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Exploring the potential of olivine-containing copper-nickel slag for carbon dioxide mineralization in cementitious materials

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International Journal of Minerals,Metallurgy and Materials 2024年第3期31卷 562-573页

作者： Qianqian wang Zequn Yao lijie Guo Xiaodong Shen College of Materials Science and Engineering Nanjing Tech UniversityNanjing 211816China State Key Laboratory of Materials-Oriented Chemical Engineering Nanjing 211816China BGRIMM Technology Group Beijing 100160China

Water-quenched copper-nickel metallurgical slag enriched with olivine minerals exhibits promising potential for the production of CO_(2)-mineralized cementitious materials.In this work,copper-nickel slag-based cementitious material(CNCM)was synthesized by using different chemical activation methods to enhance its hydration reactivity and CO_(2) mineralization capacity.Different water curing ages and carbonation conditions were explored related to their carbonation and mechanical properties development.Meanwhile,thermogravimetry differential scanning calorimetry and X-ray diffraction methods were applied to evaluate the CO_(2) adsorption amount and carbonation products of CNCM.Microstructure development of carbonated CNCM blocks was examined by backscattered electron imaging(BSE)with energy-dispersive X-ray spectrometry.Results showed that among the studied samples,the CNCM sample that was subjected to water curing for 3 d exhibited the highest CO_(2) sequestration amount of 8.51wt%at 80℃and 72 h while presenting the compressive strength of 39.07 MPa.This result indicated that 1 t of this CNCM can sequester 85.1 kg of CO_(2) and exhibit high compressive strength.Although the addition of citric acid did not improve strength development,it was beneficial to increase the CO_(2) diffusion and adsorption amount under the same carbonation conditions from BSE results.This work provides guidance for synthesizing CO_(2)-mineralized cementitious materials using large amounts of metallurgical slags containing olivine minerals.

关键词： copper-nickel slag fayalite CO_(2)sequestration cementitious material admixtures carbonation conditions

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Ultrathin Hematite Photoanode with Gradient Ti Doping

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Research 2020年第1期2020卷 883-890页

作者： Pengfei Liu Chongwu wang Lijie Wang Xuefeng Wu Lirong Zheng Hua Gui Yang Key Laboratory for Ultrafine Materials of Ministry of Education Shanghai Engineering Research Center of Hierarchical NanomaterialsSchool of Materials Science and EngineeringEast China University of Science and Technology130 Meilong RoadShanghai 200237China School of Electrical and Electronic Engineering Nanyang Technological University50 Nanyang AvenueSingaporeSingapore 639798 Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China

The poor photoelectrochemical(PEC)performance derived from insufficient charge separation in hematite photoanode crucially limits its application.Gradient doping with band bending in a large region is then considered as a promising strategy,facilitating the charge transfer ability due to the built-in electric field.Herein,we developed a synthetic strategy to prepare gradient Ti-doped ultrathin hematite photoelectrode and systematically investigated its PEC performance.The as-synthesized electrode(1.5-6.0%doping level from the surface to the substrate)delivered a photocurrent of about 1.30mAcm^(-2) at 1.23V versus the reversible hydrogen electrode(RHE),which is nearly 100%higher than that of homogeneously doped hematite electrode.The enhanced charge transfer property,induced by the energy band bending due to the built-in electric field,has been further confirmed by electrochemical measurements.This strategy of gradient doping should be adaptable and can be applied for other functional materials in various fields.

关键词： electrode doping bending

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Tuning porosity of coal-derived activated carbons for CO_(2) adsorption

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Frontiers of Chemical Science and Engineering 2022年第9期16卷 1345-1354页

作者： Zhipeng Qie Lijie Wang Fei Sun Huan Xiang Hua wang Jihui Gao Guangbo Zhao Xiaolei Fan School of Energy Science and Engineering Harbin Institute of TechnologyHarbin 150001China Department of Chemical Engineering and Analytical Science The University of ManchesterManchester M139PLUK China Datang Corporation Renewable Energy Science and Technology Research Institute Beijing 100052China Energy and Bioproducts Research Institute(EBRI) Aston UniversityBirmingham B47ETUK

A simple method was developed to tune the porosity of coal-derived activated carbons,which provided a model adsorbent system to investigate the volumetric CO_(2)adsorption performance.Specifically,the method involved the variation of the activation temperature in a K2CO3 induced chemical activation process which could yield activated carbons with defined microporous(<2 nm,including ultra-microporous<1 nm)and meso-microporous structures.CO_(2)adsorption isotherms revealed that the microporous activated carbon has the highest measured CO_(2)adsorption capacity(6.0 mmol∙g^(–1)at 0℃and 4.1 mmol∙g^(-1)at 25℃),whilst ultra-microporous activated carbon with a high packing density exhibited the highest normalized capacity with respect to packing volume(1.8 mmol∙cm−3 at 0℃and 1.3 mmol∙cm^(–3)at 25℃),which is significant.Both experimental correlation analysis and molecular dynamics simulation demonstrated that(i)volumetric CO_(2)adsorption capacity is directly proportional to the ultra-micropore volume,and(ii)an increase in micropore sizes is beneficial to improve the volumetric capacity,but may lead a low CO_(2)adsorption density and thus low pore space utilization efficiency.The adsorption experiments on the activated carbons established the criterion for designing CO_(2)adsorbents with high volumetric adsorption capacity.

关键词： coal-derived activated carbons porosity CO_(2)adsorption molecular dynamics

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Theoretical Model of Dynamic Bulk Modulus for Aerated Hydraulic Fluid

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Chinese Journal of Mechanical Engineering 2022年第5期35卷 183-193页

作者： Xiaoming Yuan Weiqi wang Xuan Zhu lijie Zhang Hebei Key Laboratory of Heavy Machinery Fluid Power Transmission and Control Yanshan UniversityQinhuangdao 066004China Key Laboratory of Advanced Forging&Stamping Technology and Science Ministry of Education of ChinaYanshan UniversityQinhuangdao 066000China State Key Laboratory of Fluid Power and Mechatronic Systems Zhejiang UniversityHangzhou 310027China

Existing models of bulk modulus for aerated hydraulic fluids primarily focus on the effects of pressure and air fraction,whereas the effect of temperature on bulk modulus is disregarded.Based on the lumped parameter method and the full cavitation model,combined with the improved Henry’s law and the air polytropic course equation,a theoretical model of dynamic bulk modulus for an aerated hydraulic fluid is derived.The effects of system pressure,air fraction,and temperature on bulk modulus are investigated using the controlled variable method.The results show that the dynamic bulk modulus of the aerated hydraulic fluid is inconsistent during the compression process.At the same pressure point,the dynamic bulk modulus during expansion is higher than that during compression.Under the same initial air faction and pressure changing period,a higher temperature results in a lower dynamic bulk modulus.When the pressure is lower,the dynamic bulk modulus of each temperature point is more similar to each other.By comparing the theoretical results with the actual dynamic bulk modulus of the Shell Tellus S ISO32 standard air-containing oil,the goodness-of-fit between the theoretical model and experimental value at three temperatures is 0.9726,0.9732,and 0.9675,which validates the theoretical model.In this study,a calculation model of dynamic bulk modulus that considers temperature factors is proposed.It predicts the dynamic bulk modulus of aerated hydraulic fluids at different temperatures and provides a theoretical basis for improving the analytical model of bulk modulus.

关键词： Aerated hydraulic fluid Dynamic bulk modulus Theory model Air fraction Pressure

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Mechanism of Structure Variations at Rifted Margins in the Central Segment of South Atlantic:Insights from Numerical Modeling

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Acta Geologica Sinica(English Edition) 2023年第4期97卷 1229-1242页

作者： wang Zhichen LI Jianghai FENG Zhiqiang wang lijie LIU Chen Key Laboratory of Orogenic Belts and Crustal Evolution School of Earth and Space SciencePeking UniversityBeijing 100871China Institute of Oil and Gas Peking UniversityBeijing 100871China Sinopec Petroleum Exploration and Production Research Institute Beijing 100871China

Rifted margins in the central South Atlantic portray spatial variability in terms of preserved width and thickness,which relates to complex rift-related fault activities.However,there is still a lack of systematic and quantitative explanations for the causes of the variations that are observed along the paired rifts.To elucidate this issue,2D viscous-plastic thermomechanical numerical models are applied to capture the behavior of deformation,in which we investigate the effects of extensional rate,crustal strength and thickness on crust-mantle coupling,and timing of transition from rifting to breakup.Our numerical experiments demonstrate that crust-mantle decoupling accounts for crustal hyperextension,and that incorporating moderate-intensity rheology into lower crust may yield insights into the hyper-extended crust and asymmetric architecture observed in the central South Atlantic.The results also suggest that undulations in lithospheric basement cause asymmetric mantle upwelling.The lower crust of fold belts takes priority to be thermally weakened over craton and induces rift migration simultaneously.A new mechanism for the formation of failed rift is described,where the mechanical decoupling derived from thermally weakened lower crust gives access to dual rift migration.These results reinforce the interpretation on how crustal rheology shapes margins architectures and highlight the first-order effects of crust-mantle coupling.

关键词： conjugate rifted margins crustal rheology crust-mantle coupling and decoupling rift migration central South Atlantic

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Self-templating synthesis of Pd_(4)S hollow nanospheres as electrocatalysts for oxygen reduction reaction

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Nano Research 2023年第2期16卷 2597-2603页

作者： Qian wang Donghui Zhao Jialong Yu lijie Shi Yawen wang Hongyu Chen Institute of Advanced Synthesis School of Chemistry and Molecular EngineeringNanjing Tech UniversityNanjing 211816China School of Science Westlake UniversityHangzhou 310023China

Hollow nanostructures with structural advantages have been widely exploited as catalysts in electrochemical reactions.However,there are only limited strategies for constructing hollow Pd-based nanostructures.In this work,Pd4S hollow nanospheres(Pd4S HNSs)are synthesized with a facile wet-chemical method via a self-templating process.Intermediate Pd-L-cysteine solid nanospheres(SNSs)were firstly obtained by the coordination of L-cysteine with Pd^(2+),and then in situ converted to hollow nanospheres in the following reduction process.The formation mechanism of the Pd4S HNSs was studied,and the size of the Pd4S HNSs can be readily adjusted by tuning the size of the SNSs.The hollow morphology would help the exposure of active sites and the prevention of aggregation during the catalytic reactions.As a result,the Pd4S HNSs exhibit improved catalytic performances in the oxygen reduction reactions,with a half-wave potential of 0.913 V vs.reversible hydrogen electrode(RHE)and impressive stability in the accelerated durability test.

关键词： Pd4S hollow nanospheres self-templating electrocatalysis oxygen reduction reaction

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Seasonal changes in gut microbiota of sea cucumber over natural aestivation cycle

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Journal of Oceanology and Limnology 2024年第3期42卷 849-864页

作者： Ye ZHAO Han wang Haona wang lijie ZHANG Hao SUN Yanying ZHANG Ocean School Yantai UniversityYantai 264005China

Sea cucumber Apostichopus japonicus is an ideal model organism for marine invertebrate aestivation;it annually enters a“sleeping state”for nearly 3 months when ambient water temperature range is 25–30℃.The natural fasting is accompanied by remodeling the intestinal biota and function,which is a part of host biology and could affect the gut microbiota.We investigatesd the impact of annual aestivation on gut microbiota using high-throughput sequencing of 16S rRNA amplicons.Results reveal a notable alteration in the composition of gut bacteria during aestivation during which various indigenous families and genera that exhibit a preference for dietary glycans(e.g.,family Rhodobacteraceae and Flavobacteriaceae)decreased,while the taxa capable of utilizing substrates derived from the host(e.g.,genus Akkermansia and Prevotella)increased,and so did certain opportunistic pathogenic bacteria.Moreover,the investigation delved into the gut morphology and immunity response of A.japonicus and reveal that the intestine of A.japonicus undergoes substantial atrophy and degeneration during aestivation.However,there was an observed augmentation in the levels of acid and neutral mucin within mucous cells,as well as an enhanced immune defense response(as evidenced by increased gene expression of AjTLR3,LITAF,Ajp105,and LYZ).These results imply that the composition of sea cucumber gut microbiota differed between aestivation and active periods,which potentially affects the intestinal functions of the host and the symbiotic relationship between host and its microbiota over the activeaestivation cycle.

关键词： Apostichopus japonicus aestivation gut microbiota diet Illumina sequencing

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HiTL-based adaptive fuzzy tracking control of MASs:A distributed fixed-time strategy

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中国科学:技术科学英文版 2023年第10期66卷 2907-2916页

作者： LIU Yang CHI RongHu LI HongYi wang lijie LIN Na College of Automation and Electronic Engineering Qingdao University of Science and TechnologyQingdao 266061China School of Automation Guangdong University of TechnologyGuangzhou 510006China Guangdong Province Key Laboratory of Intelligent Decision and Cooperative Control Guangdong University of TechnologyGuangzhou 510006China Institute of Complexity Science and the School of Automation Qingdao UniversityQingdao 266071China

Human-in-the-loop(HiTL)control is promising for the cooperative control problem of multi-agent systems(MASs)under the complicated environment.By considering the effect of human intelligence and decision making,the system robustness and security are notably enhanced.Hence,a distributed fixed-time tracking control problem is investigated in this paper for heterogeneous MASs based on the HiTL idea.First,a lemma of practically fixed-time stable is given where an explicit relationship of settling time and convergence domain is clearly shown.Then,under the framework of the adaptive backstepping approach,a series of modified intermediate control signals is designed to avoid the singularity problem by taking advantage of power transformation,fuzzy logic systems,and inequality schemes.Finally,the numerical example and comparison results are utilized to testify the effectiveness of the proposed method.

关键词： human-in-the-Loop heterogeneous MASs fixed-time stable adaptive tracking control fuzzy logic systems

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Continuous-wave operation of 1550 nm low-threshold triple-lattice photonic-crystal surface-emitting lasers

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Light(Science & Applications) 2024年第3期13卷 446-453页

作者： Ziye wang Xia Liu Pinyao wang Huanyu Lu Bo Meng Wei Zhang Lijie Wang Yanjing wang Cunzhu Tong State Key Laboratory of Luminescence and Applications Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Central Research Institute Planning Dept 2012 LabsHuawei Technologies Company Ltd.Shenzhen 518129China

Benefitting from narrow beam divergence,photonic crystal surface-emitting lasers are expected to play an essential role in the ever-growing fields of optical communication and light detection and ranging.Lasers operating with 1.55μm wavelengths have attracted particular attention due to their minimum fiber loss and high eye-safe threshold.However,high interband absorption significantly decreases their performance at this 1.55μm wavelength.Therefore,stronger optical feedback is needed to reduce their threshold and thus improve the output power.Toward this goal,photonic-crystal resonators with deep holes and high dielectric contrast are often used.Nevertheless,the relevant techniques for high-contrast photonic crystals inevitably complicate fabrication and reduce the final yield.In this paper,we demonstrate the first continuous-wave operation of 1.55μm photonic-crystal surface-emitting lasers by using a‘triple-lattice photonic-crystal resonator’,which superimposes three lattice point groups to increase the strength of in-plane optical feedback.Using this geometry,the in-plane 180°coupling can be enhanced threefold compared to the normal single-lattice structure.Detailed theoretical and experimental investigations demonstrate the much lower threshold current density of this structure compared to‘single-lattice’and‘double-lattice’photonic-crystal resonators,verifying our design principles.Our findings provide a new strategy for photonic crystal laser miniaturization,which is crucial for realizing their use in future high-speed applications.

关键词： resonator crystal lattice

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Different dietary starch patterns in lowprotein diets:effect on nitrogen efficiency,nutrient metabolism,and intestinal flora in growing pigs

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Journal of Animal Science and Biotechnology 2022年第5期13卷 1557-1575页

作者： Junyan Zhou Lu wang lijie Yang Guangxin Yang Xiangfang Zeng Shiyan Qiao State Key Laboratory of Animal Nutrition China Agricultural UniversityBeijing 100193People’s Republic of China Beijing Bio-feed additives Key Laboratory Beijing 100193People’s Republic of China

Background:Protein releases amino acids faster than starch releases glucose in digestive tract of pigs fed lowprotein(LP)diets.Poor synchronization of dietary glucose and amino acids supply leads to compromised nitrogen efficiency.Dietary starch patterns modulation may improve this situation.Methods:Growing barrows(29.7±2.0 kg)were randomly allotted into 5 dietary treatments with LP diets consisting of different purified starches.Treatments included:waxy corn starch(W LP),corn starch+waxy corn starch(C+W LP),corn starch(C LP),pea starch+waxy corn starch(P+W LP)and pea starch(P LP).In the experiment,growth performance,protein deposition,nutrient metabolism,and fecal microbial community of pigs were investigated.In vitro starch digestion was used for predicting the in vivo glucose response.Results:Dietary starch in vitro glucose release profile was determined by starch source and the ratio of amylopectin and amylose.C+W LP treatment showed decreased total nitrogen excretion and plasma citrulline concentration and improved plasma leptin concentration among treatments(P<0.05).Besides,the highest nitrogen apparent biological value,whole-body protein deposition and growth performance and lowest urinary nitrogen excretion were also observed in C+W LP treatment.Compared with the other groups,C+W LP and C LP showed increased plasma pyruvate,IGF-1,and lipase concentrations(P<0.05).The W LP group presented dramatically increased plasma alanine and urea nitrogen concentration and decreased aldolase and leptin concentrations(P<0.05).Dietary starch patterns did not make an impact on bacterial richness and diversity,but changed the taxonomic and functional structures of the microbial communities.Microbial protein fermentation product(isobutyrate and isovalerate)presented increased in P LP treatments compared with the other treatments(P<0.05).Conclusions:Dietary starch patterns modulation can regulate dietary glucose release profile,nutrient metabolism,protein turnover,and fecal microbial fermentation in pigs.The optimal dietary

关键词： Intestinal flora Low-protein diet Nitrogen efficiency Nutrient metabolism Starch patterns

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