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Confinement of ionomer for electrocatalytic CO2 reduction reaction via efficient mass transfer pathways

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National Science Review 2024年第2期11卷 168-176页

作者： Xiaowei Du Peng zhang Gong zhang Hui Gao lili zhang Mengmeng zhang Tuo Wang Jinlong Gong School of Chemical Engineering and Technology Key Laboratory for Green Chemical Technology of the Ministry of Education Tianjin University Collaborative Innovation Center of Chemical Science and Engineering(Tianjin) National Industry-Education Platform of Energy Storage Tianjin University Joint School of the National University of Singapore and Tianjin University International Campus of Tianjin University Haihe Laboratory of Sustainable Chemical Transformations

Gas diffusion electrodes（GDEs） mediate the transport of reactants, products and electrons for the electrocatalytic CO2reduction reaction（CO2RR） in membrane electrode assemblies. The random distribution of ionomer, added by the traditional physical mixing method, in the catalyst layer of GDEs affects the transport of ions and CO2. Such a phenomenon results in elevated cell voltage and decaying selectivity at high current densities. This paper describes a pre-confinement method to construct GDEs with homogeneously distributed ionomer, which enhances mass transfer locally at the active centers. The optimized GDE exhibited comparatively low cell voltages and high CO Faradaic efficiencies（FE > 90%） at a wide range of current densities. It can also operate stably for over 220 h with the cell voltage staying almost unchanged. This good performance can be preserved even with diluted CO2feeds, which is essential for pursuing a high single-pass conversion rate. This study provides a new approach to building efficient mass transfer pathways for ions and reactants in GDEs to promote the electrocatalytic CO2RR for practical applications.

关键词： CO2 electroreduction gas diffusion electrode mass transfer ionomer Ag catalyst

Biased Bi-Population Evolutionary Algorithm for Energy-Efficient Fuzzy Flexible Job Shop Scheduling with Deteriorating Jobs

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Complex System Modeling and Simulation 2024年第1期4卷 15-32页

作者： Libao Deng Yingjian Zhu Yuanzhu Di lili zhang School of Information Science and Engineering Harbin Institute of TechnologyWeihai 264209China. Department of Computer Science Maynooth UniversityMaynoothW23 F2H6 the School of Computing Dublin City UniversityDublinD09 V209Ireland.

There are many studies about flexible job shop scheduling problem with fuzzy processing time and deteriorating scheduling,but most scholars neglect the connection between them,which means the purpose of both models is to simulate a more realistic factory *** this perspective,the solutions can be more precise and practical if both issues are considered ***,the deterioration effect is treated as a part of the fuzzy job shop scheduling problem in this paper,which means the linear increase of a certain processing time is transformed into an internal linear shift of a triangle fuzzy processing *** from that,many other contributions can be stated as follows.A new algorithm called reinforcement learning based biased bi-population evolutionary algorithm(RB2EA)is proposed,which utilizes Q-learning algorithm to adjust the size of the two populations and the interaction frequency according to the quality of population.A local enhancement method which combimes multiple local search stratgies is *** interaction mechanism is designed to promote the convergence of the *** experiments are designed to evaluate the efficacy of RB2EA,and the conclusion can be drew that RB2EA is able to solve energy-efficient fuzzy flexible job shop scheduling problem with deteriorating jobs(EFFJSPD)efficiently.

关键词： bi-population evolutionary algorithm Q-learning algorithm fuzzy deteriorating effect energy flexible job shop scheduling

Wide‑field swept‑source OCT angiography of the periarterial capillary‑free zone before and after anti‑VEGF therapy for branch retinal vein occlusion

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Eye and Vision 2024年第2期10卷 31-40页

作者： Wenyi Tang Wei Liu Jingli Guo lili zhang Gezhi Xu Keyan Wang Qing Chang Department of Ophthalmology Eye and ENT Hospital of Fudan University83 Fenyang RoadShanghai 200031China Shanghai Key Laboratory of Visual Impairment and Restoration Fudan UniversityShanghaiChina NHC Key Laboratory of Myopia(Fudan University) Laboratory of MyopiaChinese Academy of Medical SciencesShanghaiChina

Background:The aim of the study was to investigate the changes in the periarterial capillary-free zone(paCFZ)after anti-vascular endothelial growth factor(VEGF)therapy in patients with branch retinal vein occlusion(BRVO)by widefield swept-source optical coherence tomography angiography(SS-OCTA)and assess their associations with clinical ***:In this retrospective observational study of 54 treatment-naive BRVO patients with macular edema,we reviewed the findings of 12×12 mm^(2)SS-OCTA at baseline,3,6,and 12 months after intravitreal ranibizumab *** paCFZ and major retinal artery areas were measured on SS-OCTA *** paCFZ area to artery area(P/A)ratio was ***:The paCFZ areas and P/A ratios of first-and second-order arteries were significantly greater in BRVO eyes than in contralateral eyes(all P<0.01),but there were no differences in the first-and second-order artery areas(P=0.20 and 0.25,respectively).The paCFZ areas and P/A ratios decreased significantly at 3,6,and 12 months after anti-VEGF therapy(all P<0.01).The baseline P/A ratio was significantly correlated with the baseline best-corrected visual acuity(BCVA),central retinal thickness,and their improvements at 3,6,and 12 months(all P<0.05).Baseline BCVA and P/A ratios of first-and second-order arteries were independently associated with the final BCVA in multivariate linear ***:Wide-field SS-OCTA shows that anti-VEGF therapy can lead to a significant improvement in the paCFZ parameters in *** baseline P/A ratios on SS-OCTA tend to predict better visual outcomes at 12 months after anti-VEGF therapy.

关键词： Swept-source optical coherence tomography angiography Branch retinal vein occlusion Periarterial capillary free zone Anti-VEGF treatment Prognosis

Progress in models for coupled human and natural systems

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Science China Earth Sciences 2024年第11期67卷 3631-3637页

作者： Tianxiang YUE Chenchen WU Wenjiao SHI Yongzhong TIAN Qing WANG Yimin LU lili zhang State Key Laboratory of Resources and Environment Information System Institute of Geographical Sciences and Natural Resources ResearchChinese Academy of Sciences College of Resources and Environment University of Chinese Academy of Sciences School of Geographical Sciences Southwest University National Institute of Environmental Health Chinese Center for Disease Control and Prevention National Engineering Research Center of Geospatial Information Technology Fuzhou University The Aerospace Information Research Institute Chinese Academy of Sciences

1. Introduction Malthus (1798) was one of the earliest researchers to propose a coupled human-natural system (CHANS) model, particularly in his analysis of the relationship between population growth and food supply. He argued that while population grows geometrically, food supply increases only arithmetically, suggesting that this imbalance could eventually lead to a food crisis due to diminishing per capita food availability (Malthus, 1798).

关键词： ECOLOGICAL-SYSTEMS SUSTAINABILITY POPULATION COMPLEXITY DECISIONS FRAMEWORK DYNAMICS EARTH

Metabolic mechanism of dietary factors and effect of dietary types associated with hyperuricemia: A review

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Food Science and Human Wellness 2024年

作者： Kaina Qiao Xuewei Zhou lili zhang Wangang zhang Baoguo Sun Yuyu zhang College of Food Science and Technology， Nanjing Agricultural University Key Laboratory of Geriatric Nutrition and Health (Beijing Technology and Business University)， Ministry of Education Key Laboratory of Flavor Science of China General Chamber of Commerce， Beijing Technology and Business University Food Laboratory of Zhongyuan， Beijing Technology and Business University

Globally， hyperuricemia is a growing health， social， and economic problem which could cause gout， chronic kidney diseases and other diseases. There are increasing evidences that a sensible diet makes sense to reduce the risk of hyperuricemia. This review aims to explore the metabolic mechanism of dietary factors and effects of dietary types associated with hyperuricemia. Recommendations for dietary modification to prevent hyperuricemia are as following: decreasing intake of animal organs， seafood， sugar-sweetened， and alcohol beverages is essential; choosing water or unsweetened tea and coffee instead of sweetened beverages is beneficial; and increasing intake of vegetables， reduced-fat dairy products， foods containing fiber， micronutrients and unsaturated fatty acids is helpful. In addition， consumption of fruits and legumes in moderation is advantageous， and low-fructose of fruits and low-purine of non-soy beans are recommended. Moreover， personalized diet needs to be emphasized for hyperuricemic patients accompanied with diverse metabolic diseases.

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Ferroptosis mechanism and Alzheimer's disease

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Neural Regeneration Research 2024年第8期19卷 1741-1750页

作者： Lina Feng Jingyi Sun Ling Xia Qiang Shi Yajun Hou lili zhang Mingquan Li Cundong Fan Baoliang Sun Shandong Key Laboratory of TCM Multi-Target Intervention and Disease Control the Second Affiliated Hospital of Shandong First Medical UniversityTaianShandong ProvinceChina Department of Internal Medicine Taian Traffic HospitalTaianShandong ProvinceChina Department of Neurology the Third Affiliated Clinical Hospital of Changchun University of Chinese MedicineChangchunJilin ProvinceChina

Regulated cell death is a genetically determined form of programmed cell death that commonly occurs during the development of living *** process plays a crucial role in modulating homeostasis and is evolutionarily conserved across a diverse range of living *** is a classic regulatory mode of cell *** studies of regulatory cell death in Alzheimer’s disease have yielded increasing evidence that fe rroptosis is closely related to the occurrence,development,and prognosis of Alzheimer’s *** review summarizes the molecular mechanisms of ferroptosis and recent research advances in the role of ferro ptosis in Alzheimer’s *** findings are expected to serve as a theoretical and experimental foundation for clinical research and targeted therapy for Alzheimer’s disease.

关键词： Alzheimer’s disease apolipoprotein E Fe^(2+) ferroptosis glial cell glutathione peroxidase 4 imbalance in iron homeostasis lipid peroxidation regulated cell death system Xc^(-)

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Application of controlled-release urea increases maize N uptake,environmental benefits and economic returns via optimizing temporal and spatial distributions of soil mineral N

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Pedosphere 2024年第1期34卷 222-235页

作者： Mingxue SUN Juan LI lili zhang Xiaomeng SU Ning LIU Xiaori HAN Songjiang WU Zhentao SUN Xiangdong YANG Institute of Agricultural Resources and Regional Planning Chinese Academy of Agricultural Sciences/State Key Laboratory of Efficient Utilization of Arid and Semi-arid Arable Land in Northern China/Key Laboratory of Plant Nutrition and FertilizerMinistry of Agriculture and Rural AffairsBeijing 100081China Agricultural Development Service Center of Zhuanghe Zhuanghe 116499China Agricultural Technology Extension Center Wafangdian 116300China College of Land and Environment Shenyang Agricultural UniversityShenyang 100866China

The creation of controlled-release urea (CRU) is a potent substitute for conventional fertilizers in order to preserve the availability of nitrogen (N) in soil,prevent environmental pollution,and move toward green *** main objectives of this study were to assess the impacts of CRU’s full application on maize production and to clarify the connection between the nutrient release pattern of CRU and maize nutrient *** order to learn more about the effects of CRU application on maize yields,N uptake,mineral N (N_(min)) dynamics,N balance in soil-crop systems,and economic returns,a series of field experiments were carried out in 2018–2020 in Dalian City,Liaoning Province,*** were 4 different treatments in the experiments:no N fertilizer input (control,CK);application of common urea at 210 kg ha^(-1)(U),the ideal fertilization management level for the study site;application of polyurethane-coated urea at the same N input rate as U (PCU);and application of PCU at a 20% reduction in N input rate (0.8PCU).Our findings showed that using CRU (i.e.,PCU and 0.8 PCU) may considerably increase maize N absorption,maintain maize yields,and increase N use efficiency (NUE) compared to *** grain yield showed considerable positive correlations with total N uptake in leaf in U and 0.8 PCU,but negative correlations with that in PCU,indicating that PCU caused excessive maize absorption while 0.8 PCU could achieve a better yield response to N ***,PCU was able to maintain N fertilizer in the soil profile 0–20 cm away from the fertilization point,and higher N_(min)content was observed in the 0–20 cm soil layer at various growth stages,particularly at the middle and late growing stages,optimizing the temporal and spatial distributions of N_(min).Additionally,compared to that in U,the apparent N loss rate in PCU was reduced by 36.2%,and applying CRU (PCU and 0.8 PCU) increased net profit by 8.5% to 15.2% with less labor and fertilization *** was co

关键词： apparent N loss fertilization management green agriculture maize yield N balance N use efficiency

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Plant virology in the 21st century in China:Recent advances and future directions

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Journal of Integrative Plant Biology 2024年第3期66卷 579-622页

作者： Jianguo Wu Yongliang zhang Fangfang Li Xiaoming zhang Jian Ye Taiyun Wei Zhenghe Li Xiaorong Tao Feng Cui Xianbing Wang lili zhang Fei Yan Shifang Li Yule Liu Dawei Li Xueping Zhou Yi Li State Key Laboratory for Ecological Pest Control of Fujian and Taiwan Crops Vector-borne Virus Research CenterCollege of Plant ProtectionFujian Agriculture and Forestry UniversityFuzhou 350002China State Key Laboratory of Plant Environmental Resilience and Ministry of Agriculture Key Laboratory of Soil Microbiology College of Biological SciencesChina Agricultural UniversityBeijing 100193China State Key Laboratory for Biology of Plant Diseases and Insect Pests Institute of Plant ProtectionChinese Academy of Agricultural SciencesBeijing 100193China State Key Laboratory of Integrated Management of Pest Insects and Rodents Institute of ZoologyChinese Academy of SciencesBeijing 100101China CAS Center for Excellence in Biotic Interactions University of Chinese Academy of SciencesBeijing 100049China State Key Laboratory of Plant Genomics Institute of MicrobiologyChinese Academy of SciencesBeijing 100101China State Key Laboratory of Rice Biology Institute of BiotechnologyZhejiang UniversityHangzhou 310058China Department of Plant Pathology The Key Laboratory of Plant ImmunityNanjing Agricultural UniversityNanjing 210095China State Key Laboratory for Managing Biotic and Chemical Threats to the Quality and Safety of Agro-products Institute of Plant VirologyNingbo UniversityNingbo 315211China MOE Key Laboratory of Bioinformatics Center for Plant BiologySchool of Life SciencesTsinghua UniversityBeijing 100084China State Key Laboratory of Protein and Plant Gene Research School of Life SciencesPeking UniversityBeijing 100871China

Plant viruses are a group of intracellular pathogens that persistently threaten global food *** advances in plant virology have been achieved by Chinese scientists over the last 20 years,including basic research and technologies for preventing and controlling plant viral ***,we review these milestones and advances,including the identification of new crop-infecting viruses,dissection of pathogenic mechanisms of multiple viruses,examination of multilayered interactions among viruses,their host plants,and virus-transmitting arthropod vectors,and in-depth interrogation of plantencoded resistance and susceptibility ***,various plant virus-based vectors have also been successfully developed for gene function studies and target gene expression in *** also recommend future plant virology studies in China.

关键词： China emerging plant viruses plant virology plant resistance/susceptibility to viral infection plant-virus transmission vector interactions plant virus-based vectors viral pathogenesis

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Highly selective growth of(6,5)single-walled carbon nanotubes from sigma phase alloy catalyst

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Nano Research 2024年第3期17卷 1999-2003页

作者： Liantao Xin Chen Ma Qianru Wu Shaokang Liu Linhai Li Xiuyun zhang Liu Qian Maoshuai He Dong Li Fangqian Han Shulan Hao Lihu Feng Yahan Li Huaping Liu lili zhang Chang Liu Jin zhang College of Chemistry and Molecular Engineering Qingdao University of Science and TechnologyQingdao 266042China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China College of Physics Science and Technology Yangzhou UniversityYangzhou 225002China Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsBeijing National Laboratory for Molecular SciencesCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China

The chirality structure of a single-walled carbon nanotube(SWNT)strongly depends on the composition of catalyst used in the chemical vapor deposition *** this study,we develop a porous magnesia supported manganese-rhenium(MnRe/MgO)catalyst for chirality-selective synthesis of *** characterizations reveal that(6,5)tubes with a selectivity higher than 70%are grown from the Re-rich MnRe/MgO *** comparing the SWNT growth results with those of monometallic Mn or Re,the formation of sigma phase,an intermetallic compound occurring in transition-metal alloy systems,is revealed to be crucial for the dominant synthesis of(6,5)*** work not only extends the application of sigma phase alloy for catalytic synthesis of SWNTs,but also sheds lights on the growth of SWNTs with a high chirality selectivity.

关键词： single-walled carbon nanotubes sigma phase manganese-rhenium catalyst selective growth transition-metal alloy