyforskolin Coleus forskohlii 12-hydroxy-8,13E-labdadien-15-oic acid labdane diterpenoid.

Feasible synthesis of porous h-BN by Mg^(2+)induced lattice dislocations for hydrogen and ammonia storage

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Nano Research 2025年第1期18卷 94-99页

作者： Xiaojia Huang Zihao Wang Yihan kong Li Jiang Baolin Wang Jiangtao Jia Heping Ma Guangshan Zhu Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Northeast Normal UniversityChangchun 130024China School of Chemical Engineering and Technology Xi’an Jiaotong University Xi’an 710049China

Hexagonal boron nitride(h-BN)is a two-dimensional(2D)layered material with a structure similar to graphite and it has potential as a hydrogen and ammonia storage ***,dense packing in the standard h-BN structure limits its surface area and prevents the B and N from being adsorption *** this study,the addition of Mg^(2+)during h-BN synthesis facilitated the growth of lattice dislocations and led to a crosslinked three-dimensional(3D)porous structure.A proposed formation mechanism for porous h-BN was confirmed by several characterization routes,most clearly by high-resolution transmission electron microscopy(HRTEM).Porous Mg/BNs exhibited high H_(2)and NH_(3)uptakes and showed potential for H_(2)and NH_(3)storage.

关键词： hexagonal boron nitride porous material dislocation gas storage