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Physicochemical properties of coconut husk activated carbon modified by Fe(N0_(3))_(3)and Mn(N0_(3))_(2)

Journal of Iron and Steel Research International 2021年第5期28卷 530-537页

作者： Hong-ming Long Bang-fu Huang Zhe Shi lan-peng liu De-fu Wang Lu Li Key Laboratory of Metallurgical Emission Reduction&Resources Recycling(Anhui University of Technology) Ministry of EducationMa'anshan 243002AnhuiChina Department of Metallurgical Engineering Kunming University of Science and TechnologyKunming 650093YunnanChina Clean Metallurgy Key Laboratory of Complex Iron Resources University of Yunnan ProvinceKunming 650093YunnanChina

Fe-loaded activated carbon(AC)has high surface acidity and more active sites,while manganese-loaded AC has high oxygen *** husk AC modified by Fe-Mn was studied with the aim of revealing the modification ***,HNO_(3)AC was prepared using the nitric acid immersion ***,Fe-Mn/AC was prepared using the Fe(N0_(3))_(3)and Mn(N0_(3))_(2)sequential *** effects of HNO_(3),Fe(N0_(3))_(3),and Mn(N0_(3))_(2)on the pore texture and surface chemical characteristics of carbon materials were examined by scanning electron microscopy,Brunauer-Emmett-Teller(BET)analysis,X-ray diffraction and Fourier-transform infrared *** surface topography,pore structure,active material,and functional groups of AC,HNO_(3)/AC,and Fe-Mn/AC were systematically *** following results were *** surface of HNO_(3)AC has more ditches and air voids;the micropores of HNO_(3)AC are deformed and flattened compared to those of *** surface of Fe-Mn/AC exhibits an accumulation ***_(2)O_(4)and FeMn_(2)O_(4)formed more pore *** and HNO_(3)AC have numerous *** higher loading quantity of Fe-Mn results in bigger specific *** active components of Fe-Mn/AC-1,Fe-Mn/AC-2,Fe-Mn/AC-3,and Fe-Mn/AC-4 are MnFe_(2)O_(4),MnO_(0.43)Fe_(2.57)O_(4),Mn_(3)O_(4),and ot-Fe_(2)O_(3)>*** surface functional groups of AC and HNO_(3)AC are oxygen-containing functional *** effect of Fe-Mn modifying conditions on functional group species is rare;however,Fe/AC has more oxygen-containing functional *** research findings can aid in the desulfurization and denitrification of the Fe-Mn/AC catalyst.

关键词： HNO_(3) Fe(N0_(3))_(3) Mn(N0_(3))_(2) Coconut husk activated carbon Physicochemical property Modification mechanism

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Interface Design Strategy for GNS/AZ91 Composites with Semi-Coherent Structure

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Acta Metallurgica Sinica(English Letters) 2024年第3期37卷 467-483页

作者： Jing-peng Xiong Yi-Qi Zeng Jin-Long liu Wei-Cheng Wang lan Luo Yong liu Key Laboratory of Lightweight and High Strength Structural Materials of Jiangxi Province School of Advanced ManufacturingNanchang UniversityNanchang 330031China School of Physics and Materials Science Nanchang UniversityNanchang 330031China

The interfacial structure plays an important role in the mechanical properties of magnesium matrix composite(MMCs)reinforced with graphene nanosheet(GNS)due to their poor wettability with the Mg *** interface design strategy was proposed to form the semi-coherent interfacial structure with superior bonding *** lattice mismatch and interfacial bonding strength between Mg/rare earth oxide/carbon were utilized as key characteristics to evaluate the interfacial *** oxide(La2O3)was selected as the intermediate candidate due to its low lattice mismatch and high interfacial bonding *** identify the interfacial structure of Mg/La2O3/graphene,first-principles calculations were conducted to calculate the ideal work of separation and electronic structure of the *** demonstrated the presence of strong ionic and covalent interactions at the interface,which theoretically verified the strong interfacial bonding strength among Mg/La2O3/graphene *** experimentally validate the interface strength,MMCs with the interface structure of Mg/La2O3/GNS were *** formation of in-situ La2O3 led to the successful attainment of semi-coherent structures between Mg/La2O3 and La2O3/GNS,resulting in high strength and good ductility of the ***,this work proposes a new approach to interface design in MMCs with an enhancement of mechanical properties.

关键词： Interface design strategy Magnesium matrix composite Graphene nanosheets Semi-coherent interface Mechanical properties

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Surrogate modeling for unsaturated infiltration via the physics and equality-constrained artificial neural networks

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第6期16卷 2282-2295页

作者： peng lan Jingjing Su Sheng Zhang School of Civil Engineering Central South UniversityChangsha410075China Discipline of Civil Surveying and Environmental EngineeringPriority Research Centre for Geotechnical Science and EngineeringThe University of NewcastleCallaghanNSW2308Australia Qinghai University Qinghai810016China

Machine learning(ML)provides a new surrogate method for investigating groundwater flow dynamics in unsaturated *** pure data-driven methods(*** neural network,DNN)can provide rapid predictions,but they do require sufficient on-site data for accurate training,and lack interpretability to the physical processes within the *** this paper,we provide a physics and equalityconstrained artificial neural network(PECANN),to derive unsaturated infiltration solutions with a small amount of initial and boundary *** takes the physics-informed neural network(PINN)as a foundation,encodes the unsaturated infiltration physical laws(*** equation,RE)into the loss function,and uses the augmented Lagrangian method to constrain the learning process of the solutions of RE by adding stronger penalty for the initial and boundary *** unsaturated infiltration cases are designed to test the training performance of PECANN,***-dimensional(1D)steady-state unsaturated infiltration,1D transient-state infiltration,two-dimensional(2D)transient-state infiltration,and 1D coupled unsaturated infiltration and *** predicted results of PECANN are compared with the finite difference solutions or analytical *** results indicate that PECANN can accurately capture the variations of pressure head during the unsaturated infiltration,and present higher precision and robustness than DNN and *** is also revealed that PECANN can achieve the same accuracy as the finite difference method with fewer initial and boundary training ***,we investigate the effect of the hyperparameters of PECANN on solving RE *** provides an effective tool for simulating unsaturated infiltration.

关键词： Richards equation(RE) Unsaturated infiltration Data-driven solutions Numerical modeling Machine learning(ML)

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New γ-Ray Sources Identified in All-sky Surveys Based on Fermipy's Advanced Algorithm

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Research in Astronomy and Astrophysics 2024年第10期24卷 81-91页

作者： Yunchuan Xiang peng Feng Xiaofei lan School of Physics and Astronomy China West Normal UniversityNanchong 637009China Department of Astronomy Yunnan Universityand Key Laboratory of Astroparticle Physics of Yunnan ProvinceKunming 650091China

We employ an efficient method for identifying γ-ray sources across the entire sky,leveraging advanced algorithms from Fermipy,and cleverly utilizing the Galactic diffuse background emission model to partition the entire sky into72 regions,thereby greatly enhancing the efficiency of discovering new sources throughout the sky through multithreaded parallel *** confirming the reliability of the new method,we applied it for the first time to analyze data from the Fermi Large Area Telescope(Fermi-LAT)encompassing approximately 15.41 yr of all-sky *** this analysis,we successfully identified 1379 new sources with significance levels exceeding 4σ,of which 497 sources exhibited higher significance levels exceeding 5σ.Subsequently,we performed a systematic analysis of the spatial extension,spectra,and light variation characteristics of these newly identified *** identified 21 extended sources and 23 sources exhibiting spectral curvature above 10 ***,we identified 44 variable sources above 1 GeV.

关键词： gamma-rays:diffuse background methods:data analysis catalogs gamma-rays:general

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Fabrication of Molecularly Imprinted Electrospun Nanofibers with Mono-amidoxime Functional Ligand for Efficient Decontamination of Toxic Organophosphates

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Chinese Journal of Polymer Science 2024年第4期42卷 446-456页

作者： lan Wang peng Jiang Ya-Lin Niu Jun-peng Cao Tian-Ying Guo Key Laboratory of Functional Polymer Materials Ministry of EducationInstitute of Polymer ChemistryCollege of Chemistry and Frontier Science Center for the Creation of New Organic SubstancesNankai UniversityTianjin300071China

There is an urgent imperative to discover practical and efficacious artificial catalysts for the expeditious decontamination of toxic organophosphates. Herein, we propose a novel molecularly imprinted approach utilizing electrospun fiber scaffolds. Specifically, an amidoxime-based functional polymer (PMAOX) has been synthesized, which contains amidoxime groups that can act as nucleophiles and ligands for the formation of catalytic active sites. This polymer was blended with polyacrylonitrile (PAN), a well-processable material, to prepare a nanofiber mat using electrospinning techniques. Then, the amidoxime side groups on fiber surface were further cross-linked after the molecular coordination of templates to complete the molecularly imprinting process. This approach can not only enhance the content of functional molecularly imprinted polymers without affecting structural stability, but also combines surface MI technology to fully expose and leverage the advantages of active sites. The as prepared molecularly imprinted electrospun nanofibers MIF-Zn-PMAOX/PAN-6/4 catalyzes the degradation of paraoxon with a half-life of 32 min, and MIF-Ag-PMAOX/PAN catalyzes the degradation of parathion with a half-life of 18 min. The maximum catalytic rate evidence rate enhancements nearly 3700-fold of the self-hydrolysis. Thus, the mono-amidoxime based molecularly imprinted fibers demonstrate the versatility and superiority as self-detoxifying for organophosphates.

关键词： Organophosphateshydrolysis Electrospinning Molecular imprinting

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Probing phase transition of band topology via radiation topology

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Photonics Research 2024年第6期12卷 1150-1157页

作者： CHANG-YIN JI WENZE lan peng FU GANG WANG CHANGZHI GU YELIANG WANG JIAFANG LI YUGUI YAO BAOLI liu Key Laboratory of Advanced Optoelectronic Quantum Architecture and Measurement(MOE) Beijing Key Laboratory of Nanophotonics&Ultrafine Optoelectronic Systemsand School of PhysicsBeijing Institute of TechnologyBeijing 100081China School of Integrated Circuits and Electronics MIIT Key Laboratory for Low-Dimensional Quantum Structure and DevicesBeijing Institute of TechnologyBeijing 100081China Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China School of Physical Sciences CAS Key Laboratory of Vacuum PhysicsUniversity of Chinese Academy of SciencesBeijing 100190China CAS Center for Excellence in Topological Quantum Computation CAS Key Laboratory of Vacuum PhysicsUniversity of Chinese Academy of SciencesBeijing 100190China

Topological photonics has received extensive attention from researchers because it provides brand new physical principles to manipulate *** topology is characterized using the Berry phase defined by Bloch *** now,the scheme for experimentally probing the topological phase transition of band topology has always been relatively lacking in topological ***,radiation topology can be aroused by the far-field polarization singularities of Bloch states,which is described by the Stokes *** such two types of topologies are both related to Bloch states on the band structures,it is rather surprising that their development is almost ***,in optical analogs of the quantum spin Hall effects(QSHEs)and Su-Schrieffer-Heeger model,we reveal the correlation between the phase transition of band topology and radiation topology and then demonstrate that the radiation topology can be employed to study the band topological *** experimentally demonstrate such an intriguing phenomenon in optical analogs of *** findings not only provide an insightful understanding of band topology and radiation topology,but also can serve as a route to manipulate light.

关键词： transition topology topological

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Microfacies and diagenetic alteration in a semi-deep to deep lacustrine shale: The Yanchang Formation in the Ordos Basin, China

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Petroleum Science 2024年第3期21卷 1524-1538页

作者： Bin Bai Jing-Yue Hao Ling Fu Yu-Xi liu Jian-peng Wang lan Wang Kevin GTaylor Lin Ma PetroChina Research Institute of Petroleum Exploration and Development Beijing100083China Department of Earth and Environmental Sciences University of ManchesterM139PLUK College of Earth Sciences Jilin UniversityChangchun130061jilinChina Department of Chemical Engineering University of ManchesterM139PLUK

The mineralogical development and diagenetic sequence of lacustrine shales in the Chang 7 Member of the Yanchang Formation in the Ordos Basin are detailed studied.A model of their depositional system and a diagenetic diagram are proposed in this *** detailed petrographic,mineralogical,and elemental analyses,four distinct shale types are identified:argillaceous shale,siliceous shale,calcareous shale,and carbonate,clay,and silt-bearing *** main diagenetic process in argillaceous shale is the transformation of illite to smectite,negatively impacting shale *** shale undergoes carbonate cementation and quartz dissolution,contributing to increased porosity,particularly in *** shale experiences diagenesis characterised by carbonate formation and dissolution,with a prevalence of *** carbonate,clay,and silt-bearing shale,the dissolution of K-feldspar contributes to illitization of *** shale,characterised by more clay minerals and lower mesopore volume,is identified as a potential hydrocarbon *** shale,with the highest pore volume and abundant inter-mineral pores,emerges as a promising shale oil *** findings contribute to a comprehensive understanding of shale properties,aiding in the prediction of shale oil exploration potential in the studied area.

关键词： Ordos Basin Yanchang Formation Chang 7 Member Diagenesis Microfacies

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Self-propelled Leidenfrost droplets on femtosecond-laser-induced surface with periodic hydrophobicity gradient

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International Journal of Extreme Manufacturing 2024年第2期6卷 502-509页

作者： Bohong Li lan Jiang Xiaowei Li Zhipeng Wang peng Yi Laser Micro/Nano Fabrication Laboratory School of Mechanical EngineeringBeijing Institute of TechnologyBeijingPeople’s Republic of China Beijing Institute of Technology Chongqing Innovation Center ChongqingPeople’s Republic of China Yangtze Delta Region Academy of Beijing Institute of Technology JiaxingPeople’s Republic of China

The controllable transfer of droplets on the surface of objects has a wide application prospect in the fields of microfluidic devices,fog collection and so *** Leidenfrost effect can be utilized to significantly reduce motion ***,the use of 3D structures limits the widespread application of self-propulsion based on Leidenfrost droplets in microelectromechanical *** manipulate Leidenfrost droplets,it is necessary to create 2D or quasi-2D *** this study,femtosecond laser is applied to fabricate a surface with periodic hydrophobicity gradient(SPHG),enabling directional self-propulsion of Leidenfrost *** field analysis within the Leidenfrost droplets reveals that the vapor layer between the droplets and the hot surface can be modulated by the SPHG,resulting in directional propulsion of the inner *** viscous force between the gas and liquid then drives the droplet to move.

关键词： self-propelled Leidenfrost droplets periodic hydrophobicity gradient femtosecond laser fabrication

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Knittable and washable aerogel fiber inspired by polar bear hair

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Science China Materials 2024年第2期67卷 705-706页

作者： Yue liu Huisheng peng State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Scienceand Institute of Fiber Materials and DevicesFudan UniversityShanghai 200438China

The advances in chemistry and materials have boosted the development of smart textiles,which are poised to revolutionize human lifestyles through multifunctional integration,such as heating,cooling,sensing and supplying energy^([1,2]).Among them,thermal insulation is an essential function of textiles to protect humans from complex and extreme environments and realize personal thermal management without energy con-sumption^([3]).

关键词： textiles insulation extreme

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Simulation of Underground Reservoir Stability of Pumped Storage Power Station Based on Fluid-Structure Coupling

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Computer Modeling in Engineering & Sciences 2024年第5期139卷 1381-1399页

作者： peng Qiao Shuangshuang lan Hongbiao Gu Zhengtan Mao Faculty of Architecture Civil and Transportation EngineeringBeijing University of TechnologyBeijing100020China College of Transportation Engineering Nanjing Tech UniversityNanjing210000China

Based on global initiatives such as the clean energy transition and the development of renewable energy,the pumped storage power station has become a new and significant way of energy storage and regulation,and its construction environment is more complex than that of a traditional *** particular,the stability of the rock strata in the underground reservoirs is affected by the seepage pressure and rock stress,which presents some challenges in achieving engineering safety and *** the advantages of the numerical simulation method in dealing deal with nonlinear problems in engineering stability,in this study,the stability of the underground reservoir of the Shidangshan(SDS)pumped storage power station was numerically calculated and quantitatively analyzed based on fluid-structure coupling theory,providing an important reference for the safe operation and management of the underground ***,using the COMSOL software,a suitablemechanicalmodel was created in accordance with the geological structure and project characteristics of the underground ***,the characteristics of the stress field,displacement field,and seepage field after excavation of the underground reservoir were simulated in light of the seepage effect of groundwater on the nearby rock of the underground ***,based on the construction specifications and Molar-Coulomb criterion,a thorough evaluation of the stability of the underground reservoir was performed through simulation of the filling and discharge conditions and anti-seepage strengthening *** findings demonstrate that the numerical simulation results have a certain level of reliability and are in accordance with the stress measured in the project *** underground reservoir excavation resulted in a maximum displacement value of the rock mass around the caverns of 3.56 mm in a typical section,and the safety coefficient of the parts,as determined using the Molar-Coulomb criterion,was highe

关键词： Underground reservoir fluid-structure coupling numerical simulation pumped storage power station filling and discharge

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