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Energy & Environmental Materials 2024年第1期7卷 301-312页

作者： Diab Khalafallah Weibo huang Mingjia Zhi Zhanglian Hong State Key Laboratory of Silicon Material School of Materials Science and EngineeringZhejiang University38 Zheda RoadHangzhou 310027China Mechanical Design and Materials Department Faculty of Energy EngineeringAswan UniversityP.O.Box 81521AswanEgypt

Herein,we demonstrate the synthesis of bifunctional nickel cobalt selenide@nickel telluride(Ni_(x)Co_(12-x)Se@NiTe)core-shell heterostructures via an electrodeposition approach for overall urea electrolysis and *** 3D vertically orientated NiTe dendritic frameworks induce the homogeneous nucleation of 2D Ni_(x)Co_(12-x)Se nanosheet arrays along similar crystal directions and bring a strong interfacial binding between the integrated active *** particular,the optimized Ni_(6)Co_(6)Se@NiTe with an interface coupling effect works in concert to tune the intrinsic *** only needs a low overpotential of 1.33 v to yield a current density of 10 mA cm^(-2)for alkaline urea ***,the full urea catalysis driven only by Ni_(6)Co_(6)Se@NiTe achieves 10 mA cm^(-2)at a potential of 1.38 v and can approach a constant level of the current response for 40 ***,the integrated Ni_(6)Co_(6)Se@NiTe electrode delivers an enhanced specific capacity(223 mA h g^(-1)at 1 A g^(-1))with a high cycling ***,a hybrid asymmetric supercapacitor(HASC)device based on Ni_(6)Co_(6)Se@NiTe exhibits a favorable rate capability and reaches a high energy density of 67.7 Wh kg^(-1)and a power density of 724.8 W kg^(-1)with an exceptional capacity retention of 92.4%after sequential 12000 cycles at 5 A g^(-1).

关键词： bifunctional Ni_(x)Co_(12-x)Se@NiTe core-shell electrodeposition heterointerfaces supercapacitors UOR

Pixel-level crack segmentation of tunnel lining segments based on an encoder–decoder network

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Frontiers of Structural and Civil Engineering 2024年第5期18卷 681-698页

作者： Shaokang HOU Zhigang OU Yuequn huang Yaoru LIU State Key Laboratory of Hydroscience and Engineering Tsinghua UniversityBeijing 100084China China Renewable Energy Engineering Institute Beijing 100120China State Key Laboratory of Stimulation and Regulation of Water Cycles in River Basins China Institute of Water Resources and Hydropower ResearchBeijing 100038China Hunan Provincial Water Resources Development&Investment Co. Ltd.Changsha 410007China

Regular detection and repair for lining cracks are necessary to guarantee the safety and stability of *** development of computer vision has greatly promoted structural health *** study proposes a novel encoder–decoder structure,CrackRecNet,for semantic segmentation of lining segment cracks by integrating improved vGG-19 into the U-Net *** image acquisition equipment is designed based on a camera,3-dimensional printing(3DP)bracket and two laser rangefinders.A tunnel concrete structure crack(TCSC)image data set,containing images collected from a double-shield tunnel boring machines(TBM)tunnel in China,was *** data preprocessing operations,such as brightness adjustment,pixel resolution adjustment,flipping,splitting and annotation,2880 image samples with pixel resolution of 448×448 were *** model was implemented by Pytorch in PyCharm processed with 4 NvIDIA TITAN v *** the experiments,the proposed CrackRecNet showed better prediction performance than U-Net,TernausNet,and *** paper also discusses GPU parallel acceleration effect and the crack maximum width quantification.

关键词： tunnel lining segment crack detection semantic segmentation convolutional neural network encoder-decoder structure

Dilute Aqueous-Aprotic Electrolyte Towards Robust Zn-Ion Hybrid Supercapacitor with High Operation voltage and Long Lifespan

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Nano-Micro Letters 2024年第9期16卷 1-12页

作者： Shuilin Wu Yibing Yang Mingzi Sun Tian Zhang Shaozhuan huang Daohong Zhang Bolong huang Pengfei Wang Wenjun Zhang Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education&Hubei Key Laboratory of Catalysis and Materials Science South-Central Minzu UniversityWuhan 430074People’s Republic of China Department of Materials Science and Engineering and Center of Super‑Diamond and Advanced FilmsCity University of Hong Kong83 Tat Chee AvenueKowloon TongHong Kong SARPeople’s Republic of China Department of Applied Biology and Chemical Technology The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Key Laboratory of Photochemical Conversion and Optoelectronic Materials Technical Institute of Physics and ChemistryChinese Academy of SciencesBeijingPeople’s Republic of China

With the merits of the high energy density of batteries and power density of supercapacitors,the aqueous Zn-ion hybrid supercapacitors emerge as a promising candidate for applications where both rapid energy delivery and moderate energy storage are ***,the narrow electrochemical window of aqueous electrolytes induces severe side reactions on the Zn metal anode and shortens its *** also limits the operation voltage and energy density of the Zn-ion hybrid ***'water in salt'electrolytes can effectively broaden their electrochemical windows,but this is at the expense of high cost,low ionic conductivity,and narrow temperature compatibility,compromising the electrochemical performance of the Zn-ion hybrid ***,designing a new electrolyte to balance these factors towards high-performance Zn-ion hybrid supercapacitors is urgent and *** developed a dilute water/acetonitrile electrolyte(0.5 m Zn(CF_(3)SO_(3))_(2)+1 m LiTFSI-H_(2)O/AN)for Zn-ion hybrid supercapacitors,which simultaneously exhibited expanded electrochemical window,decent ionic conductivity,and broad temperature *** this electrolyte,the hydration shells and hydrogen bonds are significantly modulated by the acetonitrile and *** a result,a Zn-ion hybrid supercapacitor with such an electrolyte demonstrates a high operating voltage up to 2.2 v and long lifespan beyond 120,000 cycles.

关键词： Zn-ion supercapacitors Zn metal anode Electrolyte engineering Hydrogen bonds Solvation structures

Upper and Lower Bounds of the α-Universal Triple I Method for Unified Interval Implications

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Computers, Materials & Continua 2024年第4期79卷 1063-1088页

作者： Yiming Tang Jianwei Gao Yifan huang School of Computer and Information Hefei University of TechnologyHefei230601China Department of Electrical and Computer Engineering University of AlbertaEdmontonAB T6R 2V4Canada

Theα-universal triple I(α-UTI)method is a recognized scheme in the field of fuzzy reasoning,whichwas proposed by our research group *** robustness of fuzzy reasoning determines the quality of reasoning algorithms to a large extent,which is quantified by calculating the disparity between the output of fuzzy reasoning with interference and the output without ***,in this study,the interval robustness(embodied as the interval stability)of theα-UTI method is explored in the interval-valued fuzzy *** begin with,the stability of theα-UTI method is explored for the case of an individual rule,and the upper and lower bounds of its results are estimated,using four kinds of unified interval implications(including the R-interval implication,the S-interval implication,the QL-interval implication and the interval t-norm implication).Through analysis,it is found that theα-UTI method exhibits good interval stability for an individual ***,the stability of theα-UTI method is revealed in the case of multiple rules,and the upper and lower bounds of its outcomes are *** results show that theα-UTI method is stable for multiple rules when four kinds of unified interval implications are used,***,theα-UTI reasoning chain method is presented,which contains a chain structure with multiple *** corresponding solutions and their interval perturbations are *** is found that theα-UTI reasoning chain method is stable in the case of chain *** application examples in affective computing are given to verify the stability of theα-*** summary,through theoretical proof and example verification,it is found that theα-UTImethod has good interval robustness with four kinds of unified interval implications aiming at the situations of an individual rule,multi-rule and reasoning chain.

关键词： Fuzzy reasoning the CRI method the triple I method fuzzy implication interval robustness

Pairing nitroxyl radical and phenazine with electron-withdrawing/-donating substituents in “water-in-ionic liquid” for high-voltage aqueous redox flow batteries

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Green Energy & Environment 2024年第4期9卷 713-722页

作者： Zhifeng huang Rolf Hempelmann Yiqiong Zhang Li Tao Ruiyong Chen Transfercenter Sustainable Electrochemistry Saarland University and KIST Europe66125SaarbruckenGermany State Key Laboratory of Chem/Bio-Sensing and Chemometrics College of Chemistry and Chemical Engineering Hunan University Changsha410082HunanChina College of Materials Science and Engineering Changsha University of Science and Technology Changsha410114HunanChina Materials Innovation Factory Department of ChemistryUniversity of LiverpoolLiverpoolL697ZDUnited Kingdom

Aqueous redox-active organic materials-base electrolytes are sustainable alternatives to vanadium-based electrolyte for redoxﬂow batteries(RFBs)due to the advantages of high ionic conductivity,environmentally benign,safety and low ***,the underexplored redox properties of organic materials and the narrow thermodynamic electrolysis window of water(1.23 v)hinder their wide ***,seeking suitable organic redox couples and aqueous electrolytes with a high output voltage is highly suggested for advancing the aqueous organic *** this work,the functionalized phenazine and nitroxyl radical with electron-donating and electron-withdrawing group exhibit redox potential of-0.88 v and 0.78 v ***,respectively,in“water-in-ionic liquid”supporting *** spectra reveal that the activity of water is largely suppressed in“water-in-ionic liquid”due to the enhanced hydrogen bond interactions between ionic liquid and water,enabling an electrochemical stability window above 3 v.“Water-in-ionic liquid”supporting electrolytes help to shift redox potential of nitroxyl radical and enable the redox activity of functionalized *** assembled aqueous RFB allows a theoretical cell voltage of 1.66 v and shows a practical discharge voltage of 1.5 v in the“water-in-ionic liquid”***,capacity retention of 99.91%per cycle is achieved over 500 charge/discharge cycles.A power density of 112 mW cm^(-2) is obtained at a current density of 30 mA cm^(-2).This work highlights the importance of rationally combining supporting electrolytes and organic molecules to achieve high-voltage aqueous RFBs.

关键词： Aqueous redoxﬂow batteries Water-in-ionic liquid electrolytes High-voltage aqueous batteries Organic redox-active materials

Weakly Polarized Organic Cation-Modified Hydrated vanadium Oxides for High-Energy Efficiency Aqueous Zinc-Ion Batteries

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Nano-Micro Letters 2024年第7期16卷 169-186页

作者： Xiaoxiao Jia Chaofeng Liu Zhi Wang Di huang Guozhong Cao Department of Materials Science and Engineering University of WashingtonSeattleWA 98195USA School of Materials Science and Engineering Tongji UniversityShanghai 201804People’s Republic of China

vanadium oxides,par-ticularly hydrated forms like v_(2)O_(5)·nH_(2)O(vOH),stand out as promising cathode candidates for aqueous zinc ion batteries due to their adjustable layered structure,unique electronic characteristics,and high theoretical ***,challenges such as vanadium dissolution,sluggish Zn^(2+)diffusion kinetics,and low operating voltage still hinder their direct *** this study,we present a novel vanadium oxide([C_(6)H_(6)N(CH_(3))_(3)]_(1.08)v_(8)O_(20)·0.06H_(2)O,TMPA-vOH),developed by pre-inserting trimethylphenylammonium(TMPA+)cations into *** incorporation of weakly polarized organic cations capitalizes on both ionic pre-intercalation and molecular pre-intercalation effects,resulting in a phase and morphology transition,an expansion of the interlayer distance,extrusion of weakly bonded interlayer water,and a substantial increase in v^(4+)*** modifications synergistically reduce the electrostatic interactions between Zn^(2+)and the v-O lattice,enhancing structural stability and reaction kinetics during *** a result,TMPA-vOH achieves an elevated open circuit voltage and operation voltage,exhibits a large specific capacity(451 mAh g^(-1)at 0.1 A g^(-1))coupled with high energy efficiency(89%),the significantly-reduced battery polarization,and outstanding rate capability and cycling *** concept introduced in this study holds great promise for the development of high-performance oxide-based energy storage materials.

关键词： Zinc-ion battery vanadium oxide v_(2)O_(5)·nH_(2)O Pre-intercalation Interlayer engineering

Proterozoic to Phanerozoic case studies of laser ablation microanalysis for microbial carbonate U–Pb geochronology

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Geoscience Frontiers 2024年第2期15卷 30-40页

作者： Yuxiang Jiang Simon v.Hohl Xiangtong huang Shouye Yang State Key Laboratory of Marine Geology School of Ocean and Earth SciencesTongji UniversityShanghai 200092China

Some of the earliest bio-sedimentary records of life on Earth are represented by microbial carbonates,which are also critical geochemical archives of ancient seawater chemistry and the environmental circumstances in which they *** paleo-microbial environments on Earth and potentially other planets requires precise determination of the depositional ages of these ***(abiogenic)carbonate geochemistry communities can now use developments in in-situ laser ablation U-Pb dating using inductively coupled plasma mass spectrometry(LA-ICP-MS).Due to the effects of impurity mixing and diagenesis,microbial carbonates have received little geochronological study despite their broad relevance for understanding ancient seawater’s environmental conditions and geochemical *** study demonstrates using time-of-flight mass spectrometry(TOF-MS)to perform quick,quantitative elemental mapping before U-Pb spot dating to improve experiment success rates and data reliability and offers four practical application examples.

关键词： Stromatolite Microbial carbonate Carbonate geochronology In-situ LA-ICP-MS ICP-Time Of Flight-MS Trace element mapping

Online Monitoring Method for Junction Temperature of SiC MOSFETs based on Temperature Sensitive Electrical Parameter

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CSEE Journal of Power and Energy Systems 2024年第4期10卷 1799-1807页

作者： Han Cao Puqi Ning Yunhao huang Xuhui Wen Wuhan Second Ship Design and Research Institute Wuhan 430205China Key Laboratory of Power Electronics and Electric Drive Institute of Electrical EngineeringChinese Academy of SciencesBeijing 100190China Institute of Electrical Engineering Chinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China Collaborative Innovation Center of Electric vehicles in Beijing Beijing 100081China

Compared to Si devices,the junction temperature of SiC devices is more critical due to the reliability concern introduced by immature packaging technology applied to new *** paper proposes a practical SiC MOSFET junction temperature monitoring method based on the on-state voltage$\\boldsymbol{v}_{\\mathbf{ds}(\\mathbf{on})}$*** Section II of the paper,the temperature sensitivity of the on-state voltage$\\boldsymbol{v}_{\\mathbf{ds}(\\mathbf{on})}$is *** hardware of the measurement system is set up in Section III,which consists of an On-state voltage Measurement Circuit(OvMC),the sampling and isolation ***,a calibration method based on the self-heating of the SiC MOSFET chip is presented in Section *** the final Section,the junction temperature is monitored synchronously according to the calibration *** proposed method is applied to a Buck converter and verified by both an Infrared Radiation(IR)camera and a Finite Element Analysis(FEA)tool.

关键词： Junction temperature Silicon Carbide(SiC)MOSFET TSEP

Heptagonal intramolecular-lock strategy enables high-performance thermally activated delayed fluorescence emitters

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Science China Chemistry 2024年第4期67卷 1181-1186页

作者： Zhenmei huang Dezhi Yang Dongge Ma Zhengyang Bin Jingsong You Key Laboratory of Green Chemistry and Technology of Ministry of Education College of ChemistrySichuan UniversityChengdu 610064China Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and DevicesSouth China University of TechnologyGuangzhou 510640China

The development of highly efficient thermally activated delayed fluorescence(TADF)emitters is persistently pursued for the application of organic light-emitting diodes(OLED)in full-colour display and solid-state ***,we present a heptagonal intramolecular-lock strategy to design high-performance TADF *** a proof-of-concept,a new type of tribenzotropone(TBP)acceptor has been designed and synthesized by a cascade decarboxylative cyclization of aryl oxoacetic acid derivative with biphenyl boronic *** with the unlocked benzophenone(BP)acceptor,the TBP acceptor has a highly twisted heptagonal geometry with moderate rigidity and flexibility,which enables a high-performance TADF emitter with a small single-triplet energy gap(ΔE_(ST))of 0.04 e v,a high photoluminescence quantum yield(Φ_(PL))of 99% and a large horizontal orientation factor(Θ_(//))of 84.0%.Consequently,highly efficient OLEDs with an external quantum efficiency as high as 33.8% are assembled,which is significantly higher than those of DPAC-BP with a highly rotatable BP acceptor(23.8%)as well as DPACFO with a rigid fluorenone(FO)acceptor(6.9%).

关键词： organic light-emitting diodes medium-ring intramolecular-lock thermally activated delayed fluorescence molecular orientation

Numerical investigation of dynamic characteristics of dual throat nozzle and bypass dual throat nozzle in thrust vectoring starting process

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Chinese Journal of Aeronautics 2024年第10期37卷 184-206页

作者： Yuqi ZHANG Jinglei XU Minglei CAO Ruifeng PAN Shuai huang Key Laboratory of Inlet and Exhaust System Technology of Ministry of Education Nanjing University of Aeronautics and AstronauticsNanjing 210016China College of Energy and Power Engineering Nanjing University of Aeronautics and AstronauticsNanjing 210016China State Key Laboratory of Mechanics and Control of Aeronautics and Astronautics Structures Nanjing 210016China

The Bypass Dual Throat Nozzle(BDTN)is a novel fluidic Thrust vectoring(Tv)nozzle,it switches to Tv state by opening the valve in the *** greatly manipulate the BDTN,the dynamic characteristics in the Tv starting process should be *** paper conducts numerical simulations to grasp the variation processes of performances and the flow field evolution of BDTN and Dual Throat Nozzle(DTN).The dynamic responses of Tv starting in typical DTN models are investigated at ***,the Tv starting processes of BDTN in different Nozzle Pressure Ratio(NPR)conditions are simulated,and the valve opening durations(T)are also *** the expected Tv direction is achieved in the DTN,the jet is deflected to the opposite direction at the beginning of the dynamic process,which is called the reverse Tv ***,this phenomenon disappears in the *** larger injection width of DTN intensifies unsteady oscillations,and the reverse Tv phenomenon is *** the BDTN,T determines the delay degree of performance variations compared to the static results,which is called hysteresis *** NPR=10,the hysteresis affects the final stable performance of *** study analyses the dynamic characteristics in DTN and BDTN,laying a foundation for further design of nozzles and control strategies.

关键词： Dual Throat Nozzle(DTN) Bypass Dual Throat Nozzle(BDTN) Dynamic characteristic Thrust vectoring starting process Cavity vortex Hysteresis effect